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Andrea Alú

Publications and source records attributed to Andrea Alú.

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Fostering cultural change in research through innovative knowledge sharing, evaluation, and community engagement strategies

Bringing together researchers, funders, industry partners, and publishers from 14 countries across 5 continents, we advance the debate around open-science, assessment and learning. We introduce an integrative "open knowledge system" framework linking knowledge production, validation, assessment, and reuse into one ecosystem view, and translate it into actionable recommendations for each stakeholder. Shifting focus to modular, machine-readable knowledge objects, these recommendations are intended to help diagnose misaligned incentives and guide reforms that properly value all scientific contributions.

cs.SI

Saturable time-varying mirror based on an ENZ material

We report a switchable time-varying mirror, composed of an ITO-Au stack, which can be efficiently modulated in time with over a ten-fold increase in reflectivity, with a change of 0.6. Upon interacting with the time-varying mirror, the frequency content of a reflected pulse is extended to 31 THz. This originates from the shortening of the response time of the mirror beyond saturation, as confirmed by a time-varying model and by further four-wave mixing experiments. A temporal response unbounded by the pump bandwidth opens new avenues for spectral manipulation from time-varying systems with impact for communication networks, optical switching and computing. We report a switchable time-varying mirror, composed of an ITO-Au bilayer, displaying a ten-fold modulation of reflectivity ($ΔR \approx 0.6$), which saturates for a driving pump intensity $I_{\mathrm{pump}}\approx 100$~GW/cm$^2$. Upon interacting with the saturated time-varying mirror, the frequency content of a reflected pulse is extended up to 31 THz, well beyond the pump spectral content (2.8 THz). We interpret the spectral broadening as a progressive shortening of the mirror rise time from 110 fs to sub 30 fs with increasing pump power, which is confirmed by four-wave mixing experiments and partially captured by a linear time-varying model of the mirror. A temporal response unbounded by the pump bandwidth opens new avenues for spectral manipulation from time-varying systems with impact for communication networks, optical switching and computing.

physics.optics

Unveiling Topological Charges and Their Manipulation in Electronic Circuits

Leveraging topological properties in the response of electromagnetic systems can greatly enhance their potential. Although the investigation of singularity-based electromagnetics and non-Hermitian electronics has considerably increased in recent years in the context of various scattering anomalies, their topological properties have not been fully assessed. In this work, we theoretically and experimentally demonstrate that non-Hermitian perturbations around bound states in the continuum can lead to singularities of the scattering matrix, which are topologically nontrivial and comply with charge conservation. The associated scattering matrix poles, zeros and pole-zero pairs delineate extreme scattering events, including lasing, coherent perfect absorption, and absorber-lasers. The presented framework enables a recipe for generation, annihilation and addition of these singularities in electric circuits, with potential for extreme scattering engineering across a broad range of the electromagnetic spectrum for sensing, wireless power transfer, lasing and thermal emission devices.

physics.optics

Low-Symmetry Nanophotonics

Photonics and optoelectronics are at the foundations of widespread technologies, from high-speed Internet to systems for artificial intelligence, automotive LiDAR, and optical quantum computing. Light enables ultrafast speeds and low energy for all-optical information processing and transport, especially when confined at the nanoscale level, at which the interactions of light with matter unveil new phenomena, and the role of local symmetries becomes crucial. In this Perspective, we discuss how symmetry violations provide unique opportunities for nanophotonics, tailoring wave interactions in nanostructures for a wide range of functionalities. We discuss geometrical broken symmetries for localized surface polaritons, the physics of moiré photonics, in-plane inversion symmetry breaking for valleytronics and nonradiative state control, time-reversal symmetry breaking for optical nonreciprocity, and parity-time symmetry breaking. Overall, our Perspective aims at presenting under a unified umbrella the role of symmetry breaking in controlling nanoscale light, and its widespread applications for optical technology.

physics.optics

Topological scattering singularities and embedded eigenstates for polarization control and sensing applications

