arXiv subjects

Alexey Y. Nikitin

Publications and source records attributed to Alexey Y. Nikitin.

At least 19 recordsLinked to original sources

arXiv2026

Wave Vortices Around Oscillating Subwavelength Holes: Water-Wave Observation

We consider a two-dimensional wave system containing a subwavelength hole, such as an aperture in an interface supporting surface electromagnetic or acoustic waves, or an island in a fluid surface sustaining gravity-capillary waves. Recent studies have revealed the emergence of pronounced wave vortices around such structures, termed type-II vortices, in contrast to conventional (type-I) vortices associated with phase singularities and intensity nulls. A striking natural manifestation of type-II vortices occurs in ocean tides around islands such as New Zealand, Madagascar, and Iceland, where the tidal phase increases by $\pm 2π$ around the island. Although this phenomenon is usually associated with the Coriolis effect from the rotation of the Earth, here we demonstrate the controlled generation of type-II vortices using a minimal and tunable setup: a dipole-oscillating subwavelength hole and a single incident plane wave. Using laboratory gravity-capillary waves and an oscillating subwavelength `island', we directly measure the resulting phase structure, topological charge, and wave angular momentum. We show that the emergence and handedness of the vortices can be precisely controlled via the relative phase between the dipolar source and the incident wave. Our results offer a simple and versatile mechanism for engineering subwavelength wave vortices, with potential applications in a variety of two-dimensional wave systems.

physics.flu-dyn↗

arXiv2026

Twistoptics in Planar Heterostructures with an Arbitrary Number of Rotated 3D Thin Layers and 2D Conductive Sheets

Twistoptics has recently emerged as a branch of nano-optics that explores light propagation in stacks of thin anisotropic layers rotated relative to one another. The concept is particularly relevant for polaritons -- hybrid light-matter quasiparticles -- in van der Waals (vdW) materials, where strong in-plane anisotropy and deep subwavelength confinement make the polaritonic dispersion highly sensitive to interlayer twist angles. This sensitivity enables exotic phenomena such as canalization, i.e., diffraction-free propagation, with potential applications ranging from thermal management to super-resolution imaging. Despite rapid progress, a general analytical framework to describe polariton propagation in twisted planar heterostructures has been missing. Here we present an analytical model for planar stacks comprising an arbitrary number of finite-thickness anisotropic (biaxial) layers and infinitesimally thin anisotropic conductive sheets. The formalism and its high-momentum and thin-film approximations predict key polaritonic observables, such as wavelength, propagation length, and electromagnetic field distributions. We also provide open-access numerical scripts implementing the model to support their practical use. Together, these results provide a general theoretical foundation for twistoptics and should facilitate the discovery and accelerate the implementation of twist-engineered polaritonic phenomena across the electromagnetic spectrum.

physics.optics↗

arXiv2026

Launching of Visible-Range Hyperbolic Polaritons by Gold Nanoantennas in a natural van der Waals crystal

Anisotropic van der Waals materials provide a powerful platform for nanoscale optoelectronics, enabling strong light$-$matter interaction and deep electromagnetic field confinement mediated by polaritons, hybrid light$-$matter excitations with unique dispersion properties. While polaritonic phenomena in van der Waals heterostructures have been extensively explored in the mid-infrared frequency range, their behaviour at the visible frequencies remains largely unexplored, in part due to the lack of knowledge on natural materials supporting anisotropic and highly confined visible-range polaritons. In this context, MoOCl$_2$, an anisotropic van der Waals metal, is particularly interesting, since it supports hyperbolic plasmon polaritons (PPs) that enable directional propagation and subwavelength light compression. Here, we investigate the strategy for launching anisotropic PPs in MoOCl$_2$ in the visible frequency range using gold rod nanoantennas. The nanoantennas, placed on top of the MoOCl$_2$ crystal, excite in-plane anisotropic PP modes, effectively overcoming the momentum mismatch between waves in free-space and nanoscale PPs. We demonstrate a strong electromagnetic field confinement, angle-dependent absorption, and controlled anisotropic PP launching enabled by gold nanoantennas, highlighting the potential of MoOCl$_2$ as a compact platform for nanoscale waveguiding and optical signal processing. By providing a practical antenna-based strategy for exciting visible-range PPs, this work addresses the lack of compact elements for optical signal manipulation and opens new opportunities for optoelectronic devices based on van der Waals polaritonics.

