arXiv subjects

Andreas Buchleitner

Publications and source records attributed to Andreas Buchleitner.

At least 37 records · Page 2Linked to original sources

arXiv2023

Measuring the quantum state of photoelectrons

A photoelectron, emitted due to the absorption of light quanta as described by the photoelectric effect, is often characterized experimentally by a classical quantity, its momentum. However, since the photoelectron is a quantum object, its rigorous characterization requires the reconstruction of the complete quantum state, the photoelectron's density matrix. Here, we use quantum state tomography to fully characterize photoelectrons emitted from helium and argon atoms upon absorption of ultrashort, extreme ultraviolet light pulses. While in helium we measure a pure photoelectronic state, in argon, spin-orbit interaction induces entanglement between the ion and the photoelectron, leading to a reduced purity of the photoelectron state. Our work shows how state tomography gives new insights into the fundamental quantum aspects of light-induced electronic processes in matter, bridging the fields of photoelectron spectroscopy and quantum information, and offering new spectroscopic possibilities for quantum technology.

quant-ph↗

arXiv2023

Hong-Ou-Mandel interference of composite particles

We study the Hong-Ou-Mandel interference of two identical, composite particles, each formed of two bosonic or fermionic constituents, as they scatter against a potential barrier in a one-dimensional lattice. For tightly bound composites, we show that the combination of their constituents' mutual interactions and exchange symmetry gives rise to an effective nearest-neighbour interaction between composites, which induces a reduction of the interference contrast.

quant-ph↗

arXiv2023

Hong-Ou-Mandel interference on a lattice: symmetries and interactions

We describe the Hong-Ou-Mandel interference of two identical particles evolving on a one-dimensional tight-binding lattice where a potential barrier plays the role of a beam splitter. Careful consideration of the symmetries underlying the two-particle interference effect allows us to reformulate the problem in terms of ordinary wave interference in a Michelson interferometer. This approach is easily generalized to the case where the particles interact, and we compare the resulting analytical predictions for the bunching probability to numerical simulations of the two-particle dynamics.

quant-ph↗

arXiv2023

Indistinguishability of identical bosons from a quantum information theory perspective

Using tools from quantum information theory, we present a general theory of indistinguishability of identical bosons in experiments consisting of passive linear optics followed by particle number detection. Our results do neither rely on additional assumptions on the input state of the interferometer, such as, for instance, a fixed mode occupation, nor on any assumption on the degrees of freedom that potentially make the particles distinguishable. We identify the expectation value of the projector onto the $N$-particle symmetric subspace as an operationally meaningful measure of indistinguishability, and derive tight lower bounds on it that can be efficiently measured in experiments. Moreover, we present a consistent definition of perfect distinguishability and characterize the corresponding set of states. In particular, we show that these states are diagonal in the computational basis up to a permutationally invariant unitary. Moreover, we find that convex combinations of states that describe partially distinguishable and perfectly indistinguishable particles can lead to perfect distinguishability, which itself is not preserved under convex combinations.

quant-ph↗

arXiv2023

First-detection-time statistics in many-body quantum transport

We study the transport of many partially distinguishable and possibly interacting particles under the action of repeated projective measurements on a target space and investigate how the particles' interference affects the mean first detection time. We contrast the detection of exactly $n$ versus at least $n$ particles, explain divergences in the mean first detection time through spectral properties of the generating evolution operator, and illustrate our findings by an example.

quant-ph↗

arXiv2023

Highly-transmitting modes of light in dynamic atmospheric turbulence

We show that instantaneous spatial singular modes of light in a dynamically evolving, turbulent atmosphere offer significantly improved high-fidelity signal transmission as compared to standard encoding bases corrected by adaptive optics. Their enhanced stability in stronger turbulence is associated with a subdiffusive algebraic decay of the transmitted power with evolution time.

physics.optics↗

arXiv2023

An Energy Estimation Benchmark for Quantum Computers

Certifying the performance of quantum computers requires standardized tests. We propose a simple energy estimation benchmark that is motivated from quantum chemistry. With this benchmark we statistically characterize the noisy outcome of the IBM Quantum System One in Ehningen, Germany. We find that the benchmark results hardly correlate with the gate errors and readout errors reported for the device. In a time-resolved analysis, we monitor the device over several hours and find two-hour oscillations of the benchmark results, as well as outliers, which we cannot explain from the reported device status. We then show that the implemented measurement error mitigation techniques cannot resolve these oscillations, which suggests that deviations from the theoretical benchmark outcome statistics do not stem solely from the measurement noise of the device.