Epsilon-near-zero and epsilon near-pole materials enable reflective systems supporting a class of symmetry-protected and accidental embedded eigenstates (EE) characterized by a diverging phase-resonance. Here we show that pairs of topologically protected scattering singularities necessarily emerge from EEs when a non-Hermitian parameter is introduced, lifting the degeneracy between oppositely charged singularities. The underlying topological charges are characterized by an integer winding number and appear as phase vortices of the complex reflection coefficient. By creating and annihilating them, we show that these singularities obey charge conservation, and provide versatile control of amplitude, phase and polarization in reflection, with potential applications for polarization control and sensing.

physics.optics

Quantum Embedded Superstates

Optical supercavity modes (superstates), i.e., hybrid modes emerging from the strong coupling of two nonorthogonal modes of an open cavity, can support ultranarrow lines in scattering spectra associated with quasi bound states in the continuum (quasi-BIC). These modes are of great interest for sensing applications as they enable compact systems with unprecedented sensitivity. However, these quasi-BIC sensors obey the shot-noise limit, which may be overcome only in quantum sensors. Here, we unveil that a three-level quantum system (e.g., atom, quantum dot, superconducting qubit) can be tailored to support the quantum analog of an embedded superstate with an unboundedly narrow emission line in the strong coupling regime. Remarkably, we demonstrate that the coupling of such a system with a cavity (e.g., plasmonic or dielectric nanoparticle, microcavity, microwave resonator) enables sensing properties with significantly reduced noise. Our results can be applied to a plethora of quantum platforms from microwave superconductors to cold atoms and quantum dots, opening interesting opportunities for quantum sensing and computing.

physics.optics

Berreman Embedded Eigenstates for Narrowband Absorption and Thermal Emission

Embedded eigenstates are nonradiative modes of an open structure with momentum compatible with radiation, yet characterized by unboundedly large Q-factors. Traditionally, these states originate from total destructive interference of radiation from two or more non-orthogonal modes in periodic structures. In this work, we demonstrate a novel class of embedded eigenstates based on Berreman modes in epsilon-near-zero (ENZ) layered materials and propose realistic silicon carbide (SiC) structures supporting high-Q (~10^3) resonances based on these principles. The proposed structures demonstrate strong absorption in a narrow spectral and angular range, giving rise to quasi-coherent and highly directive thermal emission.

physics.optics

Virtual Critical Coupling

Electromagnetic resonators are a versatile platform to harvest, filter and trap electromagnetic energy, at the basis of many applications from microwaves to optics. Resonators with a large intrinsic quality factor (Q) are highly desirable since they can store a large amount of energy, leading to sharp filtering and low loss. Exciting high-Q cavities with monochromatic signals, however, suffers from poor excitation efficiency, i.e., most of the impinging energy is lost in the form of reflection, since high-Q resonators are weakly coupled to external radiation. Although critical coupling eliminates reflections in steady-state by matching the intrinsic and coupling decay rates, this approach requires the introduction of loss in the resonator, causing dissipation and lowering the overall Q-factor. Here, we extend the notion of critical coupling to high-Q lossless resonators based on tailoring the temporal profile of the excitation wave. Utilizing coupled-mode theory, we demonstrate an effect analogous to critical coupling by mimicking loss with non-monochromatic excitations at complex frequencies. Remarkably, we show that this approach enables unitary excitation efficiency in open systems, even in the limit of extreme quality factors in the regime of quasi-bound states in the continuum.

physics.optics

Coherent Control of Light Scattering

Recently, a broad spectrum of exceptional scattering effects, including bound states in the continuum, exceptional points in PT-symmetrical non-Hermitian systems, and many others attainable in wisely suitably engineered structures have been predicted and demonstrated. Among these scattering effects, those that rely on coherence properties of light are of a particular interest today. Here, we have discussed coherent scattering effects in photonics. Coherent perfect absorption (CPA) generalizes the concept of perfect absorption to systems with several excitation channels. This effect allows all-optical light manipulation by tuning of parameters of coherent excitation. In its turn, the virtual perfect absorption (VPA) effect generalizes the concept of CPA to complex frequencies and Hermitian systems. In contrast to real energy dissipation in PA and CPA, in VPA the energy is trapped in a resonator till excitation continuous exponentially growth and gets released when it breaks. Additionally, VPA provides a way to perfectly couple to any even lossless high-Q resonators. Finally, employing principles of coherent excitation can boost the performance of traditional WPT systems via coherently enhanced wireless power transfer (CWPT) effect.

