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Andrea Perali

Publications and source records attributed to Andrea Perali.

At least 19 recordsLinked to original sources

Quantum Impurities as Probes of Finite-Temperature Fluctuations in Two-Dimensional Bose Gases

Two-dimensional quantum gases provide a distinctive setting in which enhanced thermal fluctuations, finite-size effects, and two-body bound-state formation are intrinsically intertwined. In this work, we study a single attractive impurity immersed in a finite, weakly interacting two-dimensional Bose gas, where finite size stabilizes a nonzero condensate fraction by introducing an infrared momentum scale, thereby enabling a Bogoliubov description of the bath. Using a hybrid approach that combines finite-temperature many-body scattering theory with input from path-integral Monte Carlo, we analyze the impurity quasiparticle energy across the condensate and normal regimes. The infrared scale generates a phonon-activation temperature below which the impurity energy remains nearly temperature independent. Once the resolved phonon modes become thermally populated, their contribution competes with condensate depletion, producing a nonmonotonic temperature dependence of the polaron energy. These results suggest that attractive Bose polarons may serve as sensitive probes of finite-size thermal fluctuations, phonon dressing, and bound-state physics in low-dimensional Bose gases.

cond-mat.quant-gas

Superconducting dome due to the Fano-Feshbach shape resonance in artificial high-Tc superlattices

In this work we provide compelling experimental validation of the Bianconi Perali Valletta (BPV) theory predicting a superconducting dome based on a quantum material design of Artificial High TC Superlattices (AHTS) made with a selected nanoscale heterostructure geometry. These AHTS are SNSN superlattices of quantum wells of period d, composed of first units, superconducting doped Mott insulator layers with Rashba spin orbit coupling (S) of thickness L, intercalated by second units, normal metal spacers (N). In these superlattices, grown by molecular beam epitaxy (MBE), the experimental superconducting dome is obtained by material quantum design changing the chemical potential via the quantum geometrical factor L/d which tunes the Fano-Feshbach shape resonance in the pair transfer between superconducting gaps in the BCS regime and different gaps in the BEC-BCS crossover. Here we present a systematic magneto-transport study of AHTS artificial superlattices across the full doping range of the superconducting dome, from the deeply underdoped to the overdoped regime, using pulsed magnetic fields up to 72 T. By varying the L/d ratio, we tune the effective hole concentration delta=0.45(1-L/d) and map the evolution of the resistive transitions, the upper critical magnetic field and the Ginzburg-Landau coherence length

cond-mat.supr-con

Signature in sound-mode of the exciton bilayer two-dimensional superfluid transition

Obtaining definitive evidence of exciton superfluidity in electron-hole bilayers in zero magnetic field remains a major longstanding challenge since the condensate is electrically neutral, making its phase coherence difficult to detect directly. We show that the Anderson-Bogoliubov sound velocity provides a dynamical signature of exciton superfluidity. Across the BCS-BEC crossover, the velocity is known to discontinuously drop to zero at the Berezinskii-Kosterlitz-Thouless (BKT) transition. The magnitude of the drop has a strong density dependence. We compute this behavior, with the inclusion of finite-temperature screening, and determine the BKT transition using a renormalization-group approach. We further identify a temperature window which is experimentally accessible, where vortex-antivortex excitations strongly renormalize both the sound velocity and the transition temperature.

cond-mat.supr-con

Deep learning recognition and analysis of Volatile Organic Compounds based on experimental and synthetic infrared absorption spectra

Volatile Organic Compounds (VOCs) are organic molecules that have low boiling points and therefore easily evaporate into the air. They pose significant risks to human health, making their accurate detection the crux of efforts to monitor and minimize exposure. Infrared (IR) spectroscopy enables the ultrasensitive detection at low-concentrations of VOCs in the atmosphere by measuring their IR absorption spectra. However, the complexity of the IR spectra limits the possibility to implement VOC recognition and quantification in real-time. While deep neural networks (NNs) are increasingly used for the recognition of complex data structures, they typically require massive datasets for the training phase. Here, we create an experimental VOC dataset for nine different classes of compounds at various concentrations, using their IR absorption spectra. To further increase the amount of spectra and their diversity in term of VOC concentration, we augment the experimental dataset with synthetic spectra created via conditional generative NNs. This allows us to train robust discriminative NNs, able to reliably identify the nine VOCs, as well as to precisely predict their concentrations. The trained NN is suitable to be incorporated into sensing devices for VOCs recognition and analysis.

