SearcharxivSearch

arXiv subjects

Amit Ghosal

Publications and source records attributed to Amit Ghosal.

At least 19 recordsLinked to original sources

Interplay of Excitonic Charge Density Wave and Superconductivity in Transition Metal Dichalcogenides

Motivated by the unique characteristics of the phase diagram of 1T-TiSe2, we investigated the complex interplay of excitonic charge density wave (CDW) and superconductivity (SC) on a two-dimensional triangular lattice, each site accommodating two orbitals. In response to various tuning parameters, such as intercalation, pressure, substitution, and gating, these materials exhibit a generic and gradual waning of CDW, followed by the emergence of SC. Intriguingly, the nature of CDW changes from commensurate to incommensurate with the appearance of SC. Setting up a minimal model based on observed excitonic CDW and electron and hole pockets in the Fermi surface, and analyzing it within a simple mean-field framework, we can comprehend some salient experimental features. We also found that the qualitative phase diagram remains insensitive to details of the band structure. These results offer crucial insights into the nature of the interplay between CDW and SC in transition-metal dichalcogenides.

cond-mat.supr-con

Evolution of inhomogeneities in two-dimensional disordered superconductors in a magnetic field

Emerging granularity in superconducting films by tuning disorder is a well-studied topic, both theoretically and experimentally. However, the orbital magnetic field generates a vortex lattice and contributes to the formation of periodic inhomogeneities. Here, we study superconducting films in the simultaneous presence of disorder and a magnetic field, examining how inhomogeneities in various superconducting correlations evolve under these two perturbations. By performing scanning tunneling spectroscopy (STS) on thin films of \ce{Sr2VO_{3-\text{x}}FeAs} layer structures under both zero and finite orbital magnetic fields, we report impressive similarities between our theoretical results and the experimental findings. Our results have strong implications for identifying the nature of vortices in disordered superconductors, demonstrating a crossover from Abrikosov to Josephson character with increasing disorder, and provide predictive guidance for interpreting STS and current mapping data in complex superconductors.

cond-mat.supr-con

Charge Modulation in the Vortex Halo of a Superconductor Enhances its Critical Magnetic Field

When an orbital magnetic field suppresses superconductivity, forming periodic vortices in type-II superconductors, subdominant orders can emerge in the vortex cores. Rather than competing with superconductivity, we find that the emergent charge order within the halo of a vortex makes superconductivity more robust by enhancing the upper critical field. We establish that charge modulations nucleate in and around the vortex core for model parameters dictated by the underlying non-superconducting state. We further show that the spectral signatures from the Caroli-de Gennes-Matricon (CdGM) bound states in vortex cores track the charge modulation. The CdGM-like peak is found to shift toward the gap edge and oscillate from particle-to-hole bias from site to site, signaling charge modulation.

cond-mat.supr-con

Cooperative motion in equilibrium phases across two-dimension melting in pure and disordered systems

We uncover the dynamics of particles with Gaussian core interactions across melting in pure and disordered two-dimensional (2D) systems. Intriguing signatures of cooperative motion of particles in string-like paths are found at low temperatures. Such a motion, while common to glasses and supercooled liquids, are realized here in traditional equilibrium phases, including in pure systems. We explore the interplay of such motion and impurities and report their repercussions on spatiotemporal correlations. In particular, cooperative motion seems to cause a departure from the diffusive dynamics, causing slow relaxation.

cond-mat.soft

Charge density wave solutions of the Hubbard model in the composite operator formalism

