arXiv subjects

Alicia Sit

Publications and source records attributed to Alicia Sit.

18 recordsLinked to original sources

arXiv2025

Ultrafast switching of telecom photon-number states

A crucial component of photonic quantum information processing platforms is the ability to modulate, route, convert, and switch quantum states of light noiselessly with low insertion loss. For instance, a high-speed, low-loss optical switch is crucial for scaling quantum photonic systems that rely on measurement-based feed-forward approaches. Such a device will also ideally be capable of operating on photon-number states, which can act as non-Gaussian resources. Here, we demonstrate ultrafast all-optical switching of heralded photon-number states, of up to 6 photons, using the optical Kerr effect in a single-mode fiber. A local birefringence is created by a high-intensity pump pulse at a center wavelength of 1030 nm which overlaps temporally with the 1550 nm photons in the fiber. A switching efficiency of $>$99 % is reached with a resolution of 2.3 ps, an insertion loss of $2.27\pm0.08$ dB, and a signal-to-noise ratio of 32,000.

quant-ph↗

arXiv2025

Ultrafast all-optical modulation of spatially structured photons

Manipulating the structure of single photons in the ultrafast domain is enabling new quantum information processing technologies. At the picosecond timescale, quantum information can be processed before decoherence can occur. In this work, we study the capabilities of few-mode cross-phase modulation via the optical Kerr effect, using ultrafast pulses. We observe a significant modulation in the spatial mode of structured photons on timescales $\leq 1.3$~ps.

quant-ph↗

arXiv2025

Terahertz electro-optic modulation of single photons

The manipulation of visible and near-infrared light at the single-photon level plays a key role in quantum communication systems where information is encoded into photonic degrees of freedom. In practical implementations, it is important to achieve this manipulation with high speeds, low loss, and low noise. In this work, we propose the use of terahertz~(THz) electric fields as a pump source for electro-optic modulation of single photons in bulk media. We demonstrate spectral modulations of single photons in the form of frequency translation and bandwidth manipulations as the terahertz field imparts linear and quadratic phases on the photons at various time delays within 1~ps. Our results show frequency translations exceeding 500~GHz at multi-THz modulation speeds and loss levels of $\approx$1~dB, complementing the current state-of-the-art electro-optic modulation techniques limited to speeds up to 100~GHz. The proposed approach leverages recent developments in terahertz generation techniques, introducing new avenues to manipulate non-classical light in an unexplored regime for quantum photonics.

quant-ph↗

arXiv2024

A genetic algorithm for the response of twisted nematic liquid crystals to an applied field

When an external field is applied across a liquid-crystal cell, the twist and tilt distributions cannot be calculated analytically and must be extracted numerically. In the standard approach, the Euler-Lagrange equations are derived from the minimization of the free energy of the system and then solved via finite-difference methods, often implemented in commercial software. These tools iterate from initial solutions that are compatible with the boundary conditions, providing limited to no flexibility for customization. Here, we present a genetic algorithm that outputs fast and accurate solutions to the integral form of the equations. In our approach, the evolutionary routine is sequentially applied at each position within the bulk of the cell, thus overcoming the necessity of assuming trial solutions. The predictions of our routine strongly support the experimental observations on different instances of spatially varying twisted nematic liquid-crystal cells, patterned with different topologies on the two alignment layers.

physics.comp-ph↗

arXiv2023

Spatially twisted liquid-crystal devices

Nematic liquid-crystal devices are a powerful tool to structure light in different degrees of freedom, both in classical and quantum regimes. Most of these devices exploit either the possibility of introducing a position-dependent phase retardation with a homogeneous alignment of the optic axis -- e.g., liquid-crystal-based spatial light modulators -- or conversely, with a uniform but tunable retardation and patterned optic axis, e.g., $q$-plates. The pattern is the same in the latter case on the two alignment layers. Here, a more general case is considered, wherein the front and back alignment layers are patterned differently. This creates a non-symmetric device which can exhibit different behaviours depending on the direction of beam propagation and effective phase retardation. In particular, we fabricate multi-$q$-plates by setting different topological charges on the two alignment layers. The devices have been characterized by spatially resolved Stokes polarimetry, with and without applied electric voltage, demonstrating new functionalities.

