arXiv subjects

Andrea Prosperetti

Publications and source records attributed to Andrea Prosperetti.

At least 19 recordsLinked to original sources

arXiv2026

Leidenfrost droplets: The roles of ambient humidity and internal droplet circulation

A volatile droplet gently deposited on a superheated substrate can sit on a thin film of its own vapour, which prevents contact between the drop and surface. This phenomenon is called the Leidenfrost effect. In this paper, through direct numerical simulations, we analyse characteristics of Leidenfrost water droplets with a single computational model over four decades of droplet radius, stitching together previous works in the limit of large and small droplets. Using the model, we show that the ambient humidity, an underappreciated factor in the Leidenfrost system, in combination with the flow in the drop has a significant impact on the geometry and drying kinetics. Our results imply the inadequacies of commonly made assumptions of a pure vapour phase and an isothermal droplet. When modelling large Leidenfrost droplets with an axisymmetric model, large discrepancies between experiments and the computational results occur. Through azimuthal stability analysis, we show that this is due to the unrealistic constraint of axisymmetry. This finding is supported by 3D simulations of a simplified model. Finally, some hypotheses are explored to account for the remaining discrepancies with experimental data.

physics.flu-dyn↗

arXiv2024

Particle Re-Suspension in Two-Phase Dispersed Rayleigh-B\'{e}nard Convection

The process by which particles are entrained by the fluid in Rayleigh-B\'{e}nard convection is studied by means of particle-resolved numerical simulations in a periodic domain at a Rayleigh number of $10^7$. The fluid Prandtl number is 1 and the particle-to-fluid density ratio 1.1. The results show that the horizontal velocity field near the bottom of the cell accumulates particles in heaps, or `dunes', at the base of ascending plumes. The dunes deflect the incoming flow, conferring to it a vertical velocity component which entrains the particles up the dune and into the plume. An experimental observation of this mechanism was briefly reported by Solomatov et al. (Earth Planet. Sc. Lett. 120, 387, 1993) but has not been considered further in the literature. By its very nature, such a process cannot be simulated by the point particle model. The final particle load carried by the convection depends both on the available gravitational energy of the fluid and on the effectiveness of the re-suspension mechanism.

physics.flu-dyn↗

arXiv2021

Crown formation from a cavitating bubble close to a free surface

A rapidly growing bubble close to a free surface induces jetting: a central jet protruding outwards and a crown surrounding it at later stages. While the formation mechanism of the central jet is known and documented, that of the crown remains unsettled. We perform axisymmetric simulations of the problem using the free software program basilisk, where a finite-volume compressible solver has been implemented, that uses a geometric Volume-of-Fluid method (VoF) for the tracking of the interface. We show that the mechanism of crown formation is a combination of a pressure distortion over the curved interface, inducing flow focusing, and of a flow reversal, caused by the second expansion of the toroidal bubble that drives the crown. The work culminates in a parametric study with the Weber number, the Reynolds number, the pressure ratio and the dimensionless bubble distance to the free surface as control parameters. Their effects on both the central jet and the crown are explored. For high Weber numbers, we observe the formation of weaker "secondary crowns", highly correlated with the third oscillation cycle of the bubble.

physics.flu-dyn↗

arXiv2021

Marangoni instability of a drop in a stably stratified liquid

Marangoni instabilities can emerge when a liquid interface is subjected to a concentration or temperature gradient. It is generally believed that for these instabilities bulk effects like buoyancy are negligible as compared to interfacial forces, especially on small scales. Consequently, the effect of a stable stratification on the Marangoni instability has hitherto been ignored. Here we report, for an immiscible drop immersed in a stably stratified ethanol-water mixture, a new type of oscillatory solutal Marangoni instability which is triggered once the stratification has reached a critical value. We experimentally explore the parameter space spanned by the stratification strength and the drop size and theoretically explain the observed crossover from levitating to bouncing by balancing the advection and diffusion around the drop. Finally, the effect of the stable stratification on the Marangoni instability is surprisingly amplified in confined geometries, leading to an earlier onset.