We investigate the charge density wave phase in the strongly correlated Hubbard model without any other broken symmetry phase. Starting from the atomic Hamiltonian with no hopping, we generate quasiparticle operators corresponding to holons and doublons in the strongly correlated limit of the repulsive Hubbard model. We develop a real space composite operator formalism using the equation of motion technique to include the intersite hopping perturbatively. Our fully self-consistent calculation stabilizes multiple unidirectional translation symmetry broken states within the doping range $\delta=0.07$ to $0.2$. The charge-ordered states become increasingly unfavorable with hole-doping. The unidirectional density waves manifest as periodic modulations of half-filled Mott regions separated by hole-rich regions. Notably, density wave solutions with periods of $3$ to $8$ lattice spacing remain energetically higher than those with larger periods. Quenched disorder on the charge-ordered states induces the merging of the Mott regions and, consequently, forms short-ranged charge modulations. The density of states shows signatures of strongly correlated Mott regions, potentially relevant to the physics of underdoped cuprates.

cond-mat.str-el

Charge modulation in the background of depleted superconductivity inside vortices

We use the Bogoliubov-de Gennes (BDG) formalism to undertake a microscopic investigation of a vortex lattice in a strongly correlated, type-II, d-wave superconductor (SC) treating strong correlation within Gutzwiller formalism. We demonstrate that in the underdoped region, the vortex core changes from metallic-type to insulating-type in the presence of subdominant charge and bond order, in contrast to Mott-type, when these orders are absent. We have investigated that such subdominant order changes the structure and spectrum of the d-wave vortex in the underdoped region. We have demonstrated the formation of charge and bond modulation at the vortex center by decreasing the doping and reaching an underdoped zone.

cond-mat.supr-con

Pinning of Vortices by impurities in Unconventional superconductors

We carry out a microscopic study of a vortex lattice in a strongly correlated, type-II, d-wave superconductor(SC) using Bogoliubov de Gennes (BDG) formalism. In weak-coupling theory, commonly accepted truism is that a vortex binds to impurity. We demonstrate that in unconventional SCs, the binding of vortex to an impurity depends on relevant parameters. In particular, we illustrate such dependency on the sign of impurity, i.e. attractive or repulsive, as well as doping. We emphasize that this seemingly unanticipated behavior arises from strong correlation effects and is absent in weak coupling descriptions.

cond-mat.supr-con

The effect of disorder on phases across two-dimensional thermal melting

We study melting in a two-dimensional system of classical particles with Gaussian-core interactions in disordered environments. The pure system validates the conventional two-step melting with a hexatic phase intervening between the solid and the liquid. This picture is modified in the presence of pinning impurities. A random distribution of pinning centers forces a hexatic-like low temperature phase that transits into a liquid at a single melting temperature $T^{\rm RP}_{\rm m}$. In contrast, pinning centers located at randomly chosen sites of a perfect crystal anchors a solid at low temperatures which undergoes a direct transition to the liquid at $T^{\rm CP}_{\rm m}$. Thus, the two-step melting is lost in either cases of disorder. We discuss the characteristics of melting depending on the nature of the impurities.

cond-mat.soft

Significance of the nature of disorder on the universal features of the spatio-temporal correlations of two-dimensional Coulomb-clusters

We comprehend the role of imperfections in materials consisting of interacting particles, arising from different origins on their universal features. Specifically, we report the static and dynamic responses in a cluster of Coulomb interacting particles in two dimensions. Confined systems with pinned impurities are studied, and results are compared with those from irregularly trapped system of particles. While the disorder of first type leads to diffusive single-particle dynamics, the motion of a single particle in an irregular trap is chaotic but ballistic. The many-particle system does not differentiate between these two models of disorder insofar as their qualitative properties are concerned -- particularly for describing the thermal melting of the underlying Coulomb-"solid". However, quantitative differences persist -- the relaxation time scales differ significantly by tuning impurity concentration.

cond-mat.dis-nn

Enigma of the vortex state in a strongly correlated d-wave superconductor

We show that strong electronic repulsion transforms a vortex core from a metallic-type in overdoped regime to a Mott-insulator at underdoping of a strongly correlated d-wave superconductor. This changeover is accompanied by an accumulation of electron density at the vortex core towards local half-filling in the underdoped region, which in turn facilitates the formation of the Mott insulating core. We find that the size of vortices evolves non-monotonically with doping. A similar non-monotonicity of critical field $H_{\rm c2}$, as extracted from superfluid stiffness, is also found. Our results explain some recent experimental puzzles of cuprate superconductors.

