arXiv subjects

Alexei Trifonov

Publications and source records attributed to Alexei Trifonov.

8 recordsLinked to original sources

arXiv2012

Multi-color correlative light and electron microscopy using nanoparticle cathodoluminescence

Correlative light and electron microscopy promises to combine molecular specificity with nanoscale imaging resolution. However, there are substantial technical challenges including reliable co-registration of optical and electron images, and rapid optical signal degradation under electron beam irradiation. Here, we introduce a new approach to solve these problems: multi-color imaging of stable optical cathodoluminescence emitted in a scanning electron microscope by nanoparticles with controllable surface chemistry. We demonstrate well-correlated cathodoluminescence and secondary electron images using three species of semiconductor nanoparticles that contain defects providing stable, spectrally-distinguishable cathodoluminescence. We also demonstrate reliable surface functionalization of the particles. The results pave the way for the use of such nanoparticles for targeted labeling of surfaces to provide nanoscale mapping of molecular composition, indicated by cathodoluminescence color, simultaneously acquired with structural electron images in a single instrument.

physics.ins-det↗

arXiv2010

Properties of nitrogen-vacancy centers in diamond: group theoretic approach

We present a procedure that makes use of group theory to analyze and predict the main properties of the negatively charged nitrogen-vacancy (NV) center in diamond. We focus on the relatively low temperatures limit where both the spin-spin and spin-orbit effects are important to consider. We demonstrate that group theory may be used to clarify several aspects of the NV structure, such as ordering of the singlets in the ($e^2$) electronic configuration, the spin-spin and the spin-orbit interactions in the ($ae$) electronic configuration. We also discuss how the optical selection rules and the response of the center to electric field can be used for spin-photon entanglement schemes. Our general formalism is applicable to a broad class of local defects in solids. The present results have important implications for applications in quantum information science and nanomagnetometry.

quant-ph↗

arXiv2007

Fast quantum key distribution with decoy number states

We investigate the use of photon number states to identify eavesdropping attacks on quantum key distribution (QKD) schemes. The technique is based on the fact that different photon numbers traverse a channel with different transmittivity. We then describe two QKD schemes that utilize this method, one of which overcomes the upper limit on the key generation rate imposed by the dead time of detectors when using a heralded source of photons.

quant-ph↗

arXiv2004

Entangled Two-Photon Wave Packet in a Dispersive Medium

We report an experimental study of group-velocity dispersion effect on an entangled two-photon wavepacket, generated via spontaneous parametric down-conversion and propagating through a dispersive medium. Even in the case of using CW laser beam for pump, the biphoton wavepacket and the second-order correlation function spread significantly. The study and understanding of this phenomenon is of great importance for quantum information applications, such as quantum communication and distant clock synchronization.

quant-ph↗

arXiv2000

Simultaneous minimum-uncertainty measurement of discrete-valued complementary observables

We have made the first experimental demonstration of the simultaneous minimum uncertainty product between two complementary observables for a two-state system (a qubit). A partially entangled two-photon state was used to perform such measurements. Each of the photons carries (partial) information of the initial state thus leaving a room for measurements of two complementary observables on every member in an ensemble.

quant-ph↗

arXiv2000

Comprehensive experimental test of quantum erasure

In an interferometer, path information and interference visibility are incompatible quantities. Complete determination of the path will exclude any possibility of interference, rendering the visibility zero. However, if the composite object and probe state is pure, it is, under certain conditions, possible to trade the path information for improved (conditioned) visibility. Such a procedure is called quantum erasure. We have performed such experiments with polarization entangled photon pairs. Using a partial polarizer we could vary the degree of entanglement between object and probe. We could also vary the interferometer splitting ratio and thereby vary the a priori path predictability. We have tested quantum erasure under a number of different experimental conditions and found good agreement between experiments and theory.

quant-ph↗

arXiv2000

Unpolarized light in quantum optics

We present a new derivation of the unpolarized quantum states of light, whose general form was first derived by Prakash and Chandra [Phys. Rev. A 4, 796 (1971)]. Our derivation makes use of some basic group theory, is straightforward, and offers some new insights.

quant-ph↗

arXiv1999

Complementarity and the uncertainty relations

We formulate a general complementarity relation starting from any Hermitian operator with discrete non-degenerate eigenvalues. We then elucidate the relationship between quantum complementarity and the Heisenberg-Robertson's uncertainty relation. We show that they are intimately connected. Finally we exemplify the general theory with some specific suggested experiments.

quant-ph↗