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Andrea Raggio

Publications and source records attributed to Andrea Raggio.

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Isomeric yield ratios and mass spectrometry of Y and Nb isotopes in the neutron-rich N=60 region: the unusual case of $^{98}$Y

The isomeric yield ratio (IYR) of fission products is an observable that carries relevant information about the fragments emerging from the scission of a fissioning nucleus. We report on IYR of $^{96,98,100}$Y and $^{100,102}$Nb, together with the previously reported values for $^{97}$Y and $^{99}$Nb, produced in the 28 MeV $\alpha$-induced fission of $^{232}$Th at the Ion Guide Isotope Separation On-Line (IGISOL) facility of the University of Jyv{\"a}skyl{\"a}. We measured the IYR using two different techniques, the phase-imaging ion-cyclotron-resonance (PI-ICR) and the multiple-reflection time-of-flight mass spectrometry (MR-TOF-MS) methods. Moreover, we measured the masses of the long-lived states in $^{98,100}$Y and $^{100,102}$Nb populated via in-trap $\beta$-decay of their precursors. Since the $\beta$-decay selectively populates states with a favourable spin-parity, we could identify the measured state and show that the ground state is the low-spin state in the cases of $^{98}$Y and $^{100}$Nb, while it is the high-spin state in the cases of $^{100}$Y and $^{102}$Nb. This measurement confirms the spin-parity assignments of all the nuclei as they are reported in the NUBASE2020 evaluations, disagreeing with the assignment for $^{100}$Y reported in the ENSDF evaluation. Making also use of previously reported data, we observe an anomalously low IYR for the $N=59$ isotope $^{98}$Y as compared to other yttrium or neighboring niobium isotopes. This behavior is very rare across the nuclear chart and is posited to be connected to the characteristic shape coexistence of $^{98}$Y, and to the change in the charge radii of the ground and excited states in the $N=58-60$ region.

nucl-ex

Disentangling the influence of excitation energy and compound nucleus angular momentum on fission fragment angular momentum

The origin of the large angular momenta observed for fission fragments is still a question under discussion. To address this, we study isomeric yield ratios (IYR), i.e. the relative population of two or more long-lived metastable states with different spins, of fission products. We report on IYR of 17 isotopes produced in the 28 MeV $\alpha$-induced fission of $^{232}$Th at the IGISOL facility of the University of Jyv\"askyl\"a. The fissioning nuclei in this reaction are $^{233,234,235}$U*. We compare our data to IYR from thermal neutron-induced fission of $^{233}$U and $^{235}$U, and we observe statistically significant larger IYR in the $^{232}$Th($\alpha$,f) reaction, where the average compound nucleus (CN) spin is 7.5 $\hbar$, than in $^{233,235}$U(n$_{th}$,f), with average spins 2.5 and 3.5 $\hbar$, respectively. To assess the influence of the excitation energy, we study literature data of IYR from photon-induced fission reactions, and find that the IYR are independent of the CN excitation energy. We conclude that the different IYR must be explained by the different CN spin alone. This implies that the FF angular momentum only partly comes from the fission process itself, and is in addition influenced by the angular momentum present in the CN.

nucl-ex

High-precision mass measurements of neutron deficient silver isotopes probe the robustness of the $N$ = 50 shell closure

High-precision mass measurements of exotic $^{95-97}$Ag isotopes close to the $N = Z$ line have been conducted with the JYFLTRAP double Penning trap mass spectrometer, with the silver ions produced using the recently commissioned inductively-heated hot cavity catcher laser ion source at the Ion Guide Isotope Separator On-Line facility. The atomic mass of $^{95}$Ag was directly determined for the first time. In addition, the atomic masses of $\beta$-decaying 2$^+$ and 8$^+$ states in $^{96}$Ag have been identified and measured for the first time, and the precision of the $^{97}$Ag mass has been improved. The newly measured masses, with a precision of $\approx$ 1 keV/c$^2$, have been used to investigate the $N =$ 50 neutron shell closure confirming it to be robust. Empirical shell-gap and pairing energies determined with the new ground-state mass data are compared with the state-of-the-art \textit{ab initio} calculations with various chiral effective field theory Hamiltonians. The precise determination of the excitation energy of the $^{96m}$Ag isomer in particular serves as a benchmark for \textit{ab initio} predictions of nuclear properties beyond the ground state, specifically for odd-odd nuclei situated in proximity to the proton dripline below $^{100}$Sn. In addition, density functional theory (DFT) calculations and configuration-interaction shell-model (CISM) calculations are compared with the experimental results. All theoretical approaches face challenges to reproduce the trend of nuclear ground-state properties in the silver isotopic chain across the $N =$50 neutron shell and toward the proton drip-line.

nucl-ex

RAPTOR: a new collinear laser ionization spectroscopy and laser-radiofrequency double-resonance experiment at the IGISOL facility

RAPTOR, Resonance ionization spectroscopy And Purification Traps for Optimized spectRoscopy, is a new collinear resonance ionization spectroscopy device constructed at the Ion Guide Isotope Separator On-Line (IGISOL) facility at the University of Jyväskylä, Finland. By operating at beam energies of under 10 keV, the footprint of the experiment is reduced compared to more traditional collinear laser spectroscopy beamlines. In addition, RAPTOR is coupled to the JYFLTRAP Penning trap mass spectrometer, opening a window to laser-assisted nuclear-state selective purification, serving not only the mass measurement program, but also supporting post-trap decay spectroscopy experiments. Finally, the low-energy ion beams used for RAPTOR will enable high-precision laser-radiofrequency double-resonance experiments, resulting in spectroscopy with linewidths below 1 MHz. In this contribution, the technical layout of RAPTOR and a selection of ion-beam optical simulations for the device are presented, along with a discussion of the current status of the commissioning experiments.

physics.ins-det