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Andrés Greco

Publications and source records attributed to Andrés Greco.

At least 19 recordsLinked to original sources

Competing Interlayer Loop Currents and Superconductivity in the Bilayer $t$-$J_\perp$-$V$ Model

The recent discovery of high-$T_c$ superconductivity in pressurized and thin-film bilayer nickelates, featuring a strong interlayer exchange coupling, and their potential similarities with cuprate superconductors, has made this a very active topic in condensed matter physics. In the present paper we study the strongly correlated one-orbital ($d_{x^2-y^2}$) bilayer $t$-$J_\perp$-$V$ model for nickelates, where $V$ denotes the Coulomb interactions, using a controlled large-$N$ expansion at and beyond the mean-field level. Focusing on the out-of-plane spin exchange interaction ($J_\perp$), we find that it triggers both out-of-plane $s$-wave superconductivity and an out-of-plane bond-order phase ($z$-BOP) instability. The $z$-BOP gives rise to a complex $z$-axis hopping dominated by its imaginary component, which drives out-of-plane currents and induces in-plane ones, spontaneously forming on the vertical plaquettes a loop-current state that breaks time-reversal symmetry. Competition between this loop-current phase and superconductivity yields a dome-shaped superconducting region, with optimal superconductivity occurring near the $z$-BOP quantum critical point. The resulting phase diagram features a pure loop-current region, a low-doping coexistence phase, a pure superconducting state at higher doping, and a correlated metallic state.

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Strongly correlated model of acousticlike plasmons persisting across the phase diagram of cuprate superconductors

Layered two-dimensional electron systems exhibit both optical and acousticlike plasmons around the Brillouin-zone center. In the layered cuprate La$_{2-x}$Sr$_x$CuO$_4$, resonant inelastic x-ray scattering (RIXS) has detected corresponding acousticlike plasmons in a low-energy regime comparable to that of other collective excitations associated with distinct regions of the cuprate phase diagram. This overlap in energy scale raises the question of whether the acousticlike plasmons are significantly influenced by phase-specific electronic phenomena, including the pseudogap, charge and spin order, superconductivity, and strange-metal behavior. Here we show that a single parameter set of the layered $t$-$J$-$V$ model, which incorporates strong correlations and the long-range Coulomb interaction $V$, consistently describes the acousticlike plasmon dispersion across all currently available RIXS data from the underdoped to the heavily overdoped regime. This transferability of a single parameter set exceeds that of earlier theoretical descriptions and supports a picture in which strong correlations persist into the heavily overdoped regime, while the collective plasmon mode exhibits only limited sensitivity to the phase-specific electronic phenomena that distinguish different regions of the phase diagram.

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Raman response in superconducting multiorbital systems with application to nickelates

The recent discovery of high-$T_c$ superconductivity in pressurized and thin film nickelates is nowadays one of the most relevant and active topics in solid-state physics. The origin of superconductivity together with the relevance of multiorbital physics are highly discussed issues in this field. Knowledge of the size of the gap and its symmetry is of fundamental interest to uncover the superconducting mechanism at play in the nickelates. Electronic Raman scattering is a powerful tool to investigate the main characteristics of the gap. Here, we investigate the Raman response in the superconducting phase for three different models: Two-orbital models, including $d_{x^2-y^2}$ and $d_{z^2}$ orbitals, with one and two layers; as well as a bilayer model with the $d_{x^2-y^2}$ orbital as the only active one. For each of these models, we consider different pairing symmetries and determine their characteristic fingerprints in the Raman response. For the two-orbital models, we perform full multiorbital calculations including interorbital and intraorbital scattering, and compare the results with those obtained using the additive Raman response where each band is considered separately. Our results should be useful for discussing the minimal model for superconductivity and its pairing symmetry in nickelates. The obtained results and discussions, as well as the presented formalism, are also of general interest for other multiorbital systems.