cond-mat.supr-con

Charge, bond, and pair density wave orders in a strongly correlated system

The coexistence of multiple quasi-degenerate orders is the hallmark of the strongly correlated materials. Experiments often reveal several spatially modulated orders in the underdoped cuprates. This has come to the forefront with the possible detection of the pair density wave states. However, microscopic calculations often struggle to stabilize such spatially modulating orders as the ground state in the strong correlation limit. This work uses the $t-t^\prime-J$-model with an additional nearest-neighbor repulsion to stabilize spatially oscillating charge, bond, and pairing orders in the underdoped regime. We employ the standard Gutzwiller approach while treating the inhomogeneity for the spatial orders using the self-consistent Hartree-Fock-Bogoliubov methodology. Our calculations reveal that unidirectional bond density states coexisting with charge and pairing modulations can have lower energy than the uniform superconducting state over an extensive doping range. These modulating states vanish monotonically as the modulation wavevector becomes shorter with increased dopings. The finite momentum orders melt upon increasing doping to a vestigial nematic state which breaks the rotational symmetry of the system. The spatial features of the ground state at each doping reveal multiple wavevectors, which potentially drives the incommensuration of charge orders. Interestingly, the spatially modulating states are absent when the strong correlations criteria are relaxed, suggesting that the removal of double occupancy aids the stabilization of density wave orders.

cond-mat.supr-con

New paradigm for a disordered superconductor in a magnetic field

We show that while orbital magnetic field and disorder, acting individually weaken superconductivity, acting together they produce an intriguing evolution of a two-dimensional type-II s-wave superconductor. For weak disorder, the critical field H_c at which the superfluid density collapses is coincident with the field at which the superconducting energy gap gets suppressed. However, with increasing disorder these two fields diverge from each other creating a pseudogap region. The nature of vortices also transform from Abrikosov vortices with a metallic core for weak disorder to Josephson vortices with gapped and insulating cores for higher disorder. Our results naturally explain two outstanding puzzles: (1) the gigantic magnetoresistance peak observed as a function of magnetic field in thin disordered superconducting films; and (2) the disappearance of the celebrated zero-bias Caroli-de Gennes-Matricon peak in disordered superconductors.

cond-mat.supr-con

Fulde-Ferrell-Larkin-Ovchinnikov state in strongly correlated d-wave superconductors

The Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) phase is an unconventional superconducting state found under the influence of strong Zeeman field. This phase is identified by finite center-of-mass momenta in the Cooper pairs, causing the pairing amplitude to oscillate in real space. Repulsive correlations, on the other hand, smear out spatial inhomogeneities in d-wave superconductors. We investigate the FFLO state in a strongly correlated d-wave superconductor within a consolidated framework of Hartree-Fock-Bogoliubov theory and Gutzwiller approximation. We find that the profound effects of strong correlations lie in shifting the BCS-FFLO phase boundary towards a lower Zeeman field and thereby enlarging the window of the FFLO phase. In the FFLO state, our calculation features a sharp mid-gap peak in the density of states, indicating the formation of strongly localized Andreev bound states. We also find that the signatures of the FFLO phase survive even in the presence of an additional translational symmetry breaking competing order in the ground state. This is demonstrated by considering a broken symmetry ground state with a simultaneous presence of the d-wave superconducting order and a spin-density wave order, often found in unconventional superconductors.