physics.optics↗

arXiv2023

Full spatial characterization of entangled structured photons

Vector beams (VBs) are fully polarized beams with spatially varying polarization distributions, and they have found widespread use in numerous applications such as microscopy, metrology, optical trapping, nano-photonics, and communications. The entanglement of such beams has attracted significant interest, and it has been shown to have tremendous potential in expanding existing applications and enabling new ones. However, due to the complex spatially varying polarization structure of entangled VBs (EVBs), a complete entanglement characterization of these beams remains challenging and time-consuming. Here, we have used a time-tagging event camera to demonstrate the ability to simultaneously characterize approximately $2.6\times10^6$ modes between a bi-partite EVB using only 16 measurements. This achievement is an important milestone in high-dimensional entanglement characterization of structured light, and it could significantly impact the implementation of related quantum technologies. The potential applications of this technique are extensive, and it could pave the way for advancements in quantum communication, quantum imaging, and other areas where structured entangled photons play a crucial role.

quant-ph↗

arXiv2021

Polychromatic Electric Field Knots

The polarization of a monochromatic optical beam lies in a plane, and in general, is described by an ellipse, known as the polarization ellipse. The polarization ellipse in the tight focusing (non-paraxial) regime forms non-trivial three-dimensional topologies, such as Möbius and ribbon strips, as well as knots. The latter is formed when the dynamics of specific polarization states, e.g., circular polarization states, are studied upon propagation. However, there is an alternative method to generate optical knots: the electric field's tip can be made to evolve along a knot trajectory in time locally. We propose an intuitive technique to generate and engineer the path traced by the electric field vector of polychromatic beams to form different knots. In particular, we show examples of how tightly focused beams with at least three frequency components and different spatial modes can cause the tip of the electric field vector to follow, locally, a knotted trajectory. Furthermore, we characterize the generated knots and explore different knot densities upon free-space propagation in the focal volume. Our study may provide insight for designing current densities when structured polychromatic electromagnetic fields interact with materials.

physics.optics↗

arXiv2020

Two-photon interference: the Hong-Ou-Mandel effect

Nearly 30 years ago, two-photon interference was observed, marking the beginning of a new quantum era. Indeed, two-photon interference has no classical analogue, giving it a distinct advantage for a range of applications. The peculiarities of quantum physics may now be used to our advantage to outperform classical computations, securely communicate information, simulate highly complex physical systems and increase the sensitivity of precise measurements. This separation from classical to quantum physics has motivated physicists to study two-particle interference for both fermionic and bosonic quantum objects. So far, two-particle interference has been observed with massive particles, among others, such as electrons and atoms, in addition to plasmons, demonstrating the extent of this effect to larger and more complex quantum systems. A wide array of novel applications to this quantum effect is to be expected in the future. This review will thus cover the progress and applications of two-photon (two-particle) interference over the last three decades.

quant-ph↗

arXiv2020

Orbital angular momentum and energy loss characterization of plasmonic excitations in metallic nanostructures in TEM

Recently, a new device to measure the Orbital Angular Momentum (OAM) electronic spectrum after elastic/inelastic scattering in a transmission electron microscope has been introduced. We modified the theoretical framework needed to describe conventional low loss electron energy loss spectroscopy (EELS) experiments in transmission electron microscopes (TEM) to study surface plasmons in metallic nanostructures, to allow for an OAM post selection and devise new experiments for the analysis of these excitations in nanostructures. We found that unprecedented information on the symmetries and on the chirality of the plasmonic modes can be retrieved even with limited OAM and energy resolutions.