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Detecting pairing symmetry of bilayer nickelates using electronic Raman scattering

The recent discovery of high-temperature superconductivity in both bulk and thin-film bilayer nickelates La$_3$Ni$_2$O$_7$ has garnered significant attention. However, the corresponding pairing symmetry remains debated in both experiments and theoretical studies due to conflicting experimental evidence from bulk and thin-film materials. In this work, we examine the electronic Raman response across different channels for various pairing symmetries within a two-orbital bilayer model. By comparing Raman susceptibilities obtained from multiorbital and band-additive approaches, we demonstrate that Raman response can distinguish between different pairing symmetries and identify pocket-dependent gap amplitudes for both fully gapped and nodal superconducting states. Specifically, the nodal $d_{x^2-y^2}/d_{xy}$-wave pairing exhibits robust low-energy power-law behavior, distinct from a fully gapped pairing. Additionally, for the $s_{\pm}$-wave pairing, the detailed gap anisotropy on the $β$ pocket can be determined. Possible experimental implications are also discussed. Our results highlight the crucial role of multiorbital effects in shaping the Raman spectra and establish electronic Raman scattering as a powerful and symmetry-resolved probe for determining the superconducting gap in unconventional superconductors.

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Strong-coupling theory of bilayer plasmon excitations

Recently plasmon excitations in bilayer lattice systems were studied extensively in the weak-coupling regime. Unlike single-layer systems, these bilayers exhibit two distinct modes, $ω_{\pm}$, which show characteristic dependences upon the momentum and hopping integrals along the $z$ direction. To apply them to cuprates, strong correlation effects should be considered, but a comprehensive analysis has not yet been investigated. In this work, we present a strong-coupling theory to analyze the charge dynamics of a bilayer system, utilizing the $t$-$J$-$V$ model, which includes the long-range Coulomb interaction, $V$, on a lattice. Although our theoretical framework is fundamentally different from the weak-coupling approach, we find that resulting plasmon excitations are similar to those of a weak-coupling theory. A key distinction is that our strong-coupling framework reveals a noticeable suppression of particle-hole excitations, which allows the plasmon modes to remain well-defined over a wider region of momentum. We suggest that the experimentally reported plasmon excitations in Y-based cuprates can be described by the $ω_{-}$ mode, although we call for more systematic experiments to verify this.

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Out-of-plane bond-order phase, superconductivity, and their competition in the $t$-$J_\parallel$-$J_\perp$ model: Possible implications for bilayer nickelates

Almost four decades of intense research have been invested to study the physics of high-T$_c$ cuprate superconductors. The recent discovery of high-T$_c$ superconductivity in pressurized bilayer nickelates and its potential similarities with cuprate superconductors may open a new window to understand this long-standing problem. We have studied the proposed bilayer $t$-$J_\parallel$-$J_\perp$ model [where $J_\parallel$ ($J_\perp$) is the in-plane (out-of-plane) magnetic exchange] in a large-$N$ approach on the basis of the path integral representation for Hubbard operators, which allows to obtain results at mean-field and beyond mean-field level. We find that $J_\perp$ is a candidate for triggering high superconducting $T_c$ values at quarter filling (hole doping $δ=0.5$) of the $d_{x^2-y^2}$ orbitals. Beyond mean-field level, we find a new phase, an out-of-plane bond-order phase (z-BOP), triggered also by $J_\perp$. z-BOP develops below a critical temperature which decreases with increasing doping and vanishes at a quantum critical point below quarter filling. The occurrence of this phase and its competition with superconductivity leads to a superconducting dome-shaped behavior as a function of doping and as a function of $J_\perp$. Qualitative comparisons with the physics of cuprates and the recent literature on the new pressurized nickelates are given along the paper.

