arXiv subjects

Alfred B. U'Ren

Publications and source records attributed to Alfred B. U'Ren.

At least 19 recordsLinked to original sources

arXiv2024

Spatio-Spectral Quantum State Estimation of Photon Pairs from Optical Fiber Using Stimulated Emission

Developing a quantum light source that carries more than one bit per photon is pivotal for expanding quantum information applications. Characterizing a high-dimensional multiple-degree-of-freedom source at the single-photon level is challenging due to the large parameter space as well as limited emission rates and detection efficiencies. Here, we characterize photon pairs generated in optical fiber in the transverse-mode and frequency degrees of freedom by applying stimulated emission in both degrees of freedom while detecting in one of them at a time. This method may be useful in the quantum state estimation and optimization of various photon-pair source platforms in which complicated correlations across multiple degrees of freedom may be present.

quant-ph↗

arXiv2024

Generation of heralded vector-polarized single photons in remotely controlled topological classes

We demonstrate an experimental protocol for the preparation and control of heralded single photons in inhomogeneously polarized states, such as Vector Vortex and Full Poincaré beam states. A laser beam is shaped by a voltage-controlled spin-to-orbital angular momentum converter q-plate device which eliminates the need for an interferometer for the robust preparation of high-quality inhomogeneously polarized beams. Such a beam is then used as pump in a spontaneous parametric downconversion (SPDC) photon-pair source. We demonstrate the full pump to heralded single photon transfer of the intensity/phase distributions, as well as of the vector polarization structure. Additionally, we show that by controlling the polarization to which the heralding idler photon is projected before detection, we can toggle between the direct and basis-switched pump-single photon transfer. We show that this non-local control of the heralded single photon pertains also to the topological class of the resulting heralded single photon. We believe that our work will lead to new opportunities in photons-based quantum information processing science.

quant-ph↗

arXiv2023

Quantum enhanced probing of multilayered-samples

Quantum sensing exploits quantum phenomena to enhance the detection and estimation of classical parameters of physical systems and biological entities, particularly so as to overcome the inefficiencies of its classical counterparts. A particularly promising approach within quantum sensing is Quantum Optical Coherence Tomography which relies on non-classical light sources to reconstruct the internal structure of multilayered materials. Compared to traditional classical probing, Quantum Optical Coherence Tomography provides enhanced-resolution images and is unaffected by even-order dispersion. One of the main limitations of this technique lies in the appearance of artifacts and echoes, i.e. fake structures that appear in the coincidence interferogram, which hinder the retrieval of information required for tomography scans. Here, by utilizing a full theoretical model, in combination with a fast genetic algorithm to post-process the data, we successfully extract the morphology of complex multilayered samples and thoroughly distinguish real interfaces, artifacts, and echoes. We test the effectiveness of the model and algorithm by comparing its predictions to experimentally-generated interferograms through the controlled variation of the pump wavelength. Our results could potentially lead to the development of practical high-resolution probing of complex structures and non-invasive scanning of photo-degradable materials for biomedical imaging/sensing, clinical applications, and materials science.

quant-ph↗

arXiv2022

Fiber-based photon pair generation: a tutorial

The purpose of this tutorial paper is to present a broad overview of photon-pair generation through the spontaneous four wave mixing (SFWM) process in optical fibers. Progress in optical fiber technology means that today we have at our disposal a wide variety of types of fiber, which together with the fact that SFWM uses two pump fields, implies a truly remarkable versatility in the resulting possible photon-pair properties. We discuss how the interplay of the frequency, transverse mode, and polarization degrees of freedom, the first linked to the latter two through fiber dispersion, leads to interesting entanglement properties both in individual degrees of freedom and also permitting hybrid and hyper entanglement in combinations of degrees of freedom. This tutorial covers methods for photon pair factorability, frequency tunability, and SFWM bandwidth control, the effect of frequency non-degenerate and counter-propagating pumps, as well methods for characterizing photon pairs generated in optical fibers.

quant-ph↗

arXiv2022

Witnessing Entangled Two-Photon Absorption via Quantum Interferometry

Recent investigations suggest that the use of non-classical states of light, such as entangled photon pairs, may open new and exciting avenues in experimental two-photon absorption spectroscopy. Despite several experimental studies of entangled two-photon absorption (eTPA), there is still a heated debate on whether eTPA has truly been observed. This interesting debate has arisen, mainly because it has been recently argued that single-photon-loss mechanisms, such as scattering or hot-band absorption may mimic the expected entangled-photon linear absorption behavior. In this work, we focus on transmission measurements of eTPA, and explore three different two-photon quantum interferometers in the context of assessing eTPA. We demonstrate that the so-called N00N-state configuration is the only one amongst those considered insensitive to linear (single-photon) losses. Remarkably, our results show that N00N states may become a potentially powerful tool for quantum spectroscopy, and place them as a strong candidate for the certification of eTPA in an arbitrary sample.

