arXiv subjects

Alisa Javadi

Publications and source records attributed to Alisa Javadi.

34 records · Page 2Linked to original sources

arXiv2021

Suppression of surface-related loss in a gated semiconductor microcavity

We present a surface passivation method that reduces surface-related losses by almost two orders of magnitude in a highly miniaturized GaAs open microcavity. The microcavity consists of a curved dielectric distributed Bragg reflector (DBR) with radius $\sim 10$ $μ$m paired with a GaAs-based heterostructure. The heterostructure consists of a semiconductor DBR followed by an n-i-p diode with a layer of quantum dots in the intrinsic region. Free-carrier absorption in the highly doped n- and p-layers is minimized by positioning them close to a node of the vacuum electromagnetic-field. The surface, however, resides at an anti-node of the vacuum field and results in significant loss. These losses are much reduced by surface passivation. The strong dependence on wavelength implies that the main effect of the surface passivation is to eliminate the surface electric field, thereby quenching below-bandgap absorption via a Franz-Keldysh-like effect. An additional benefit is that the surface passivation reduces scattering at the GaAs surface. These results are important in other nano-photonic devices which rely on a GaAs-vacuum interface to confine the electromagnetic field.

physics.optics↗

arXiv2021

Radiative Auger Process in the Single-Photon Limit

In a multi-electron atom, an excited electron can decay by emitting a photon. Typically, the leftover electrons are in their ground state. In a radiative Auger process, the leftover electrons are in an excited state and a redshifted photon is created. In a semiconductor quantum dot, radiative Auger is predicted for charged excitons. Here we report the observation of radiative Auger on trions in single quantum dots. For a trion, a photon is created on electron-hole recombination, leaving behind a single electron. The radiative Auger process promotes this additional (Auger) electron to a higher shell of the quantum dot. We show that the radiative Auger effect is a powerful probe of this single electron: the energy separations between the resonance fluorescence and the radiative Auger emission directly measure the single-particle splittings of the electronic states in the quantum dot with high precision. In semiconductors, these single-particle splittings are otherwise hard to access by optical means as particles are excited typically in pairs, as excitons. After the radiative Auger emission, the Auger carrier relaxes back to the lowest shell. Going beyond the original theoretical proposals, we show how applying quantum optics techniques to the radiative Auger photons gives access to the single-electron dynamics, notably relaxation and tunneling. This is also hard to access by optical means: even for quasi-resonant $p$-shell excitation, electron relaxation takes place in the presence of a hole, complicating the relaxation dynamics. The radiative Auger effect can be exploited in other semiconductor nanostructures and quantum emitters in the solid state to determine the energy levels and the dynamics of a single carrier.

cond-mat.mes-hall↗

arXiv2020

Narrow optical linewidths and spin pumping on charge-tunable, close-to-surface self-assembled quantum dots in an ultra-thin diode

We demonstrate full charge control, narrow optical linewidths, and optical spin pumping on single self-assembled InGaAs quantum dots embedded in a $162.5\,\text{nm}$ thin diode structure. The quantum dots are just $88\,\text{nm}$ from the top GaAs surface. We design and realize a p-i-n-i-n diode that allows single-electron charging of the quantum dots at close-to-zero applied bias. In operation, the current flow through the device is extremely small resulting in low noise. In resonance fluorescence, we measure optical linewidths below $2\,μ\text{eV}$, just a factor of two above the transform limit. Clear optical spin pumping is observed in a magnetic field of $0.5\,\text{T}$ in the Faraday geometry. We present this design as ideal for securing the advantages of self-assembled quantum dots -- highly coherent single photon generation, ultra-fast optical spin manipulation -- in the thin diodes required in quantum nano-photonics and nano-phononics applications.

cond-mat.mes-hall↗

arXiv2020

Low-Noise GaAs Quantum Dots for Quantum Photonics

Quantum dots are both excellent single-photon sources and hosts for single spins. This combination enables the deterministic generation of Raman-photons -- bandwidth-matched to an atomic quantum-memory -- and the generation of photon cluster states, a resource in quantum communication and measurement-based quantum computing. GaAs quantum dots in AlGaAs can be matched in frequency to a rubidium-based photon memory, and have potentially improved electron spin coherence compared to the widely used InGaAs quantum dots. However, their charge stability and optical linewidths are typically much worse than for their InGaAs counterparts. Here, we embed GaAs quantum dots into an $n$-$i$-$p$-diode specially designed for low-temperature operation. We demonstrate ultra-low noise behaviour: charge control via Coulomb blockade, close-to lifetime-limited linewidths, and no blinking. We observe high-fidelity optical electron-spin initialisation and long electron-spin lifetimes for these quantum dots. Our work establishes a materials platform for low-noise quantum photonics close to the red part of the spectrum.

