arXiv subjects

Ali Yazdani

Publications and source records attributed to Ali Yazdani.

At least 19 recordsLinked to original sources

arXiv2026

Local spectroscopy of anyons bound to charge traps

Fractional quantum Hall states host anyons, emergent quasiparticles with fractional charge and nontrivial exchange statistics. Controlling, trapping, and braiding anyons are central goals for both fundamental physics and topological quantum computation. A key step toward such control is understanding how anyons behave when confined in local potentials, where their internal structure can become relevant. Here, we use the scanning tunneling microscopy/spectroscopy (STM/STS) to study the excitation spectrum in integer and fractional quantum Hall states of monolayer graphene near individual charged impurities. In the integer quantum Hall states, the STS spectra show lifting of orbital degeneracy near defects, appearing as a band of discrete energy levels. In fractional states, (v=1/3 and 2/5), however, we observe an additional energy splitting of the lowest-energy spectral feature that occurs only when the chemical potential lies within a fractional gap and is absent in compressible or integer regimes. We attribute this to many-body configurations of anyons trapped by an impurity potential. Strikingly, numerical calculations show that the splitting requires an anisotropic confining potential, vanishing for a rotationally symmetric trap. The competing multi-anyon states carry nearly identical charge within the core of the potential but differ in how that charge is redistributed at larger radius. Our results establish local tunneling spectroscopy as a direct probe of anyon bound states, providing a key step toward understanding and controlling their behavior in confined geometries relevant for braiding and fusion.

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arXiv2026

Visualizing Symmetry Broken Chern Insulators and their Quantum Melting

In the presence of a magnetic field, electronic states of moir\'e quantum materials develop a Hofstadter spectrum that provides a unique setting for studying the interplay between band topology and strong electron-electron interaction. Using scanning tunneling microscopy, we study Hofstadter's states in bilayer graphene aligned with hexagonal BN and directly visualize the formation of interaction-driven symmetry breaking Chern insulators. Our measurements reveal the formation of phases that double, triple or quadruple the moir\'e unit cell at fractional filling of the Hofstadter bands, as well as states with complex intra-unit-cell wave functions. We visualize two distinct quantum phenomena in different Chern states, including quantum melting driven by the appearance and proliferation of topological defects, and a quantum transition co-occurring with phase competition and separation.

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arXiv2026

Qumus: Realization of An Embodied AI Quantum Material Experimentalist

While modern Large Language Models (LLMs) and agentic artificial intelligence (AI) have demonstrated transformative capabilities in digital domains, the realization of embodied AI capable of real-world scientific discovery remains a difficult frontier. The advancements are hindered by the inherent complexity of integrating high-level reasoning, multimodal information processing and real-time physical execution. Here we introduce Qumus, the first AI quantum materials experimentalist. Physically embodied within a robotic mini-laboratory, Qumus is an intelligent, multimodal, and multi-agent system designed for the creation and nano-processing of atomically thin two-dimensional (2D) materials and stacked van der Waals (vdW) structures. Qumus autonomously navigates the full scientific cycle, from hypothesis generation and protocol planning to multi-step experimental execution, result analysis and reporting, acting as an experimentalist. Markedly, the system has achieved, for the first time, the AI-creation of graphene, as well as the first AI-fabrication of complex nanodevices including atomically thin field-effect transistors via vdW stacking. Qumus excels at these tasks by demonstrating autonomous error correction and closed-loop experimentation. Our results establish a generalizable framework for self-improving embodied AI systems that learn directly from the quantum world, opening a pathway toward accelerated discovery in quantum materials, electronics and beyond.

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arXiv2025

tritonBLAS: Triton-based Analytical Approach for GEMM Kernel Parameter Selection

We present tritonBLAS, a fast and deterministic analytical model that uses architectural parameters like the cache hierarchy, and relative code and data placement to generate performant GPU GEMM kernels. tritonBLAS explicitly models the relationship between architectural topology, matrix shapes, and algorithmic blocking behavior to predict near-optimal configurations without runtime autotuning. Based on this model, we developed and implemented a lightweight GEMM framework entirely within Triton. We evaluate the performance of tritonBLAS across a diverse set of GEMM problem sizes on modern GPUs. tritonBLAS achieves over 95% of the performance of autotuning solutions, while reducing autotuning time to zero. This makes tritonBLAS a practical drop-in replacement for empirical tuning in production HPC and ML workloads.

