arXiv subjects

Alexander von Reppert

Publications and source records attributed to Alexander von Reppert.

4 recordsLinked to original sources

arXiv2025

Experimental evidence of dominant ultrafast diffusive energy transport by hot electrons in Cu

When the dimensions of structures shrink to the order of the inelastic mean free path of the energy-carrying quasi-particles, the character of energy transport changes from diffusive to ballistic. However, the point of transition remains a matter of debate. Here, we determine the dominant channel of energy transport through a nanoscale Cu layer as a function of its thickness. The energy rapidly transferred across Cu via hot electrons from a photo-excited Pt layer into a buried Ni detection layer translates into a rapid expansion of the Ni layer probed via ultrafast x-ray diffraction. The non-linear dependence of the Ni strain amplitude on the absorbed laser fluence indicates that the transport through Cu becomes more efficient with increasing fluence. This fluence-dependent transport efficiency is reproduced by a diffusive energy transport model and serves as a generally applicable experimental approach to distinguish diffusion from ballistic transport. Following this approach, we identify diffusive electronic energy transport to govern the spatial energy distribution for Cu layer thicknesses larger than twice the electronic inelastic mean free path.

cond-mat.mtrl-sci↗

arXiv2025

Rapid heat assisted polarization reversal in ferroelectric thin films

We demonstrate that switching of ferroelectric thin-films sandwiched between metallic electrodes can be controlled by laser-assisted heating, reminiscent of heat-assisted magnetic recording. We employ electrical switching cycles that quantify the electrically switchable remanent polarization $P_\mathrm{r}$ and show that 300\,ns voltage pulses alone change the polarization by less than $ΔP P_\mathrm{r}$ of the average polarization. The transient average temperature modeled by the heat equation can rationalize the polarization change observed for different relative timing $Δt$ of the laser pulse, if it arrives before the electrical pulse.

cond-mat.mtrl-sci↗

arXiv2024

Controlling effective field contributions to laser-induced magnetization precession by heterostructure design

Nanoscale heterostructure design can control laser-induced heat dissipation and strain propagation as well as their efficiency for driving magnetization precession. We use insulating MgO layers incorporated into metallic Pt-Cu-Ni heterostructures to block the propagation of hot electrons. Ultrafast x-ray diffraction (UXRD) experiments quantify how this enables controlling the spatio-temporal shape of the transient heat and strain, which drive the magnetization dynamics in the Ni layer. The frequency of the magnetization precession observed by the time-resolved magneto-optical Kerr effect (MOKE) in polar geometry is systematically tuned by the magnetic field orientation. The combined experimental analysis (UXRD and MOKE) and modeling of transient strain, heat and magnetization uniquely highlights the importance of quasi-static strain as a driver of precession, when the magnetic material is rapidly heated via electrons. The concomitant effective field change originating from demagnetization partially compensates the change induced by quasi-static strain. Tailored strain pulses shaped via the nanoscale heterostructure design provide an equally efficient, phase-matched driver of precession, paving the way for opto-magneto-acoustic devices with low heat energy deposited in the magnetic layer.

cond-mat.mtrl-sci↗

arXiv2023

Concepts and use cases for picosecond ultrasonics with x-rays

This review discusses picosecond ultrasonics experiments using ultrashort hard x-ray probe pulses to extract the transient strain response of laser-excited nanoscopic structures from Bragg-peak shifts. This method provides direct, layer-specific, and quantitative information on the picosecond strain response for structures down to few-nm thickness. We model the transient strain using the elastic wave equation and express the driving stress using Grüneisen parameters stating that the laser-induced stress is proportional to energy density changes in the microscopic subsystems of the solid, i.e., electrons, phonons and spins. The laser-driven strain response can thus serve as an ultrafast proxy for local energy-density and temperature changes, but we emphasize the importance of the nanoscale morphology for an accurate interpretation due to the Poisson effect. The presented experimental use cases encompass ultrathin and opaque metal heterostructures, continuous and granular nanolayers as well as negative thermal expansion materials, that each pose a challenge to established all-optical techniques.

cond-mat.mtrl-sci↗