physics.flu-dyn↗

arXiv2021

Plasmonic Microbubble Dynamics in Binary Liquids

The growth of surface plasmonic microbubbles in binary water/ethanol solutions is experimentally studied. The microbubbles are generated by illuminating a gold nanoparticle array with a continuous wave laser. Plasmonic bubbles exhibit ethanol concentration-dependent behaviors. For low ethanol concentrations (f_e) of < 67.5%, bubbles do not exist at the solid-liquid interface. For high f_e values of >80%, the bubbles behave as in pure ethanol. Only in an intermediate window of 67.5% < f_e < 80% do we find sessile plasmonic bubbles with a highly nontrivial temporal evolution, in which as a function of time three phases can be discerned. (1) In the first phase, the microbubbles grow, while wiggling. (2) As soon as the wiggling stops, the microbubbles enter the second phase in which they suddenly shrink, followed by (3) a steady reentrant growth phase. Our experiments reveal that the sudden shrinkage of the microbubbles in the second regime is caused by a depinning event of the three phase contact line. We systematically vary the ethanol concentration, laser power, and laser spot size to unravel water recondensation as the underlying mechanism of the sudden bubble shrinkage in phase 2.

cond-mat.soft↗

arXiv2020

Dynamics of a toroidal bubble on a cylinder surface with an application to geophysical exploration

During the operation of a seismic airgun source, a certain amount of compressed high-pressure air is released from the airgun chamber into the surrounding water, generating an expanding toroidal bubble attached to the airgun-body. The subsequent oscillations of the bubble generate low-frequency pressure waves, which are used to map the ocean subbottom, e.g., to locate oil and gas reserves. The bubble dynamic behavior and the emitted pressure waves are inevitably influenced by the airgun-body. However, the bubble-airgun-body interaction is far from well understood. This paper investigates the strong interaction between a long cylinder and an attached toroidal bubble via hundreds of boundary integral simulations, aiming to provide new physical insights for airgun-bubble dynamics. Firstly, the overall physical phenomena are discussed and three types of bubble collapse patterns are identified, namely (i) upward jetting due to gravity, (ii) annular jet toward the cylinder body and (iii) weak/no jet. Thereafter, we investigate the effects of the cylinder radius, initial bubble pressure and Froude number on the bubble oscillation period and the pressure wave induced by the bubble. At last, the impact of a cylinder on a Sercel type airgun-bubble is discussed with a particular focus on the spectrum of the pressure waves.

physics.flu-dyn↗

arXiv2020

Gas-Vapor Interplay in Plasmonic Bubble Shrinkage

The understanding of the shrinkage dynamics of plasmonic bubbles formed around metallic nanoparticles immersed in liquid and irradiated by a resonant light source is crucial for the usage of these bubbles in numerous applications. In this paper we experimentally show and theoretically explain that a plasmonic bubble during its shrinkage undergoes two different phases: first, a rapid partial bubble shrinkage governed by vapor condensation and, second, a slow diffusion-controlled bubble dissolution. The history of the bubble formation plays an important role in the shrinkage dynamics during the first phase, as it determines the gas-vapor ratio in the bubble composition. Higher laser powers lead to more vaporous bubbles, while longer pulses and higher dissolved air concentrations lead to more gaseous bubbles. The dynamics of the second phase barely depends on the history of bubble formation, i.e. laser power and pulse duration, but strongly on the dissolved air concentration, which defines the concentration gradient at the bubble interface. Finally, for the bubble dissolution in the second phase, with decreasing dissolved air concentration, we observe a gradual transition from a $R(t) \propto (t_0 - t) ^{1/3}$ scaling law to a $R(t) \propto (t_0 - t) ^{1/2}$ scaling law, where $t_0$ is the lifetime of the bubble and theoretically explain this transition.

physics.flu-dyn↗

arXiv2020

Modelling large scale airgun-bubble dynamics with highly non-spherical features

A thorough understanding of the dynamics of meter-sized airgun-bubbles is very crucial to seabed geophysical exploration. In this study, we use the boundary integral method to investigate the highly non-spherical airgun-bubble dynamics and its corresponding pressure wave emission. Moreover, a model is proposed to also consider the process of air release from the airgun port, which is found to be the most crucial factor to estimate the initial peak of the pressure wave. The numerical simulations show good agreement with experiments, in terms of non-spherical bubble shapes and pressure waves. Thereafter, the effects of the port opening time $T\rm_{open}$, airgun firing depth, heat transfer, and gravity are numerically investigated. We find that a smaller $T\rm_{open}$ leads to a more violent air release that consequently causes stronger high-frequency pressure wave emissions; however, the low-frequency pressure waves are little affected. Additionally, the non-spherical bubble dynamics is highly dependent on the Froude number $Fr$. Starting from $Fr=2$, as $Fr$ increases, the jet contains lower kinetic energy, resulting in a stronger energy focusing of the bubble collapse itself and thus a larger pressure peak during the bubble collapse phase. For $Fr \ge 7$, the spherical bubble theory becomes an appropriate description of the airgun-bubble. The new findings of this study may provide a reference for practical operations and designing environmentally friendly airguns in the near future.

