arXiv subjects

Ana Predojević

Publications and source records attributed to Ana Predojević.

At least 19 recordsLinked to original sources

arXiv2025

Rabi oscillations of a monolayer quantum emitter driven through its excited state

The interaction of a quantum two-level system with a resonant driving field results in the emergence of Rabi oscillations, which are the hallmark of a controlled manipulation of a quantum state on the Bloch sphere. This all-optical coherent control of solid-state two-level systems is crucial for quantum applications. In this work we study Rabi oscillations emerging in a WSe2 monolayer-based quantum dot. The emitter is driven coherently using picosecond laser pulses to a higher-energy state, while photoluminescence is probed from the ground state. The theoretical treatment based on a three-level exciton model reveals the population transfer between the exciton ground and excited states coupled by Coulomb interaction. Our calculations demonstrate that the resulting exciton ground state population can be controlled by varying driving pulse area and detuning which is evidenced by the experimental data. Our results pave the way towards the coherent control of quantum emitters in atomically thin semiconductors, a crucial ingredient for monolayer-based high-performance, on-demand single photon sources.

cond-mat.mes-hall↗

arXiv2025

Universal computational super-resolution framework for imaging of quantum dots

We present a universal deep-learning method that reconstructs super-resolved images of quantum emitters from a single camera frame measurement. Trained on physics-based synthetic data spanning diverse point-spread functions, aberrations, and noise, the network generalizes across experimental conditions without system-specific retraining. We validate the approach on low- and high-density In(Ga)As quantum dots and strain-induced dots in 2D monolayer WSe$_2$, resolving overlapping emitters even under low signal-to-noise and inhomogeneous backgrounds. By eliminating calibration and iterative acquisitions, this single-shot strategy enables rapid, robust computational super-resolution for nanoscale characterization and quantum photonic device fabrication.

quant-ph↗

arXiv2025

Extraction of coherence times of biexciton and exciton photons emitted by a single resonantly excited quantum dot under controlled dephasing

The visibility of two-photon interference is limited by the indistinguishability of the photons. In the cascaded emission of a three-level system, such as a single quantum dot, the indistinguishability of each photon in the pair is primarily affected by two main factors: the temporal correlation between paired photons and dephasing. Investigating the individual effects of these factors on photon indistinguishability is challenging, as both factors affect it simultaneously. In this study, we investigate the temperature-dependent two-photon interference visibility of the biexciton and exciton photons emitted from a single quantum dot under two-photon resonant excitation, while keeping temporal correlation between the paired photons intact. Finally, we simultaneously extract the coherence times of the biexciton and exciton photons as a function of temperature.

quant-ph↗

arXiv2024

Losses resistant verification of quantum non-Gaussian photon statistics

Quantum non-Gaussian states of light have fundamental properties that are essential for a multitude of applications in quantum technology. However, many of these features are difficult to detect using standard criteria due to optical losses and detector inefficiency. As the statistics of light are unknown, the loss correction on the data is unreliable, despite the fact that the losses can be precisely measured. To address this issue, we employ a loss-mitigated verification technique utilising quantum non-Gaussian witnesses, which incorporate the known optical losses and detector inefficiency into their derivation. This approach allows us to address the considerable challenge of experimentally demonstrating unheralded quantum non-Gaussian states of single photons and photon pairs.

quant-ph↗

arXiv2024

Women for Quantum -- Manifesto of Values

Data show that the presence of women in quantum science is affected by a number of detriments and their percentage decreases even further for higher positions. Beyond data, from our shared personal experiences as female tenured quantum physics professors, we believe that the current model of scientific leadership, funding, and authority fails to represent many of us. It is time for a real change that calls for a different kind of force and for the participation of everyone. Women for quantum calls for a joint effort and aims with this initiative to contribute to such a transformation.

physics.soc-ph↗

arXiv2024

Engineering the impact of phonon dephasing on the coherence of a WSe$_{2}$ single-photon source via cavity quantum electrodynamics

Emitter dephasing is one of the key issues in the performance of solid-state single photon sources. Among the various sources of dephasing, acoustic phonons play a central role in adding decoherence to the single photon emission. Here, we demonstrate, that it is possible to tune and engineer the coherence of photons emitted from a single WSe$_2$ monolayer quantum dot via selectively coupling it to a spectral cavity resonance. We utilize an open cavity to demonstrate spectral enhancement, leveling, and suppression of the highly asymmetric phonon sideband, finding excellent agreement with a microscopic description of the exciton-phonon dephasing in a truly two-dimensional system. Moreover, the impact of cavity tuning on the dephasing is directly assessed via optical interferometry, which points out the capability to utilize light-matter coupling to steer and design dephasing and coherence of quantum emitters in atomically thin crystals.

