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Andrea Alù

Publications and source records attributed to Andrea Alù.

At least 19 recordsLinked to original sources

Asymmetric Negative Refraction in Nonlocal Double-Wire Metamaterials

We demonstrate that heterogeneous double-wire metamaterials, comprising two dissimilar and nonconnected wire arrays, enable loss-asymmetric hyperbolic dispersion and strongly asymmetric negative refraction. We unveil that, owing to their strongly nonlocal response and distinctive microstructure, such geometry supports two independent hyperbolic propagation channels with unequal losses, which can be selectively excited by free-space propagating waves incident at opposite angles. This angular selectivity gives rise to asymmetric negative refraction at the air-metamaterial interfaces, characterized by strong angular asymmetry in transmission and absorption, while preserving reciprocity. This phenomenon is scalable and can be realized with metallic wire arrays over a broad frequency spectrum extending from microwave to infrared frequencies, showing that nonlocality can emulate shear-like dissipative asymmetry that, in local media, requires lower spatial symmetry. Our findings open new avenues for directional energy transport and angle-selective wave control in photonic platforms.

physics.optics↗

All-Optical Control over Nonlocality for Ultrafast Image Processing with an Excitonic Metasurface

Image processing lies at the foundation of many modern technologies, such as augmented reality and autonomous driving, yet conventional digital approaches remain energy-intensive and limited in speed. Nonlocal metasurfaces - 2D structures engineered at the nanoscale to support delocalized, dispersion engineered resonances - provide a fast, energy-efficient and ultrathin platform to perform image processing directly on the light path. Introducing tunability in this platform is an outstanding challenge, and would enable dynamic real-time control over the implemented processing operation, facilitating flexible integration into adaptive and multifunctional photonic architectures. Here, we demonstrate optically tunable edge detection at ultrafast speeds by integrating a dielectric nonlocal metasurface with multilayer WS2, whose strong exciton-driven optical response enables dynamic control of the metasurface nonlocality at sub-ps speeds. Using resonant optical pumping of the A-exciton in WS2, the metasurface transfer function is rapidly switched from edge detection to bright-field imaging by tuning its spatial nonlocality. Operating in the visible spectral range at a wavelength around 700 nm, the device shows ultrafast switching times and reaches an amplitude modulation depth of 11.5 dB for normal incident light. This approach provides a reconfigurable, ultrathin, all-optical platform for adaptive optical computing systems and highlights the potential of the highly nonlinear properties of 2D materials for active metasurfaces at ultrafast speeds.

physics.optics↗

Ultrafast Control of Lifetime in High Q Anisotropic Plasmon Polaritons

Losses are a major roadblock in the technological implementation of surface plasmons at optical frequencies. The recent emergence of MoOCl2, a correlated van-der-Waals material with strongly anisotropic optical properties, offers new avenues to circumvent this limit. We report the far-field observation of high-Q surface plasmon polaritons in this material, arising from the anisotropic hybridisation of surface plasmons and dielectric modes. We then explore nonlinear pumping of intraband electrons to the conduction band in these structures, leading, contrary to intuition, to an abrupt increase in the lifetime of the polariton resonance, despite the injection of hot electrons. This counterintuitive phenomenon stems from the competition between photon and plasmon excitations in a lenticular polariton resonance, yielding a largely tuneable lifetime at ultrafast speeds.

physics.optics↗

Aperiodic temporal modulation for distortionless broadband impedance matching beyond the Bode-Fano limit

The Bode-Fano bound sets a fundamental trade-off between bandwidth and reflection in passive, linear, time-invariant matching networks. We show that an aperiodically time-modulated reactive element can emulate the non-Foster response required to match a prescribed pulse, achieving reflectionless, nearly distortionless energy transfer beyond the Bode-Fano limit. The approach introduces a new constraint: a minimum dc bias that scales with pulse bandwidth, derived from the requirement that the modulated capacitance remain positive at all times. This modulation-bias bound replaces the classical bandwidth-reflection trade-off with a bandwidth-energy trade-off. A realistic circuit simulation confirms broadband matching with preserved waveform fidelity, demonstrating that the scheme is physically realizable and not merely a mathematical circumvention.