cs.LG

Berezinskii-Kosterlitz-Thouless transition with enhanced phase stiffness in $d$-wave strongly coupled two-dimensional superconductors

We reveal the key role of the $d$-wave symmetry of the superconducting gap in strongly coupled two-dimensional superconductors in determining the properties of the Berezinskii-Kosterlitz-Thouless (BKT) transition, associated with a sizable enhancement of the phase stiffness compared to nodeless-gap superconductors. The enhanced stiffness originates from extended regions of vanishing gap around the nodal lines of the Brillouin zone (BZ). Our study, based on mean-field and BKT theory, presents a comparative analysis of $s$-wave and $d$-wave scenarios, highlighting the features of the latter that boost the stiffness and the BKT transition temperature (T$_{BKT}$). The comparison focuses on two quantities: the mean-field critical temperature and the maximum superconducting gap related to the pairing strengths. We present a phase diagram showing the scaling of T$_{BKT}$ with respect to the mean-field critical temperature across the BCS-BEC crossover and the evolution of the pseudogap. We also present a zero-temperature phase-stiffness intensity map over the Brillouin zone, displaying a two-component structure consisting of low- and high-stiffness regions whose extent depends on microscopic parameters. These results identify the nodal gap structure of strongly coupled two-dimensional superconductors as a key mechanism enabling enhanced stiffness and elevated T$_{BKT}$ compared to their $s$-wave counterparts.

cond-mat.supr-con

Beyond Random Phase Approximation in electron-hole bilayer superfluidity

We derive the normal and anomalous proper polarization functions and the screened Coulomb interactions in a two-dimensional superfluid electron-hole bilayer, including all first-order corrections beyond the Random Phase Approximation (RPA). This requires a modification of the perturbation method as first noted by Nozières and Schrieffer [1, 2]. We discuss the physical origin and magnitude of the first-order corrections in a superfluid system with long-range Coulomb interactions. Unlike conventional superconductivity, Migdal's theorem does not apply here, so exchange vertex corrections cannot be neglected. The screened electron-electron, hole-hole, and electron-hole interactions in the superfluid state are evaluated as functions of the carrier density. We find that at low density, the strong cancellations between the normal and anomalous components that make screening of the interactions negligible, apply not only within RPA but also with the first-order corrections included. As the density is increased, the normal-anomalous cancellation weakens and screening becomes increasingly significant. We find that the first-order corrections amplify the normal-anomalous difference but only at large momenta exchanged in the two-particle scattering, so their effect on the interactions remains modest. We conclude that the superfluid state RPA is an excellent approximation for the screening and for the effective electron-hole pairing in this superfluid system over the range of densities up to the maximum of the superfluid gap.

cond-mat.str-el

The Lunar Gravitational-wave Antenna: Mission Studies and Science Case

The Lunar Gravitational-wave Antenna (LGWA) is a proposed array of next-generation inertial sensors to monitor the response of the Moon to gravitational waves (GWs). Given the size of the Moon and the expected noise produced by the lunar seismic background, the LGWA would be able to observe GWs from about 1 mHz to 1 Hz. This would make the LGWA the missing link between space-borne detectors like LISA with peak sensitivities around a few millihertz and proposed future terrestrial detectors like Einstein Telescope or Cosmic Explorer. In this article, we provide a first comprehensive analysis of the LGWA science case including its multi-messenger aspects and lunar science with LGWA data. We also describe the scientific analyses of the Moon required to plan the LGWA mission.

gr-qc

Amplitude, phase, and topological fluctuations shaping the complex phase diagram of two-dimensional superconductors

