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Alexey V. Kavokin

Publications and source records attributed to Alexey V. Kavokin.

At least 19 recordsLinked to original sources

Quantized topological transport mediated by the long-range couplings

Certain topological systems with time-varying Hamiltonian enable quantized and disorder-robust transport of excitations. Here, we introduce the modification of the celebrated Thouless pump when the on-site energies remain fixed, while the nearest and next-nearest neighbor couplings vary in time. We demonstrate quantized transport of excitations and propose an experimental implementation using an array of evanescently coupled optical waveguides.

physics.optics↗

Semiconductor-Semimetal Transition in van der Waals Carbyne Crystals

Freestanding van der Waals crystals made of single-atom carbon chains (carbynes) have been recently realized technologically. Here we investigate their electronic and optical properties experimentally, by continuous-wave and time-resolved photoluminescence spectroscopy, and theoretically. Employing a fully three-dimensional tight-binding formalism benchmarked against density functional theory calculations we predict the semimetal-semiconductor transition to occur in van der Waals carbyne crystals composed by the chains of about 42 atoms long. The semiconductor phase is characterized by a hyperbolic van Hove singularity which gives rise to unconventional hyperbolic exciton states. Experimentally, we access the semiconductor phase, where resonant features associated with hyperbolic excitons are clearly visible. The exciton oscillator strength is found to be strongly sensitive to the length of carbon chains: our experiments show that it decreases with the increasing chain length. This tendency, confirmed by the theoretical modeling, manifests the evolution of the hyperbolic exciton state on the way to the semiconductor-semimetal crossover. Our approach accounts for the actual crystalline geometry, including alternating intra-chain hoppings and inter-chain couplings. By fitting tight-binding dispersions to density functional theory data we extract consistent parameters and establish a comprehensive framework for the physics of carbyne crystals. This study paves the way towards efficient band-gap engineering in ultimate one-dimensional carbon crystals.

cond-mat.mes-hall↗

Spatial coherence of room-temperature monolayer WSe$_2$ exciton-polaritons in a trap

The emergence of spatial and temporal coherence of light emitted from solid-state systems is a fundamental phenomenon, rooting in a plethora of microscopic processes. It is intrinsically aligned with the control of light-matter coupling, and canonical for laser oscillation. However, it also emerges in the superradiance of multiple, phase-locked emitters, and more recently, coherence and long-range order have been investigated in bosonic condensates of thermalized light, as well as in exciton-polaritons driven to a ground state via stimulated scattering. Here, we experimentally show that the interaction between photons in a Fabry-Perot microcavity and excitons in an atomically thin WSe$_2$ layer is sufficient such that the system enters the hybridized regime of strong light-matter coupling at ambient conditions. Via Michelson interferometry, we capture clear evidence of increased spatial and temporal coherence of the emitted light from the spatially confined system ground-state. The coherence build-up is accompanied by a threshold-like behaviour of the emitted light intensity, which is a fingerprint of a polariton laser effect. Valley-physics is manifested in the presence of an external magnetic field, which allows us to manipulate K and K' polaritons via the Valley-Zeeman-effect. Our findings are of high application relevance, as they confirm the possibility to use atomically thin crystals as simple and versatile components of coherent light-sources, and in valleytronic applications at room temperature.

cond-mat.mes-hall↗

Bosonic condensation of exciton-polaritons in an atomically thin crystal

The emergence of two-dimensional crystals has revolutionized modern solid-state physics. From a fundamental point of view, the enhancement of charge carrier correlations has sparked enormous research activities in the transport- and quantum optics communities. One of the most intriguing effects, in this regard, is the bosonic condensation and spontaneous coherence of many-particle complexes. Here, we find compelling evidence of bosonic condensation of exciton-polaritons emerging from an atomically thin crystal of MoSe2 embedded in a dielectric microcavity under optical pumping. The formation of the condensate manifests itself in a sudden increase of luminescence intensity in a threshold-like manner, and a significant spin-polarizability in an externally applied magnetic field. Spatial coherence is mapped out via highly resolved real-space interferometry, revealing a spatially extended condensate. Our device represents a decisive step towards the implementation of coherent light-sources based on atomically thin crystals, as well as non-linear, valleytronic coherent devices.