physics.optics

Nanophotonics with 2D Transition Metal Dichalcogenides

Two-dimensional transition metal dichalcogenides (TMDCs) have recently become attractive semiconductor materials for several optoelectronic applications, such as photodetection, light harvesting, phototransistors, light-emitting diodes, and lasers. They are particularly appealing because their bandgap lies in the visible and near-IR range, and they possess strong excitonic resonances, high oscillator strengths, and valley-selective response. Coupling these materials to optical nanocavities enhances the quantum yield of exciton emission, enabling advanced quantum optics and nanophotonic devices. Here, we review state-of-the-art advances on hybrid exciton-polariton structures based on monolayer TMDCs coupled to plasmonic and dielectric nanocavities. We first generally discuss the optical properties of 2D WS2, WSe2, MoS2 and MoSe2 materials, paying special attention to their energy and photoluminescence/absorption spectra, excitonic fine structure, and to the dynamics of exciton formation and valley depolarization. We then discuss light-matter interactions in hybrid exciton-polariton structures. Finally, we focus on weak and strong coupling regimes in monolayer TMDCs-based exciton-polariton systems, envisioning research directions and future opportunities based on this novel material platform.

physics.optics

Spectroscopy and Biosensing with Optically Resonant Dielectric Nanostructures

Resonant dielectric nanoparticles (RDNs) made of materials with large positive dielectric permittivity, such as Si, GaP, GaAs, have become a powerful platform for modern light science, enabling various fascinating applications in nanophotonics and quantum optics. In addition to light localization at the nanoscale, dielectric nanostructures provide electric and magnetic resonant responses throughout the visible and infrared spectrum, low dissipative losses and optical heating, low doping effect and absence of quenching, which are interesting for spectroscopy and biosensing applications. In this review, we present state-of-the-art applications of optically resonant high-index dielectric nanostructures as a multifunctional platform for light-matter interactions. Nanoscale control of quantum emitters and applications for enhanced spectroscopy including fluorescence spectroscopy, surface-enhanced Raman scattering (SERS), biosensing, and lab-on-a-chip technology are surveyed. We describe the theoretical background underlying these effects, overview realizations of specific resonant dielectric nanostructures and hybrid excitonic systems, and outlook the challenges in this field, which remain open to future research.

physics.optics

Tunable Resonance Coupling in Single Si Nanoparticle-Monolayer WS2 Structures

Two-dimensional semiconducting transition metal dichalcogenides (TMDCs) are extremely attractive materials for optoelectronic applications in the visible and near-IR range. Here, we address for the first time to the best of our knowledge the issue of resonance coupling in hybrid exciton-polariton structures based on single Si nanoparticles coupled to monolayer WS2. We predict a transition from weak to strong coupling regime , with a Rabi splitting energy exceeding 200 meV for a Si nanoparticle covered by monolayer WS 2 at the magnetic optical Mie resonance. This large transition is achieved due to the symmetry of magnetic dipole Mie mode and by changing the surrounding dielectric material from air to water. The prediction is based on the experimental estimation of TMDC dipole moment variation obtained from measured photoluminescence (PL) spectra of WS2 monolayers in different solvents. An ability of such a system to tune the resonance coupling is realized experimentally for optically resonant spherical Si nanoparticles placed on a WS2 monolayer. The Rabi splitting energy obtained for this scenario increases from 49.6 meV to 86.6 meV after replacing air by water. Our findings pave the way to develop high-efficiency optoelectronic, nanophotonic and quantum optical devices.

physics.optics

Analytical Study of Sub-Wavelength Imaging by Uniaxial Epsilon-Near-Zero Metamaterial Slabs

We discuss the imaging properties of uniaxial epsilon-near-zero metamaterial slabs with possibly tilted optical axis, analyzing their sub-wavelength focusing properties as a function of the design parameters. We derive in closed analytical form the associated two-dimensional Green's function in terms of special cylindrical functions. For the near-field parameter ranges of interest, we are also able to derive a small-argument approximation in terms of simpler analytical functions. Our results, validated and calibrated against a full-wave reference solution, expand the analytical tools available for computationally-efficient and physically-incisive modeling and design of metamaterial-based sub-wavelength imaging systems.

physics.optics