arXiv subjects

Amar C. Vutha

Publications and source records attributed to Amar C. Vutha.

At least 19 recordsLinked to original sources

arXiv2024

Comagnetometry using mirror-symmetric ions in a crystal

Searches for physics beyond the Standard Model using spin sensors are susceptible to spurious frequency shifts and noise due to magnetic fields. Therefore a comagnetometer -- an auxiliary sensor that allows mundane magnetic field effects to be differentiated from new physics -- is an essential feature of many precision searches. Here we demonstrate the operation of a novel type of comagnetometer using nuclear spins of dopant ions in a crystal, comparing four different sub-ensembles of ions. We demonstrate rejection of magnetic-field-induced shifts to better than 1 part in 10$^5$ using this system, laying the groundwork for improved searches of time-reversal symmetry violation using solid-state systems.

physics.atom-ph↗

arXiv2023

Nuclear T-violation search using octupole-deformed nuclei in a crystal

Precision measurements with atoms and molecules can search for subtle violations of time-reversal symmetry (T) in nuclei, and thereby probe a variety of new physics models. We present a detailed scheme for a nuclear T-violation search experiment using $^{153}$Eu$^{3+}$ ions doped in non-centrosymmetric sites within a Y$_2$SiO$_5$ crystal. The ions in this solid contain nuclei that are highly sensitive to T-violation, and avail of large atomic enhancements by being polarized within the solid. But in particular, the system and methods that we discuss here enable the use of vast numbers of nuclei trapped in crystals, while also offering a number of stringent tests to ward off systematic errors. Our approach maps out a path to probe new physics at the PeV energy scale.

physics.atom-ph↗

arXiv2023

Coherent quantum beats: spectroscopy of energy differences masked by inhomogeneous broadening

Precision spectroscopy of solid-state systems is challenging due to inhomogeneous broadening. We describe a technique -- coherent quantum beats -- that enables the measurement of small frequency shifts within an inhomogeneously broadened distribution while addressing the full ensemble. We show that the technique can be used to obtain improvements in signal size and spectral resolution, offering advantages for precision measurements in solids.

physics.atom-ph↗

arXiv2023

BaF molecules in neon ice: trapping, spectroscopy and optical control of electron spins

We have trapped BaF molecules in neon ice, and used laser-induced fluorescence spectroscopy to map out optical transitions in the trapped molecules. Our measurements show that the neon lattice does not significantly perturb certain optical transitions in the trapped molecules. We used one of these transitions to polarize the electron spins, detect spin flips and measure hyperfine transitions in the trapped molecules, entirely using lasers. This demonstration with heavy polar molecules opens up new opportunities for precision measurements of beyond-standard-model physics.

physics.atom-ph↗

arXiv2020

Electron electric dipole moment searches using clock transitions in ultracold molecules

Permanent electric dipole moments (EDMs) of fundamental particles such as the electron are signatures of parity and time-reversal violation due to physics beyond the standard model. EDM measurements probe new physics at energy scales well beyond the reach of present-day colliders. Recent advances in assembling molecules from ultracold atoms have opened up new opportunities for improving the reach of EDM experiments. But better measurement techniques, that are not limited by the magnetic field sensitivity of such molecules, are necessary before these opportunities can be fully exploited. We present a technique that takes advantage of magnetically-insensitive hyperfine clock transitions in polar molecules, and offers new ways to improve both the precision and accuracy of EDM searches with ultracold assembled molecules.

physics.atom-ph↗

arXiv2020

Nd$^+$ isotope shift measurements in a cryogenically-cooled neutral plasma

We report measurements of the isotope shifts of two transitions ($4f^46s\rightarrow [25044.7]^{\circ}_{7/2}$ and $4f^46s\rightarrow [25138.6]^{\circ}_{7/2}$) in neodymium ions (Nd$^+$) with hundredfold improved accuracy, using laser spectroscopy of a cryogenically-cooled neutral plasma. The isotope shifts were measured across a set of five spin-zero isotopes that spans a nuclear shape transition. We discuss the prospects for further improvements to the accuracy of Nd$^+$ isotope shifts using optical clock transitions, which could enable higher precision tests of King plot linearity for new physics searches.

physics.atom-ph↗

arXiv2019

Improved estimate of the collisional frequency shift in Al$^+$ optical clocks

Collisions between background gas particles and the trapped ion in an atomic clock can subtly shift the frequency of the clock transition. The uncertainty in the correction for this effect makes a significant contribution to the total systematic uncertainty budget of trapped-ion clocks. Using a non-perturbative analytic framework that was developed for this problem, we estimate the frequency shift in Al$^+$ ion clocks due to collisions with helium and hydrogen. Our calculations significantly improve the uncertainties in the collisional shift coefficients, and show that the collisional frequency shifts for Al$^+$ are zero to within uncertainty.

physics.atom-ph↗

arXiv2019

Direct observation of a highly forbidden optical transition in Sm:SrF$_2$

The $4f^6$ $^{7}F_0$ $\to 4f^6$ $^{5}D_0$ intra-configuration transition in Sm:SrF$_2$ is forbidden for Sm$^{2+}$ ions in the octahedrally symmetric substitution sites in SrF$_2$. We report the direct observation of this transition using laser-induced fluorescence at cryogenic temperatures, and measurements of the excited state lifetime and the excitation cross section. To the best of our knowledge, this optical transition has the longest lived excited state ever observed in a solid.