We study the amplitude and phase fluctuations of the Ginzburg-Landau quasiorder parameter for superconductors in two spatial dimensions. Starting from the mean-field critical temperature $T_{\mathrm{c}0}$, we calculate the beyond-mean-field critical temperature $T_{\rm c}$ by including thermal fluctuations of the quasiorder parameter within the Gaussian level. Moreover, from our beyond-mean-field results, we derive the Berezinskii-Kosterlitz-Thouless critical temperature $T_{\rm BKT}$, which takes into account topological vortex-antivortex excitations in the phase fluctuations as well as the amplitude fluctuations, to obtain the shifts of transition temperatures. We elucidate how the Gaussian thermal fluctuations and phase fluctuations associated with vortex excitations affect thermodynamic properties by determining the $H$-$T$ phase diagram for a type-II superconductor and computing the critical behaviors of the heat capacity, which are experimentally accessible, allowing the characterization of the cascade of different kinds of fluctuations in 2D superconductors.

cond-mat.supr-con

High-Tc superconducting dome in artificial heterostructures made of nanoscale quantum building blocks

While the search of high Tc superconductivity was driven mostly by trial and error methodology searching for novel materials, here we provide a quasi-first-principle quantum theory for engineering superconductivity in artificial high-Tc superlattices (AHTS) with period d, ranging from 5.28 down to 3 nanometers, made of superconducting quantum wells of variable thickness L. An important feature of our quantum design is the key role of the interface internal electric field giving Rashba spin-orbit coupling (SOC) in the nanoscale quantum superconducting building blocks. By tuning the geometrical conformational parameter L/d around its magic ratio 2/3 we predict the superconducting dome of Tc versus doping characteristic of unconventional superconductors. Quantum size effects, controlled by L/d, change the energy width and splitting of two quantum subbands formed by the electronic space charge confined in superconducting nano-layers. The theoretical superconducting dome Tc versus charge density controlled by the Fano-Feshbach resonance between two superconducting gaps has been able to predict experimental results on cuprate AHTS by tuning the geometry of superlattices of quantum wells made of superconducting layers (S) of thickness L of modulation doped stoichiometric Mott insulator La2CuO4 with no chemical dopants, with interface space charge confined within normal metal (N) overdoped cuprate layers

cond-mat.supr-con

Berezinskii-Kosterlitz-Thouless to BCS-like superconducting transition crossover driven by weak magnetic fields in ultra-thin NbN films

The Berezinskii-Kosterlitz-Thouless (BKT) transition in ultra-thin NbN films is investigated in the presence of weak perpendicular magnetic fields. A jump in the phase stiffness at the BKT transition is detected up to 5 G, while the BKT features are smeared between 5 G and 50 G, disappearing altogether at 100 G, where conventional current-voltage behaviour is observed. Our findings demonstrate that weak magnetic fields, insignificant in bulk systems, deeply affect our ultra-thin system, promoting a crossover from Halperin-Nelson fluctuations to a BCS-like state with Ginzburg-Landau fluctuations, as the field increases. This behavior is related to field-induced free vortices that screen the vortex-antivortex interaction and smear the BKT transition.

cond-mat.supr-con

Pairing amplification induced by nonadiabatic effects on the electron-phonon interaction throughout the BCS-BEC crossover

Nonadiabatic effects in the electron-phonon coupling are important whenever the ratio between the phononic and the electronic energy scales, the adiabatic ratio, is non negligible. For superconducting systems, this gives rise to additional diagrams in the superconducting self-energy, the vertex and cross corrections. In this work we explore these corrections in a two-dimensional single-band system through the crossover between the weak-coupling BCS and strong-coupling Bose-Einstein regimes. By focusing on the pseudogap phase, we identify the parameter range in which the pairing amplitude is amplified by nonadiabatic effects and map them throughout the BCS-BEC crossover. These effects become stronger as the system is driven deeply in the crossover regime, for phonon frequencies of the order of the hopping energy and for large enough electron-phonon coupling. Finally, we provide the phase space regions in which the effects of nonadiabaticity are more relevant for unconventional superconductors.

cond-mat.supr-con

High-$T_c$ Berezinskii-Kosterlitz-Thouless transition in 2D superconducting systems with coupled deep and quasi-flat electronic bands with van Hove singularities