physics.flu-dyn↗

arXiv2018

A bouncing oil droplet in a stratified liquid and its sudden death

Droplets can self-propel when immersed in another liquid in which a concentration gradient is present. Here we report the experimental and numerical study of a self-propelling oil droplet in a vertically stratified ethanol/water mixture: At first, the droplet sinks slowly due to gravity, but then, before having reached its density matched position, jumps up suddenly. More remarkably, the droplet bounces repeatedly with an ever increasing jumping distance, until all of a sudden it stops after about 30 min. We identify the Marangoni stress at the droplet/liquid interface as responsible for the jumping: its strength grows exponentially because it pulls down ethanol-rich liquid, which in turn increases its strength even more. The jumping process can repeat because gravity restores the system. Finally, the sudden death of the jumping droplet is also explained. Our findings have demonstrated a type of prominent droplet bouncing inside a continuous medium with no wall or sharp interface.

physics.flu-dyn↗

arXiv2016

Tribonucleation of bubbles

We report on the nucleation of bubbles on solids that are gently rubbed against each other in a liquid. The phenomenon is found to depend strongly on the material and roughness of the solid surfaces. For a given surface, temperature, and gas content, a trail of growing bubbles is observed if the rubbing force and velocity exceed a certain threshold. Direct observation through a transparent solid shows that each bubble in the trail results from the early coalescence of several microscopic bubbles, themselves detaching from microscopic gas pockets forming between the solids. From a detailed study of the wear tracks, with atomic force and scanning electron microscopy imaging, we conclude that these microscopic gas pockets originate from a local fracturing of the surface asperities, possibly enhanced by chemical reactions at the freshly created surfaces. Our findings will be useful either for preventing undesired bubble formation or, on the contrary, for "writing with bubbles," i.e., creating controlled patterns of microscopic bubbles.

physics.flu-dyn↗

arXiv2016

Dynamic Leidenfrost effect: relevant time- and length-scales

When a liquid droplet impacts a hot solid surface, enough vapor may be generated under it as to prevent its contact with the solid. The minimum solid temperature for this so-called Leidenfrost effect to occur is termed the Leidenfrost temperature, or the dynamic Leidenfrost temperature when the droplet velocity is non-negligible. We observe the wetting/drying and the levitation dynamics of the droplet impacting on an (isothermal) smooth sapphire surface using high speed total internal reflection imaging, which enables us to observe the droplet base up to about 100 nm above the substrate surface. By this method we are able to reveal the processes responsible for the transitional regime between the fully wetting and the fully levitated droplet as the solid temperature increases, thus shedding light on the characteristic time- and length-scales setting the dynamic Leidenfrost temperature for droplet impact on an isothermal substrate.

physics.flu-dyn↗

arXiv2014

Heat transport in boiling turbulent Rayleigh-Bénard convection

Boiling is an extremely effective way to promote heat transfer from a hot surface to a liquid due to several mechanisms many of which are not understood in quantitative detail. An important component of the overall process is that the buoyancy of the bubbles compounds with that of the liquid to give rise to a much enhanced natural convection. In this paper we focus specifically on this enhancement and present a numerical study of the resulting two-phase Rayleigh-Bénard convection process. We make no attempt to model other aspects of the boiling process such as bubble nucleation and detachment. We consider a cylindrical cell with a diameter equal to its height. The cell base and top are held at temperatures above and below the boiling point of the liquid, respectively. By keeping the temperature difference constant and changing the liquid pressure we study the effect of the liquid superheat in a Rayleigh number range that, in the absence of boiling, would be between $2\times10^6$ and $5\times10^9$. We find a considerable enhancement of the heat transfer and study its dependence on the bubble number, the degree of superheat of the hot cell bottom and the Rayleigh number. The increased buoyancy provided by the bubbles leads to more energetic hot plumes detaching from the hot cell bottom and, as a consequence, the strength of the circulation in the cell is significantly increased. Our results are in general agreement with recent experimental results of Zhong et al., Phys. Rev. Lett. {\bf 102}, 124501 (2009) for boiling Rayleigh-Bénard convection.

physics.flu-dyn↗

arXiv2013

Leidenfrost temperature increase for impacting droplets on carbon-nanofiber surfaces