cond-mat.mes-hall↗

arXiv2020

A bright and fast source of coherent single photons

A single photon source is a key enabling technology in device-independent quantum communication, quantum simulation for instance boson sampling, linear optics-based and measurement-based quantum computing. These applications involve many photons and therefore place stringent requirements on the efficiency of single photon creation. The scaling on efficiency is an exponential function of the number of photons. Schemes taking full advantage of quantum superpositions also depend sensitively on the coherence of the photons, i.e. their indistinguishability. It is therefore crucial to maintain the coherence over long strings of photons. Here, we report a single photon source with an especially high system efficiency: a photon is created on-demand at the output of the final optical fibre with a probability of 57%. The coherence of the photons is very high and is maintained over a stream consisting of thousands of photons; the repetition rate is in the GHz regime. We break with the established semiconductor paradigms, such as micropillars, photonic crystal cavities and waveguides. Instead, we employ gated quantum dots in an open, tunable microcavity. The gating ensures low-noise operation; the tunability compensates for the lack of control in quantum dot position and emission frequency; the output is very well-matched to a single-mode fibre. An increase in efficiency over the state-of-the-art by more than a factor of two, as reported here, will result in an enormous decrease in run-times, by a factor of $10^{7}$ for 20 photons.

quant-ph↗

arXiv2020

A coherent spin-photon interface with waveguide induced cycling transitions

Solid-state quantum dots are promising candidates for efficient light-matter interfaces connecting internal spin degrees of freedom to the states of emitted photons. However, selection rules prevent the combination of efficient spin control and optical cyclicity in this platform. By utilizing a photonic crystal waveguide we here experimentally demonstrate optical cyclicity up to $\approx15$ through photonic state engineering while achieving high fidelity spin initialization and coherent optical spin control. These capabilities pave the way towards scalable multi-photon entanglement generation and on-chip spin-photon gates.

quant-ph↗

arXiv2019

A wave-function ansatz method for calculating field correlations and its application to the study of spectral filtering and quantum dynamics of multi-emitter systems

We develop a formalism based on a time-dependent wave-function ansatz to study correlations of photons emitted from a collection of two-level quantum emitters. We show how to simulate the system dynamics and evaluate the intensity of the scattered photons and the second-order correlation function $g^{(2)}$ in terms of the amplitudes of the different components of the wave function. Our approach is efficient for considering systems that contain up to two excitations. To demonstrate this we first consider the example of spectral filtering of photons emitted from a single quantum emitter. We show how our formalism can be used to study spectral filtering of the two-photon component of the emitted light from a single quantum emitter for various kinds of filters. Furthermore, as a general application of our formalism, we show how it can be used to study photon-photon correlations in an optically dense ensemble of two-level quantum emitters. In particular we lay out the details of simulating correlated photon transport in such ensembles reported recently by S. Mahmoodian {\it et.al.} [Phys. Rev. Lett. {\bf 121}, 143601 (2018)]. Compared to other existing techniques, the advantage of our formalism is that it is applicable to any generic spectral filter and quantum many-body systems involving a large number of quantum emitters while requiring only a modest computational resource.

quant-ph↗

arXiv2018

Coherent optical control of a quantum-dot spin-qubit in a waveguide-based spin-photon interface

Waveguide-based spin-photon interfaces on the GaAs platform have emerged as a promising system for a variety of quantum information applications directly integrated into planar photonic circuits. The coherent control of spin states in a quantum dot can be achieved by applying circularly polarized laser pulses that may be coupled into the planar waveguide vertically through radiation modes. However, proper control of the laser polarization is challenging since the polarization is modified through the transformation from the far field to the exact position of the quantum dot in the nanostructure. Here we demonstrate polarization-controlled excitation of a quantum-dot electron spin and use that to perform coherent control in a Ramsey interferometry experiment. The Ramsey interference reveals a pure dephasing time of $ 2.2\pm0.1 $ ns, which is comparable to the values so far only obtained in bulk media. We analyze the experimental limitations in spin initialization fidelity and Ramsey contrast and identify the underlying mechanisms.