physics.app-ph↗

A generalized Kirchhoff's law of thermal radiation for Floquet media

Kirchhoff's law fundamentally relates thermal emission to absorption. For linear, static, reciprocal media, it equates the emissivity and absorptivity for each direction and frequency, while in nonreciprocal systems emission and absorption are equal when the bias is time-reversed. In time-varying media, however, temporal modulation breaks time-translation invariance, converts frequencies, and enables energy exchange with the modulation drive. As a result, a same-frequency relation between absorptivity and emissivity can no longer be expected. Here, we derive a generalized Kirchhoff's law for linear time-varying Floquet media. We show that the emissivity at a given frequency equals a weighted sum of harmonic-resolved absorptivities of the adjoint system, with weights accounting for thermal occupation and photon-flux conversion. This relation has both practical and fundamental consequences. In practical terms, it allows emissivity to be calculated from absorption, simplifying the design of time-varying thermal emitters. More fundamentally, it reveals thermal radiation regimes inaccessible in static media. In particular, we identify time-varying structures that exhibit strong emission with negligible absorption at the same frequency for all directions, yielding a near-maximal violation of the conventional form of Kirchhoff's law.

physics.optics↗

Bode-Fano Limits to Broadband Absorption by Small Particles

Nanostructures can be designed to absorb light efficiently at resonance despite their subwavelength footprint, but causality and passivity fundamentally limit the bandwidth over which strong absorption can be maintained. Here we derive fundamental absorption-bandwidth limits for passive, causal, linear, and temporally dispersive subwavelength objects by rigorously casting electromagnetic scattering as an equivalent impedance-matching problem. This mapping yields ultimate Bode-Fano-type constraints for optical absorption and provides rational synthesis guidelines for the material dispersion of passive nanoparticles that can approach the bounds. Our results clarify the ultimate limits for broadband light harvesting and dissipation, with implications for solar-energy conversion, photothermal hyperthermia, thermal management, and related nanophotonic technologies.

physics.optics↗

Symmetry-driven Phononic Metamaterials

Phonons are quasiparticles associated with mechanical vibrations in materials. They are at the root of the propagation of sound and elastic waves, as well as of thermal phenomena, which are pervasive in our everyday life and in many technologies. The fundamental understanding and control of phonon responses in natural and artificial media are key in the context of communications, isolation, energy harvesting and control, sensing and imaging. It has recently been realized that controlling different symmetry classes at the microscopic and mesoscopic scales in synthetic media offers a powerful tool to precisely tailor phononic responses for advanced acoustic and elastodynamic wave control. In this Review, we survey the recent progress in the design and synthesis of artificial phononic media, namely phononic crystals and metamaterials, guided by symmetry principles. Starting from tailored broken spatial symmetries, we discuss their interplay with time symmetries for non-reciprocal and non-conservative phenomena. We also address broader concepts that combine multiple symmetry classes to induce exotic phononic wave transport. We conclude with an outlook on future research directions based on symmetry engineering for the advanced control of phononic waves.

physics.app-ph↗

Microwave-to-optical transduction using magnon-exciton coupling in a layered antiferromagnet