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arXiv2025

Visualizing interaction-driven restructuring of quantum Hall edge states

Many topological phases host gapless boundary modes that can be dramatically modified by electronic interactions. Even for the long-studied edge modes of quantum Hall phases, forming at the boundaries of two-dimensional (2D) electron systems, the nature of such interaction-induced changes has been elusive. Despite advances made using local probes, key experimental challenges persist: the lack of direct information about the internal structure of edge states on microscopic scales, and complications from edge disorder. Here, we use scanning tunneling microscopy (STM) to image pristine electrostatically defined quantum Hall edge states in graphene with high spatial resolution and demonstrate how correlations dictate the structures of edge channels on both magnetic and atomic length scales. For integer quantum Hall states in the zeroth Landau level, we show that interactions renormalize the edge velocity, dictate the spatial profile for copropagating modes, and induce unexpected edge valley polarization that differ from those of the bulk. While some of our findings can be understood by mean-field theory, others show breakdown of this picture, highlighting the roles of edge fluctuations and inter-channel couplings. We also extend our measurements to spatially resolve the edge state of fractional quantum Hall phases and detect spectroscopic signatures of interactions in this chiral Luttinger liquid. Our study establishes STM as a promising tool for exploring edge physics of the rapidly expanding 2D topological phases, including newly realized fractional Chern insulators.

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arXiv2025

Spectroscopy of the Fractal Hofstadter Energy Spectrum

Hofstadter's butterfly, the predicted energy spectrum for non-interacting electrons confined to a two-dimensional lattice in a magnetic field, is one of the most remarkable fractal structures in nature. At rational ratios of magnetic flux quanta per lattice unit cell, this spectrum shows self-similar distributions of energy levels that reflect its recursive construction. For most materials, Hofstadter's butterfly is predicted under experimental conditions that are unachievable using laboratory-scale magnetic fields. More recently, electrical transport studies have provided evidence for Hofstadter's butterfly in materials engineered to have artificially large lattice constants, such as those with moir\'e superlattices. Yet to-date, direct spectroscopy of the fractal energy spectrum predicted by Hofstadter nearly 50 years ago has remained out of reach. Here we use high-resolution scanning tunneling microscopy / spectroscopy (STM / STS) to probe the flat electronic bands in twisted bilayer graphene near the predicted second magic angle, an ideal setting for spectroscopic studies of Hofstadter's spectrum. Our study shows the fractionalization of flat moir\'e bands into discrete Hofstadter subbands and discerns experimental signatures of self-similarity of this spectrum. Moreover, our measurements uncover a spectrum that evolves dynamically with electron density, displaying phenomena beyond that of Hofstadter's original model due to the combined effects of strong correlations, Coulomb interactions, and the quantum degeneracy of electrons in twisted bilayer graphene.

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arXiv2024

High spatial resolution charge sensing of quantum Hall states

Charge distribution offers a unique fingerprint of important properties of electronic systems, including dielectric response, charge ordering and charge fractionalization. We develop a new architecture for charge sensing in two-dimensional electronic systems in a strong magnetic field. We probe local change of the chemical potential in a proximitized detector layer using scanning tunneling microscopy (STS), allowing us to infer the chemical potential and the charge profile in the sample. Our technique has both high energy (<0.3 meV) and spatial (<10 nm) resolution exceeding that of previous studies by an order of magnitude. We apply our technique to study the chemical potential of quantum Hall liquids in monolayer graphene under high magnetic fields and their responses to charge impurities. The chemical potential measurement provides a local probe of the thermodynamic gap of quantum Hall ferromagnets and fractional quantum Hall states. The screening charge profile reveals spatially oscillatory response of the quantum Hall liquids to charge impurities, and is consistent with the composite Fermi liquid picture close to the half-filling. Our technique also paves the way to map moir\'e potentials, probe Wigner crystals, and investigate fractional charges in quantum Hall and Chern insulators.