quant-ph↗

arXiv2018

Quantum optics with near lifetime-limited quantum-dot transitions in a nanophotonic waveguide

Establishing a highly efficient photon-emitter interface where the intrinsic linewidth broadening is limited solely by spontaneous emission is a key step in quantum optics. It opens a pathway to coherent light-matter interaction for, e.g., the generation of highly indistinguishable photons, few-photon optical nonlinearities, and photon-emitter quantum gates. However, residual broadening mechanisms are ubiquitous and need to be combated. For solid-state emitters charge and nuclear spin noise is of importance and the influence of photonic nanostructures on the broadening has not been clarified. We present near lifetime-limited linewidths for quantum dots embedded in nanophotonic waveguides through a resonant transmission experiment. It is found that the scattering of single photons from the quantum dot can be obtained with an extinction of $66 \pm 4 \%$, which is limited by the coupling of the quantum dot to the nanostructure rather than the linewidth broadening. This is obtained by embedding the quantum dot in an electrically-contacted nanophotonic membrane. A clear pathway to obtaining even larger single-photon extinction is laid out, i.e., the approach enables a fully deterministic and coherent photon-emitter interface in the solid state that is operated at optical frequencies.

quant-ph↗

arXiv2017

Indistinguishable and efficient single photons from a quantum dot in a planar nanobeam waveguide

We demonstrate a high-purity source of indistinguishable single photons using a quantum dot embedded in a nanophotonic waveguide. The source features a near-unity internal coupling efficiency and the collected photons are efficiently coupled off-chip by implementing a taper that adiabatically couples the photons to an optical fiber. By quasi-resonant excitation of the quantum dot, we measure a single-photon purity larger than 99.4% and a photon indistinguishability of up to 94+-1% by using p-shell excitation combined with spectral filtering to reduce photon jitter. A temperature-dependent study allows pinpointing the residual decoherence processes notably the effect of phonon broadening. Strict resonant excitation is implemented as well as another mean of suppressing photon jitter, and the additional complexity of suppressing the excitation laser source is addressed. The study opens a clear pathway towards the long-standing goal of a fully deterministic source of indistinguishable photons, which is integrated on a planar photonic chip.

quant-ph↗

arXiv2017

Two mechanisms of disorder-induced localization in photonic-crystal waveguides

Unintentional but unavoidable fabrication imperfections in state-of-the-art photonic-crystal waveguides lead to the spontaneous formation of Anderson-localized modes thereby limiting slowlight propagation and its potential applications. On the other hand, disorder-induced cavities offer an approach to cavity-quantum electrodynamics and random lasing at the nanoscale. The key statistical parameter governing the disorder effects is the localization length, which together with the waveguide length determines the statistical transport of light through the waveguide. In a disordered photonic-crystal waveguide, the localization length is highly dispersive, and therefore, by controlling the underlying lattice parameters, it is possible to tune the localization of the mode. In the present work, we study the localization length in a disordered photonic-crystal waveguide using numerical simulations. We demonstrate two different localization regimes in the dispersion diagram where the localization length is linked to the density of states and the photon effective mass, respectively. The two different localization regimes are identified in experiments by recording the photoluminescence from quantum dots embedded in photonic-crystal waveguides.

physics.optics↗

arXiv2017

Spin-photon interface and spin-controlled photon switching in a nanobeam waveguide

Access to the electron spin is at the heart of many protocols for integrated and distributed quantum-information processing [1-4]. For instance, interfacing the spin-state of an electron and a photon can be utilized to perform quantum gates between photons [2,5] or to entangle remote spin states [6-9]. Ultimately, a quantum network of entangled spins constitutes a new paradigm in quantum optics [1]. Towards this goal, an integrated spin-photon interface would be a major leap forward. Here we demonstrate an efficient and optically programmable interface between the spin of an electron in a quantum dot and photons in a nanophotonic waveguide. The spin can be deterministically prepared with a fidelity of 96\%. Subsequently the system is used to implement a "single-spin photonic switch", where the spin state of the electron directs the flow of photons through the waveguide. The spin-photon interface may enable on-chip photon-photon gates [2], single-photon transistors [10], and efficient photonic cluster state generation [11].

quant-ph↗

arXiv2017

Numerical modelling of the coupling efficiency of single quantum emitters in photonic-crystal waveguides