physics.optics↗

arXiv2026

MoOCl$_2$ as a Hyperbolic Planar Platform for Nanooptics at Telecom Frequencies

On-chip optoelectronics is fundamental to modern telecommunication, yet the diffraction limit of light remains a major obstacle to the extreme miniaturization of photonic integrated circuits (PICs). Hyperbolic polaritons (HPs) $-$ hybrid light-matter excitations in materials with opposite-signed dielectric permittivity tensor components $-$ offer a solution through their ability to support deep sub-wavelength confinement and unique optical phenomena such as canalization and negative refraction. To date, however, the most widely studied hyperbolic van der Waals (vdW) crystals, including hBN and $α$-MoO$_3$, operate mainly in the mid-infrared, leaving the telecommunication bands (1260$-$1675 nm) largely uncovered. Here, we predict HPs operating directly in the telecommunication window in the vdW crystal molybdenum oxychloride (MoOCl$_2$). Building on recent evidence that MoOCl$_2$ can support plasmon polaritons in the visible, we theoretically investigate its optical response at telecom wavelengths and identify the conditions under which strongly confined, canalized HPs modes emerge. Beyond establishing a telecom platform, we outline device-level opportunities enabled by these modes, including diffraction-free waveguides based on canalization, tunable polaritonic crystals, and high-efficiency spontaneous emission-enhancement platforms. These paradigms cover the essential pillars of on-chip information processing: emission, propagation, modulation and detection. Our results establish MoOCl$_2$ as a potentially transformative material that bridges physics of hyperbolic PPs with potential practical implementations, opening avenues for ultra-compact, high-density, and low-power photonic components.

physics.optics↗

arXiv2026

Size-dependent Dielectric Permittivity of Perovskite Nanocrystals

Perovskite nanocrystals (PNCs) are promising building blocks for quantum photonic devices. Optical properties of PNCs can be enhanced by integration with optical cavities or nanoantennas. Designing such structures requires accurate size dependent dielectric permittivity of PNCs. However, current reports provide primarily ensemble averaged values with limited access to the intrinsic response of individual PNCs. Here we suggest a methodology to reconstruct the size dependent complex dielectric permittivity of CsPbBr3 PNCs from the measured absorbance spectrum of colloidal solution. The permittivity of PNCs is modeled as a sum of Voigt profile oscillators, with the size dependent transition energies governed by the exciton effective mass. Using a transmission electron microscopy derived size distribution of the PNCs, the solution permittivity is obtained via Maxwell Garnett effective medium approximation. This permittivity is used in a transfer matrix method to simulate and fit the absorbance spectrum, from which the permittivity of PNCs is reconstructed. The extracted spectral linewidth from the imaginary part of the permittivity (78.4 meV) is consistent with single nanocrystal emission linewidths at room temperature. Finite element simulations show enhanced absorption cross section of a single PNC coupled to a nanoantenna, demonstrating applicability of the extracted permittivity. More generally, these findings provide a route to extract intrinsic permittivity of individual nanocrystals from absorbance measurements of their ensembles.

physics.optics↗

arXiv2025

Quantitative Analytical Model for Scattering-type Scanning Near-field Optical Spectroscopy

Scattering-type scanning near-field optical microscopy (s-SNOM) is a versatile technique in nanooptics, enabling local probing of optical responses beyond the diffraction limit from vis to THz frequencies. Its theoretical modeling based on tip-sample interactions typically relies on computationally intensive numerical methods or phenomenological models with empiric fitting parameters, complicating spectral analysis and interpretation. Developing a rigorous quantitative analytical model remains a significant challenge in near-field microscopy. Here, we introduce an accurate analytical solution for the prolate spheroid model of s-SNOM in the quasi-electrostatic limit. We validate our solution through comparisons with numerical simulations and experimental spectra. Due to its higher computational efficiency compared to numerical simulation and higher accuracy compared to phenomenological solutions, our solution for spheroid model facilitates spectrum prediction and interpretation for homogeneous bulk samples, enables systematic exploration of parameter effects, and supports data generation for machine learning applications. Furthermore, the generality of our approach allows straightforward extension to more complex nanostructures.