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arXiv2024

Fingerprints of Composite Fermion Lambda Levels in Scanning Tunneling Microscopy

Composite fermion (CF) is a topological quasiparticle that emerges from a non-perturbative attachment of vortices to electrons in strongly correlated two-dimensional materials. Similar to non-interacting fermions that form Landau levels in a magnetic field, CFs can fill analogous ``Lambda'' levels, giving rise to the fractional quantum Hall (FQH) effect of electrons. Here, we show that Lambda levels can be directly visualized through the characteristic peak structure in the signal obtained via spectroscopy with the scanning tunneling microscopy (STM) on a FQH state. Complementary to transport, which probes low-energy properties of CFs, we show that \emph{high-energy} features in STM spectra can be interpreted in terms of Lambda levels. We numerically demonstrate that STM spectra can be accurately modeled using Jain's CF theory. Our results show that STM provides a powerful tool for revealing the anatomy of FQH states and identifying physics beyond the non-interacting CF paradigm.

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arXiv2024

A Microscopic Perspective on Moiré Materials

Contemporary quantum materials research is guided by themes of topology and of electronic correlations. A confluence of these two themes is engineered in "moiré materials", an emerging class of highly tunable, strongly correlated two-dimensional (2D) materials designed by the rotational or lattice misalignment of atomically thin crystals. In moiré materials, dominant Coulomb interactions among electrons give rise to collective electronic phases, often with robust topological properties. Identifying the mechanisms responsible for these exotic phases is fundamental to our understanding of strongly interacting quantum systems, and to our ability to engineer new material properties for potential future technological applications. In this Review, we highlight the contributions of local spectroscopic, thermodynamic, and electromagnetic probes to the budding field of moiré materials research. These techniques have not only identified many of the underlying mechanisms of the correlated insulators, generalized Wigner crystals, unconventional superconductors, moiré ferroelectrics, and topological orbital ferromagnets found in moiré materials, but they have also uncovered fragile quantum phases that have evaded spatially averaged global probes. Furthermore, we highlight recently developed local probe techniques, including local charge sensing and quantum interference probes, that have uncovered new physical observables in moiré materials.

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arXiv2024

Wave-function engineering on superconducting substrates: Chiral Yu-Shiba-Rusinov molecules

Magnetic adatoms on superconductors give rise to Yu-Shiba-Rusinov (YSR) states that hold considerable interest for the design of topological superconductivity. Here, we show that YSR states are also an ideal platform to engineer structures with intricate wave-function symmetries. We assemble structures of iron atoms on the quasi-two-dimensional superconductor $2H$-NbSe$_2$. The Yu-Shiba-Rusinov wave functions of individual atoms extend over several nanometers enabling hybridization even at large adatom spacing. We show that the substrate can be exploited to deliberately break symmetries of the adatom structure in ways unachievable in the gas phase. We highlight this potential by designing chiral wave functions of triangular adatom structures confined within a plane. Our results significantly expand the range of interesting quantum states that can be engineered using arrays of magnetic adatoms on superconductors.

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arXiv2023

Direct observation of a magnetic field-induced Wigner crystal

Eugene Wigner predicted long ago that when the Coulomb interactions between electrons become much stronger than their kinetic energy, electrons crystallize into a closely packed lattice. A variety of two-dimensional systems have shown evidence for Wigner crystals; however, a spontaneously formed classical or quantum Wigner crystal (WC) has never been directly visualized. Neither the identification of the WC symmetry nor direct investigation of its melting has been accomplished. Here we use high-resolution scanning tunneling microscopy (STM) measurements to directly image a magnetic field-induced electron WC in Bernal-stacked bilayer graphene (BLG), and examine its structural properties as a function of electron density, magnetic field, and temperature. At high fields and the lowest temperature, we observe a triangular lattice electron WC in the lowest Landau Level (LLL) of BLG. The WC possesses the expected lattice constant and is robust in a range of filling factors between $\nu\sim$ 0.13 and $\nu\sim$ 0.38 except near fillings where it competes with fractional quantum Hall (FQH) states. Increasing the density or temperature results in the melting of the WC into a liquid phase that is isotropic but has a modulated structure characterized by the WC's Bragg wavevector. At low magnetic fields, the WC unexpectedly transitions into an anisotropic stripe phase, which has been commonly anticipated to form in higher LLs. Analysis of individual lattice sites reveals signatures that may be related to the quantum zero-point motion of electrons in the WC lattice.

