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Alexey Belyanin

Publications and source records attributed to Alexey Belyanin.

At least 55 records · Page 3Linked to original sources
arXiv2018

Watt-level widely tunable single-mode emission by injection-locking of a multimode Fabry-Perot quantum cascade laser

Free-running Fabry-Perot lasers normally operate in a single-mode regime until the pumping current is increased beyond the single-mode instability threshold, above which they evolve into a multimode state. As a result of this instability, the single-mode operation of these lasers is typically constrained to few percents of their output power range, this being an undesired limitation in spectroscopy applications. In order to expand the span of single-mode operation, we use an optical injection seed generated by an external-cavity single-mode laser source to force the Fabry-Perot quantum cascade laser into a single-mode state in the high current range, where it would otherwise operate in a multimode regime. Utilizing this approach we achieve single-mode emission at room temperature with a tuning range of $36 \, \mathrm{cm}^-1$ and stable continuous-wave output power exceeding 1 W. Far-field measurements show that a single transverse mode is emitted up to the highest optical power indicating that the beam properties of the seeded Fabry-Perot laser remain unchanged as compared to free-running operation.

physics.optics↗
arXiv2018

Enhancement of the spontaneous emission in subwavelength quasi-two-dimensional waveguides and resonators

We consider a quantum-electrodynamic problem of the spontaneous emission from a two-dimensional (2D) emitter, such as a quantum well or a 2D semiconductor, placed in a quasi-2D waveguide or cavity with subwavelength confinement in one direction. We apply the Heisenberg-Langevin approach which includes dissipation and fluctuations in the electron ensemble and in the electromagnetic field of a cavity on equal footing. The Langevin noise operators that we introduce do not depend on any particular model of dissipative reservoir and can be applied to any dissipation mechanism. Moreover, our approach is applicable to nonequilibrium electron systems, e.g. in the presence of pumping, beyond the applicability of the standard fluctuation-dissipation theorem. We derive analytic results for simple but practically important geometries: strip lines and rectangular cavities. Our results show that a significant enhancement of the spontaneous emission, by a factor of order 100 or higher, is possible for quantum wells and other 2D emitters in a subwavelength cavity.

quant-ph↗
arXiv2017

Enhanced third-order optical nonlinearity driven by surface-plasmon field gradients

Achieving efficient nonlinear optical frequency conversion in small volumes is key for future on-chip photonic devices that would provide a higher-speed alternative to modern electronics. However, the already intrinsically low conversion efficiency severely limits miniaturization to nanoscale dimensions. Here we demonstrate that gradient-field effects can provide for an efficient, conventionally dipole-forbidden nonlinear response, offering a new approach for enhanced nonlinear optics in nanostructures. We show that a {\em longitudinal} nonlinear source current can dominate the third-order optical nonlinearity of the free electron response in gold in the technologically important near-IR frequency range where the nonlinearities due to other mechanisms are particularly small. Using adiabatic nanofocusing to spatially confine the excitation fields, from measurements of the $2ω_1 - ω_2$ four-wave mixing response as a function of detuning $ω_1 - ω_2$, we find up to $10^{-5}$ conversion efficiency with a gradient field contribution to $χ^{(3)}_{\mathrm{Au}}$ of up to $10^{-19}~\mathrm{m}^2 / \mathrm{V}^2$. The results are in good agreement with theory based on plasma hydrodynamics. Our results demonstrate an increase in nonlinear conversion efficiency with decreasing sample size that can offset and even overcompensate the volume decrease of conventional dipolar pathways. This will enable more efficient nonlinear optical devices and frequency converters and facilitate the extension of coherent multidimensional spectroscopies to the nanoscale.

cond-mat.mes-hall↗
arXiv2017

Observation of Diode Behavior and Gate Voltage Control of Hybrid Plasmon-Phonon Polaritons in Graphene-Hexagonal Boron Nitride Heterostructures