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Impact of electron correlations on two-particle charge response in electron- and hole-doped cuprates

Estimating many-body effects that deviate from an independent particle approach, has long been a key research interest in condensed matter physics. Layered cuprates are prototypical systems, where electron-electron interactions are found to strongly affect the dynamics of single-particle excitations. It is however, still unclear how the electron correlations influence charge excitations, such as plasmons, which have been variously treated with either weak or strong correlation models. In this work, we demonstrate the hybridised nature of collective valence charge fluctuations leading to dispersing acoustic-like plasmons in hole-doped La$_{1.84}$Sr$_{0.16}$CuO$_{4}$ and electron-doped La$_{1.84}$Ce$_{0.16}$CuO$_{4}$ using the two-particle probe, resonant inelastic x-ray scattering. We then describe the plasmon dispersions in both systems, within both the weak mean-field Random Phase Approximation (RPA) and strong coupling $t$-$J$-$V$ models. The $t$-$J$-$V$ model, which includes the correlation effects implicitly, accurately describes the plasmon dispersions as resonant excitations outside the single-particle intra-band continuum. In comparison, a quantitative description of the plasmon dispersion in the RPA approach is obtained only upon explicit consideration of re-normalized electronic band parameters. Our comparative analysis shows that electron correlations significantly impact the low-energy plasmon excitations across the cuprate doping phase diagram, even at long wavelengths. Thus, complementary information on the evolution of electron correlations, influenced by the rich electronic phases in condensed matter systems, can be extracted through the study of two-particle charge response.

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Crossover between electron-electron and electron-phonon mediated pairing on the Kagome lattice

We study electron-electron and electron-phonon mediated pairing in the Holstein extended Hubbard model on the Kagome lattice near the van Hove fillings, and investigate their combined effects on electron pairing states. We find that their combination can promote exotic pairings in a crossover region, where the filling is close to a van Hove singularity. In particular, at the $p$-type van Hove filling the $E_{1u}$ ($p$-wave) and $B_{2u}$ ($f_{y^3-3yx^2}$-wave) pairings become leading, and at the $m$-type van Hove filling the $E_{1u}$ and $A_{2g}$ ($i$-wave) pairings get promoted. Moreover, we show that the electron-phonon interaction acquires a significant momentum dependence, due to the sublattice texture of the Fermi surfaces, which can promote non $s$-wave pairing. We present a detailed analysis of these pairing propensities and discuss implications for the vanadium-based kagome superconductors AV$_3$Sb$_5$.

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Low-energy plasmon excitations in infinite-layer nickelates

The discovery of superconductivity in infinite-layer nickelates is presently an important topic in condensed-matter physics, and potential similarities to and differences from cuprates are under intense debate. We determine general features of the charge excitation spectrum in nickelates from two opposite viewpoints: (i) Nickelates are regarded as strongly correlated electron systems like cuprate superconductors and thus can be described by the $t$-$J$ model, and (ii) electron correlation effects are not as strong as in cuprates, and thus, random-phase approximation (RPA) calculations may capture the essential physics. We find that in both cases, plasmon excitations are realized around the momentum transfer $\vq=(0,0,q_z)$, although they tend to be damped more strongly in the RPA. In particular, this damping is enhanced by the relatively large interlayer hopping expected in nickelates. Besides reproducing the optical plasmon at $\vq=(0,0,0)$ observed in Nd$_{0.8}$Sr$_{0.2}$NiO$_2$, we obtain low-energy plasmons with gaps of $\sim 360$ and $\sim 560$ meV at $\vq=(0,0,q_z)$ for finite $q_z$ in cases (i) and (ii), respectively. The present work offers a possible theoretical hint to answer whether nickelates are cupratelike or not and contributes to the general understanding of the charge dynamics in nickelates.