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arXiv2023

High-Resolution Tunneling Spectroscopy of Fractional Quantum Hall States

Strong interaction between electrons in two-dimensional systems in the presence of a high magnetic field gives rise to fractional quantum Hall states that host quasiparticles with fractional charge and fractional exchange statistics. Here, we demonstrate high-resolution scanning tunneling microscopy and spectroscopy of fractional quantum Hall states in ultra clean Bernal-stacked bilayer graphene devices. Spectroscopy measurements show sharp excitations that have been predicted to emerge when electrons fractionalize into bound states of quasiparticles. We find energy gaps for candidate non-abelian fractional states that are larger by a factor of five than other related systems - for example semiconductor heterostructures - and this suggests bilayer graphene is an ideal platform for the manipulation of these quasiparticles and for the creation of a topological quantum bit. We also find previously unobserved fractional states in our very clean graphene samples.

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arXiv2023

Hunting for Majoranas

Over the last decade, there have been considerable efforts to observe non-abelian quasi-particles in novel quantum materials and devices. These efforts are motivated by the goals of demonstrating quantum statistics of quasi-particles beyond those of fermions and bosons and of establishing the underlying science for the creation of topologically protected quantum bits. In this review, we focus on efforts to create topological superconducting phases hosting Majorana zero modes. We consider the lessons learned from existing experimental efforts, which are motivating both improvemensts to current platforms and exploration of new approaches. Although the experimental detection of non-abelian quasi-particles remains challenging, the knowledge gained thus far and the opportunities ahead offer high potential for discovery and advances in this exciting area of quantum physics.

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arXiv2023

Broken symmetries and excitation spectra of interacting electrons in partially filled Landau levels

Interacting electrons in flat bands give rise to a variety of quantum phases. One fundamental aspect of such states is the ordering of the various flavours - such as spin or valley - that the electrons can undergo and the excitation spectrum of the broken symmetry states that they form. These properties cannot be probed directly with electrical transport measurements. The zeroth Landau level of monolayer graphene with four-fold spin-valley degeneracy is a model system for such investigations, but the nature of its broken symmetry states - particularly at partial fillings - is still not understood. Here we demonstrate a non-invasive spectroscopic technique with a scanning tunneling microscope and use it to perform measurements of the valley polarization of the electronic wavefunctions and their excitation spectrum in the partially filled zeroth Landau level of graphene. We can extract information such as the strength of Haldane pseudopotentials that characterize the repulsive interactions underlying the fractional quantum states. Our experiments also demonstrate that fractional quantum Hall phases are built upon broken symmetry states that persist at partial filling. Our experimental approach quantifies the valley phase diagram of the partially filled Landau level as a model flat band platform which is applicable to other graphene-based electronic systems.

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arXiv2023

Strong Inter-valley Electron-Phonon Coupling in Magic-Angle Twisted Bilayer Graphene

The unusual properties of superconductivity in magic-angle twisted bilayer graphene (MATBG) have sparked enormous research interest. However, despite the dedication of intensive experimental efforts and the proposal of several possible pairing mechanisms, the origin of its superconductivity remains elusive. Here, utilizing angle-resolved photoemission spectroscopy with micrometer spatial resolution, we have revealed flat band replicas in superconducting MATBG, where MATBG is unaligned with its hexagonal boron nitride (hBN) substrate11. These replicas exhibit uniform energy spacing, approximately 150 +- 15 meV apart, indicative of strong electron-boson coupling. Strikingly, these replicas are absent in non-superconducting twisted bilayer graphene (TBG) systems, either when MATBG is aligned to hBN or when TBG deviates from the magic angle. Calculations suggest that the formation of these flat band replicas in superconducting MATBG are attributed to the strong coupling between flat band electrons and an optical phonon mode at the graphene K point, facilitated by inter-valley scattering. These findings, although do not necessarily put electron phonon coupling as the main driving force for the superconductivity in MATBG, unravel the unique electronic structure inherent in superconducting MATBG, thereby providing crucial information for understanding the unusual electronic landscape from which the superconductivity is derived.