physics.optics↗

arXiv2025

Perovskite Nanocrystals as Emerging Single-Photon Emitters: Progress, Challenges, and Opportunities

Metal-halide perovskite nanocrystals (PNCs) have emerged as leading candidates for next-generation quantum emitters, offering a unique combination of high photoluminescence quantum yield, tunable emission, short radiative lifetimes, and record-high single-photon purity under ambient conditions. These properties, together with low-cost and scalable solution-phase fabrication, position PNCs as attractive alternatives to traditional epitaxial and colloidal quantum dots. In this Review, we outline the physical parameters that define quantum emission in PNCs, compare their performance to other established and emerging quantum emitters, and assess the key figures of merit, including photostability, single-photon purity, and photon indistinguishability, required for practical quantum applications. We discuss underlying mechanisms affecting PNC emission behavior and highlight recent advances in improving their quantum emitting properties through synthetic and photonic engineering approaches. While challenges related to environmental stability and photon indistinguishability remain, emerging strategies, such as surface passivation, metal ion doping, and coupling with electromagnetic nano- and micro-cavities, are steadily closing the gap between PNCs and ideal quantum light sources.

physics.optics↗

arXiv2025

Tunable hyperbolic Landau-level polaritons in charge-neutral graphene nanoribbon metasurfaces

Magnetized charge-neutral graphene supports collective hybrid electronic excitations - polaritons - which have quantum origin. In contrast to polaritons in doped graphene, which arise from intraband electronic transitions, those in charge-neutral graphene originate from interband transitions between Landau levels, enabled by the applied magnetic field. Control of such quantum polaritons and shaping their wavefronts remains totally unexplored. Here we design an artificial two-dimensional quantum material formed by charge-neutral graphene nanoribbons exposed to an external magnetic field. In such metasurface, quantum polaritons acquire a hyperbolic dispersion. We find that the topology of the isofrequency curves of quantum hyperbolic magnetoexciton polaritons excited in this quantum material can change, so that the shape of isofrequency curves transforms from a closed to open one by tuning the external magnetic field strength. At the topological transition, we observe canalization phenomena, consisting of the propagation of all the polaritonic plane waves in the continuum along the same direction when excited by a point source. From a general perspective, our fundamental findings introduce a novel type of actively-tunable quantum polaritons with hyperbolic dispersion and can be further generalized to other types of quantum materials and polaritons in them. In practice, quantum hyperbolic polaritons can be used for applications related to quantum sensing and computing.

cond-mat.mes-hall↗

arXiv2025

Directional strong coupling at the nanoscale between hyperbolic polaritons and organic molecules

Strong coupling (SC) is a fundamental concept in physics that describes extreme interactions between light and matter. Recent experiments have demonstrated SC at the nanometer scale, where strongly confined polaritons, rather than photons, couple to quantum emitters or molecular vibrations. Coupling with the latter is generally referred to as vibrational SC (VSC) and is of significant fundamental and technological interest, as it can be an effective tool for modifying molecular properties. However, the implementation of VSC, especially at the nanoscale, depends on the development of tuning mechanisms that allow control over the coupling strength and, eventually, its directionality, opening the door for the selective coupling of specific molecular vibrations. Here we report the observation of directional VSC. Specifically, we show nanoscale images of propagating hyperbolic phonon polaritons (PhPs) coupled to pentacene molecules revealing that the fingerprint of VSC for propagating polaritons -- a marked anti-crossing in their dispersion at the vibrational resonance -- can be modulated as a function of the direction of propagation. In addition, we show that VSC can exhibit an optimal condition for thin molecular layers, characterized by a maximum coupling strength along one single direction. This phenomenon is understood by analysing the overlap of the polariton field with molecular layers of varying thicknesses. Apart from their fundamental importance, our findings promise novel applications for directional sensing or local directional control of chemical properties at the nanoscale.