cond-mat.mes-hall↗

Pseudo-drag of a polariton superfluid

The drag of half-light half-mater quasiparticles, exciton-polaritons, by an electric current is a peculiar mechanism of light-matter interaction in solids. While an ideal superfluid is protected from being dragged by its zero viscosity, here we argue that the state of the superfluid polariton condensate formed by a non-resonant optical pumping can be controlled by the electric current. The proposed mechanism is based on the stimulated relaxation of moving uncondensed excitons dragged by the electric current. The stimulated relaxation process favors the formation of a moving condensate in a quantum state that is characterised by the lowest condensation threshold. We also show that the electron-mediated inelastic scattering of the reservoir excitons to the condensate leads to the transfer of a non-zero mean momentum to the electron gas thus contributing to the electric current. We predict the generation of circular electric currents in a micropillar cavity in the presence of a nonresonant laser pumping at normal incidence.

cond-mat.mes-hall↗

Optical valley Hall effect for highly valley-coherent exciton-polaritons in an atomically thin semiconductor

Spin-orbit coupling is a fundamental mechanism that connects the spin of a charge carrier with its momentum. Likewise, in the optical domain, a synthetic spin-orbit coupling is accessible, for instance, by engineering optical anisotropies in photonic materials. Both, akin, yield the possibility to create devices directly harnessing spin- and polarization as information carriers. Atomically thin layers of transition metal dichalcogenides provide a new material platform which promises intrinsic spin-valley Hall features both for free carriers, two-particle excitations (excitons), as well as for photons. In such materials, the spin of an exciton is closely linked to the high-symmetry point in reciprocal space it emerges from. Here, we demonstrate, that spin, and hence valley selective propagation is accessible in an atomically thin layer of MoSe2, which is strongly coupled to a microcavity photon mode. We engineer a wire-like device, where we can clearly trace the flow, and the helicity of exciton-polaritons expanding along a channel. By exciting a coherent superposition of K and K- tagged polaritons, we observe valley selective expansion of the polariton cloud without neither any applied external magnetic fields nor coherent Rayleigh scattering. Unlike the valley Hall effect for TMDC excitons, the observed optical valley Hall effect (OVHE) strikingly occurs on a macroscopic scale, and clearly reveals the potential for applications in spin-valley locked photonic devices.

cond-mat.mes-hall↗

Observation of bosonic condensation in a hybrid monolayer MoSe2-GaAs microcavity

Condensation of bosons into a macroscopic quantum state belongs to the most intriguing phenomena in nature. It was first realized in quantum gases of ultra-cold atoms, but more recently became accessible in open-dissipative, exciton-based solid-state systems at elevated temperatures. Semiconducting monolayer crystals have emerged as a new platform for studies of strongly bound excitons in ultimately thin materials. Here, we demonstrate the formation of a bosonic condensate driven by excitons hosted in an atomically thin layer of MoSe2, strongly coupled to light in a solid-state resonator. The structure is operated in the regime of collective strong coupling, giving rise to hybrid exciton-polariton modes composed of a Tamm-plasmon resonance, GaAs quantum well excitons and two-dimensional excitons confined in a monolayer of MoSe2. Polariton condensation in a monolayer crystal manifests by a superlinear increase of emission intensity from the hybrid polariton mode at injection powers as low as 4.8 pJ/pulse, as well as its density-dependent blueshift and a dramatic collapse of the emission linewidth as a hallmark of temporal coherence. Importantly, we observe a significant spin-polarization in the injected polariton condensate, a fingerprint of the core property of monolayer excitons subject to spin-valley locking. The observed effects clearly underpin the perspective of building novel highly non-linear valleytronic devices based on light-matter fluids, coherent bosonic light sources based on atomically thin materials, and paves the way towards studying materials with unconventional topological properties in the framework of bosonic condensation.

cond-mat.quant-gas↗

The interplay of phonon and exciton-mediated superconductivity in hybrid semiconductor-superconductor structures

We predict a strong enhancement of the critical temperature in a conventional Bardeen-Cooper-Schrieffer (BCS) superconductor in the presence of a bosonic condensate of exciton-polaritons. The effect depends strongly on the ratio of the cutoff frequencies for phonon and exciton-polariton mediated BCS superconductivity, respectively. We also discuss a possible design of hybrid semiconductor-superconductor structures suitable for the experimental observation of such an effect.

