arXiv subjects

Alexandra Tofful

Publications and source records attributed to Alexandra Tofful.

5 recordsLinked to original sources

arXiv2026

International Optical Clock Comparison Using the European Optical Fiber Network

Optical clocks have achieved remarkable estimated fractional frequency uncertainties reaching the $10^{-18}$ level and below, enabling applications in fundamental physics, general relativity, and geodesy. However, the challenge of verifying the international consistency of optical clocks remains critical as efforts intensify toward redefining the SI second based on an optical transition or transitions. We report on a two-month international clock comparison campaign involving seven optical clocks in four national metrology institutes (INRIM, LNE-OP, NPL, and PTB) connected via the optical fiber network established in Europe. The campaign resulted in optical frequency ratios with uncertainties ranging from $7.7\times10^{-18}$ to $6.1\times10^{-17}$. Among the results, the $^{171}$Yb$^+$(E3) clocks at NPL and PTB demonstrated agreement within an uncertainty of $7.7\times10^{-18}$, marking the first international verification of two independently developed optical clocks below one part in $10^{17}$. The operation of the $^{199}$Hg clock at LNE-OP (formerly LNE-SYRTE) resulted in frequency ratios with improved uncertainties with $^{171}$Yb$^+$(E3), $^{171}$Yb, and $^{87}$Sr optical clocks. These results provide input for the redefinition of the second and underscore how fiber-linked clock networks can advance metrology and scientific applications.

physics.atom-ph↗

arXiv2025

Coordinated international comparisons between optical clocks connected via fiber and satellite links

Optical clocks provide ultra-precise frequency references that are vital for international metrology as well as for tests of fundamental physics. To investigate the level of agreement between different clocks, we simultaneously measured the frequency ratios between ten optical clocks in six different countries, using fiber and satellite links. This is the largest coordinated comparison to date, from which we present a subset of 38 optical frequency ratios and an evaluation of the correlations between them. Four ratios were measured directly for the first time, while others had significantly lower uncertainties than previously achieved, supporting the advance towards a redefinition of the second and the use of optical standards for international time scales.

physics.atom-ph↗

arXiv2024

$^{171}$Yb$^+$ optical clock with $2.2\times 10^{-18}$ systematic uncertainty and absolute frequency measurements

A full evaluation of the uncertainty budget for the ytterbium ion optical clock at the National Physical Laboratory (NPL) was performed on the electric octupole (E3) $^2\mathrm{S}_{1/2}\,\rightarrow\, ^2\mathrm{F}_{7/2}$ transition. The total systematic frequency shift was measured with a fractional standard systematic uncertainty of $2.2\times 10^{-18}$. Furthermore, the absolute frequency of the E3 transition of the $^{171}$Yb$^+$ ion was measured between 2019 and 2023 via a link to International Atomic Time (TAI) and against the local caesium fountain NPL-CsF2. The absolute frequencies were measured with fractional standard uncertainties between $3.7 \times 10^{-16}$ and $1.1 \times 10^{-15}$, and all were in agreement with the 2021 BIPM recommended frequency.

physics.atom-ph↗

arXiv2023

Analysis of atomic-clock data to constrain variations of fundamental constants

We present a new framework to study the time variation of fundamental constants in a model-independent way. Model independence implies more free parameters than assumed in previous studies. Using data from atomic clocks based on $^{87}$Sr, $^{171}$Yb$^+$ and $^{133}$Cs, we set bounds on parameters controlling the variation of the fine-structure constant, $\alpha$, and the electron-to-proton mass ratio, $\mu$. We consider variations on timescales ranging from a minute to almost a day. In addition, we use our results to derive some of the tightest limits to date on the parameter space of models of ultralight dark matter and axion-like particles.

physics.atom-ph↗

arXiv2022

The mechanism of high harmonic generation in liquid alcohol

The observation of non-perturbative harmonic emission in solids from ultrashort laser pulses [1] sparked a wave of studies [2,3] as a probe of charge carrier dynamics in solids under strong fields and a route to extreme ultraviolet (XUV) attosecond photonic devices [4]. High harmonic generation (HHG) in liquids [5,6] is far less explored, despite their relevance to biological media, and the mechanism is hotly debated. Using few-cycle pulses below the breakdown threshold, we demonstrate HHG in alcohol with data showing carrier-envelope-phase-dependent XUV spectra extending to 50 eV from isopropanol. We study the mechanism of the harmonic emission through its dependence on the driving field and find it to be consistent with a strong-field recombination mechanism. This maps emitted photon energy to the electron trajectories. We explore the role of the liquid environment in scattering the trajectories and find evidence that information on electron scattering from neighbouring molecules is encoded in the harmonic spectra. Using simulations we exploit this to estimate the scattering cross section and we confirm that the cross-section in liquid isopropanol is significantly reduced compared to vapour. Our findings suggest an \textit{in situ} measurement strategy for retrieving accurate values of scattering cross sections in liquids, and also a pathway to liquid-based attosecond XUV devices.

physics.optics↗