quant-ph↗

arXiv2022

Quantum optical coherence microscopy for bioimaging applications

Quantum-optical coherence tomography (QOCT) is an optical sectioning modality based on the quantum interference of photon pairs, obtained from a spontaneous parametric downconversion (SPDC) source. The promise of QOCT derives from two quantum-conferred advantages when compared to equivalent classical optical coherence tomography (OCT) systems: a factor of 2 axial resolution enhancement, as well as dispersion cancellation. However, the technique is far from being competitive with current OCT devices due to the long required acquisition times. Here, we on the one hand demonstrate a quantum optical coherence microscopy (QOCM) technique that is designed to overcome some of the limitations of previous QOCT implementations, and on the other hand test it on representative samples, including glass layers with manufactured transverse patterns and metal-coated biological specimens. We use a collinear SPDC source, so that the entire emitted photon pair flux may contribute to the measurements, together with a multi-mode detection design. We employ a Michelson interferometer with the sample placed as end-mirror in one of the interferometer arms, instead of the more typical Hong-Ou-Mandel used in QOCT implementations. In order to probe biological samples we transition from a Michelson to a Linnik interferometer by placing a microscope objective in the sample arm. In our setup, while the idler photon is collected with a multi-mode fiber, the signal photon is detected by an ICCD camera, leading to full-field transverse reconstruction through a single axial acquisition sequence. Interestingly, our setup permits concurrent OCT and QOCT trace acquisition, the former with greater counts and the latter with the benefit of quantum-conferred advantages. We hope that our current results will represent a significant step forward towards the actual applicability of QOCT, e.g. in clinical settings.

physics.optics↗

arXiv2021

Submegahertz spectral width photon pair source based on fused silica microspheres

High efficiency, sub-MHz bandwidth photon pair generators will enable the field of quantum technology to transition from laboratory demonstrations to transformational applications involving information transfer from photons to atoms. While spontaneous parametric processes are able to achieve high efficiency photon pair generation, the spectral bandwidth tends to be relatively large, as defined by phase-matching constraints. To solve this fundamental limitation, we use an ultra-high quality factor (Q) fused silica microsphere resonant cavity to form a photon pair generator. We present the full theory for the SWM process in these devices, fully taking into account all relevant source characteristics in our experiments. The exceptionally narrow (down to kHz-scale) linewidths of these devices in combination with the device size results in a reduction in the bandwidth of the photon pair generation, allowing sub-MHz spectral bandwidth to be achieved. Specifically, using a pump source centered around 1550nm, photon pairs with the signal and idler modes at wavelengths close to 1540nm and 1560nm, respectively, are demonstrated. We herald a single idler-mode photon by detecting the corresponding signal photon, filtered via transmission through a wavelength division multiplexing channel of choice. We demonstrate the extraction of the spectral profile of a single peak in the single-photon frequency comb from a measurement of the signal-idler time of emission distribution. These improvements in device design and experimental methods enabled the narrowest spectral width (366kHz) to date in a heralded single photon source basedon SFWM.

quant-ph↗

arXiv2021

Experimental study on the effects of photon-pair temporal correlations in entangled two-photon absorption

Entangled two-photon absorption (ETPA) has recently become a topic of lively debate, mainly due to the apparent inconsistencies in the experimentally-reported ETPA cross sections of organic molecules. In this work, we provide a thorough experimental study of ETPA in the organic molecules Rhodamine B (RhB) and Zinc Tetraphenylporphirin (ZnTPP). The goal of this contribution is twofold: on one hand, it seeks to reproduce the results of previous experimental reports and, on the other, it aims to determine the effects of different temporal correlations -- introduced as a controllable time-delay between the photons to be absorbed -- on the strength of the ETPA signal. In our experiment, the samples are excited by entangled pairs produced by type-I SPDC, with a spectral distribution centered at 810 nm. Surprisingly, and contrary to what was expected, the time delay did not produce in our experiments any systematic change in the cross-sections when monitoring the ETPA signal using a transmission measurement scheme. As a plausible cause of this unexpected result, we argue that the photon-pair flux, typically-used in these experiments, is not sufficient to promote the two-photon absorption process in these molecules. This suggests that the actual absorption cross-section values are lower than those previously reported, and therefore do not lead to a measurable ETPA effect for the transmission method.

quant-ph↗

arXiv2020

Interference effects in quantum-optical coherence tomography using spectrally engineered photon pairs