Light-matter interaction in two-dimension photonic materials allows for confinement and control of free-space radiation on sub-wavelength scales. Most notably, the van der Waals heterostructure obtained by stacking graphene (G) and hexagonal Boron Nitride (hBN) can provide for hybrid hyperbolic plasmon phonon-polaritons (HP3). Here, we present a polariton diode effect and low-bias control of HP3 modes confined in G-hBN. Using broadband infrared synchrotron radiation coupled to a scattering-type near-field optical microscope, we launch HP3 waves over both hBN Reststrahlen bands and observe the unidirectional propagation of HP3 modes at in-plane heterointerfaces associated with the transition between different substrate dielectrics. By electric gating we further control the HP3 hybridization modifying the coupling between the continuum graphene plasmons and the discrete hyperbolic phonon polaritons of hBN as described by an extended Fano model. This is the first demonstration of unidirectional control of polariton propagation, with break in reflection/transmission symmetry for HP3 modes. G-hBN and related hyperbolic metamaterial nanostructures can therefore provide the basis for novel logic devices of on-chip nano-optics communication and computing.

cond-mat.mes-hall↗
arXiv2017

Single-mode instability in standing-wave lasers: The quantum cascade laser as a self-pumped parametric oscillator

We report the observation of a clear single-mode instability threshold in continuous-wave Fabry-Perot quantum cascade lasers (QCLs). The instability is characterized by the appearance of sidebands separated by tens of free spectral ranges (FSR) from the first lasing mode, at a pump current not much higher than the lasing threshold. As the current is increased, higher-order sidebands appear that preserve the initial spacing, and the spectra are suggestive of harmonically phase-locked waveforms. We present a theory of the instability that applies to all homogeneously broadened standing-wave lasers. The low instability threshold and the large sideband spacing can be explained by the combination of an unclamped, incoherent Lorentzian gain due to the population grating, and a coherent parametric gain caused by temporal population pulsations that changes the spectral gain line shape. The parametric term suppresses the gain of sidebands whose separation is much smaller than the reciprocal gain recovery time, while enhancing the gain of more distant sidebands. The large gain recovery frequency of the QCL compared to the FSR is essential to observe this parametric effect, which is responsible for the multiple-FSR sideband separation. We predict that by tuning the strength of the incoherent gain contribution, for example by engineering the modal overlap factors and the carrier diffusion, both amplitude-modulated (AM) or frequency-modulated emission can be achieved from QCLs. We provide initial evidence of an AM waveform emitted by a QCL with highly asymmetric facet reflectivities, thereby opening a promising route to ultrashort pulse generation in the mid-infrared. Together, the experiments and theory clarify a deep connection between parametric oscillation in optically pumped microresonators and the single-mode instability of lasers, tying together literature from the last 60 years.

physics.optics↗
arXiv2017

Self-starting harmonic frequency comb generation in a quantum cascade laser

Optical frequency combs establish a rigid phase-coherent link between microwave and optical domains and are emerging as high-precision tools in an increasing number of applications. Frequency combs with large intermodal spacing are employed in the field of microwave photonics for radiofrequency arbitrary waveform synthesis and for generation of THz tones of high spectral purity in the future wireless communication networks. We demonstrate for the first time self-starting harmonic frequency comb generation with a THz repetition rate in a quantum cascade laser. The large intermodal spacing caused by the suppression of tens of adjacent cavity modes originates from a parametric contribution to the gain due to temporal modulations of the population inversion in the laser. The mode spacing of the harmonic comb is shown to be uniform to within $5\times 10^{-12}$ parts of the central frequency using multiheterodyne self-detection. This new harmonic comb state extends the range of applications of quantum cascade laser frequency combs.

physics.optics↗
arXiv2017

Magneto-polaritons in Weyl semimetals in a strong magnetic field

Exotic topological and transport properties of Weyl semimetals generated a lot of excitement in the condensed matter community. Here we show that Weyl semimetals in a strong magnetic field are highly unusual optical materials. The propagation of electromagnetic waves is affected by an interplay between plasmonic response of chiral Weyl fermions and extreme anisotropy induced by a magnetic field. The resulting magneto-polaritons possess a number of peculiar properties, such as hyperbolic dispersion, photonic stop bands, coupling-induced transparency, and broadband polarization conversion. These effects can be used for optical spectroscopy of these materials including detection of the chiral anomaly, or for broadband terahertz/infrared applications.

