SearcharxivSearch

arXiv subjects

Anatoli Kheifets

Publications and source records attributed to Anatoli Kheifets.

11 recordsLinked to original sources

Continuous rainbow RABBITT investigation of resonant states in He and H$_2$

We employ Reconstruction of Attosecond Beating By Interference of Two-photon Transitions with an advanced energy resolution (rainbow RABBITT) to resolve under-threshold discrete excitations and above-threshold auto-ionizing states in the He atom and the H$_2$ molecule. Both below and above the threshold, the whole series of resonances is reconstructed continuously and at once by the parity based separation of the two-photon ionization amplitude. This allows for an efficient extraction of the RABBITT magnitude and phase parameters without the need for adjusting the laser photon frequency. The latter parameters are then used to test the validity of the logarithmic Hilbert transform which relates the RABBITT phase and magnitude in the resonant region.

physics.atom-ph

Wide-bandgap optical materials for high-harmonics generation at the nanoscale

High-order harmonics generation (HHG) is the only process that enables table-top-size sources of extreme-ultraviolet (XUV) light. The HHG process typically involves light interactions with gases or plasma-material phases that hinder wider adoption of such sources. This motivates the research in HHG from nanostructured solids. Here we investigate theoretically material platforms for HHG at the nanoscale using first-principle supercomputer simulations. We reveal that wide bandgap semiconductors, aluminium nitride AlN and silicon nitride SiN, are highly promising for XUV light generation when compared to one of the most common nonlinear nanophotonic material -- silicon. In our calculations we assume excitation with 100 fs pulse duration, 10^13 W/cm^2 peak power and 800 nm central wavelength. We demonstrate that in AlN material the interplay between the crystal symmetry and the incident light direction and polarization can enable the generation of both even and odd harmonics. Our results should advance the developments of high-harmonics generation of XUV light from nanostructured solids.

physics.optics

Extraction of XUV+IR ionization amplitudes from the circular dichroic phase

A strong helicity dependence of reconstruction of attosecond bursts by beating of two-photon transitions (RABBITT) with circularly polarized XUV and IR pulses was reported by Han et al. [Nature Physics 19, 230 and arXiv 2302.04137 (2023)]. They attributed a circular dichroic phase in RABBITT to the helical structure of the photoelectron wave packets in the final state. We exploit this effect to determine the magnitude and phase of two-photon XUV+IR ionization amplitudes. In s-electron targets (H, He, Li), such a determination is fully ab initio and free from any instrumental limitations. In heavier noble gases like Ar, characterization of two-photon ionization amplitudes can be made from the circular dichroic phase with minimal and very realistic assumptions.

physics.atom-ph

Propagation effects in high-harmonic generation from dielectric thin films

Theoretical investigation is conducted of high-order harmonic generation (HHG) in silicon thin films to elucidate the effect of light propagation in reflected and transmitted waves. The first-principles simulations are performed of the process in which an intense pulsed light irradiates silicon thin films up to 3 $μ$m thickness. Our simulations are carried within the time-dependent density functional theory (TDDFT) with the account of coupled dynamics of the electromagnetic fields and the electronic motion. It was found that the intensity of transmission HHG gradually decreases with the thickness, while the reflection HHG becomes constant from a certain thickness. Detailed analyses show that transmission HHG have two origins: the HHG generated near the front edge and propagating to the back surface, and that generated near the back edge and emitted directly. The dominating mechanism of the transmission HHG is found to depend on the thickness of the thin film and the frequency of the HHG. At the film thickness of 1 $μ$m, the transmission HHG with the frequency below 20 eV is generated near the back edge, while that with the frequency above 20 eV is generated near the front edge and propagates from there to the back surface.

cond-mat.mtrl-sci

High order harmonic generation in semiconductors driven at near- and mid-IR wavelengths

We study high order harmonics generation (HHG) in crystalline silicon and diamond subjected to near and mid-infrared laser pulses. We employ time-dependent density functional theory and solve the time-dependent Kohn-Sham equation in the single-cell geometry. We demonstrate that clear and clean HHG spectra can be generated with careful selection of the pulse duration. In addition, we simulate dephasing effects in a large silicon super-cell through displacement of atomic positions prepared by a molecular dynamics simulation. We compare our results with the previous calculations by Floss et al. [arXiv:1705.10707] [Phys. Rev. A 97, 011401(R) (2018)] on Diamond at 800 nm and by Tancogne-Dejean et al. [arXiv:1609.09298] [Phys. Rev. Lett. 118, 087403 (2017)] on Si at 3000 nm.

