arXiv subjects

Anatoly V. Zayats

Publications and source records attributed to Anatoly V. Zayats.

At least 37 records · Page 2Linked to original sources

arXiv2023

Hot-electron dynamics in plasmonic nanostructures

The coherent oscillations of mobile charge carriers near the surface of good conductors-surface plasmons-are been exploited in many applications in information technologies, clean energy, high-density data storage, photovoltaics, chemistry, biology, medicine and security. Light can be coupled to surface plasmons and trapped near the interface between a metal and an adjacent material. This leads to the nanoscale confinement of light, impossible by any other means, and a related electromagnetic field enhancement. Microscopic electron dynamic effects associated with surface plasmons are capable of significantly influencing physical and chemical processes near a conductor surface, not only as a result of the high electric fields, but also via the excitation of energetic charge carriers: holes below Fermi level or electrons above it. When remaining inside plasmonic media, these so-called hot carriers result in nonlinear, Kerr-type, optical effects important for controlling light with light. They can also transfer into the surroundings of the nanostructures, resulting in photocurrent, or they can interact with adjacent molecules and materials, inducing photochemical transformations. Understanding the dynamics of hot carriers and related effects in plasmonic nanostructures is essential for the development of ultrafast detectors and nonlinear optical components, broadband photocatalysis, enhanced nanoscale optoelectronic devices, nanoscale and ultrafast temperature control, and other technologies of tomorrow. This review will discuss the basics of plasmonically-engendered hot electrons, theoretical descriptions and experimental methods to study them, and describe prototypical processes and examples of the most promising applications of hot-electron processes at the metal interfaces.

cond-mat.mes-hall↗

arXiv2023

Large-area, freestanding single-crystal gold of single nanometer thickness

Two-dimensional single-crystal metals are highly sought after for next-generation technologies. Here, we report large-area (>10^4 μm2), single-crystal two-dimensional gold with thicknesses down to a single-nanometer level, employing an atomic-level-precision chemical etching approach. The ultrathin thickness and single-crystal quality endow two-dimensional gold with unique properties including significantly quantum-confinement-augmented optical nonlinearity, low sheet resistance, high transparency and excellent mechanical flexibility. By patterning the two-dimensional gold into nanoribbon arrays, extremely-confined near-infrared plasmonic resonances are further demonstrated with quality factors up to 5. The freestanding nature of two-dimensional gold allows its straightforward manipulation and transfer-printing for integration with other structures. The developed two-dimensional gold provides an emerging platform for fundamental studies in various disciplines and opens up new opportunities for applications in high-performance ultrathin optoelectronic, photonic and quantum devices.

physics.optics↗

arXiv2023

Dynamic dielectric metasurfaces via control of surface lattice resonances in non-homogeneous environment

Dynamic control of metamaterials and metasurfaces is crucial for many photonic technologies, such as flat lenses, displays, augmented reality devices, and beam steering, to name a few. The dynamic response is typically achieved by controlling the phase and/or amplitude of individual meta-atom resonances using electro-optic, phase-change or nonlinear effects. Here, we propose and demonstrate a new practical strategy for the dynamic control of the resonant interaction of light with dielectric metasurfaces, exploiting the dependence of the interaction between meta-atoms in the array on the inhomogeneity of the surrounding medium. The revealed tuning mechanisms are based on the concept of the surface lattice resonance (SLR), the development of which strongly depends on the difference between permittivities of superstrate and substrate materials. We experimentally demonstrate surface lattice resonances in dielectric (Si) metasurfaces, and reveal two tuning mechanisms corresponding to shifting or damping of the SLR in optofluidic environment. The demonstrated dynamic tuning effect with the observed vivid colour changes may provide a dynamic metasurface approach with high spectral selectivity and enhanced sensitivity for sensors, as well as high-resolution for small pixel size displays.

physics.optics↗

arXiv2022

Non-Diffractive 3D Polarisation Features of Optical Vortex Beams

Vector optical vortices exhibit complex polarisation patterns due to the interplay between spin and orbital angular momenta. Here we demonstrate, both analytically and with simulations, that certain polarisation features of optical vortex beams maintain constant transverse spatial dimensions independently of beam divergence due to diffraction. These polarisation features appear in the vicinity of the phase singularity and are associated with the presence of longitudinal electric fields. The predicted effect may prove important in metrology and high resolution imaging applications.