Coherent interfaces between microwave-frequency quantum systems and low-loss optical links are essential for quantum networks. However, existing microwave-optical transducers often trade conversion efficiency against added noise, bandwidth, and device integrability. Here, we demonstrate coherent microwave-to-optical transduction based on magnon-exciton coupling in the layered antiferromagnet CrSBr. Driving the antiferromagnetic resonance with microwave signals imprints coherent modulation on a reflected optical probe, generating optical sidebands that are resonantly enhanced near excitonic transitions. While prior magnon-based approaches to microwave-to-optical transduction have typically relied on intrinsically weak off-resonant magneto-optical effects (e.g., Faraday rotation), our scheme exploits strong light-matter interactions at exciton resonances. Even in a bulk crystal without cavity enhancement, we observe coherent conversion over an intrinsically broadband window of ~ 300 MHz. We further show that multiple exciton-polariton resonances inherit the magnon-coupled response, suggesting a route to broaden the usable optical detuning range and to mitigate optical dissipation. Our results establish magnon-coupled excitons in layered magnets as a scalable platform for broadband microwave-optical interfaces, with pathways to higher cooperativity via reduced magnetic volume and cavity integration.

cond-mat.mtrl-sci↗

Minkowski-Space Modeling of Hyperbolic Lenses

The extreme anisotropy of hyperbolic materials enables extreme wave confinement, but it is also associated with an inherent misalignment between phase and energy flow, which complicates device modeling and design. Here we introduce a Minkowski-space approach to describe hyperbolic wave propagation, showing that this complexity is geometric rather than physical. By embedding anisotropy into an effective Lorentzian metric, we establish a rational design framework for hyperbolic interfaces and lenses, and analytically derive their transfer function and resolution limits, enabling ultra-large numerical apertures and deep sub-diffraction focusing. We validate our theory with the design and full-wave modeling of a planar van der Waals polaritonic lens operating in the mid-infrared frequency range.

physics.optics↗

Freeform Spectrally Stable Topological Photonic Vortex Resonators

Topological concepts have been at the forefront of materials research in recent years, driving a revolution in our understanding of the response of quantum materials and enabling new ways to manipulate light and sound in topological metamaterials. Topological defects and topological boundaries of different dimensions have driven a paradigm shift in photonics, where topological photonic crystals and metamaterials can be engineered to create one-way flow of energy robust to defects or to control such flows with synthetic degrees of freedom along topological domain walls. More recently, topological point singularities encoded into photonic structures have been shown to enable confinement of optical modes with the topologically nontrivial nature of the cavity imprinted into the vorticity of optical far fields. Here we demonstrate that the two latter concepts - domain wall and point singularities - can be unified into an even more powerful tool to enable arbitrarily shaped resonant cavities of any dimension supporting spectrally stable zero-energy modes. We experimentally confirm that such modes, whose existence is guaranteed by topological principles, allow an unprecedented degree of control over the optical field, which appears to have no phase modulation across space, can have any desirable radiation pattern, and enables spectral stability regardless of shape or length.

physics.optics↗

Dynamical Drexhage Effect: Amplified Emission in Time-Modulated Electromagnetic Environments

We investigate the effect of nonrelativistic motion on the emission dynamics of a dipole emitter moving next to a reflecting interface. Within the formalism of macroscopic QED, we obtain a general equation of motion for the dipole amplitude in terms of the dyadic Green's function, yielding a dynamical extension of the Drexhage effect. At short dipole-surface distances, the dipole can be described as a parametric oscillator featuring time-dependent dampings and Lamb shifts, both arising from the self-induced modulation of the surrounding electromagnetic environment. Importantly, these time-dependent parameters do not always average out, leading to amplification of the dipole amplitude and the radiated intensity when considering certain sinusoidal trajectories with specific modulation amplitudes and frequencies. We derive threshold modulation amplitudes as function of the relative permittivities at the interface. Qualitatively, in the vicinity of certain epsilon-near-zero materials, amplification is possible purely by modulation of the damping. Our findings open up avenues for the dynamic control of light-matter interaction in nanophotonic environments.