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Ring-like shaped charge modulations in the t-J model with long-range Coulomb interaction

The study of the charge excitations in cuprates is presently an interesting topic because of the development of new and precise x-ray experiments. Based on a large-$N$ formulation of the two-dimensional $t$-$J$ model, which allows us to consider all possible charge excitations on an equal footing, we investigate the charge spectrum for both electron- and hole-doped cases. In both cases, the instability toward phase separation, which has momentum modulation ${\bf q}=(0,0)$, is found to be robust in a large region of the doping-temperature phase diagram. If a short-range Coulomb repulsion is included the phase separation region shrinks, but the instability remains at ${\bf q}=(0,0)$. If on the other hand a two-dimensional long-range Coulomb interaction is included the instability sets in at ${\bf q}$ momenta forming a ring around ${\bf q}=(0,0)$. The computed charge spectrum in the translation-invariant phase shows well-formed rings. We discuss our results in the light of recent x-ray experiments in electron- and hole-doped cuprates, where ring-like shaped charge modulations have been reported.

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Electron self-energy from quantum charge fluctuations in the layered t-J model with long-range Coulomb interaction

Employing a large-N scheme of the layered t-J model with the long-range Coulomb interaction, which captures fine details of the charge excitation spectra recently observed in cuprate superconductors, we explore the role of the charge fluctuations on the electron self-energy. We fix temperature at zero and focus on quantum charge fluctuations. We find a pronounced asymmetry of the imaginary part of the self-energy Im$Σ({\bf k}, ω)$ with respect to $ω= 0$, which is driven by strong electron correlation effects. The quasiparticle weight is reduced dramatically, which occurs almost isotropically along the Fermi surface. Concomitantly an incoherent band and a sharp side band are newly generated and acquire sizable spectral weight. All these features are driven by usual on-site charge fluctuations, which are realized in a rather high-energy region and yield plasmon excitations. On the other hand, the low-energy region with the scale of the superexchange interaction J is dominated by bond-charge fluctuations. Surprisingly, compared with the effect of the on-site charge fluctuations, their effect on the electron self-energy is much weaker even if the system approaches close to bond-charge instabilities. Furthermore, quantum charge dynamics does not produce a clear kink nor a pseudogap in the electron dispersion.

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Superconductivity with and without glue and the role of the double-occupancy forbidding constraint in the t-J-V model

The occurrence of retarded (with glue) and unretarded (without glue) pairing is thoroughly discussed in cuprates. We analyze some aspects of this problem in the context of the t-J-V model in a large-N approximation. When 1/N renormalizations are neglected the mean-field result is recovered, where the unretarded d-wave superconducting pairing triggered by the spin-exchange interaction J is obtained. However, the presence of a non-negligible nearest-neighbors Coulomb interaction V(q) kills superconductivity. If the non-double-occupancy constraint and its fluctuations are considered, the situation changes drastically. In this case, V(q) is screened making d-wave superconductivity very robust. In addition, we show that the early proposal for the presence of an unretarded pairing contribution triggered by the spin-exchange interaction J can be discussed in this context.

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Close inspection of plasmon excitations in cuprate superconductors

Recently resonant inelastic x-ray scattering experiments reported fine details of the charge excitations around the in-plane momentum ${\bf q}_{\parallel}=(0,0)$ for various doping rates in electron-doped cuprates ${\rm La_{2-x}Ce_xCuO_4}$. We find that those new experimental data are well captured by acoustic-like plasmon excitations in a microscopic study of the layered $t$-$J$ model with the long-range Coulomb interaction. The acoustic-like plasmon is not a usual plasmon typical to the two-dimensional system, but has a small gap proportional to the interlayer hopping $t_z$.

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Ferromagnetic fluctuations in the Rashba-Hubbard model

We study the occurrence and the origin of ferromagnetic fluctuations in the longitudinal spin susceptibility of the $t$-$t'$-Rashba-Hubbard model on the square lattice. The combined effect of the second-neighbor hopping $t'$ and the spin-orbit coupling leads to ferromagnetic fluctuations in a broad filling region. The spin-orbit coupling splits the energy bands, leading to two van Hove fillings, where the sheets of the Fermi surface change their topology. Between these two van Hove fillings the model shows ferromagnetic fluctuations. We find that these ferromagnetic fluctuations originate from interband contributions to the spin susceptibility. These interband contributions only arise if there is one holelike and one electronlike Fermi surface, which is the case for fillings in between the two van Hove fillings. We discuss implications for experimental systems and propose a test on how to identify these types of ferromagnetic fluctuations in experiments.