cond-mat.supr-con↗

Room temperature Tamm-Plasmon Exciton-Polaritons with a WSe2 monolayer

Solid state cavity quantum electrodynamics is a rapidly advancing field which explores the frontiers of light-matter coupling. Plasmonic approaches are of particular interest in this field, since they carry the potential to squeeze optical modes to spaces significantly below the diffraction limit1,2, enhancing light-matter coupling. They further serve as an architecture to design ultra-fast, non-linear integrated circuits with smallest footprints3. Transition metal dichalcogenides are ideally suited as the active material in such circuits as they interact strongly with light at the ultimate monolayer limit4. Here, we implement a Tamm-plasmon-polariton structure, and study the coupling to a monolayer of WSe2, hosting highly stable excitons5. Exciton-Polariton formation at room temperature is manifested in the characteristic energy-momentum dispersion relation studied in photoluminescence, featuring an anti-crossing between the exciton and photon modes with a Rabi-splitting of 23.5 meV. Creating polaritonic quasi-particles in plasmonic architectures with atomic monolayers under ambient conditions is a crucial step towards compact, highly non-linear integrated photonic and polaritonic circuits6,7.

cond-mat.mes-hall↗

Magnetization Currents of Fluctuative Cooper Pairs

Recent experiments show that the Nernst-Ettingshausen effect is orders of magnitude stronger than the thermoelectric Seebeck effect in superconductors above the critical temperature. We explain different magnitudes of the two effects accounting for the magnetization current of virtual Cooper pairs. The method allows for detailed understanding of the surprising non-monotonic dependence of the Nernst-Ettingshausen coefficient on the magnetic field.

cond-mat.supr-con↗

Enhanced thermoelectric coupling near electronic phase transition: the role of fluctuation Cooper pairs

Thermoelectric energy conversion is a direct but low-efficiency process, which precludes the development of long-awaited wide-scale applications. As a breakthrough permitting a drastic performance increase is seemingly out of reach, we fully reconsider the problem of thermoelectric coupling enhancement. The corner stone of our approach is the observation that heat engines are particularly efficient when their operation involves a phase transition of their working fluid. We derive and compute the thermoelastic coefficients of various systems, including Bose and Fermi gases, and fluctuation Cooper pairs. Combination of these coefficients yields the definition of the thermodynamic figure of merit, the divergence of which at $finite$ temperature indicates that conditions are fulfilled for the best possible use of the thermoelectric working fluid. Here, this situation occurs in the fluctuation regime only, as a consequence of the increased compressibility of the working fluid near its phase transition. Our results and analysis clearly show that efforts in the field of thermoelectricity can now be productively directed towards systems where electronic phase transitions are possible.

cond-mat.other↗

Crossover from exciton-polariton to photon Bose-Einstein condensation

BEC of exciton-polaritons and related effects such as superfluidity1,2, spontaneous symmetry breaking3,4 and quantised vortices5,6 open way to creation of novel light sources7 and optical logic elements8. Remarkable observations of exciton-polariton BEC in microcavities9-12 have been reported in the recent ten years. Very recently, thermalisation and subsequent condensation of cavity photons in a dye-filled microcavity have been observed13. Here we show that BEC of both exciton-polaritons and photons can be created in the same system under different optical excitation conditions. A dynamic phase transition between a photon and a polariton BEC takes place after a single high-power excitation pulse and we find both condensed states in thermal equilibrium with the excited states. At the crossover, photons and polaritons coexist, which results in a decrease in the long-range spatial coherence. Build-up and successive depinning of polarisation is observed at the threshold of both polariton and photon condensation.