quant-ph↗

arXiv2024

Impact of temporal correlations, coherence, and postselection on two-photon interference

Two-photon interference is an indispensable resource in quantum photonics, but it is not straightforward to achieve. The cascaded generation of photon pairs contains intrinsic temporal correlations that negatively affect the ability of such sources to perform two-photon interference, thus hindering applications. We report on how such correlation interplays with decoherence and temporal postselection, and under which conditions temporal postselection could improve two-photon interference visibility. Our study identifies crucial parameters and points the way to a source with optimal performance.

quant-ph↗

arXiv2023

Multipartite entanglement encoded in the photon-number basis by sequential excitation of a three-level system

We propose a general scheme to generate entanglement encoded in the photon-number basis, via a sequential resonant two-photon excitation of a three-level system. We apply it to the specific case of a quantum dot three-level system, which can emit a photon pair through a biexciton-exciton cascade. The state generated in our scheme constitutes a tool for secure communication, as the multipartite correlations present in the produced state may provide an enhanced rate of secret communication with respect to a perfect GHZ state.

quant-ph↗

arXiv2023

Deep learning of quantum entanglement from incomplete measurements

The quantification of the entanglement present in a physical system is of para\-mount importance for fundamental research and many cutting-edge applications. Currently, achieving this goal requires either a priori knowledge on the system or very demanding experimental procedures such as full state tomography or collective measurements. Here, we demonstrate that by employing neural networks we can quantify the degree of entanglement without needing to know the full description of the quantum state. Our method allows for direct quantification of the quantum correlations using an incomplete set of local measurements. Despite using undersampled measurements, we achieve a quantification error of up to an order of magnitude lower than the state-of-the-art quantum tomography. Furthermore, we achieve this result employing networks trained using exclusively simulated data. Finally, we derive a method based on a convolutional network input that can accept data from various measurement scenarios and perform, to some extent, independently of the measurement device.

quant-ph↗

arXiv2023

Hyperfine-interaction limits polarization entanglement of photons from semiconductor quantum dots

Excitons in quantum dots are excellent sources of polarization-entangled photon pairs, but a quantitative understanding of their interaction with the nuclear spin bath is still missing. Here we investigate the role of hyperfine energy shifts using experimentally accessible parameters and derive an upper limit to the achievable entanglement fidelity. Our results are consistent with all available literature, indicate that spin-noise is often the dominant process limiting the entanglement in InGaAs quantum dots, and suggest routes to alleviate its effect.

quant-ph↗

arXiv2023

Optimal and tight Bell inequalities for state-independent contextuality sets

Two fundamental quantum resources, nonlocality and contextuality, can be connected through Bell inequalities that are violated by state-independent contextuality (SI-C) sets. These Bell inequalities allow for applications that require simultaneous nonlocality and contextuality. However, for existing Bell inequalities, the nonlocality produced by SI-C sets is very sensitive to noise. This precludes experimental implementation. Here we identify the Bell inequalities for which the nonlocality produced by SI-C sets is optimal, i.e., maximally robust to either noise or detection inefficiency, for the simplest SI-C [S. Yu and C. H. Oh, Phys. Rev. Lett. 108, 030402 (2012)] and Kochen-Specker sets [A. Cabello et al., Phys. Lett. A 212, 183 (1996)] and show that, in both cases, nonlocality is sufficiently resistant for experiments. Our work enables experiments that combine nonlocality and contextuality and therefore paves the way for applications that take advantage of their synergy.

quant-ph↗

arXiv2022

Steady-state entanglement generation for non-degenerate qubits

We propose a scheme to dissipatively produce steady-state entanglement in a two-qubit system, via an interaction with a bosonic mode. The system is driven into a stationary entangled state, while we compensate the mode dissipation by injecting energy via a coherent pump field. We also present a scheme which allows us to adiabatically transfer all the population to the desired entangled state. The dynamics leading to the entangled state in these schemes can be understood in analogy with electromagnetically induced transparency (EIT) and stimulated Raman adiabatic passage (STIRAP), respectively.

quant-ph↗

arXiv2021

High extraction efficiency source of photon pairs based on a quantum dot embedded in a broadband micropillar cavity

The generation of photon pairs in single quantum dots is based on a process that is, in its nature, deterministic. However, an efficient extraction of these photon pairs from a high-index semiconductor host material requires engineering of the photonic environment. We report on a micropillar-based device featuring an extraction efficiency of 69.4(10)$\%$ that is achieved by harnessing a broadband operation suitable for extraction of photon pairs emitted from a single quantum dot. Opposing the approaches that rely solely on Purcell enhancement to realize the enhancement of the extraction efficiency, our solution exploits a suppression of the emission into the modes other than the cavity mode. Our technological implementation requires modest fabrication effort enabling higher device yields that can be scaled up to meet the growing needs of quantum technologies. Furthermore, the design of the device can be further optimized to allow for an extraction efficiency of 85$\%$.