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Doping dependence of d-wave bond-charge excitations in electron-doped cuprates

Motivated by the recent experiments reporting the doping dependence of the short-range charge order (CO) in electron-doped cuprates, we study the resonant x-ray scattering spectrum from d-wave bond-charge fluctuations obtained in the two-dimensional t-J model. We find that (i) the CO is short-range, (ii) the CO peak is pronounced at low temperature, (iii) the peak intensity increases with decreasing carrier doping $δ$ down to $δ\approx$ 0.10 and is substantially suppressed below $δ\approx$ 0.10 due to strong damping, and (iv) the momentum of the CO decreases monotonically down to $δ\approx$ 0.10 and goes up below $δ\approx$ 0.10. These results reasonably capture the major features of the experimental data, and the observed short-range CO can be consistently explained in terms of bond-charge fluctuations with an internal d-wave symmetry.

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Origin of the high-energy charge excitations observed by resonant inelastic x-ray scattering in cuprate superconductors

The recent development of x-ray scattering techniques revealed the charge-excitation spectrum in high-$T_c$ cuprate superconductors. While the presence of a dispersive signal in the high-energy charge-excitation spectrum is well accepted in the electron-doped cuprates, its interpretation and universality are controversial. Since charge fluctuations are observed ubiquitously in cuprate superconductors, the understanding of its origin is a pivotal issue. Here, we employ the layered $t$-$J$ model with the long-range Coulomb interaction and show that an acoustic-like plasmon mode with a gap at in-plane momentum (0,0) captures the major features of the high-energy charge excitations. The high-energy charge excitations, therefore, should be a universal feature in cuprate superconductors and are expected also in the hole-doped cuprates. Acoustic-like plasmons in cuprates have not been recognized yet in experiments. We propose several experimental tests to distinguish different interpretations of the high-energy charge excitations.

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Mechanism for unconventional superconductivity in the hole-doped Rashba-Hubbard model

Motivated by the recent resurgence of interest in topological superconductivity, we study in this paper superconducting pairing instabilities of the hole-doped Rashba-Hubbard model on the square lattice with first- and second-neighbor hopping. Within a weak-coupling approach based on the random phase approximation, we compute the spin-fluctuation mediated paring interactions as a function of spin-orbit coupling and hole doping. Rashba spin-orbit coupling splits the spin degeneracies of the bands, which leads to two van Hove singularities at two different fillings. We find that for a broad doping region in between these two van Hove fillings the spin fluctuations exhibit a strong ferromagnetic contribution. Because of these ferromagnetic fluctuations, the triplet $f$-wave pairing channel is dominant within this filling region, resulting in a topologically nontrival phase. We discuss possible experimental realizations of this phase in heavy-fermion hybrid structures.

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Isotope effect on the superconducting critical temperature of cuprates in the presence of charge order

Using the large-$N$ limit of the $t$-$J$ model and allowing also for phonons and the electron-phonon interaction we study the isotope effect $α$ for coupling constants appropriate for YBCO. We find that $α$ has a minimum at optimal doping and increases strongly (slightly) towards the underdoped (overdoped) region. Using values for the electron phonon interaction from the local density approximation we get good agreement for $α$ as a function of $T_c$ and doping $δ$ with recent experimental data in YBCO. Our results strongly suggest that the large increase of $α$ in the underdoped region is (a) caused by the shift of electronic spectral density from low to high energies associated with a competing phase (in our case a charge density wave) and the formation of a gap, and (b) compatible with the small electron phonon coupling constants obtained from the local density approximation. We propose a similar explanation for the anomalous behavior of $α$ in Sr doped La$_2$CuO$_4$ near the doping 1/8.

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