arXiv subjects

Alexey Akimov

Publications and source records attributed to Alexey Akimov.

7 recordsLinked to original sources

arXiv2026

Tune-out wavelength for the thulium atom near 576 nm

We report the theoretical prediction and measurement of a tune-out wavelength for the ground state of the thulium atom in a linearly polarized optical dipole trap with a wavelength of approximately 576 nm. The measurements were conducted using a combination of trap frequency and RF loss spectroscopy, thus making it possible to separate the scalar and tensor parts of the total polarizability without measurements in the range of negative total polarizability. The calculated tune-out wavelength is consistent with the measured one of $575.646_{-0.014}^{+0.016}$ nm in air. The existence of the zero in the polarizability for the Tm ground state was confirmed by the trap loss experiment, which also made it possible to refine the tune-out wavelength to $575.646_{-0.004}^{+0.004}$. Despite the presence of an imaginary part of the polarizability at some wavelengths, it was experimentally demonstrated that, with a proper choice of the dipole trap polarization, it was possible to achieve Bose-Einstein condensation of thulium atoms in the range from 575.348 to 575.689 nm, covering the tune-out wavelength.

physics.atom-ph↗

arXiv2024

Transport of magnetically sensitive atoms in a magnetic environment

Among interesting applications of cold atoms, quantum simulations attract a lot of attention. In this context, rare-earth ultracold atoms are particularly appealing for such simulators due to their numerous Fano-Feshbach resonances and magnetic dipole moments in the ground state. Creating a quantum gas microscope requires a large optical access that may be achieved using transport of atoms between separate vacuum volumes. We demonstrate that in case of the transport of magnetic atoms the magnetic field can be directly measured and adjusted to reduce additional losses after the transport therefore increasing the efficiency of subsequent evaporation cooling. This approach allows to transfer over 85% of the atoms from the main chamber to the scientific chamber, located 38 cm away with moderate laser power of 26 W without atomic polarization decay.

cond-mat.quant-gas↗

arXiv2022

Control of NV center radiation in nanodiamonds by silicon nanoantennas

The development of nanophotonics systems for the manipulation of the luminescent properties of single quantum emitters is essential for quantum communication and computing. Dielectric nanosystems enable various opportunities for light control through inherent electric and magnetic resonances, however their full potential has not yet been discovered. Here, the emission properties of NV centers in nanodiamonds placed in the near-field zone of silicon nanoresonators are investigated. It is demonstrated experimentally that the spontaneous emission rate of single NV centers in 50 nm nanodiamonds can be modified by their coupling to spherical nanoantennas, reducing the mode of the lifetime distribution by approximately 2 times from 16 ns to 9 ns. It is also shown that the collected intensity of photoluminescence emission from the multiple NV centers in 150 nm nanodiamond coupled to a cylindrical nanoantenna is increased by more than 50% compared to the intensity from the same nanodiamond on a bare substrate

physics.optics↗

arXiv2021

Roadmap on Integrated Quantum Photonics

Integrated photonics is at the heart of many classical technologies, from optical communications to biosensors, LIDAR, and data center fiber interconnects. There is strong evidence that these integrated technologies will play a key role in quantum systems as they grow from few-qubit prototypes to tens of thousands of qubits. The underlying laser and optical quantum technologies, with the required functionality and performance, can only be realized through the integration of these components onto quantum photonic integrated circuits (QPICs) with accompanying electronics. In the last decade, remarkable advances in quantum photonic integration and a dramatic reduction in optical losses have enabled benchtop experiments to be scaled down to prototype chips with improvements in efficiency, robustness, and key performance metrics. The reduction in size, weight, power, and improvement in stability that will be enabled by QPICs will play a key role in increasing the degree of complexity and scale in quantum demonstrations. In the next decade, with sustained research, development, and investment in the quantum photonic ecosystem (i.e. PIC-based platforms, devices and circuits, fabrication and integration processes, packaging, and testing and benchmarking), we will witness the transition from single- and few-function prototypes to the large-scale integration of multi-functional and reconfigurable QPICs that will define how information is processed, stored, transmitted, and utilized for quantum computing, communications, metrology, and sensing. This roadmap highlights the current progress in the field of integrated quantum photonics, future challenges, and advances in science and technology needed to meet these challenges.

quant-ph↗

arXiv2020

Photoinduced Vibrations Drive Ultrafast Structural Distortion in Lead Halide Perovskite

Organic-inorganic perovskites have shown great promise towards their application in optoelectronics. The success of this class of material is dictated by the complex interplay between various underlying microscopic phenomena. The structural dynamics of organic cations and the inorganic sublattice after photoexcitation is hypothesized to have a direct effect on the material properties, thereby affecting the overall device performance. Here, we use two-dimensional (2D) electronic spectroscopy to reveal impulsively excited vibrational modes of methylammonium (MA) lead iodide perovskite, which drive the structural distortion after photoexcitation. The vibrational analysis of the measured data allows us to directly monitor the time evolution of the librational motion of the MA cation along with the vibrational coherences of inorganic sublattice. Wavelet analysis of the observed vibrational coherences uncovers the interplay between these two types of phonons. It reveals the coherent generation of the librational motion of the MA cation within ~300 fs, which is complemented by the coherent evolution of the skeletal motion of the inorganic sublattice. We have employed time-dependent density functional theory (TDDFT) to study the atomic motion of the MA cation and the inorganic sublattice during the process of photoexcitation. The TDDFT calculations support our experimental observations of the coherent generation of librational motions in the MA cation and highlight the importance of the anharmonic interaction between the MA cation and the inorganic sublattice. Our calculations predict the transfer of the photoinduced vibrational coherence from the MA cation to the inorganic sublattice, which drives the skeleton motion to form a polaronic state leading to long lifetimes of the charge carriers. This work may lead to novel design principles for next generation of solar cell materials.

physics.chem-ph↗

arXiv2020

Intense Dark Exciton Emission from Strongly Quantum Confined CsPbBr$_3$ Nanocrystals

Dark ground state exciton in semiconductor nanocrystals has been a subject of much interest due to its long lifetime attractive for applications requiring long-lived electronic or spin states. Significant effort has been made recently to explore and access the dark exciton level in metal halide perovskite nanocrystals, which are emerging as a superior source of photons and charges compared to other existing semiconductor nanocrystals. However, the direct observation of long-lived photoluminescence from dark exciton has remained elusive in metal halide perovskite nanocrystals. Here, we report the observation of the intense emission from dark ground state exciton with 1-10 us lifetime in strongly quantum confined CsPbBr3 nanocrystals, which contrasts the behavior of weakly confined system explored so far. The study in CsPbBr3 nanocrystals with varying degree of confinement has revealed the crucial role of quantum confinement in enhancing the bright-dark exciton level splitting which is important for accessing the dark exciton. Our work demonstrates the future potential of strongly quantum-confined perovskite nanocrystals as a new platform to utilize dark excitons.

physics.app-ph↗

arXiv2017

Electron spin contrast of Purcell-enhanced nitrogen-vacancy ensembles in nanodiamonds

Nitrogen-vacancy centers in diamond allow for coherent spin state manipulation at room temperature, which could bring dramatic advances to nanoscale sensing and quantum information technology. We introduce a novel method for the optical measurement of the spin contrast in dense nitrogen-vacancy (NV) ensembles. This method brings a new insight into the interplay between the spin contrast and fluorescence lifetime. We show that for improving the spin readout sensitivity in NV ensembles, one should aim at modifying the far field radiation pattern rather than enhancing the emission rate.

cond-mat.mes-hall↗