quant-ph↗

arXiv2021

Effect of source statistics on utilizing photon entanglement in quantum key distribution

A workflow for evaluation of entanglement source quality is proposed. Based on quantum state density matrices obtained from theoretical models and experimental data, we make an estimate of a potential performance of a quantum entanglement source in quantum key distribution protocols. This workflow is showcased for continuously pumped spontaneous parametric down-conversion (SPDC) source, where it highlights the trade-off between entangled pair generation rate and entanglement quality caused by multiphoton nature of the generated quantum states. We employ this characterization technique to show that secure key rate of down-converted photon pairs is limited to 0.029 bits per detection window due to intrinsic multiphoton contributions. We also report that there exists one optimum gain for continuous-wave down-conversion sources. We find a bound for secure key rate extracted from SPDC sources and make a comparison with perfectly single-pair quantum states, such as those produced by quantum dots.

quant-ph↗

arXiv2021

Device-independent quantum key distribution based on Bell inequalities with more than two inputs and two outputs

Device-independent quantum key distribution (DI-QKD) offers the strongest form of security against eavesdroppers bounded by the laws of quantum mechanics. However, a practical implementation is still pending due to the requirement of combinations of visibility and detection efficiency that are beyond those possible with current technology. This mismatch motivates the search for DI-QKD protocols that can close the gap between theoretical and practical security. In this work, we present two DI-QKD protocols whose security relies on Bell inequalities with more than two inputs and two outputs. We show that, for maximally entangled states and perfect visibility, a protocol based on a Bell inequality with three inputs and four outputs requires a slightly lower detection efficiency than the protocols based on Bell inequalities with two inputs and two outputs.

quant-ph↗

arXiv2020

Entangled photon pairs from quantum dots embedded in a self-aligned cavity

We introduce a scalable photonic platform that enables efficient generation of entangled photon pairs from a semiconductor quantum dot. Our system, which is based on a self-aligned quantum dot-micro-cavity structure, erases the need for complex steps of lithography and nanofabrication. We experimentally show collection efficiency of 0.17 combined with a Purcell enhancement of up to 1.7 in the pair emission process. We harness the potential of our device to generate photon pairs entangled in time bin, reaching a fidelity of 0.84(5) with the maximally entangled state. The achieved pair collection efficiency is 4 times larger than the state-of-the art. The device, which theoretically supports pair extraction efficiencies of nearly 0.5 is a promising candidate for the implementation of bright sources of time-bin, polarization- and hyper entangled photon pairs in a straightforward manner.

quant-ph↗

arXiv2020

Technological implementation of a photonic Bier-Glass cavity

In this paper, we introduce a novel quantum photonic device, which we term photonic Bier-Glass cavity. We discuss its fabrication and functionality, which is based on the coupling of integrated In(Ga)As quantum dots to a broadband photonic cavity resonance. By design, the device architecture uniquely combines the Purcell enhancement of a photonic micropillar structure with broadband photonic mode shaping of a vertical, tapered waveguide, making it an interesting candidate to enable the efficient extraction of entangled photon pairs. We detail the epitaxial growth of the heterostructure and the necessary lithography steps to approach a GaAs-based photonic device with a height exceeding 15 $μ$m, supported on a pedestal that can be as thin as 20 nm. We present an optical characterization, which confirms the presence of broadband optical resonances, in conjunction with amplified spontaneous emission of single photons.

physics.app-ph↗

arXiv2020

Opto-Mechanical Tuning of the Polarization Properties of Micropillar Cavity Systems with embedded Quantum Dots

Strain tuning emerged as an appealing tool to tune fundamental optical properties of solid state quantum emitters. In particular, the wavelength and fine structure of quantum dot states could be tuned using hybrid semiconductor-piezoelectric devices. Here, we show how an applied external stress can directly impact the polarization properties of coupled InAs quantum dot-micropillar cavity systems. In our experiment, we find that we can reversibly tune the anisotropic polarization splitting of the fundamental microcavity mode by approximately 60 $μ\text{eV}$. We discuss the origin of this tuning mechanism, which arises from an interplay between elastic deformation and the photoelastic effect in our micropillar. Finally, we exploit this effect to tune the quantum dot polarization opto-mechanically via the polarization-anisotropic Purcell effect. Our work paves the way for optomechanical and reversible tuning of the polarization and spin properties of light-matter coupled solid state systems.

cond-mat.mes-hall↗