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Allan S. Johnson

Publications and source records attributed to Allan S. Johnson.

21 records · Page 2Linked to original sources

Direct characterisation of tuneable few-femtosecond dispersive-wave pulses in the deep UV

Dispersive wave emission (DWE) in gas-filled hollow-core dielectric waveguides is a promising source of tuneable coherent and broadband radiation, but so far the generation of few-femtosecond pulses using this technique has not been demonstrated. Using in-vacuum frequency-resolved optical gating, we directly characterise tuneable 3fs pulses in the deep ultraviolet generated via DWE. Through numerical simulations, we identify that the use of a pressure gradient in the waveguide is critical for the generation of short pulses.

physics.optics↗

Practical Witness for Electronic Coherences

The origin of the coherences in two-dimensional spectroscopy of photosynthetic complexes remains disputed. Recently it has been shown that in the ultrashort-pulse limit, oscillations in a frequency-integrated pump-probe signal correspond exclusively to electronic coherences, and thus such experiments can be used to form a test for electronic vs. vibrational oscillations in such systems. Here we demonstrate a method for practically implementing such a test, whereby pump-probe signals are taken at several different pulse durations and used to extrapolate to the ultrashort-pulse limit. We present analytic and numerical results determining requirements for pulse durations and the optimal choice of pulse central frequency, which can be determined from an absorption spectrum. Our results suggest that for numerous systems the required experiment could be implemented by many ultrafast spectroscopy laboratories using pulses of tens of femtoseconds in duration. Such experiments could resolve the standing debate over the nature of coherences in photosynthetic complexes.

quant-ph↗

Full characterisation of polarisation states of light via direct measurement

Ascertaining the physical state of a system is vital in order to understand and predict its behaviour. Tomography is a standard approach used to determine the form of an unknown state. Here we show that an alternative approach, based on sequential weak and strong measurements, can be used to determine the density matrix in a simple, fast, and general style. We directly measure the probability amplitudes of a variety of pure polarisation states of light. We then generalise this experiment to directly measure the Dirac distribution and consequently determine the density matrix. Our work is the first to demonstrate the direct measurement of the full description of the state of a two-dimensional system, and it has applications to measurements in foundational quantum mechanics, quantum information, and physical chemistry.

quant-ph↗