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arXiv2023

Electron-K-Phonon Interaction In Twisted Bilayer Graphene

We develop an analytic theory to describe the interaction between electrons and K-phonons and study its influence on superconductivity in the bare bands of twisted bilayer graphene (TBG). We find that, due to symmetry and the two-center approximation, only one optical K-phonon (~ 160meV) of graphene is responsible for inter-valley electron-phonon interaction. This phonon has recently been found in angular-resolved photo-emission spectroscopy to be responsible for replicas of the TBG flat bands. By projecting the interaction to the TBG flat bands, we perform the full symmetry analysis of phonon-mediated attractive interaction and pairing channels in the Chern basis, and show that several channels are guaranteed to have gapless order parameters. From the linearized gap equations, we find that the highest Tc pairing induced by this phonon is a singlet gapped s-wave inter-Chern-band order parameter, followed closely by a gapless nematic d-wave intra-Chern-band order parameter. We justify these results analytically, using the topological heavy fermion mapping of TBG which has allowed us to obtain an analytic form of phonon-mediated attractive interaction and to analytically solve the linearized and T=0 gap equations. For the intra-Chern-band channel, the nematic state with nodes is shown to be stabilized in the chiral flat band limit. While the flat band Coulomb interaction can be screened sufficiently enough - around Van-Hove singularities - to allow for electron-phonon based superconductivity, it is unlikely that this effect can be maintained in the lower density of states excitation bands around the correlated insulator states.

cond-mat.supr-con↗

arXiv2023

Insulators at Fractional Fillings in Twisted Bilayer Graphene Partially Aligned to Hexagonal Boron Nitride

At partial fillings of its flat electronic bands, magic-angle twisted bilayer graphene (MATBG) hosts a rich variety of competing correlated phases that show sample to sample variations. Divergent phase diagrams in MATBG are often attributed to the sublattice polarization energy scale, tuned by the degree of alignment of the hexagonal boron nitride (hBN) substrates typically used in van der Waals devices. Unaligned MATBG exhibits unconventional superconductivity and correlated insulating phases, while nearly perfectly aligned MATBG/hBN exhibits zero-field Chern insulating phases and lacks superconductivity. Here we use scanning tunneling microscopy and spectroscopy (STM/STS) to observe gapped phases at partial fillings of the flat bands of MATBG in a new intermediate regime of sublattice polarization, observed when MATBG is only partially aligned ($θ_{Gr-hBN}$ $\approx$ 1.65$^\circ$) to the underlying hBN substrate. Under this condition, MATBG hosts not only phenomena that naturally interpolate between the two sublattice potential limits, but also unexpected gapped phases absent in either of these limits. At charge neutrality, we observe an insulating phase with a small energy gap ($Δ$ < 5 meV) likely related to weak sublattice symmetry breaking from the hBN substrate. In addition, we observe new gapped phases near fractional fillings $ν$ = $\pm 1/3$ and $ν$ = $\pm 1/6$, which have not been previously observed in MATBG. Importantly, energy-resolved STS unambiguously identifies these fractional filling states to be of single-particle origin, possibly a result of the super-superlattice formed by two moiré superlattices. Our observations emphasize the power of STS in distinguishing single-particle gapped phases from many-body gapped phases in situations that could be easily confused in electrical transport measurements.

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arXiv2023

Quantum textures of the many-body wavefunctions in magic-angle graphene

Interactions among electrons create novel many-body quantum phases of matter with wavefunctions that often reflect electronic correlation effects, broken symmetries, and novel collective excitations. A wide range of quantum phases has been discovered in MATBG, including correlated insulating, unconventional superconducting, and magnetic topological phases. The lack of microscopic information, including precise knowledge of possible broken symmetries, has thus far hampered our understanding of MATBG's correlated phases. Here we use high-resolution scanning tunneling microscopy to directly probe the wavefunctions of the correlated phases in MATBG. The squares of the wavefunctions of gapped phases, including those of the correlated insulators, pseudogap, and superconducting phases, show distinct patterns of broken symmetry with a $\sqrt{3}$ x $\sqrt{3}$ super-periodicity on the graphene atomic lattice that has a complex spatial dependence on the moiré superlattice scale. We introduce a symmetry-based analysis to describe our measurements of the wavefunctions of MATBG's correlated phases with a set of complex-valued local order parameters. For the correlated insulators in MATBG, at fillings of $ν$ = $\pm$ 2 electrons per moiré unit cell relative to charge neutrality, we compare the observed quantum textures to those expected for proposed theoretical ground states. In typical MATBG devices, the textures of correlated insulators' wavefunctions closely match those of the theoretically proposed IKS order, while in ultra-low-strain samples our data has local symmetries like those of a T-IVC phase. We also study the wavefunction of MATBG's superconducting state, revealing strong signatures of intervalley coherence that can only be distinguished from those of the insulator with our phase-sensitive measurements.

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