arXiv subjects

Alvaro Bermejillo-Seco

Publications and source records attributed to Alvaro Bermejillo-Seco.

6 recordsLinked to original sources

arXiv2026

Strain-controlled magnetism and magnetoelasticity in monolayer NiPS$_3$ and CrPS$_4$

We develop a first-principles framework for magnetoelastic coupling in two-dimensional magnets based on a strain-dependent Heisenberg model. In this approach, strain derivatives of the exchange interactions provide direct access to magnetostriction and to the magnetic renormalization of the elastic tensor, establishing a microscopic link between spin interactions and elastic response. We apply the method to monolayer NiPS$_3$ and CrPS$_4$, which exhibit contrasting magnetoelastic behavior. NiPS$_3$ shows weak and nearly isotropic spin-lattice coupling, consistent with a robust zigzag antiferromagnetic ground state. In contrast, CrPS$_4$ displays strong anisotropic coupling, leading to strain-driven transitions between spin-spiral and ferromagnetic phases and significant changes in the critical temperature and elastic response. Our results demonstrate a general route to quantify magnetoelastic effects in low-dimensional magnets and highlight CrPS$_4$ as a promising platform for strain engineering of magnetic order.

cond-mat.mtrl-sci↗

arXiv2026

Magnetic ground states of CrPS$_4$ and NiPS$_3$ monolayers from long-range exchange interactions

We investigate the magnetic properties of monolayer CrPS$_4$ and NiPS$_3$ by combining first-principles calculations, second-principles spin models, and Monte Carlo simulations. Unlike conventional approaches that truncate exchange interactions after only a few shells and determine them by fitting total energies, we extract the magnetic exchange tensors directly from density functional theory using the LKAG formalism and include interactions until numerical convergence is achieved. We show that long-range exchange interactions qualitatively modify the magnetic behavior of both materials. In CrPS$_4$, they destabilize the previously predicted ferromagnetic ground state and stabilize a spin-spiral phase, reducing the critical temperature to about 21\,K, in agreement with available experiments. The resulting magnetic phase diagram contains multiple collinear and non-collinear phases that can be tuned by temperature and external magnetic fields. In NiPS$_3$, the experimentally observed zigzag antiferromagnetic order only emerges when exchange interactions up to the fifth shell are included. These results demonstrate that quantitatively predictive spin models for thiophosphate monolayers require long-range exchange interactions and provide a predictive framework for accurately describing two-dimensional van der Waals magnets.

cond-mat.mtrl-sci↗

arXiv2026

Magnon polaritons in a van der Waals ferromagnet coupled to a superconducting resonator

Achieving magnon-photon hybridization in the microwave regime is essential for integrating magnetic excitations with superconducting circuits. While this has been extensively demonstrated in bulk magnetic systems, realizing it in two-dimensional van der Waals materials remains challenging due to their reduced magnetic volume and increased dissipation. Here, magnon-photon hybridization is observed in exfoliated flakes of the van der Waals ferromagnet Cr$_2$Ge$_2$Te$_6$, with thicknesses down to 30 nm. The resulting magnon polaritons-hybrid excitations of cavity photons and magnons-are evidenced by reproducible avoided crossings across six devices, enabled by a low-impedance superconducting resonator design. The coupling strength follows the expected square-root dependence on thickness, and extrapolation of this scaling indicates that hybridization in the monolayer limit is within reach.

cond-mat.mes-hall↗

arXiv2026

Magnomechanical Coupling in Suspended 2D van der Waals Ferromagnets

Magnomechanical systems provide a promising route for exploring coherent hybrid magnon-phonon interactions and hybrid information processing, but their realization has so far been limited by weak magnon-phonon coupling in conventional bulk platforms. We show that a suspended membrane of a two-dimensional van der Waals ferromagnet with in-plane magnetization and out-of-plane mechanical oscillations exhibits large magnomechanical coupling dominated by magnetoelastic interactions. The parametric single magnon-phonon coupling rate scales linearly with pre-strain and can reach hundreds of Hertz to low kiloHertz in suspended membranes of van der Waals ferromagnets such as CrGeTe_3 under experimentally realistic conditions. This rate exceeds typical values reported for YIG spheres by more than three orders of magnitude. Our results demonstrate that suspended membranes of van der Waals magnets provide a robust and highly tunable platform for magnomechanics.

cond-mat.mes-hall↗

arXiv2025

Magnon-magnon interaction induced by nonlinear spin wave dynamics

We experimentally and theoretically demonstrate that nonlinear spin-wave dynamics can induce an effective resonant interaction between non-resonant magnon modes in a yttrium iron garnet disk. Under strong pumping near the ferromagnetic resonance mode, we observe a spectral splitting that emerges with increasing drive amplitude. This phenomenon is well captured by a theoretical framework based on the linearization of a magnon three-wave mixing Hamiltonian, which at high power leads to parametric Suhl instabilities. The access and control of nonlinear magnon-parametric processes enables the development of experimental platforms in an unexplored parameter regime for both classical and quantum computation protocols.

cond-mat.mes-hall↗

arXiv2025

Thermoelastic Damping Across the Phase Transition in van der Waals Magnets

A quantitative understanding of the microscopic mechanisms responsible for damping in van der Waals nanomechanical resonators remains elusive. In this work, we investigate van der Waals magnets, where the thermal expansion coefficient exhibits an anomaly at the magnetic phase transition due to magnetoelastic coupling. Thermal expansion mediates the coupling between mechanical strain and heat flow and determines the strength of thermoelastic damping (TED). Consequently, variations in the thermal expansion coefficient are reflected directly in TED, motivating our focus on this mechanism. We extend existing TED models to incorporate anisotropic thermal conduction, a critical property of van der Waals materials. By combining the thermodynamic properties of the resonator material with the anisotropic TED model, we examine dissipation as a function of temperature. Our findings reveal a pronounced impact of the phase transition on dissipation, along with transitions between distinct dissipation regimes controlled by geometry and the relative contributions of in-plane and out-of-plane thermal conductivity. These regimes are characterized by the resonant interplay between strain and in-plane or through-plane heat propagation. To validate our theory, we compare it to experimental data of the temperature-dependent mechanical resonances of FePS$_3$ resonators.

cond-mat.mes-hall↗