cond-mat.mtrl-sci↗

arXiv2025

Misalignment between the Directions of Propagation and Decay of Nanoscale-confined Polaritons

Anisotropic van der Waals crystals have gained significant attention in nanooptics and optoelectronics due to their unconventional optical properties, including anomalous reflection, canalization, and nanofocusing. Polaritons -- light coupled to matter excitations -- govern these effects, with their complex wavevector encoding key parameters such as wavelength, lifetime, field confinement, and propagation direction. However, determining the complex wavevector, particularly the misalignment between its real and imaginary parts, has remained a challenge due to the complexity of the dispersion relation. Here, using near-field nanoimaging, we introduce a self-consistent method to extract the complex wavevector from polaritonic near-field images. We experimentally reveal a strong misalignment between the real and imaginary components of the wavevector, significantly impacting the interpretation of near-field experiments. Our findings establish a new paradigm for optical nanoimaging, providing a robust framework for accurately extracting polariton parameters and advancing the broader field of nanooptics of lossy anisotropic crystals.

physics.optics↗

arXiv2025

Bloch phonon-polaritons with anomalous dispersion in polaritonic Fourier crystals

The recently suggested concept of a polaritonic Fourier crystal (PFC) is based on a harmonically-corrugated mirror substrate for a thin pristine polaritonic crystal layer. The propagating polaritons in PFC experience a harmonic and mode-selective momentum modulation leading to a manifestation of Bloch modes with practically zero inter-mode scattering. PFC was first demonstrated for the hyperbolic phonon-polaritons in hexagonal boron nitride (hBN) within its Type II Reststrahlen band (RB-II) where the in-plane components of the dielectric permittivity tensor are isotropic and negative, while the out-of-plane component is positive. By contrast, a Type I Reststrahlen band (RB-I) is characterized by negative out-of-plane and positive in-plane permittivity components, and consequently, the inversion of field symmetry of phonon-polaritons compared to RB-II. Behavior of such RB-I modes in a polaritonic crystal is yet to be explored. Here, we employ a biaxial crystal alpha-phase molybdenum trioxide (α-MoO3) and near-field imaging to study polaritonic Bloch modes in a one-dimensional PFC within the RB-I where the mid-infrared phonon-polaritons in α-MoO3 have anomalous dispersion and negative phase velocity. Surprisingly, we observe a manifestation of Bloch waves as a dispersionless near-field pattern across the first Brillouin zone, in contrast to RB-II case demonstrated with in-plane isotropic hBN. We attribute this difference to the opposite field symmetry of the lowest-order phonon-polariton mode in the two RBs, leading to a different momentum modulation regime in the polaritonic Fourier crystal. Our results reveal the importance of mode symmetry for polaritonic crystals in general and for the emerging field of Fourier crystals in particular, which promise new ways to manipulate the nanolight.

physics.optics↗

arXiv2025

Roadmap for Photonics with 2D Materials

Triggered by the development of exfoliation and the identification of a wide range of extraordinary physical properties in self-standing films consisting of one or few atomic layers, two-dimensional (2D) materials such as graphene, transition metal dichalcogenides (TMDs), and other van der Waals (vdW) crystals currently constitute a wide research field protruding in multiple directions in combination with layer stacking and twisting, nanofabrication, surface-science methods, and integration into nanostructured environments. Photonics encompasses a multidisciplinary collection of those directions, where 2D materials contribute with polaritons of unique characteristics such as strong spatial confinement, large optical-field enhancement, long lifetimes, high sensitivity to external stimuli (e.g., electric and magnetic fields, heating, and strain), a broad spectral range from the far infrared to the ultraviolet, and hybridization with spin and momentum textures of electronic band structures. The explosion of photonics with 2D materials as a vibrant research area is producing breakthroughs, including the discovery and design of new materials and metasurfaces with unprecedented properties as well as applications in integrated photonics, light emission, optical sensing, and exciting prospects for applications in quantum information, and nanoscale thermal transport. This Roadmap summarizes the state of the art in the field, identifies challenges and opportunities, and discusses future goals and how to meet them through a wide collection of topical sections prepared by leading practitioners.