physics.optics↗

arXiv2022

Topological Transformation and Free-Space Transport of Photonic Hopfions

Structured light fields embody strong spatial variations of polarisation, phase and amplitude. Understanding, characterization and exploitation of such fields can be achieved through their topological properties. Three-dimensional (3D) topological solitons, such as hopfions, are 3D localized continuous field configurations with nontrivial particle-like structures, that exhibit a host of important topologically protected properties. Here, we propose and demonstrate photonic counterparts of hopfions with exact characteristics of Hopf fibration, Hopf index, and Hopf mapping from real-space vector beams to homotopic hyperspheres representing polarisation states. We experimentally generate photonic hopfions with on-demand high-order Hopf indices and independently controlled topological textures, including Néel-, Bloch-, and anti-skyrmionic types. We also demonstrate a robust free-space transport of photonic hopfions, thus, showing potential of hopfions for developing optical topological informatics and communications.

physics.optics↗

arXiv2022

Atomically smooth single-crystalline platform for low-loss plasmonic nanocavities

Nanoparticle-on-mirror plasmonic nanocavities, capable of extreme optical confinement and enhancement, have triggered state-of-the-art progress in nanophotonics and development of applications in enhanced spectroscopies and molecular detection. However, the optical quality factor and thus performance of these nanoconstructs are undermined by the granular polycrystalline metal films used as a mirror. Here, we report an atomically smooth single-crystalline platform for low-loss nanocavities using chemically-synthesized gold microflakes as a mirror. Nanocavities constructed using gold nanorods on such microflakes exhibit a rich structure of plasmonic modes, which are highly sensitive to the thickness of optically-thin (down to ~15 nm) microflakes. The atomically smooth single-crystalline microflakes endow nanocavities with significantly improved quality factor (~2 times) and scattering intensity (~3 times) compared with their counterparts based on deposited films. The developed low-loss nanocavities further allow for the integration with a mature platform of fiber optics, opening opportunities for realizing nanocavity-based miniaturized photonic devices with high performance.

physics.optics↗

arXiv2021

Photonic spin lattices: symmetry constraints for skyrmion and meron topologies

Symmetry governs many electronic and photonic phenomena in optics and condensed matter physics. Skyrmions and merons are prominent topological structures in magnetic materials, with the topological features determined by the interplay between anisotropy of a material and its magnetization. Here we theoretically show and experimentally demonstrate that the symmetry of the electromagnetic field determines the spin topological properties of the guided modes via spin-orbit coupling and may only result in either hexagonal spin-skyrmion or square spin-meron lattices. We also show that in the absence of spin-orbit coupling these spin topologies are degenerated in dynamic field-skyrmions, unifying description of electromagnetic field topologies. The results provide new understanding of electromagnetic field topology and its transformations as well as new opportunities for applications in quantum optics, spin-optics and topological photonics.

physics.optics↗

arXiv2020

Transverse spin dynamics of light: the generalized spin-momentum locking for structured guided modes

Quantum spin-Hall effect, a manifestation of topological properties that govern the behavior of surface states, was studied intensively in condensed matter physics resulting in the discovery of topological insulators. The quantum spin-Hall effect of light was introduced for surface plane-waves which intrinsically carry transverse optical spin, leading to many intriguing phenomena and applications in unidirectional waveguiding, metrology and quantum technologies. In addition to spin, optical waves can exhibit complex topological properties of vectorial electromagnetic fields, associated with orbital angular momentum or nonuniform intensity variations. Here, by considering both spin and angular momentum, we demonstrate a generalized spin-momentum relationship that governs vectorial properties of guided electromagnetic waves, extending optical quantum spin-Hall effect to a two-dimensional vector field of structured guided wave. The effect results in the appearance of the out-of-plane transverse optical spins, which vary progressively from the 'up' state to the 'down' state around the energy flow, and their variation is uniquely locked to the energy propagation direction. The related spin-momentum locking in a chiral spin swirl is demonstrated with four kinds of surface structured waves and proven both theoretically and experimentally. The results provide understanding of the spin dynamics in electromagnetic guided waves and show great importance in spin optics, topological photonics and optical spin-based devices and techniques.