Optical-coherence tomography (OCT) is a technique that employs light in order to measure the internal structure of semi-transparent, e.g. biological, samples. It is based on the interference pattern of low-coherence light. Quantum-OCT (QOCT), instead, employs the correlation properties of entangled photon pairs, for example, generated by the process of spontaneous parametric downconversion (SPDC). The usual QOCT scheme uses photon pairs characterised by a joint-spectral amplitude with strict spectral anti-correlations. It has been shown that, in contrast with its classical counterpart, QOCT provides resolution enhancement and dispersion cancellation. In this paper, we revisit the theory of QOCT and extend the theoretical model so as to include photon pairs with arbitrary spectral correlations. We present experimental results that complement the theory and explain the physical underpinnings appearing in the interference pattern. In our experiment, we utilize a pump for the SPDC process ranging from continuous wave to pulsed in the femtosecond regime, and show that cross-correlation interference effects appearing for each pair of layers may be directly suppressed for a sufficiently large pump bandwidth. Our results provide insights and strategies that could guide practical implementations of QOCT.

physics.optics↗

arXiv2020

Spectrally-resolved Hong-Ou-Mandel interferometry for Quantum-Optical Coherence Tomography

In this paper, we revisit the well-known Hong-Ou-Mandel (HOM) effect in which two photons, which meet at a beamsplitter, can interfere destructively, leading to null in coincidence counts. In a standard HOM measurement, the coincidence counts across the two output ports of the beamsplitter are monitored as the temporal delay between the two photons prior to the beamsplitter is varied, resulting in the well-known HOM dip. We show, both theoretically and experimentally, that by leaving the delay fixed at a particular value while relying on spectrally-resolved coincidence photon-counting, we can reconstruct the HOM dip, which would have been obtained through a standard delay-scanning, non-spectrally-resolved HOM measurement. We show that our numerical reconstruction procedure exhibits a novel dispersion cancellation effects, to all orders. We discuss how our present work can lead to a drastic reduction in the time required to acquire a HOM interferogram, and specifically discuss how this could be of particular importance for the implementation of efficient quantum-optical coherence tomography devices.

physics.optics↗

arXiv2020

Third order parametric downconversion: a stimulated approach

We study the process of seeded, or stimulated, third-order parametric down-conversion, as an extension of our previous work on spontaneous parametric downconversion (TOSPDC). We present general expressions for the spectra and throughputs expected for the cases where the seed field or fields overlap either only one or two of the TOSPDC modes, and also allow for both pump and seed to be either monochromatic or pulsed. We present a numerical study for a particular source design, showing that doubly-overlapped seeding can lead to a considerably greater generated flux as compared with singly-overlapped seeding. We furthermore show that doubly-overlapped seeding permits stimulated emission tomography for the reconstruction of the three-photon TOSPDC joint spectral intensity. We hope that our work will guide future experimental efforts based on the process of third-order parametric downconversion.

quant-ph↗

arXiv2019

Towards third-order parametric down-conversion in optical fibers

Optical fibers have been considered an optimal platform for third-order parametric down-conversion since they can potentially overcome the weak third-order nonlinearity by their long interaction length. Here we present, in the first part, a theoretical derivation for the conversion rate both in the case of spontaneous generation and in the presence of a seed beam. Then we review three types of optical fibers and we examine their properties in terms of conversion efficiency and practical feasibility.

quant-ph↗

arXiv2019

Temperature-Controlled Entangled-Photon Absorption Spectroscopy

Entangled two-photon absorption spectroscopy (TPA) has been widely recognized as a powerful tool for revealing relevant information about the structure of complex molecular systems. However, to date, the experimental implementation of this technique has remained elusive, mainly because of two major difficulties. First, the need to perform multiple experiments with two-photon states bearing different temporal correlations, which translates in the necessity to have at the experimenter's disposal tens, if not hundreds, of sources of entangled photons. Second, the need to have \emph{a priori} knowledge of the absorbing medium's lowest-lying intermediate energy level. In this work, we put forward a simple experimental scheme that successfully overcomes these two limitations. By making use of a temperature-controlled entangled-photon source, which allows the tuning of the central frequencies of the absorbed photons, we show that the TPA signal, measured as a function of the temperature of the nonlinear crystal that generates the paired photons, and a controllable delay between them, carries all information about the electronic level structure of the absorbing medium, which can be revealed by a simple Fourier transformation.

