arXiv subjects

Alexander V. Balatsky

Publications and source records attributed to Alexander V. Balatsky.

At least 37 records · Page 2Linked to original sources

arXiv2025

Large inverse Faraday effect for Rydberg states of free atoms and isolated donors in semiconductors

We report on the induction of magnetization in Rydberg systems by means of the inverse Faraday effect, and propose the appearance of the effect in two such systems, Rydberg atoms proper and shallow dopants in semiconductors. Rydberg atoms are characterized by a large orbital radius. This large radius gives such excited states a large angular moment, which when driven with circularly polarized light, translates to a large effective magnetic field ${B}_{\text{eff}}$. We calculate this effect to generate effective magnetic fields of $O(1\,μ\text{T})\times\left( \fracω{1\,\text{THz}} \right)^{-1} \left( \frac{I}{10\,\text{W cm}^{-2}} \right) n^4$ in the Rydberg states of atoms such as Rb and Cs for off-resonant photon beams with frequency omega and intensity ${I}$ expressed in units of the denominators and $n$ the principal quantum number. Additionally, terahertz spectroscopy of phosphorus doped silicon reveals a large cross-section for excitation of shallow dopants to Rydberg-like states, which even for small $n$ have the potential to be driven similarly with circularly polarized light to produce an even larger magnetization. Our theoretical calculations estimate ${B}_{\text{eff}}$ as $O(10^2\,\text{T})$ for Si:P with a beam intensity of $10^8\,\text{W cm}^{-2}$.

physics.atom-ph↗

arXiv2024

Ultrafast pseudomagnetic fields from electron-nuclear quantum geometry

Recent experiments demonstrate precise control over coherently excited circular phonon modes using high-intensity terahertz lasers, opening new pathways towards dynamical, ultrafast design of magnetism in functional materials. While the phonon Zeeman effect enables a theoretical description of phonon-induced magnetism, it lacks efficient angular momentum transfer from the phonon to the electron sector. In this work, we put forward a coupling mechanism based on electron-nuclear quantum geometry, with the inverse Faraday effect as a limiting case. This effect is rooted in the phase accumulation of the electronic wavefunction under a circular evolution of nuclear coordinates. An excitation pulse then induces a transient level splitting between electronic orbitals that carry angular momentum. First-principle simulations on SrTiO$_3$ demonstrate that in parts of the Brillouin zone, this splitting between orbitals carrying angular momentum can easily reach 50 meV.

cond-mat.mtrl-sci↗

arXiv2024

Probing multi-mobility edges in quasiperiodic mosaic lattices

The mobility edge (ME) is a crucial concept in understanding localization physics, marking the critical transition between extended and localized states in the energy spectrum. Anderson localization scaling theory predicts the absence of ME in lower dimensional systems. Hence, the search for exact MEs, particularly for single particles in lower dimensions, has recently garnered significant interest in both theoretical and experimental studies, resulting in notable progress. However, several open questions remain, including the possibility of a single system exhibiting multiple MEs and the continual existence of extended states, even within the strong disorder domain. Here, we provide experimental evidence to address these questions by utilizing a quasiperiodic mosaic lattice with meticulously designed nanophotonic circuits. Our observations demonstrate the coexistence of both extended and localized states in lattices with broken duality symmetry and varying modulation periods. By single site injection and scanning the disorder level, we could approximately probe the ME of the modulated lattice. These results corroborate recent theoretical predictions, introduce a new avenue for investigating ME physics, and offer inspiration for further exploration of ME physics in the quantum regime using hybrid integrated photonic devices.

cond-mat.dis-nn↗

arXiv2024

Light Induced Orbital Magnetism in Metals via Inverse Faraday Effect

We present a microscopic calculation of the inverse Faraday effect in metals. We derive a static local magnetic moment induced on the application of high-frequency light, using the Eilenberger formulation of quasiclassical theory. We include the effect of disorder and formulate a theory applicable across the entire temperature range, in the absence of external applied fields. For light-induced electric fields of amplitude $\sim 100 kV/cm$, the induced fields are large, $\sim 0.1 T$ for metallic Nb! The predictions of our theory agree with recent experimental and theoretical results [1]. An extension of this approach to superconductors would open a new route of inducing orbital magnetic field and potentially vortices in superconductors.