physics.optics↗

arXiv2020

Machine learning -- based diffractive imaging with subwavelength resolution

Far-field characterization of small objects is severely constrained by the diffraction limit. Existing tools achieving sub-diffraction resolution often utilize point-by-point image reconstruction via scanning or labelling. Here, we present a new imaging technique capable of fast and accurate characterization of two-dimensional structures with at least wavelength/25 resolution, based on a single far-field intensity measurement. Experimentally, we realized this technique resolving the smallest-available to us 180-nm-scale features with 532-nm laser light. A comprehensive analysis of machine learning algorithms was performed to gain insight into the learning process and to understand the flow of subwavelength information through the system. Image parameterization, suitable for diffractive configurations and highly tolerant to random noise was developed. The proposed technique can be applied to new characterization tools with high spatial resolution, fast data acquisition, and artificial intelligence, such as high-speed nanoscale metrology and quality control, and can be further developed to high-resolution spectroscopy

physics.optics↗

arXiv2019

Amplitude and phase control of guided modes excitation from a single dipole source:engineering far- and near-field directionality

The design of far-field radiation diagrams from combined electric and magnetic dipolar sources has recently found applications in nanophotonic metasurfaces that realize tailored reflection and refraction. Such dipolar sources also exhibit important near-field evanescent coupling properties with applications in polarimetry and quantum optics. Here we introduce a rigorous theoretical framework for engineering the angular spectra encompassing both far- and near-fields of electric and magnetic sources and develop a unified description of both free space and guided mode directional radiation. The approach uses the full parametric space of six complex-valued components of magnetic and electric dipoles in order to engineer constructive or destructive near-field interference. Such dipolar sources can be realized with dielectric or plasmonic nanoparticles. We show how a single dipolar source can be designed to achieve the selective coupling to multiple waveguide modes and far-field simultaneously with a desired amplitude, phase, and direction.

physics.optics↗

arXiv2019

Optical forces from near-field directionalities in planar structures

Matter manipulation with optical forces has become commonplace in a wide range of research fields and is epitomized by the optical trap. Calculations of optical forces on small illuminated particles typically neglect multiple scattering on nearby structures. However, this scattering can result in large recoil forces, particularly when the scattering includes directional near-field excitations. Near-field recoil forces have been studied in the case of electric, magnetic and circularly polarized dipoles, but they exist for any type of directional near-field excitation. We use the force angular spectrum as a concise and intuitive analytical expression for the force on any dipole near planar surfaces, which allows us to clearly distinguish the effect due to the dipole, and due to the surface. We relate this directly to the coupling efficiency of surface or guided modes via Fermi's golden rule. To exemplify this, a near-field force transverse to the illumination is computationally calculated for a Huygens dipole near a metallic waveguide. We believe this formalism will prove insightful for various nanomanipulation systems within areas such as nanofluidics, sensing, biotechnology and nano-assembly of nanostructures.

physics.optics↗

arXiv2019

Spontaneous photon-pair generation at the nanoscale

Optical nanoantennas have shown a great capacity for efficient extraction of photons from the near to the far-field, enabling directional emission from nanoscale single-photon sources. However, their potential for the generation and extraction of multi-photon quantum states remains unexplored. Here we demonstrate experimentally the nanoscale generation of two-photon quantum states at telecommunication wavelengths based on spontaneous parametric down-conversion in an optical nanoantenna. The antenna is a crystalline AlGaAs nanocylinder, possessing Mie-type resonances at both the pump and the bi-photon wavelengths and when excited by a pump beam generates photonpairs with a rate of 35 Hz. Normalized to the pump energy stored by the nanoantenna, this rate corresponds to 1.4 GHz/Wm, being one order of magnitude higher than conventional on-chip or bulk photon-pair sources. Our experiments open the way for multiplexing several antennas for coherent generation of multi-photon quantum states with complex spatial-mode entanglement and applications in free-space quantum communications and sensing.

quant-ph↗

arXiv2019

Experimental demonstration of linear and spinning Janus dipoles for polarisation and wavelength selective near-field coupling

The electromagnetic field scattered by nano-objects contains a broad range of wave vectors and can be efficiently coupled to waveguided modes. The dominant contribution to scattering from subwavelength dielectric and plasmonic nanoparticles is determined by electric and magnetic dipolar responses. Here, we experimentally demonstrate spectral and phase selective excitation of Janus dipoles, sources with electric and magnetic dipoles oscillating out of phase, in order to control near-field interference and directional coupling to waveguides. We show that by controlling the polarisation state of the dipolar excitations and the excitation wavelength to adjust their relative contributions, directionality and coupling strength can be fully tuned. Furthermore, we introduce a novel spinning Janus dipole featuring cylindrical symmetry in the near and far field, which results in either omnidirectional coupling or noncoupling. Controlling the propagation of guided light waves via fast and robust near-field interference between polarisation components of a source is required in many applications in nanophotonics and quantum optics.