In the pursuit of higher critical temperature of superconductivity, quasi-flat electronic bands and van Hove singularities in two dimensions (2D) have emerged as a potential approach to enhance Cooper pairing on the basis of mean-field expectations. However, these special electronic features suppress the superfluid stiffness and, hence, the Berezinskii-Kosterlitz-Thouless (BKT) transition in 2D superconducting systems, leading to the emergence of a significant pseudogap regime due to superconducting fluctuations. In the strong-coupling regime, one finds that superfluid stiffness is inversely proportional to the superconducting gap, which is the predominant factor contributing to the strong suppression of superfluid stiffness. Here we reveal that the aforementioned limitation is avoided in a 2D superconducting electronic system with a quasi-flat electronic band with a strong pairing strength coupled to a deep band with weak electronic pairing strength. Owing to the multiband effects, we demonstrate a screening-like mechanism that circumvents the suppression of the superfluid stiffness. We report the optimal conditions for achieving a large enhancement of the BKT transition temperature and a substantial shrinking of the pseudogap regime by tuning the intraband couplings and the pair-exchange coupling between the two band-condensates.

cond-mat.supr-con

Emergent Fano-Feshbach resonance in two-band superconductors with an incipient quasi-flat band: Enhanced critical temperature evading particle-hole fluctuations

In superconductivity, a surge of interests in enhancing $T_{\rm c}$ is ever mounting, where a recent focus is toward multi-band superconductivity. In $T_{\rm c}$ enhancements specific to two-band cases, especially around the Bardeen-Cooper-Schrieffer (BCS) to Bose-Einstein condensate (BEC) crossover considered here, we have to be careful about how quantum fluctuations affect the many-body states, i.e., particle-hole fluctuations suppressing the pairing for attractive interactions. Here we explore how to circumvent the suppression by examining multichannel pairing interactions in two-band systems. With the Gor'kov-Melik-Barkhudarov (GMB) formalism for particle-hole fluctuations in a continuous space, we look into the case of a deep dispersive band accompanied by an incipient heavy-mass (i.e., quasi-flat) band. We find that, while the GMB corrections usually suppress $T_{\rm c}$ significantly, this in fact competes with the enhanced pairing arising from the heavy band, with the trade-off leading to a peaked structure in $T_{\rm c}$ against the band-mass ratio when the heavy band is incipient. The system then plunges into a strong-coupling regime with the GMB screening vastly suppressed. This occurs prominently when the chemical potential approaches the bound state lurking just below the heavy band, which can be viewed as a Fano-Feshbach resonance, with its width governed by the pair-exchange interaction. The diagrammatic structure comprising particle-particle and particle-hole channels is heavily entangled, so that the emergent Fano-Feshbach resonance dominates all the channels, suggesting a universal feature in multiband superconductivity.

cond-mat.supr-con

Predictive power of the Berezinskii-Kosterlitz-Thouless theory based on Renormalization Group throughout the BCS-BEC crossover in 2D superconductors

Recent experiments on 2D superconductors allow the characterization of the critical temperature and of the phase diagram across the BCS-BEC crossover as a function of density. We obtain from these experiments the microscopic parameters of the superconducting state at low temperatures by the BCS mean-field approach. For Li$_x$ZrNCl, the extracted parameters are used to evaluate the superconducting phase stiffness and the Berezinskii-Kosterlitz-Thouless (BKT) critical temperature throughout the BCS-BEC crossover, by implementing the corresponding Renormalization Group (RG) approach. In this way, we make a quantitative test of the predictive power of the BKT theory for evaluating the critical temperature. The RG flow equations turn out to give a sizable renormalization of the phase stiffness and of the critical temperature, which is crucial to obtain a satisfactory agreement between the BKT theory and the experiments, in particular in the BCS-BEC crossover regime. We predict the temperature range where phase stiffness renormalization can be measured in Li$_x$ZrNCl across the BCS-BEC crossover. Contrary to other microscopic theories of superconductivity, we find that the BKT theory can be exploited to evaluate quantitatively the critical temperature of 2D superconductors in different pairing regimes.

cond-mat.supr-con

Giant amplification of Berezinskii-Kosterlitz-Thouless transition temperature in superconducting systems characterized by cooperative interplay of small-gapped valence and conduction bands