cond-mat.supr-con↗

arXiv2024

Quantum Nonlinear Acoustic Hall Effect and Inverse Acoustic Faraday Effect in Dirac Insulators

We propose to realize the quantum nonlinear Hall effect and the inverse Faraday effect through the acoustic wave in a time-reversal invariant but inversion broken Dirac insulator. We focus on the acoustic frequency much lower than the Dirac gap such that the interband transition is suppressed and these effects arise solely from the intrinsic valley-contrasting band topology. The corresponding acoustoelectric conductivity and magnetoacoustic susceptibility are both proportional to the quantized valley Chern number and independent of the quasiparticle lifetime. The linear and nonlinear components of the longitudinal and transverse topological currents can be tuned by adjusting the polarization and propagation directions of the surface acoustic wave. The static magnetization generated by a circularly polarized acoustic wave scales linearly with the acoustic frequency as well as the strain-induced charge density. Our results unveil a quantized nonlinear topological acoustoelectric response of gapped Dirac materials, like hBN and transition-metal dichalcogenide, paving the way toward room-temperature acoustoelectric devices due to their large band gaps.

cond-mat.mes-hall↗

arXiv2024

Electron-phonon coupling in copper-substituted lead phosphate apatite

Recent reports of room-temperature, ambient pressure superconductivity in copper-substituted lead phosphate apatite, commonly referred to as LK99, have prompted numerous theoretical and experimental studies into its properties. As the electron-phonon interaction is a common mechanism for superconductivity, the electron-phonon coupling strength is an important quantity to compute for LK99. In this work, we compare the electron-phonon coupling strength among the proposed compositions of LK99. The results of our study are in alignment with the conclusion that LK99 is not a likely candidate for room-temperature superconductivity if electron-phonon interaction is to serve as the mechanism.

cond-mat.supr-con↗

arXiv2024

Screening the organic materials database for superconducting metal-organic frameworks

The increasing financial and environmental cost of many inorganic materials has motivated study into organic and "green" alternatives. However, most organic compounds contain a large number of atoms in the primitive unit cell, posing a significant barrier to high-throughput screening for functional properties. In this work, we attempt to overcome this challenge and identify superconducting candidates among the metal-organic-frameworks in the organic materials database using a recently proposed proxy for the electron-phonon coupling. We then isolate the most promising candidate for in-depth analysis, C$_{9}$H$_{8}$Mn$_{2}$O$_{11}$, providing evidence for superconductivity below $100$mK.

cond-mat.mtrl-sci↗

arXiv2024

P-wave pairing near a spin-split Josephson junction

Superconductivity and magnetism are competing effects that can coexist in certain regimes. Their co-existence leads to unexpected new behaviors that include the onset of exotic electron pair mechanisms and topological phases. In this work, we study the properties of a Josephson junction between two spin-split superconductors. The spin-splitting in the superconductors can arise from either the coupling to a ferromagnetic material or an external magnetic field. The properties of the junction are dominated by the Andreev bound states that are also split. One of these states can cross the superconductor's Fermi level, leading to a ground state transition characterized by a suppressed supercurrent. We interpret the supercurrent blockade as coming from a dominance of p-wave pairing close to the junction, where electrons at both sides of the junction pair. To support this interpretation, we analyze the different pairing channels and show that p-wave pairing is favored in the case where the magnetization of the two superconductors is parallel and suppressed in the anti-parallel case. We also analyze the noise spectrum that shows signatures of the ground state transition in the form of an elevated zero-frequency noise.