quant-ph↗

arXiv2018

Testing Randomness in Quantum Mechanics

Pseudo-random number generators are widely used in many branches of science, mainly in applications related to Monte Carlo methods, although they are deterministic in design and, therefore, unsuitable for tackling fundamental problems in security and cryptography. The natural laws of the microscopic realm provide a fairly simple method to generate non-deterministic sequences of random numbers, based on measurements of quantum states. In practice, however, the experimental devices on which quantum random number generators are based are often unable to pass some tests of randomness. In this review, we briefly discuss two such tests, point out the challenges that we have encountered and finally present a fairly simple method that successfully generates non-deterministic maximally random sequences.

quant-ph↗

arXiv2018

Joint Spectral Characterization of Photon-Pair Sources

The ability to determine the joint spectral properties of photon pairs produced by the processes of spontaneous parametric downconversion (SPDC) and spontaneous four wave mixing (SFWM) is crucial for guaranteeing the usability of heralded single photons and polarization-entangled pairs for multi-photon protocols. In this paper, we compare six different techniques that yield either a characterization of the joint spectral intensity or of the closely-related purity of heralded single photons. These six techniques include: i) scanning monochromator measurements, ii) a variant of Fourier transform spectroscopy designed to extract the desired information exploiting a resource-optimized technique, iii) dispersive fibre spectroscopy, iv) stimulated-emission-based measurement, v) measurement of the second-order correlation function $g^{(2)}$ for one of the two photons, and vi) two-source Hong-Ou-Mandel interferometry. We discuss the relative performance of these techniques for the specific cases of a SPDC source designed to be factorable and SFWM sources of varying purity, and compare the techniques' relative advantages and disadvantages.

quant-ph↗

arXiv2017

Improving randomness characterization through Bayesian model selection

Nowadays random number generation plays an essential role in technology with important applications in areas ranging from cryptography, which lies at the core of current communication protocols, to Monte Carlo methods, and other probabilistic algorithms. In this context, a crucial scientific endeavour is to develop effective methods that allow the characterization of random number generators. However, commonly employed methods either lack formality (e.g. the NIST test suite), or are inapplicable in principle (e.g. the characterization derived from the Algorithmic Theory of Information (ATI)). In this letter we present a novel method based on Bayesian model selection, which is both rigorous and effective, for characterizing randomness in a bit sequence. We derive analytic expressions for a model's likelihood which is then used to compute its posterior probability distribution. Our method proves to be more rigorous than NIST's suite and the Borel-Normality criterion and its implementation is straightforward. We have applied our method to an experimental device based on the process of spontaneous parametric downconversion, implemented in our laboratory, to confirm that it behaves as a genuine quantum random number generator (QRNG). As our approach relies on Bayesian inference, which entails model generalizability, our scheme transcends individual sequence analysis, leading to a characterization of the source of the random sequences itself.

physics.data-an↗

arXiv2016

Counter-propagating spontaneous four wave mixing: photon-pair factorability and ultra-narrowband single photon

We introduce a new kind of spontaneous four wave mixing process for the generation of photon pairs, in which the four waves involved counter-propagate in a guided-wave χ^{(3)} medium; we refer to this process as counter-propagating spontaneous four wave mixing (CP-SFWM). We show that for the simplest CP-SFWM source, in which all waves propagate in the same polarization and transverse mode and in which self- and cross-phase modulation effects are negligible, phasematching is attained automatically regardless of dispersion in the fiber or waveguide. Furthermore, we show that in two distinct versions of this source (both pumps pulsed, or one pump pulsed and the remaining one monochromatic), the two-photon state is automatically factorable provided that the length of the nonlinear medium exceeds a certain threshold, easily achievable in practice since this threshold length tends to be in the range of mm to cm. We also show that if one of the pumps approaches the monochromatic limit, and for a sufficient nonlinear medium length, the bandwidth of one of the two photons in a given pair may be reduced to the level of MHz, compatible with electronic transitions for the implementation of atom-photon interfaces, without the use of optical cavities.

quant-ph↗

arXiv2016

Heralded single-photon source utilizing highly nondegenerate, spectrally factorable spontaneous parametric downconversion

We report on the generation of an indistinguishable heralded single-photon state, using highly nondegenerate spontaneous parametric downconversion (SPDC). Spectrally factorable photon pairs can be generated by incorporating a broadband pump pulse and a group-velocity matching (GVM) condition in a periodically-poled potassium titanyl phosphate (PPKTP) crystal. The heralding photon is in the near IR, close to the peak detection efficiency of off-the-shelf Si single-photon detectors; meanwhile, the heralded photon is in the telecom L-band where fiber losses are at a minimum. We observe spectral factorability of the SPDC source and consequently high purity (90%) of the produced heralded single photons by several different techniques. Because this source can also realize a high heralding efficiency (> 90%), it would be suitable for time-multiplexing techniques, enabling a pseudo-deterministic single-photon source, a critical resource for optical quantum information and communication technology.

quant-ph↗