cond-mat.mes-hall↗
arXiv2016

Stability of High-Density Two-Dimensional Excitons against a Mott Transition in High Magnetic Fields Probed by Coherent Terahertz Spectroscopy

We have performed time-resolved terahertz absorption measurements on photoexcited electron-hole pairs in undoped GaAs quantum wells in magnetic fields. We probed both unbound- and bound-carrier responses via cyclotron resonance and intraexciton resonance, respectively. The stability of excitons, monitored as the pair density was systematically increased, was found to dramatically increase with increasing magnetic field. Specifically, the 1$s$-2$p_-$ intraexciton transition at 9 T persisted up to the highest density, whereas the 1$s$-2$p$ feature at 0 T was quickly replaced by a free-carrier Drude response. Interestingly, at 9 T, the 1$s$-2$p_-$ peak was replaced by free-hole cyclotron resonance at high temperatures, indicating that 2D magnetoexcitons do dissociate under thermal excitation, even though they are stable against a density-driven Mott transition.

cond-mat.quant-gas↗
arXiv2016

Second-order nonlinear optical response of graphene

Although massless Dirac fermions in graphene constitute a centrosymmetric medium for in-plane excitations, their second-order nonlinear optical response is nonzero if the effects of spatial dispersion are taken into account. Here we present a rigorous quantum-mechanical theory of the second-order nonlinear response of graphene beyond the electric dipole approximation, which includes both intraband and interband transitions. The resulting nonlinear susceptibility tensor satisfies all symmetry and permutation properties, and can be applied to all three-wave mixing processes. We obtain useful analytic expressions in the limit of a degenerate electron distribution, which reveal quite strong second-order nonlinearity at long wavelengths, Fermi-edge resonances, and unusual polarization properties.

cond-mat.mes-hall↗
arXiv2016

Dicke Superradiance in Solids

Recent advances in optical studies of condensed matter have led to the emergence of phenomena that have conventionally been studied in the realm of quantum optics. These studies have not only deepened our understanding of light-matter interactions but also introduced aspects of many-body correlations inherent in optical processes in condensed matter systems. This article is concerned with superradiance (SR), a profound quantum optical process predicted by Dicke in 1954. The basic concept of SR applies to a general $N$-body system where constituent oscillating dipoles couple together through interaction with a common light field and accelerate the radiative decay of the system. In the most fascinating manifestation of SR, known as superfluorescence (SF), an incoherently prepared system of $N$ inverted atoms spontaneously develops macroscopic coherence from vacuum fluctuations and produces a delayed pulse of coherent light whose peak intensity $\propto N^2$. Such SF pulses have been observed in atomic and molecular gases, and their intriguing quantum nature has been unambiguously demonstrated. Here, we focus on the rapidly developing field of research on SR in solids, where not only photon-mediated coupling but also strong Coulomb interactions and ultrafast scattering exist. We describe SR and SF in molecular centers in solids, molecular aggregates and crystals, quantum dots, and quantum wells. In particular, we will summarize a series of studies we have recently performed on quantum wells in strong magnetic fields. These studies show that cooperative effects in solid-state systems are not merely small corrections that require exotic conditions to be observed; rather, they can dominate the nonequilibrium dynamics and light emission processes of the entire system of interacting electrons.

cond-mat.quant-gas↗
arXiv2016

Laser-driven parametric instability and generation of entangled photon-plasmon states in graphene and topological insulators

We show that a strong infrared laser beam obliquely incident on graphene can experience a parametric instability with respect to decay into lower-frequency (idler) photons and THz surface plasmons. The instability is due to a strong in-plane second-order nonlinear response of graphene which originates from its spatial dispersion. The parametric decay leads to efficient generation of THz plasmons and gives rise to quantum entanglement of idler photons and surface plasmon states. A similar process can be supported by surface states of topological insulators such as Bi$_2$Se$_3$.