physics.optics↗

arXiv2018

Multilevel nonvolatile optoelectronic memory based on memristive plasmonic tunnel junctions

Highly efficient information processing in brain is based on processing and memory components called synapses, whose output is dependent on the history of the signals passed through them. Here we have developed an artificial synapse with both electrical and optical memory effects using reactive tunnel junctions based on plasmonic nanorods. In an electronic realization, the electrons tunneled into plasmonic nanorods under low bias voltage are harvested to write information into the tunnel junctions via hot-electron-mediated chemical reactions with the environment. In an optical realization, the information can also be written optically by external light illumination to excite hot electrons in plasmonic nanorods. The stored information is non-volatile and can be read in both realizations either electrically or optically by measuring the resistance or inelastic-tunnelling-induced light emission, respectively. These memristive light-emitting plasmonic tunnel junctions can be used as memory, logic units or artificial synapses in future optoelectronic or neuromorphic information systems.

physics.app-ph↗

arXiv2018

Efficient energy propagation through self-assembled gold nanoparticle chain waveguides

The strong interaction of light with metallic nanoparticles enables field confinement well below the diffraction limit. Plasmonic waveguides consisting of metal nanoparticle chains could be used for the propagation of energy or information on the nanoscale, but high losses have thus far impeded practical applications. Here we demonstrate that efficient waveguiding is possible through gold nanoparticle chains despite the high dissipative losses of gold. A DNA origami directed self-assembly of monocrystalline, spherical nanoparticles allows the interparticle spacing to be decreased to 2 nm or below, which gives rise to lower-energy plasmon resonance modes. Our simulations imply that these lower energy modes allow efficient waveguiding but collapse if interparticle gap sizes are increased. Individual waveguides are characterized with nanometer-resolution by electron energy loss spectroscopy, and directed propagation of energy towards a fluorescent nanodiamond and nanoscale energy conversion is shown by cathodoluminescence imaging spectroscopy on a single-device level. With this approach, micrometer-long propagation lengths might be achieved, enabling applications in information technology, sensing and quantum optics.

physics.optics↗

arXiv2018

Deep-subwavelength features of photonic skyrmions in a confined electromagnetic field with orbital angular momentum

In magnetic materials, skyrmions are nanoscale regions where the orientation of electron spin changes in a vortex-type manner. Here we show that spin-orbit coupling in a focused vector beam results in a skyrmion-like photonic spin distribution of the excited waveguided fields. While diffraction limits the spatial size of intensity distributions, the direction of the field, defining photonic spin, is not subject to this limitation. We demonstrate that the skyrmion spin structure varies on the deep-subwavelength scales down to 1/60 of light wavelength, which corresponds to about 10 nanometre lengthscale. The application of photonic skyrmions may range from high-resolution imaging and precision metrology to quantum technologies and data storage where the spin structure of the field, not its intensity, can be applied to achieve deep-subwavelength optical patterns.

physics.optics↗

arXiv2018

Interferometric evanescent wave excitation of nano-antenna for ultra-sensitive displacement and phase metrology

We propose a method for ultra-sensitive displacement and phase metrology based on the interferometric evanescent wave excitation of nano-antennas. We show that with a proper choice of nano-antenna, tiny displacements or relative phase variations can be converted into sensitive scattering direction changes in the Fourier $k$-space. These changes stem from the strong position dependence of the imaginary Poynting vector orientation within interfering evanescent waves. Using strongly-evanescent standing waves, high sensitivity is achieved in the nano-antenna's zero scattering direction, which varies linearly with displacement over a long range. With weakly-evanescent wave interference, even higher sensitivity to tiny displacement or phase changes can be reached around chosen location. The high sensitivity of the proposed method can form the basis for many applications.

physics.optics↗

arXiv2018

Directional scattering from particles under evanescent wave illumination: the role of reactive power

Study of photonic spin-orbital interactions, which involves control of the propagation and spatial distributions of light with the polarization of electromagnetic fields, is not only important at the fundamental level but also has significant implications for functional photonic applications that require active tuning of directional light propagation. Many of the experimental demonstrations have been attributed to the spin-momentum locking characteristic of evanescent waves. In this letter, we show another property of evanescent waves: the polarization dependent direction of the imaginary part of the Poynting vector, i.e. reactive power. Based on this property, we propose a simple and robust way to tune the directional far-field scattering from nanoparticles near a surface under evanescent wave illumination by controlling linear polarization and direction of the incident light.

physics.optics↗