cond-mat.mtrl-sci

Revealing the target electronic structure with under-threshold RABBIITT

The process of reconstruction of attosecond beating by interference of two-photon transitions (RABBITT) reveals the target atom electronic structure when one of the transitions proceeds from below the ionization threshold. Such an under-threshold RABBITT resonates with the target bound states and thus maps faithfully the discrete energy levels and the corresponding oscillator strengths. We demonstrate this sensitivity by considering the Ne atom driven by the combination of the XUV and IR pulses at the fundmanetal laser frequency in the 800 and 1000~nm ranges.

physics.atom-ph

Attosecond angular streaking and tunnelling time in atomic hydrogen

Tunnelling, one of the key features of quantum mechanics, ignited an ongoing debate about the value, meaning and interpretation of 'tunnelling time'. Until recently the debate was purely theoretical, with the process considered to be instantaneous for all practical purposes. This changed with the development of ultrafast lasers and in particular, the 'attoclock' technique that is used to probe the attosecond dynamics of electrons. Although the initial attoclock measurements hinted at instantaneous tunnelling, later experiments contradicted those findings, claiming to have measured finite tunnelling times. In each case these measurements were performed with multi-electron atoms. Atomic hydrogen (H), the simplest atomic system with a single electron, can be 'exactly' (subject only to numerical limitations) modelled using numerical solutions of the 3D-TDSE with measured experimental parameters and acts as a convenient benchmark for both accurate experimental measurements and calculations. Here we report the first attoclock experiment performed on H and find that our experimentally determined offset angles are in excellent agreement with accurate 3D-TDSE simulations performed using our experimental pulse parameters. The same simulations with a short-range Yukawa potential result in zero offset angles for all intensities. We conclude that the offset angle measured in the attoclock experiments originates entirely from electron scattering by the long-range Coulomb potential with no contribution from tunnelling time delay. That conclusion is supported by empirical observation that the electron offset angles follow closely the simple formula for the deflection angle of electrons undergoing classical Rutherford scattering by the Coulomb potential. Thus we confirm that, in H, tunnelling is instantaneous (with an upperbound of 1.8 as) within our experimental and numerical uncertainty.

physics.atom-ph

Interpreting Attoclock Measurements of Tunnelling Times

Resolving in time the dynamics of light absorption by atoms and molecules, and the electronic rearrangement this induces, is among the most challenging goals of attosecond spectroscopy. The attoclock is an elegant approach to this problem, which encodes ionization times in the strong-field regime. However, the accurate reconstruction of these times from experimental data presents a formidable theoretical challenge. Here, we solve this problem by combining analytical theory with ab-initio numerical simulations. We apply our theory to numerical attoclock experiments on the hydrogen atom to extract ionization time delays and analyse their nature. Strong field ionization is often viewed as optical tunnelling through the barrier created by the field and the core potential. We show that, in the hydrogen atom, optical tunnelling is instantaneous. By calibrating the attoclock using the hydrogen atom, our method opens the way to identify possible delays associated with multielectron dynamics during strong-field ionization.

physics.atom-ph

Laser-sub-cycle two-dimensional electron momentum mapping using orthogonal two-color fields

The two-dimensional sub-cycle-time to electron momentum mapping provided by orthogonal two-color laser fields is applied to photoelectron spectroscopy. Using neon as the example we gain experimental access to the dynamics of emitted electron wave packets in electron momenta spectra measured by coincidence momentum imaging. We demonstrate the opportunities provided by this time-to-momentum mapping by investigating the influence of the parent ion on the emitted electrons on laser-sub-cycle times. It is found that depending on their sub-cycle birth time the trajectories of photoelectrons are affected differently by the ion's Coulomb field.

physics.atom-ph

Review of Strong Field Approximation and Investigating Semiclassical Evolution Approach

This paper theoretically analyzes the behavior of an atom driven by a strong electro-magnetic field. Moreover, besides traditional quantum mechanics method, we also investigate semiclassical approaches to this problem. We first performed strong field approximation for system of an atom driven by a strong electromagnetic field in velocity gauge. Our simulation result is consistent with theories and close to experiments except some reasonable difference caused by different parameters and omitted bound and final states in the transition amplitude. Next, a new semiclassical approach is used to solve Volkov wave function. We prove that semiclassical approximation works well in predicting the particle evolution in quantum world, especially for system in a strong electromagnetic field with low frequency. Finally, we also briefly illustrated how to use semiclassical approximation to get the same results as strong field approximation and also partly tested the viability of the semiclassical approach to Teller Potential. This part needs future work to accomplish. But still, semiclassical approximation provides a potentially new method to solve complicated system, which might be more effective than traditional quantum mechanics recipe.

physics.atom-ph