cond-mat.supr-con↗

arXiv2024

Kapitza stabilization of quantum critical order

Dynamical perturbations modify the states of classical systems in surprising ways and give rise to important applications in science and technology. For example, Floquet engineering exploits the possibility of band formation in the frequency domain when a strong, periodic variation is imposed on parameters such as spring constants. We describe here Kapitza engineering, where a drive field oscillating at a frequency much higher than the characteristic frequencies for the linear response of a system changes the potential energy surface so much that maxima found at equilibrium become local minima, in precise analogy to the celebrated Kapitza pendulum where the unstable inverted configuration, with the mass above rather than below the fulcrum, actually becomes stable. Our starting point is a quantum field theory of the Ginzburg-Devonshire type, suitable for many condensed matter systems, including particularly ferroelectrics and quantum paralectrics. We show that an off-resonance oscillatory electric field generated by a laser-driven THz source can induce ferroelectric order in the quantum-critical limit. Heating effects are estimated to be manageable using pulsed radiation; ``hidden" radiation-induced order can persist to low temperatures without further pumping due to stabilization by strain. We estimate the Ginzburg-Devonshire free-energy coefficients in SrTiO${}_{3}$ using density-functional theory (DFT) and the stochastic self-consistent harmonic approximation accelerated by a machine-learned force field. Although we find that SrTiO${}_{3}$ is not an optimal choice for Kapitza stabilization, we show that scanning for further candidate materials can be performed at the computationally convenient density-functional theory level. We suggest second-harmonic-generation, soft-mode-spectroscopy, and X-ray-diffraction experiments to characterize the induced order.

cond-mat.str-el↗

arXiv2023

Mobile Topological Su-Schrieffer-Heeger Soliton in a Josephson Metamaterial

Circuits involving arrays of Josephson junctions have emerged as a new platform for exploring and simulating complex bosonic systems. Motivated by this advance, we develop and theoretically analyze a one-dimensional bosonic system with sublattice symmetry, a bosonic Su-Schrieffer-Heeger model. The system features electrostatically controlled topological mid-gap states that we call soliton states. These modes can be measured using either spectroscopy through a normal lead or admittance measurements. We develop a protocol to adiabatically shuttle the position of these topological soliton states using local electrostatic gates. We demonstrate a nearly perfect fidelity of soliton shuttling for timescales within experimental reach.

cond-mat.supr-con↗

arXiv2023

Coexistence of extended and localized states in finite-sized mosaic Wannier-Stark lattices

Quantum transport and localization are fundamental concepts in condensed matter physics. It is commonly believed that in one-dimensional systems, the existence of mobility edges is highly dependent on disorder. Recently, there has been a debate over the existence of an exact mobility edge in a modulated mosaic model without quenched disorder, the so-called mosaic Wannier-Stark lattice. Here, we experimentally implement such disorder-free mosaic photonic lattices using a silicon photonics platform. By creating a synthetic electric field, we could observe energy-dependent coexistence of both extended and localized states in a finite number of waveguides. The Wannier-Stark ladder emerges when the resulting potential is strong enough, and can be directly probed by exciting different spatial modes of the lattice. Our studies provide the experimental proof of coexisting sets of strongly localized and conducting (though weakly localized) states in finite-sized mosaic Wannier-Stark lattices, which hold the potential to encode high-dimensional quantum resources with compact and robust structures.

cond-mat.dis-nn↗

arXiv2023

Appearance of Odd-Frequency Superconductivity in a Relativistic Scenario

Odd-frequency superconductivity is an exotic superconducting state in which the symmetry of the gap function is odd in frequency. Here we show that an inherent odd-frequency mode emerges dynamically under application of a Lorentz transformation of the anomalous Green function with the general frequency-dependent gap function. To see this, we consider a Dirac model with quartic potential and perform a mean-field analysis to obtain a relativistic Bogoliubov-de Gennes system. Solving the resulting Gor'kov equations yields expressions for relativistic normal and anomalous Green functions. The form of the relativistically invariant pairing term is chosen such that it reduces to BCS form in the non-relativistic limit. We choose an ansatz for the gap function in a particular frame which is even-frequency and analyze the effects on the anomalous Green function under a boost into a relativistic frame. The odd-frequency pairing emerges dynamically as a result of the boost. In the boosted frame the order parameter contains terms which are both even and odd in frequency. The relativistic correction to the anomalous Green function to first order in the boost parameter is completely odd in frequency. This work provides evidence that odd-frequency pairing may form intrinsically within relativistic superconductors.