physics.optics↗

Enhanced Interband Optical Nonlinearities from Coupled Quantum Wells

The recent, rapid advances in nonlinear chipscale nanophotonics in the visible and near-infrared have been largely driven by manipulating the local dielectric environment proximate to decades-old workhorse bulk nonlinear optical materials, rather than increasing the inherent strength of their nonlinear response. While proposed decades ago, we demonstrate the first experimental realization of a new class of designer nonlinear materials that leverage the interband optical transition in asymmetric structures to provide strong second order susceptibility, $χ^{(2)}$. Using simple AlGaAs/GaAs coupled quantum wells operating in the near-infrared as a prototype, we observed strong second harmonic generation enhancement of 1550 nm to 775 nm over bulk controls. Extracted $χ^{(2)}$ values were as high as 2750 pm/V, which is $>$7x that of bulk GaAs. Furthermore, measured susceptibilities agreed well with quantum mechanical calculations of $χ^{(2)}$ using layer profiles extracted from electron microscopy. Growth interruptions were employed to improve interfacial abruptness in response to electron microscopy characterization, resulting in increased $χ^{(2)}$ toward the simulation predictions for ideal heterointerfaces. More complex layer designs showed predicted $χ^{(2)}$ up to 7 nm/V. Such materials are anticipated to find myriad applications, including entangled photon generation at telecommunications wavelengths for chipscale quantum information processing.

physics.optics↗

Fourier transform of the hyperbola and its role in hyperbolic photonics

Motivated by recent breakthrough studies of wave hyperbolicity in extremely anisotropic natural materials and artificial composites, we investigate the radiation pattern of a localized emitter in a hyperbolic medium. Since the emission of a point source is associated with the Fourier transform of the iso-frequency contours of a medium, we derive and analyze the properties of the Fourier transform of hyperbolic dispersion, which sheds light into the emission properties in the presence of hyperbolic bands. Our analysis leads to a generalized form of Huygens' principle for hyperbolic waves, connecting to the emergence of negative refraction and focusing with hyperbolic media. We also highlight the occurrence of aliasing artifacts in polariton imaging. More broadly, our findings provide analytical tools to model polariton propagation in materials with extreme anisotropy, and may be applied to several other physical platforms featuring hyperbolic responses, from astrophysics to seismology.

physics.optics↗

On-chip electrically reconfigurable octave-bandwidth optical amplification from visible to near-infrared

Achieving broadband on-chip optical amplification spanning the visible and near-infrared (NIR) can enable diverse quantum sensing, metrology, and classical communication applications within a single unified device. However, conventional semiconductor and ion-doped amplifiers suffer from limited gain bandwidths set by fixed energy levels, while optical parametric amplifiers (OPAs) operating continuously from the visible to the NIR have remained elusive due to dispersion-limited bandwidth and the high pump powers required in the visible or ultraviolet (UV). Here, we overcome these limitations by introducing an electrically reconfigurable OPA architecture on lithium niobate integrated photonics. By synergistically combining ultra-high effective $χ^{(2)}$ nonlinearity ($\sim$7,000\%/W-cm$^2$), high-order dispersion engineering, and local electro-thermal tuning of quasi-phase matching, our device achieves record gain spectral spanning more than an optical octave, from 770 to 1650 nm. This range covers key transitions of many photonic quantum systems and all telecommunication bands. Moreover, our approach eliminates the need for high-power, wavelength-tunable visible or UV pumps, delivering a peak on-chip gain of 23.67 dB with a single 1060 nm pump at 90 mW average on-chip power. This work opens new avenues for multi-functional, reconfigurable photonics unifying the visible and infrared regimes, with broad implications for quantum sensing and communications.