cond-mat.quant-gas↗

Spontaneous symmetry breaking in a polariton and photon laser

We report on the simultaneous observation of spontaneous symmetry breaking and long-range spatial coherence both in the strong and the weak-coupling regime in a semiconductor microcavity. Under pulsed excitation, the formation of a stochastic order parameter is observed in polariton and photon lasing regimes. Single-shot measurements of the Stokes vector of the emission exhibit the buildup of stochastic polarization. Below threshold, the polarization noise does not exceed 10%, while above threshold we observe a total polarization of up to 50% after each excitation pulse, while the polarization averaged over the ensemble of pulses remains nearly zero. In both polariton and photon lasing regimes, the stochastic polarization buildup is accompanied by the buildup of spatial coherence. We find that the Landau criterion of spontaneous symmetry breaking and Penrose-Onsager criterion of long-range order for Bose-Einstein condensation are met in both polariton and photon lasing regimes.

cond-mat.mes-hall↗

The Non-linear Optical Spin Hall Effect and Long-Range Spin Transport in Polariton Lasers

We report on the experimental observation of the non-linear analogue of the optical spin Hall effect under highly non-resonant circularly polarized excitation of an exciton polariton condensate in a GaAs/AlGaAs microcavity. Initially circularly polarized polariton condensates propagate over macroscopic distances while the collective condensate spins coherently precess around an effective magnetic field in the sample plane performing up to four complete revolutions.

cond-mat.mes-hall↗

Exciton supersolidity in hybrid Bose-Fermi systems

We investigate the ground states of a Bose-Einstein condensate of indirect excitons coupled to an electron gas. We show that in a properly designed system, the crossing of a roton minimum into the negative energy domain can result in the appearance of the supersolid phase, characterized by periodicity in both real and reciprocal space. Accounting for the spin-dependent exchange interaction of excitons we obtain ferromagnetic supersolid domains. The Fourier spectra of excitations of weakly perturbed supersolids show pronounced diffraction maxima which may be detected experimentally.

cond-mat.mes-hall↗

Spontaneous Coherence in a Cold Exciton Gas

Excitons, bound pairs of electrons and holes, form a model system to explore the quantum physics of cold bosons in solids. Cold exciton gases can be realized in a system of indirect excitons, which can cool down below the temperature of quantum degeneracy due to their long lifetimes. Here, we report on the measurement of spontaneous coherence in a gas of indirect excitons. We found that extended spontaneous coherence of excitons emerges in the region of the macroscopically ordered exciton state and in the region of vortices of linear polarization. The coherence length in these regions is much larger than in a classical gas, indicating a coherent state with a much narrower than classical exciton distribution in momentum space, characteristic of a condensate. We also observed phase singularities in the coherent exciton gas. Extended spontaneous coherence and phase singularities emerge when the exciton gas is cooled below a few Kelvin.

cond-mat.mes-hall↗

Giant Nernst-Ettingshausen oscillations in Semiclassically strong magnetic fields

We consider the Nernst-Ettingshausen (NE) effect in the presence of semiclassically strong magnetic fields for a quasi-two dimensional system with a parabolic or linear dispersion of carriers. We show that the occurring giant oscillations of the NE coefficient are coherent with the recent experimental observation in graphene, graphite and bismuth. In the 2D case we find the exact shape of these oscillations and show that their magnitude decreases/increases with enhancement of the Fermi energy for Dirac fermions/normal carriers. With a crossover to 3D spectrum the phase of oscillations shifts, their amplitude decreases and the peaks become asymmetric.

cond-mat.mes-hall↗

Spontaneous formation and optical manipulation of extended polariton condensates

Cavity exciton-polaritons (polaritons) are bosonic quasi-particles offering a unique solid-state system to investigate interacting condensates. Up to now, disorder induced localization and short lifetimes have prevented the establishment of long range off diagonal order needed for any quantum manipulation of the condensate wavefunction. In this work, using a wire microcavity with polariton lifetimes ten times longer than in all previously existing samples, we show that polariton condensates can propagate over macroscopic distances outside the excitation area, while preserving their spontaneous spatial coherence. An extended condensate wave-function builds-up with a degree of spatial coherence larger than 50% over distances 50 times the polariton De Broglie wavelength. The expansion of the condensate is shown to be governed by the repulsive potential induced by photo-generated excitons within the excitation area. The control of this local potential offers a new and versatile method to manipulate extended polariton condensates. As an illustration, we demonstrate synchronization of extended condensates via controlled tunnel coupling and localization of condensates in a trap with optically controlled dimensions.

cond-mat.other↗