physics.ins-det↗

arXiv2020

Underwater quantum communication over a 30-meter flume tank

Underwater quantum communication has recently been explored using polarization and orbital angular momentum. Here, we show that spatially structured modes, e.g., a coherent superposition of beams carrying both polarization and orbital angular momentum, can also be used for underwater quantum cryptography. We also use the polarization degree of freedom for quantum communication in an underwater channel having various lengths, up to $30$ meters. The underwater channel proves to be a difficult environment for establishing quantum communication as underwater optical turbulence results in significant beam wandering and distortions. However, the errors associated to the turbulence do not result in error rates above the threshold for establishing a positive key in a quantum communication link with both the polarization and spatially structured photons. The impact of the underwater channel on the spatially structured modes is also investigated at different distances using polarization tomography.

quant-ph↗

arXiv2019

Characterization of an underwater channel for quantum communications in the Ottawa River

We examine the propagation of optical beams possessing different polarization states and spatial modes through the Ottawa River in Canada. A Shack-Hartmann wavefront sensor is used to record the distorted beam's wavefront. The turbulence in the underwater channel is analysed, and associated Zernike coefficients are obtained in real-time. Finally, we explore the feasibility of transmitting polarization states as well as spatial modes through the underwater channel for applications in quantum cryptography.

quant-ph↗

arXiv2019

Quantum process tomography of a high-dimensional quantum communication channel

The characterization of quantum processes, e.g. communication channels, is an essential ingredient for establishing quantum information systems. For quantum key distribution protocols, the amount of overall noise in the channel determines the rate at which secret bits are distributed between authorized partners. In particular, tomographic protocols allow for the full reconstruction, and thus characterization, of the channel. Here, we perform quantum process tomography of high-dimensional quantum communication channels with dimensions ranging from 2 to 5. We can thus explicitly demonstrate the effect of an eavesdropper performing an optimal cloning attack or an intercept-resend attack during a quantum cryptographic protocol. Moreover, our study shows that quantum process tomography enables a more detailed understanding of the channel conditions compared to a coarse-grained measure, such as quantum bit error rates. This full characterization technique allows us to optimize the performance of quantum key distribution under asymmetric experimental conditions, which is particularly useful when considering high-dimensional encoding schemes.

quant-ph↗

arXiv2018

Interaction-Free Ghost-Imaging of Structured Objects

Quantum - or classically correlated - light can be employed in various ways to improve resolution and measurement sensitivity. In an "interaction-free" measurement, a single photon can be used to reveal the presence of an object placed within one arm of an interferometer without being absorbed by it. This method has previously been applied to imaging. With a technique known as "ghost imaging", entangled photon pairs are used for detecting an opaque object with significantly improved signal-to-noise ratio while preventing over-illumination. Here, we integrate these two methods to obtain a new imaging technique which we term "interaction-free ghost-imaging" that possesses the benefits of both techniques. While maintaining the image quality of conventional ghost-imaging, this new technique is also sensitive to phase and polarisation changes in the photons introduced by a structured object. Furthermore, thanks to the "interaction-free" nature of this new technique, it is possible to reduce the number of photons required to produce a clear image of the object (which could be otherwise damaged by the photons) making this technique superior for probing light-sensitive materials and biological tissues.

quant-ph↗

arXiv2018

Round-Robin Differential Phase-Shift Quantum Key Distribution with Twisted Photons

Quantum key distribution (QKD) offers the possibility for two individuals to communicate a securely encrypted message. From the time of its inception in 1984 by Bennett and Brassard, QKD has been the result of intense research. One technical challenge is the monitoring of signal disturbance in a QKD system to bound the information leakage towards an unwanted eavesdropper. Recently, the round-robin differential phase-shift (RRDPS) protocol, which encodes bits of information in a high-dimensional state space, was proposed to solve this exact problem. Since its introduction, many realizations of the RRDPS protocol were demonstrated using trains of coherent pulses. Here, we propose and experimentally demonstrate an implementation of the RRDPS protocol using the photonic orbital angular momentum degree of freedom. In particular, we show that Alice's generation stage and Bob's detection stage can each be reduced to a single phase element, greatly simplifying its implementation. Our scheme offers a practical demonstration of the RRDPS protocol which will suppress the need for monitoring signal disturbance in free-space channels.