physics.optics↗

Passive harmonic mode-locked laser on lithium niobate integrated photonics

Mode-locked lasers (MLLs) are essential for a wide range of photonic applications, such as frequency metrology, biological imaging, and high-bandwidth coherent communications. The growing demand for compact and scalable photonic systems is driving the development of MLLs on various integrated photonics material platforms. Along these lines, developing MLLs on the emerging thin-film lithium niobate (TFLN) platform holds the promise to greatly broaden the application space of MLLs by harnessing TFLN 's unique electro-optic (E-O) response and quadratic optical nonlinearity. Here, we demonstrate the first electrically pumped, self-starting passive MLL in lithium niobate integrated photonics based on its hybrid integration with a GaAs quantum-well gain medium and saturable absorber. Our demonstrated MLL generates 4.3-ps optical pulses centered around 1060 nm with on-chip peak power exceeding 44 mW. The pulse duration can be further compressed to 1.75 ps via linear dispersion compensation. Remarkably, passive mode-locking occurs exclusively at the second harmonic of the cavity free spectral range, exhibiting a high pulse repetition rate $\sim$20 GHz. We elucidate the temporal dynamics underlying this self-starting passive harmonic mode-locking behavior using a traveling-wave model. Our work offers new insights into the realization of compact, high-repetition-rate MLLs in the TFLN platform, with promising applications for monolithic ultrafast microwave waveform sampling and analog-to-digital conversion.

physics.optics↗

Nonreciprocity in Quantum Technology

Nonreciprocity-the ability to transmit signals in one direction while blocking them in the reverse-has become a powerful resource in quantum technologies, enabling directional amplification, routing of quantum information, and topologically protected quantum states. Recent experimental advances have demonstrated nonreciprocal behavior in low-loss, fully integrated devices operating with weak or no magnetic bias, enabled by synthetic gauge fields, optomechanical interactions, and chiral light-matter coupling. These achievements overcome the limitations of more traditional approaches, making nonreciprocity compatible with superconducting circuits and scalable quantum photonic architectures as well as an integral part of the next generation of modular quantum computers, distributed quantum networks, and precision metrology. Here we highlight the key concepts for engineering nonreciprocity in quantum systems and describe how this functionality can be employed for high-fidelity qubit readout, robust quantum state transfer, and boosting the sensitivity of quantum sensors.

quant-ph↗

Near-field optical mode engineering-enabled freeform nonlocal metasurfaces

Nanophotonic technologies inherently rely on tailoring light-matter interactions through the excitation and interference of deeply confined optical resonances. However, existing concepts in optical mode engineering remain heuristic and are challenging to extend towards complex and multi-functional resonant phenomena. Here, we introduce an inverse design framework that optimizes near-field distributions, ideally suited to tailor Mie-type modes within dielectric nanophotonic structures, and we demonstrate its powerful opportunities to facilitate the discovery of new classes of nonlocal metasurfaces. We show that freeform nonlocal metasurfaces supporting accidental bound states in the continuum can be readily optimized to tackle tailored illumination conditions, modal properties and quality factors. We further extend our approach to multifunctional and multipolar mode engineering, and experimentally demonstrate freeform planar nonlocal multi-wavelength and chiral metasurfaces. Our versatile and robust framework for freeform mode engineering has applications in a broad range of high quality-factor metasurface platforms relevant to sensing, nonlinear optics, optomechanics and quantum information processing.

physics.optics↗

Selective Excitation of Coupled Resonators via Complex Frequency Driving: Enhanced Efficiency and Crosstalk Suppression

Controlling individual elements of coupled resonator systems poses a significant challenge, as conventional real-frequency pulses suffer from inefficiency and crosstalk, limiting fidelity and scalability. To address this challenge, we propose and explore the use of complex frequency excitations, tailoring the driving signal waveform to match the target complex reflection zeros. We demonstrate that complex frequency driving can achieve near-unity selected energy storage efficiency (100%) in a single resonator, substantially exceeding the performance of optimized Gaussian pulses (~80%). In a coupled three-resonator system, our method yields significantly higher efficiency (92-95%) along with vastly improved selectivity and crosstalk suppression compared to conventional Gaussian pulse excitations of the same duration. Our technique achieves dynamic critical coupling, providing a powerful paradigm for high-fidelity, selective control, crucial for advancing scalable complex systems for sensing and computing.

physics.optics↗