Two-dimensional superconductors and electron-hole superfluids in van der Waals heterostructures having tunable valence and conduction bands in the electronic spectrum are emerging as rich platforms to investigate novel quantum phases and topological phase transitions. In this work, by adopting a mean-field approach considering multiple-channel pairings and the Kosterlitz-Nelson criterion, we demonstrate giant amplifications of the Berezinskii-Kosterlitz-Thouless (BKT) transition temperature and a shrinking of the pseudogap for small energy separations between the conduction and valence bands and small density of carriers in the conduction band. The presence of the holes in the valence band, generated by intra-band and pair-exchange couplings, contributes constructively to the phase stiffness of the total system, adding up to the phase stiffness of the conduction band electrons that is boosted as well, due to the presence of the valence band electrons. This strong cooperative effect avoids the suppression of the BKT transition temperature for low density of carriers, that occurs in single-band superconductors where only the conduction band is present. Thus, we predict that in this regime, multi-band superconducting and superfluid systems with valence and conduction bands can exhibit much larger BKT critical temperatures with respect to single-band and single-condensate systems.

cond-mat.supr-con

Effects of intra-layer correlations on electron-hole double-layer superfluidity

We investigate the correlations acting within the layers in a superfluid system of electron-hole spatially separated layers. In this system of quasi-dipoles, the dominant correlations are Hartree--Fock. We find in the BEC regime of the superfluid where screening is negligible, that the effect of the correlations on superfluid properties is also negligible. However, in the BCS-BEC crossover regime, where the screening plays a crucial role, we find that the superfluid gap is significantly weakened because the correlations significantly boost the number of low-energy particle-hole excitations participating in the screening process. Finally, the intralayer correlations are found in this system to suppress a predicted phenomenon in which the average pair size passes through a minimum as the crossover regime is traversed. In the presence of intralayer correlations, the minimum is either extremely weak or completely absent.

cond-mat.supr-con

Berezinskii-Kosterlitz-Thouless phase transition with Rabi-coupled bosons

We theoretically investigate the superfluid-normal-state Berezinskii-Kosterlitz-Thouless transition in a binary mixture of bosonic atoms with Rabi coupling under balanced densities. We find the nonmonotonic behavior of the transition temperature with respect to the intercomponent coupling and amplification of the transition temperature for finite values of Rabi coupling, but for small intracomponent couplings. We develop the Nelson-Kosterlitz renormalization-group equations in the two-component Bose mixture and obtain the Nelson-Kosterlitz criterion modified by a fractional parameter, which is responsible for half-integer vortices, and by Rabi coupling. Adopting the renormalization-group approach, we clarify the dependence of the Berezinskii-Kosterlitz-Thouless transition temperature on the Rabi coupling and the intercomponent coupling. Analysis of the first and second sound velocities also reveals the suppression of quasicrossing of the two sound modes with a finite Rabi coupling in the low-temperature regime. Our results for a two-dimensional binary Bose superfluid contribute to the understanding of a broad range of multicomponent quantum systems such as two-dimensional multiband superconductors.

cond-mat.quant-gas

Kuramoto synchronization of quantum tunneling polarons for describing the dynamic structure in cuprate superconductors

A major open topic in cuprates is the interplay between the lattice and electronic dynamics and the importance of their coupling to the mechanism of high-temperature superconductivity (HTSC). As evidenced by Extended X-ray Absorption Fine Structure experiments (EXAFS), anharmonic structural effects are correlated with the charge dynamics and the transition to a superconducting phase in different HTSC compounds. Here we describe how structural anharmonic effects can be coupled to electronic and lattice dynamics in cuprate systems by performing the exact diagonalization of a prototype anharmonic many-body Hamiltonian on a relevant six-atom cluster and show that the EXAFS results can be understood as a Kuramoto synchronization between coupled internal quantum tunneling polarons associated with the two-site distribution of the copper-apical-oxygen ($Cu-O_{ap}$) pair in the dynamic structure. Furthermore, we find that this first order, anti-phase synchronization transition can be fine tuned by temperature and anharmonicity of the lattice vibrations, and promotes the pumping of charge, initially stored at the apical oxygen reservoirs, into the copper-oxide planes. Simultaneously, the internal quantum tunneling polaron extends to the copper-planar-oxygen ($Cu-O_{pl}$) pair. All these findings support an interpretation of the EXAFS data in terms of an effective, quantum mechanical triple-well-potential, which accurately represents the anti-phase synchronization of apical oxygens displacements and lattice-assisted charge transfer to the $CuO_2$ plane.

cond-mat.supr-con