cond-mat.supr-con

Emergent superconductivity upon disordering a charge density wave ground state

We explore the interplay of a charge density wave (CDW) order and s-wave superconductivity (sSC) in a disordered system. Recent experiments on 1T-TiSe_2, where the pristine sample has a commensurate CDW order and the superconductivity appears upon copper intercalation, motivates our study. Starting with an extended Hubbard model, with parameters which yield a CDW ground state within Hartree-Fock-Bogoliubov formalism in pure systems, we show that the addition of disorder quickly wipes out the global charge order by disrupting periodic modulation of density at some (low) strength of disorder. Along with this, the subdominant superconducting order emerges in regions that spatially anti-correlates with islands of strong local CDW order. The short-range density modulations, however, continue to persist and show discernible effects up to a larger disorder strength. The local CDW puddles reduce in size with increasing disorder and they finally lose their relevance in effecting the properties of the system. Our results have strong implications for the experimental phase diagram of transition metal dichalcogenides.

cond-mat.supr-con

Analysis of vibrational normal modes for Coulomb clusters

We study various properties of the vibrational normal modes for Coulomb-interacting particles in two-dimensional irregular confinement using numerical simulations. By analyzing the participation ratio and spectral statistics, we characterize the vibrational modes for Coulomb clusters as localized, quasi-localized and delocalized. We also study a novel correlation function to understand the spatial structure of these different kinds of modes and subsequently extract the associated characteristic length scales. We further demonstrate that, at any given temperature, particles exhibiting larger displacement over a time interval comparable to the structural relaxation time, are strongly correlated with the low-frequency quasi-localized modes of the inherent structure corresponding to the initial configuration. Establishing this correlation for Coulomb clusters paves the path to identify the particular feature of the initial configuration that determines the previously observed heterogeneous dynamics of the particles at low temperatures in these systems.

cond-mat.dis-nn

Effective pairing theory for strongly correlated d-wave superconductors

Motivated by recent proposals of correlation induced insensitivity of d-wave superconductors to impurities, we develop a simple pairing theory for these systems for up to a moderate strength of disorder. Our description implements the key ideas of Anderson, originally proposed for disordered s-wave superconductors, but in addition takes care of the inherent strong electronic repulsion in these compounds, as well as disorder induced inhomogeneities. We first obtain the self-consistent one-particle states, that capture the effects of disorder exactly, and strong correlations using Gutzwiller approximation. These `normal states', representing the interplay of strong correlations and disorder, when coupled through pairing attractions following the path of Bardeen-Cooper-Schrieffer (BCS), produce results nearly identical to those from a more sophisticated Gutzwiller augmented Bogoliubov-de Gennes analysis.

cond-mat.supr-con

Magnetic field induced emergent inhomogeneity in a superconducting film with weak and homogeneous disorder

When a magnetic field is applied, the mixed state of a conventional Type II superconductor gets destroyed at the upper critical field Hc2, where the normal vortex cores overlap with each other. Here, we show that in the presence weak and homogeneous disorder the destruction of superconductivity with field follows a different route. Starting with a weakly disordered NbN thin film ( Tc ~ 9K ), we show that under the application of magnetic field the superconducting state becomes increasingly granular, where lines of vortices separate the superconducting islands. Consequently, phase fluctuations between these islands give rise to a field induced pseudogap phase, which has a gap in the electronic density of states but where the global zero resistance state is destroyed.

cond-mat.supr-con

Static and Dynamic Properties of Two Dimensional Coulomb Clusters

We study the temperature dependence of static and dynamic responses of Coulomb interacting particles in two-dimensional traps across the thermal crossover from an amorphous solid- to liquid-like behaviors. While static correlations, that investigate the translational and bond orientational order in the confinements, show the footprints of hexatic-like phase at low temperature, dynamics of the particles slow down considerably in this state -- reminiscent of a supercooled liquid. Using density correlations, we probe intriguing signatures of long-lived inhomogeneities due to the interplay of the irregularity in the confinement and long-range Coulomb interactions. The relaxation at multiple time scales show stretched-exponential decay of spatial correlations in irregular traps. Temperature dependence of characteristic time scales, depicting the structural relaxation of the system, show striking similarities with those observed for the glassy systems indicating that, some of the key signatures of supercooled liquids emerge in confinements with lower spatial symmetries.

cond-mat.dis-nn