physics.atom-ph↗

arXiv2019

Cold, dense atomic ion clouds produced by cryogenic buffer gas cooling

We produce cold and dense clouds of atomic ions (Ca$^+$, Dy$^+$) by laser ablation of metal targets and cryogenic buffer gas cooling of the resulting plasma. We measure the temperature and density of the ion clouds using laser absorption spectroscopy. We find that large ion densities can be obtained at temperatures as low as 6 K. Our method opens up new ways to study cold neutral plasmas, and to perform survey spectroscopy of ions that cannot be laser-cooled easily.

physics.atom-ph↗

arXiv2019

Magic polarization for light shift cancellation in two-photon optical clocks

We find a simple solution to the problem of probe laser light shifts in two-photon optical atomic clocks. We show that there exists a magic polarization at which the light shifts of the two atomic states involved in the clock transition are identical. We calculate the differential polarizability as a function of laser polarization for two-photon optical clocks based on neutral calcium and strontium, estimate the magic polarization angle for these clocks, and determine the extent to which probe laser light shifts can be suppressed. We show that the light shift and the two-photon excitation rate can be independently controlled using the probe laser polarization.

physics.atom-ph↗

arXiv2018

Laser frequency stabilization using a transfer interferometer

We present a laser frequency stabilization system that uses a transfer interferometer to stabilize slave lasers to a reference laser. Our implementation uses off-the-shelf optical components along with microcontroller-based digital feedback, and offers a simple, flexible and robust way to stabilize multiple laser frequencies to better than 1 MHz.

physics.atom-ph↗

arXiv2017

The collisional frequency shift of a trapped-ion optical clock

Collisions with background gas can perturb the transition frequency of trapped ions in an optical atomic clock. We develop a non-perturbative framework based on a quantum channel description of the scattering process, and use it to derive a master equation which leads to a simple analytic expression for the collisional frequency shift. As a demonstration of our method, we calculate the frequency shift of the Sr$^+$ optical atomic clock transition due to elastic collisions with helium.

physics.atom-ph↗

arXiv2017

Displacement operators: the classical face of their quantum phase

In quantum mechanics, the operator representing the displacement of a system in position or momentum is always accompanied by a path-dependent phase factor. In particular, two non-parallel displacements in phase space do not compose together in a simple way, and the order of these displacements leads to different displacement composition phase factors. These phase factors are often attributed to the nonzero commutator between quantum position and momentum operators, but such a mathematical explanation might be unsatisfactory to students who are after more physical insight. We present a couple of simple demonstrations, using classical wave mechanics and classical particle mechanics, that provide some physical intuition for the phase associated with displacement operators.

quant-ph↗

arXiv2016

Methods, Analysis, and the Treatment of Systematic Errors for the Electron Electric Dipole Moment Search in Thorium Monoxide

We recently set a new limit on the electric dipole moment of the electron (eEDM) (J. Baron et al., ACME collaboration, Science 343 (2014), 269-272), which represented an order-of-magnitude improvement on the previous limit and placed more stringent constraints on many CP-violating extensions to the Standard Model. In this paper we discuss the measurement in detail. The experimental method and associated apparatus are described, together with the techniques used to isolate the eEDM signal. In particular, we detail the way experimental switches were used to suppress effects that can mimic the signal of interest. The methods used to search for systematic errors, and models explaining observed systematic errors, are also described. We briefly discuss possible improvements to the experiment.

physics.atom-ph↗

arXiv2016

Broadband low-noise photodetector for Pound-Drever-Hall laser stabilization

The Pound-Drever-Hall laser stabilization technique requires a fast, low-noise photodetector. We present a simple photodetector design that uses a transformer as an intermediary between a photodiode and cascaded low-noise radio-frequency amplifiers. Our implementation using a silicon photodiode yields a detector with 50 MHz bandwidth, gain $> 10^5$ V/A, and input current noise $< 4$ pA/$\sqrt{\mathrm{Hz}}$, allowing us to obtain shot-noise-limited performance with low optical power.

physics.ins-det↗

arXiv2015

Optical frequency standards for gravitational wave detection using satellite Doppler velocimetry

Gravitational waves imprint apparent Doppler shifts on the frequency of photons propagating between an emitter and detector of light. This forms the basis of a method to detect gravitational waves using Doppler velocimetry between pairs of satellites. Such detectors, operating in the milli-hertz gravitational frequency band, could lead to the direct detection of gravitational waves. The crucial component in such a detector is the frequency standard on board the emitting and receiving satellites. We point out that recent developments in atomic frequency standards have led to devices that are approaching the sensitivity required to detect gravitational waves from astrophysically interesting sources. The sensitivity of satellites equipped with optical frequency standards for Doppler velocimetry is examined, and a design for a robust, space-capable optical frequency standard is presented.

physics.atom-ph↗

arXiv2015

Optical frequency standard based on a two-photon transition in calcium

A two-photon transition in laser-cooled and trapped calcium atoms is proposed as the atomic reference in an optical frequency standard. An efficient scheme for interrogation of the frequency standard is described, and the sensitivity of the clock transition to systematic effects is estimated. Frequency standards based on this transition could lead to compact and portable devices that are capable of rapidly averaging down to $< 10^{-16}$.

physics.atom-ph↗

arXiv2014

Electric dipoles on the Bloch sphere

The time evolution of a two-level quantum mechanical system can be geometrically described using the Bloch sphere. By mapping the Bloch sphere evolution onto the dynamics of oscillating electric dipoles, we provide a physically intuitive link between classical electromagnetism and the electric dipole transitions of atomic & molecular physics.

quant-ph↗