Droplets impacting on a superheated surface can either exhibit a contact boiling regime, in which they make direct contact with the surface and boil violently, or a film boiling regime, in which they remain separated from the surface by their own vapor. The transition from the contact to the film boiling regime depends not only on the temperature of the surface and kinetic energy of the droplet, but also on the size of the structures fabricated on the surface. Here we experimentally show that surfaces covered with carbon-nanofibers delay the transition to film boiling to much higher temperature compared to smooth surfaces. We present physical arguments showing that, because of the small scale of the carbon fibers, they are cooled by the vapor flow just before the liquid impact, thus permitting contact boiling up to much higher temperatures than on smooth surfaces. We also show that, as long as the impact is in the film boiling regime, the spreading factor of impacting droplets follows the same $\We^{3/10}$ scaling (with $\We$ the Weber number) found for smooth surfaces, which is caused by the vapor flow underneath the droplet.

physics.flu-dyn↗

arXiv2013

Growing bubbles in a slightly supersaturated liquid solution

We have designed and constructed an experimental system to study gas bubble growth in slightly supersatu- rated liquids. This is achieved by working with carbon dioxide dissolved in water, pressurized at a maximum of 1 MPa and applying a small pressure drop from saturation conditions. Bubbles grow from hydrophobic cavities etched on silicon wafers, which allows us to control their number and position. Hence, the experiment can be used to investigate the interaction among bubbles growing in close proximity when the main mass transfer mechanism is diffusion and there is a limited availability of the dissolved species.

physics.flu-dyn↗

arXiv2012

Oscillations of a gas pocket on a liquid-covered solid surface

The dynamic response of a gas bubble entrapped in a cavity on the surface of a submerged solid subject to an acoustic field is investigated in the linear approximation. We derive semi-analytical expressions for the resonance frequency, damping and interface shape of the bubble. For the liquid phase, we consider two limit cases: potential flow and unsteady Stokes flow. The oscillation frequency and interface shape are found to depend on two dimensionless parameters: the ratio of the gas stiffness to the surface tension stiffness, and the Ohnesorge number, representing the relative importance of viscous forces. We perform a parametric study and show, among others, that an increase in the gas pressure or a decrease in the surface tension leads to an increase in the resonance frequency until an asymptotic value is reached.

physics.flu-dyn↗

arXiv2012

Taming Acoustic Cavitation

In this fluid dynamics video we show acoustic cavitation occurring from pits etched on a silicon surface. By immersing the surface in a liquid, gas pockets are entrapped in the pits which upon ultrasonic insonation, are observed to shed cavitation bubbles. Modulating the driving pressure it is possible to induce different behaviours based on the force balance that determines the interaction among bubbles and the silicon surface. This system can be used for several applications like sonochemical water treatment, cleaning of surfaces with deposited materials such as biofilms.

physics.flu-dyn↗

arXiv2012

Highly focused supersonic microjets: numerical simulations

By focusing a laser pulse inside a capillary partially filled with liquid, a vapour bubble is created which emits a pressure wave. This pressure wave travels through the liquid and creates a fast, focused axisymmetric microjet when it is reflected at the meniscus. We numerically investigate the formation of this microjet using axisymmetric boundary-integral simulations, where we model the pressure wave as a pressure pulse applied on the bubble. We find a good agreement between the simulations and experimental results in terms of the time evolution of the jet and on all parameters that can be compared directly. We present a simple analytical model that accurately predicts the velocity of the jet after the pressure pulse and its maximum velocity.

physics.flu-dyn↗

arXiv2012

Efficient Sonochemistry through Microbubbles Generated with Micromachined Surfaces

Sonochemical reactors are used in water treatment, the synthesis of fine chemicals, pharmaceutics and others. The low efficiency of sonoreactors have prevented its massive usage at industrial scales. Controlling the appearance of bubbles in place and time is the most limiting factor. A novel type of sonochemical reactor was designed making use of micro-fabrication techniques to control the nucleation sites of micro-bubbles. The efficiency was increased first by locating the nucleation sites in the most active region of a micro-chamber; additionally the desired chemical effect was significantly higher at the same powers than when not controlled. Silicon substrates were micromachined with "artificial nucleation sites" or pits, and placed at the bottom of the micro-chamber. The pits entrap gas which, upon ultrasonic excitation, sheds off a stream of microbubbles. The gas content of the pits is not depleted but is replenished by diffusion and the emission of microbubbles can continue for hours.

physics.chem-ph↗