cond-mat.mtrl-sci↗

arXiv2025

High-intensity wave vortices around subwavelength holes: from ocean tides to nanooptics

Vortices are ubiquitous in nature; they appear in a variety of phenomena ranging from galaxy formation in astrophysics to topological defects in quantum fluids. In particular, wave vortices have attracted enormous attention and found applications in optics, acoustics, electron microscopy, etc. Such vortices carry quantized phase singularities accompanied by zero intensity in the center, and quantum-like orbital angular momentum, with the minimum localization scale of the wavelength. Here we describe a conceptually novel type of wave vortices, which can appear around arbitrarily small `holes' (i.e., excluded areas or defects) in a homogeneous 2D plane. Such vortices are characterized by high intensity and confinement at the edges of the hole and hence subwavelength localization of the angular momentum. We demonstrate the appearance of such vortices in: (i) optical near fields around metallic nanodiscs on a dielectric substrate, (ii) phonon-polariton fields around nanoholes in a polaritonic slab, and (iii) ocean tidal waves around islands of New Zealand and Madagascar. We also propose a simple toy model of the generation of such subwavelength vortices via the interference of a point-dipole source and a plane wave, where the vortex sign is controlled by the mutual phase between these waves. Our findings open avenues for subwavelength vortex/angular-momentum-based applications in various wave fields.

physics.optics↗

arXiv2024

Low-loss twist-tunable in-plane anisotropic polaritonic crystals

Van der Waals (vdW) materials supporting phonon polaritons (PhPs) - light coupled to lattice vibrations - have gathered significant interest because of their intrinsic anisotropy and low losses. In particular, $α$-MoO$_3$ supports PhPs with in-plane anisotropic propagation, which has been exploited to tune the optical response of twisted bilayers and trilayers. Additionally, various studies have explored the realization of polaritonic crystals (PCs) - lattices with periods comparable to the polariton wavelength -. PCs consisting of hole arrays etched in $α$-MoO$_3$ slabs exhibit Bragg resonances dependent on the angle between the crystallographic axes and the lattice vectors. However, such PC concept, with a fixed orientation and size of its geometrical parameters, constrains practical applications and introduces additional scattering losses due to invasive fabrication processes. Here we demonstrate a novel PC concept that overcomes these limitations, enabling low-loss optical tuning. It comprises a rotatable pristine $α$-MoO$_3$ layer located on a periodic hole array fabricated in a metallic layer. Our design prevents degradation of the $α$-MoO$_3$ optical properties caused by fabrication, preserving its intrinsic low-loss and in-plane anisotropic propagation of PhPs. The resulting PC exhibits rotation of the Bloch modes, which is experimentally visualized by scanning near-field microscopy. In addition, we experimentally determine the polaritons momentum and reconstruct their band structure. These results pave the way for mechanically tunable nanooptical components based on polaritons for potential lasing, sensing, or energy harvesting applications.

physics.optics↗

arXiv2024

Unveiling the Mechanism of Phonon-Polariton Damping in α-MoO_3

Phonon polaritons (PhPs) (light coupled to lattice vibrations) in the highly anisotropic polar layered material molybdenum trioxide (α-MoO_3) are currently the focus of intense research efforts due to their extreme subwavelength field confinement, directional propagation and unprecedented low losses. Nevertheless, prior research has primarily concentrated on exploiting the squeezing and steering capabilities of α-MoO_3 PhPs, without inquiring much into the dominant microscopic mechanism that determines their long lifetimes, key for their implementation in nanophotonic applications. This study delves into the fundamental processes that govern PhP damping in α-MoO_3 by combining ab initio calculations with scattering-type scanning near-field optical microscopy (s-SNOM) and Fourier-transform infrared (FTIR) spectroscopy measurements across a broad temperature range (from 8 to 300 K). The remarkable agreement between our theoretical predictions and experimental observations allows us to identify third-order anharmonic phonon-phonon scattering as the main damping mechanism of α-MoO_3 PhPs. These findings shed light on the fundamental limits of low-loss PhPs, a crucial factor for assessing their implementation into nanophotonic devices.