Planar photonic nanostructures have recently attracted a great deal of attention for quantum optics applications. In this article, we carry out full 3D numerical simulations to fully account for all radiation channels and thereby quantify the coupling efficiency of a quantum emitter embedded in a photonic-crystal waveguide. We utilize mixed boundary conditions by combining active Dirichlet boundary conditions for the guided mode and perfectly-matched layers for the radiation modes. In this way, the leakage from the quantum emitter to the surrounding environment can be determined and the spectral and spatial dependence of the coupling to the radiation modes can be quantified. The spatial maps of the coupling efficiency, the $β$-factor, reveal that even for moderately slow light, near-unity $β$ is achievable that is remarkably robust to the position of the emitter in the waveguide. Our results show that photonic-crystal waveguides constitute a suitable platform to achieve deterministic interfacing of a single photon and a single quantum emitter, which has a range of applications for photonic quantum technology.

quant-ph↗

arXiv2015

Theory and experiments of disorder-induced resonance shifts and mode edge broadening in deliberately disordered photonic crystal waveguides

We study both theoretically and experimentally the effects of introducing deliberate disorder in a slow-light photonic crystal waveguide on the photon density of states. We first introduce a theoretical model that includes both deliberate disorder through statistically moving the hole centres in the photonic crystal lattice and intrinsic disorder caused by manufacturing imperfections. We demonstrate a disorder-induced mean blueshift and an overall broadening of the photonic density of states for various amounts of deliberate disorder. By comparing with measurements from a GaAs photonic crystal waveguide, we find good qualitative agreement between theory and experiment which highlights the importance of carefully including local field effects for modelling high-index contrast perturbations. Our work also demonstrates the importance of using asymmetric dielectric polarizabilities for modelling positive and negative dielectric perturbations when modelling a perturbed dielectric interface in photonic crystal platforms.

physics.optics↗

arXiv2015

Deterministic photon-emitter coupling in chiral photonic circuits

The ability to engineer photon emission and photon scattering is at the heart of modern photonics applications ranging from light harvesting, through novel compact light sources, to quantum-information processing based on single photons. Nanophotonic waveguides are particularly well suited for such applications since they confine photon propagation to a 1D geometry thereby increasing the interaction between light and matter. Adding chiral functionalities to nanophotonic waveguides lead to new opportunities enabling integrated and robust quantum-photonic devices or the observation of novel topological photonic states. In a regular waveguide, a quantum emitter radiates photons in either of two directions, and photon emission and absorption are reverse processes. This symmetry is violated in nanophotonic structures where a non-transversal local electric field implies that both photon emission and scattering may become directional. Here we experimentally demonstrate that the internal state of a quantum emitter determines the chirality of single-photon emission in a specially engineered photonic-crystal waveguide. Single-photon emission into the waveguide with a directionality of more than 90\% is observed under conditions where practically all emitted photons are coupled to the waveguide. Such deterministic and highly directional photon emission enables on-chip optical diodes, circulators operating at the single-photon level, and deterministic quantum gates. Based on our experimental demonstration, we propose an experimentally achievable and fully scalable deterministic photon-photon CNOT gate, which so far has been missing in photonic quantum-information processing where most gates are probabilistic.

quant-ph↗

arXiv2013

Statistical measurements of quantum emitters coupled to Anderson-localized modes in disordered photonic-crystal waveguides

Optical nanostructures have proven to be meritorious for tailoring the emission properties of quantum emitters. However, unavoidable fabrication imperfections may represent a nuisance. Quite remarkably, disorder offers new opportunities since light can be efficiently confined by random multiple scattering leading to Anderson localization. Here we investigate the effect of such disorder-induced cavities on the emission dynamics of single quantum dots embedded in disordered photonic-crystal waveguides. We present time-resolved measurements of both the total emission from Anderson-localized cavities and from single emitters that are coupled to the cavities. We observe both strongly inhibited and enhanced decay rates relative to the rate of spontaneous emission in a homogeneous medium. From a statistical analysis, we report an average Purcell factor of 2 in without any control on the quantum dot - cavity detuning. By spectrally tuning individual quantum dots into resonance with Anderson-localized modes, a maximum Purcell factor of 23.8 is recorded, which lies at the onset of the strong coupling regime. The presented data quantify the potential of naturally occurring Anderson-localized cavities for controlling and enhancing the light-matter interaction strength, which is of relevance not only for cavity quantum-electrodynamics experiments but potentially also for efficient energy harvesting and controllable random lasing.

physics.optics↗