cond-mat.supr-con↗

arXiv2023

Inducing Quantum Phase Transitions in Non-Topological Insulators Via Atomic Control of Sub-Structural Elements

Topological insulators (TIs) are an important family of quantum materials that exhibit a Dirac point (DP) in the surface band structure but have a finite band gap in bulk. A large degree of spin-orbit interaction and low bandgap is a prerequisite for stabilizing DPs on selective atomically flat cleavage planes. Tuning of the DP in these materials has been suggested via modifications to the atomic structure of the entire system. Using the example of As$_2$Te$_3$ and ZnTe$_5$, which are not TIs, we show that a quantum phase transition can be induced in atomically flat and stepped surfaces, for As$_2$Te$_3$ and ZrTe$_5$, respectively. This is achieved by establishing a framework for controlling electronic properties that is focused on local perturbations at key locations that we call sub-structural elements (SSEs). We exemplify this framework through a novel method of isovalent sublayer anion doping and biaxial strain.

cond-mat.mtrl-sci↗

arXiv2022

Obstructions to odd-frequency superconductivity in Eliashberg theory

We present a necessary condition for odd-frequency (odd-f) superconductivity (SC) to occur in a large class of materials described by Eliashberg theory. We use this condition to prove a no-go theorem ruling out the occurrence of odd-f SC in standard one-band superconductors with pairing interactions mediated by phonon exchange. We also present a corresponding no-go theorem for superconductors with interactions mediated by spin-fluctuations. Our results explain why odd-f SC is rare in conventional materials, and they open up the possibility for a search for materials with interactions designed so as to allow for odd-f SC.

cond-mat.supr-con↗

arXiv2021

Persistent current noise in narrow Josephson junctions

Josephson junctions have broad applications in metrology, quantum information processing, and remote sensing. For these applications, the electronic noise is a limiting factor. In this work we study the thermal noise in narrow Josephson junctions using a tight-binding Hamiltonian. For a junction longer than the superconducting coherence length, several self-consistent gap profiles appear close to a phase difference $π$. They correspond to two stable solutions with an approximately constant phase gradient over the thin superconductor connected by a $2π$ phase slip, and a solitonic branch. The current noise power spectrum has pronounced peaks at the transition frequencies between the different states in each branch. We find that the noise is reduced in the gradient branches in comparison to the zero-length junction limit. In contrast, the solitonic branch exhibits an enhanced noise and a reduced current due to the pinning of the lowest excitation energy to close to zero energy.

cond-mat.supr-con↗

arXiv2021

Shifting computational boundaries for complex organic materials

Methodology adapted from data science sparked the field of materials informatics, and materials databases are at the heart of it. Applying artificial intelligence to these databases will allow the prediction of properties of complex organic crystals.

cond-mat.mtrl-sci↗

arXiv2021

Axion-matter coupling in multiferroics

Multiferroics (MFs) are materials with two or more ferroic orders, like spontaneous ferroelectric and ferromagnetic polarizations. Such materials can exhibit a magnetoelectric effect whereby magnetic and ferroelectric polarizations couple linearly, reminiscent of, but not identical to the electromagnetic $\boldsymbol{E}\cdot \boldsymbol{B}$ axion coupling. Here we point out a possible mechanism in which an external dark matter axion field couples linearly to ferroic orders in these materials without external applied fields. We find the magnetic response to be linear in the axion-electron coupling. At temperatures close to the ferromagnetic transition fluctuations can lead to an enhancement of the axion-induced magnetic response. Relevant material candidates such as the Lu-Sc hexaferrite family are discussed.

hep-ph↗

arXiv2021

Hidden, entangled and resonating order

In condensed matter systems, the atoms, electrons or spins can sometimes arrange themselves in ways that result in unexpected properties but that cannot be detected by conventional experimental probes. Several historical and contemporary examples of such hidden orders are known and more are awaiting discovery, perhaps in the form of more complex composite, entangled or dynamical hidden orders.

cond-mat.mtrl-sci↗