cond-mat.mtrl-sci↗

arXiv2024

Polaritonic Fourier crystal

Polaritonic crystals - periodic structures where the hybrid light-matter waves called polaritons can form Bloch states - promise a deeply subdiffractional nanolight manipulation and enhanced light-matter interaction. In particular, polaritons in van der Waals materials boast extreme field confinement and long lifetimes allowing for the exploitation of wave phenomena at the nanoscale. However, in conventionally patterned nanostructures, polaritons are prone to severe scattering loss at the sharp material edges, making it challenging to create functional polaritonic crystals. Here, we introduce a new concept of a polaritonic Fourier crystal based on a harmonic modulation of the polariton momentum in a pristine polaritonic waveguide with minimal scattering. We employ hexagonal boron nitride (hBN) and near-field imaging to reveal a neat and well-defined band structure of phonon-polaritons in the Fourier crystal, stemming from the dominant excitation of the first-order Bloch mode. Furthermore, we show that the fundamental Bloch mode possesses a polaritonic bandgap even in the relatively lossy naturally abundant hBN. Thus, our work provides a new paradigm for polaritonic crystals essential for enhanced light-matter interaction, dispersion engineering, and nanolight guiding.

physics.optics↗

arXiv2024

Canalization-based super-resolution imaging using a single van der Waals layer

Canalization is an optical phenomenon that enables unidirectional propagation of light in a natural way, i.e., without the need for predefined waveguiding designs. Predicted years ago, it was recently demonstrated using highly confined phonon polaritons (PhPs) in twisted layers of the van der Waals (vdW) crystal alpha-MoO3, offering unprecedented possibilities for controlling light-matter interactions at the nanoscale. However, despite this finding, applications based on polariton canalization have remained elusive so far, which can be explained by the complex sample fabrication of twisted stacks. In this work, we introduce a novel canalization phenomenon, arising in a single vdW thin layer (alpha-MoO3) when it is interfaced with a substrate exhibiting a given negative permittivity, that allows us to demonstrate a proof-of-concept application based on polariton canalization: super-resolution (up to ~λ0/220) nanoimaging. Importantly, we find that canalization-based imaging transcends conventional projection constraints, allowing the super-resolution images to be obtained at any desired location in the image plane. This versatility stems from the synergetic manipulation of three distinct parameters: incident frequency, rotation angle of the thin vdW layer, and thickness. These results provide valuable insights into the fundamental properties of canalization and constitute a seminal step towards multifaceted photonic applications, encompassing imaging, data transmission, and ultra-compact photonic integration.

physics.optics↗

arXiv2023

Fundamentals of polaritons in strongly anisotropic thin crystal layers

Polaritons in strongly anisotropic thin layers have recently captured the attention in nanophotonics because of their directional propagation at the nanoscale, which offers unique possibilities for nanooptical applications. However, exploiting the full potential of anisotropic polaritons requires a thorough understanding of their properties, including field confinement, energy and phase propagation direction and losses. Here we fill this critical gap by providing fundamental insights into the propagation of anisotropic polaritons in thin biaxial layers. In particular, we introduce a novel methodology that allows us to represent isofrequency curves of polaritons in strongly anisotropic materials considering that the real and imaginary parts of the wavevector are not parallel. In fact, we analytically show that the direction of the imaginary part of the wavevector is parallel to the group velocity, which can have different, even perpendicular or opposite, directions with respect to the phase velocity. This finding is crucial for understanding polaritonic phenomena in anisotropic media, yet it has so far been widely overlooked in the literature. Additionally, we introduce a criterion for classifying the polaritonic modes in biaxial layers into volume and surface categories, and analyze their dispersion, field structure, and losses. Finally, we discover the existence of anisotropic transverse electric modes, which can exhibit natural canalization. Taken together, our results shed light on hitherto unexplored areas of the theory of electromagnetic modes in thin biaxial layers. Although exemplified for van der Waals MoO3 layers, our findings are general for polaritons in other strongly anisotropic biaxial hyperbolic crystals.

physics.optics↗