quant-ph↗
arXiv2015

Valley entanglement of excitons in monolayers of transition-metal dichalcogenides

We show that excitons and free carriers in K and K' valleys of transition metal dichalcogenide monolayers can be entangled with respect to their valley degree of freedom by absorbing linearly polarized single photons. This effect does not require any interaction between K and K' excitons in contrast to conventional mechanisms of entanglement that are mediated by coupling between quantum systems (e.g.~entanglement of photons in nonlinear optical interactions). The valley entanglement of excitons and free carriers can be verified by measuring the polarization of their photoluminescence or fluctuations of the photocurrent under an applied in-plane DC bias.

cond-mat.mes-hall↗
arXiv2015

Continuous wave lasing between Landau levels in graphene

We predict the general feasibility and demonstrate the specific design of the THz laser operating between Landau levels in graphene placed on a polar substrate in a magnetic field of order 1 T. Steady state operation under a continuous wave optical pumping is possible due to an interplay between Auger and surface-phonon mediated relaxation of carriers. The scheme is scalable to other materials with massless Dirac fermions, for example surface states in 3D topological insulators such as Bi$_2$Se$_3$ or Bi$_2$Te$_3$.

cond-mat.mes-hall↗
arXiv2014

Superradiant Decay of Cyclotron Resonance of Two-Dimensional Electron Gases

We report on the observation of collective radiative decay, or superradiance, of cyclotron resonance (CR) in high-mobility two-dimensional electron gases in GaAs quantum wells using time-domain terahertz magnetospectroscopy. The decay rate of coherent CR oscillations increases linearly with the electron density in a wide range, which is a hallmark of superradiant damping. Our fully quantum mechanical theory provides a universal formula for the decay rate, which reproduces our experimental data without any adjustable parameter. These results firmly establish the many-body nature of CR decoherence in this system, despite the fact that the CR frequency is immune to electron-electron interactions due to Kohn's theorem.

cond-mat.mes-hall↗
arXiv2013

Efficient nonlinear generation of THz plasmons in graphene and topological insulators

Surface plasmons in graphene may provide an attractive alternative to noble-metal plasmons due to their tighter confinement, peculiar dispersion, and longer propagation distance. We present theoretical studies of the nonlinear difference frequency generation of terahertz surface plasmon modes supported by two-dimensional layers of massless Dirac electrons, which includes graphene and surface states in topological insulators. Our results demonstrate strong enhancement of the DFG efficiency near the plasmon resonance and the feasibility of phase-matched nonlinear generation of plasmons over a broad range of frequencies.

cond-mat.mes-hall↗
arXiv2012

Generation of entangled photons in graphene in a strong magnetic field

Entangled photon states attract tremendous interest as the most vivid manifestation of nonlocality of quantum mechanics and also for emerging applications in quantum information. Here we propose a mechanism of generation of polarization-entangled photons, which is based on the nonlinear optical interaction (four-wave mixing) in graphene placed in a magnetic field. Unique properties of quantized electron states in a magnetized graphene and optical selection rules near the Dirac point give rise to a giant optical nonlinearity and a high rate of photon production in the mid/far-infrared range.

cond-mat.mes-hall↗
arXiv2012

Nonlinear optics of graphene in a strong magnetic field

Graphene placed in a magnetic field possesses an extremely high mid/far-infrared optical nonlinearity originating from its unusual band structure and selection rules for the optical transitions near the Dirac point. Here we study the linear and nonlinear optical response of graphene in strong magnetic and optical fields using quantum- mechanical density-matrix formalism. We calculate the power of coherent terahertz radiation generated as a result of four-wave mixing in graphene. We show that even one monolayer of graphene gives rise to appreciable nonlinear frequency conversion efficiency and Raman gain for modest intensities of incident infrared radiation.

cond-mat.mes-hall↗