quant-ph↗

arXiv2018

Underwater Quantum Key Distribution in Outdoor Conditions with Twisted Photons

Quantum communication has been successfully implemented in optical fibres and through free-space [1-3]. Fibre systems, though capable of fast key rates and low quantum bit error rates (QBERs), are impractical in communicating with destinations without an established fibre link [4]. Free-space quantum channels can overcome such limitations and reach long distances with the advent of satellite-to-ground links [5-8]. Shorter line-of-sight free-space links have also been realized for intra-city conditions [2, 9]. However, turbulence, resulting from local fluctuations in refractive index, becomes a major challenge by adding errors and losses [10]. Recently, an interest in investigating the possibility of underwater quantum channels has arisen, which could provide global secure communication channels among submersibles and boats [11-13]. Here, we investigate the effect of turbulence on an underwater quantum channel using twisted photons in outdoor conditions. We study the effect of turbulence on transmitted QBERs, and compare different QKD protocols in an underwater quantum channel showing the feasibility of high-dimensional encoding schemes. Our work may open the way for secure high-dimensional quantum communication between submersibles, and provides important input for potential submersibles-to-satellite quantum communication.

quant-ph↗

arXiv2017

General Lossless Spatial Polarization Transformations

Liquid crystals allow for the real-time control of the polarization of light. We describe and provide some experimental examples of the types of general polarization transformations, including universal polarization transformations, that can be accomplished with liquid crystals in tandem with fixed waveplates. Implementing these transformations with an array of liquid crystals, e.g., a spatial light modulator, allows for the manipulation of the polarization across a beam's transverse plane. We outline applications of such general spatial polarization transformations in the generation of exotic types of vector polarized beams, a polarization magnifier, and the correction of polarization aberrations in light fields.

physics.optics↗

arXiv2017

Nondestructive Measurement of Orbital Angular Momentum for an Electron Beam

Free electrons with a helical phase front, referred to as "twisted" electrons, possess an orbital angular momentum (OAM) and, hence, a quantized magnetic dipole moment along their propagation direction. This intrinsic magnetic moment can be used to probe material properties. Twisted electrons thus have numerous potential applications in materials science. Measuring this quantity often relies on a series of projective measurements that subsequently change the OAM carried by the electrons. In this Letter, we propose a nondestructive way of measuring an electron beam's OAM through the interaction of this associated magnetic dipole with a conductive loop. Such an interaction results in the generation of induced currents within the loop, which are found to be directly proportional to the electron's OAM value. Moreover, the electron experiences no OAM variations and only minimal energy losses upon the measurement, and, hence, the nondestructive nature of the proposed technique.

quant-ph↗

arXiv2016

High-Dimensional Intra-City Quantum Cryptography with Structured Photons

Quantum key distribution (QKD) promises information-theoretically secure communication, and is already on the verge of commercialization. Thus far, different QKD protocols have been proposed theoretically and implemented experimentally [1, 2]. The next step will be to implement high-dimensional protocols in order to improve noise resistance and increase the data rate [3-7]. Hitherto, no experimental verification of high-dimensional QKD in the single-photon regime has been conducted outside of the laboratory. Here, we report the realization of such a single-photon QKD system in a turbulent free-space link of 0.3 km over the city of Ottawa, taking advantage of both the spin and orbital angular momentum photonic degrees of freedom. This combination of optical angular momenta allows us to create a 4-dimensional state [8]; wherein, using a high-dimensional BB84 protocol [3, 4], a quantum bit error rate of 11\% was attained with a corresponding secret key rate of 0.65 bits per sifted photon. While an error rate of 5\% with a secret key rate of 0.43 bits per sifted photon is achieved for the case of 2-dimensional structured photons. Even through moderate turbulence without active wavefront correction, it is possible to securely transmit information carried by structured photons, opening the way for intra-city high-dimensional quantum communications under realistic conditions.

quant-ph↗