quant-ph↗

arXiv2022

Many-body coherence and entanglement probed by randomized correlation measurements

We show how coherences between identical constituents of a many-body quantum state can be interrogated by suitable correlation functions, and identify sufficient conditions under which low-order correlators fully characterize many-body coherences, as controlled by the constituents' mutual distinguishability. Comparison of correlators of different order detects many-body entanglement.

quant-ph↗

arXiv2022

Quantized fields for optimal control in the strong coupling regime

We tailor the quantum statistics of a bosonic field to deterministically drive a quantum system into a target state. Experimentally accessible states of the field achieve good control of multi-level or -qubit systems, notably also at coupling strengths beyond the rotating-wave approximation. This extends optimal control theory to the realm of fully quantized, strongly coupled control and target degrees of freedom.

quant-ph↗

arXiv2022

Many-body quantum non-Markovianity

We port the concept of non-Markovian quantum dynamics to the many-particle realm, by a suitable decomposition of the many-particle Hilbert space. We show how the specific structure of many-particle states determines the observability of non-Markovianity by single- or many-particle observables, and discuss a realization in a readily implementable few-particle set-up.

quant-ph↗

arXiv2022

Optimal route to quantum chaos in the Bose-Hubbard model

The dependence of the chaotic phase of the Bose-Hubbard Hamiltonian on particle number $N$, system size $L$ and particle density is investigated in terms of spectral and eigenstate features. We analyze the development of the chaotic phase as the limit of infinite Hilbert space dimension is approached along different directions, and show that the fastest route to chaos is the path at fixed density $n \lesssim 1$. The limit $N \to \infty$ at constant $L$ leads to a slower convergence of the chaotic phase towards the random matrix theory benchmarks. In this case, from the distribution of the eigenstate generalized fractal dimensions, the ergodic phase becomes more distinguishable from random matrix theory for larger $N$, in a similar way as along trajectories at fixed density.

quant-ph↗

arXiv2022

Continuous variable quantum state tomography of photoelectrons

We propose a continuous variable quantum state tomography protocol of electrons which result from the ionization of atoms or molecules by the absorption of extreme ultraviolet light pulses. Our protocol is benchmarked against a direct calculation of the quantum state of photoelectrons ejected from helium and argon in the vicinity of a Fano resonance. In the latter case, we furthermore distill ion-photoelectron entanglement due to spin-orbit splitting. This opens new routes towards the investigation of quantum coherence and entanglement properties on the ultrafast timescale.

physics.atom-ph↗

arXiv2022

Chaos in the Bose-Hubbard model and random two-body Hamiltonians

We investigate the chaotic phase of the Bose-Hubbard model [L. Pausch et al, Phys. Rev. Lett. 126, 150601 (2021)] in relation to the bosonic embedded random matrix ensemble, which mirrors the dominant few-body nature of many-particle interactions, and hence the Fock space sparsity of quantum many-body systems. The energy dependence of the chaotic regime is well described by the bosonic embedded ensemble, which also reproduces the Bose-Hubbard chaotic eigenvector features, quantified by the expectation value and eigenstate-to-eigenstate fluctuations of fractal dimensions. Despite this agreement, in terms of the fractal dimension distribution, these two models depart from each other and from the Gaussian orthogonal ensemble as Hilbert space grows. These results provide further evidence of a way to discriminate among different many-body Hamiltonians in the chaotic regime.

quant-ph↗

arXiv2021

Theory of multiple quantum coherence signals in dilute thermal gases

Manifestations of dipole-dipole interactions in dilute thermal gases are difficult to sense because of strong inhomogeneous broadening. Recent experiments reported signatures of such interactions in fluorescence detection-based measurements of multiple quantum coherence (MQC) signals, with many characteristic features hitherto unexplained. We develop an original open quantum systems theory of MQC in dilute thermal gases, which allows us to resolve this conundrum. Our theory accounts for the vector character of the atomic dipoles as well as for driving laser pulses of arbitrary strength, includes the far-field coupling between the dipoles, which prevails in dilute ensembles, and effectively incorporates atomic motion via a disorder average. We show that collective decay processes -- which were ignored in previous treatments employing the electrostatic form of dipolar interactions -- play a key role in the emergence of MQC signals.

quant-ph↗

arXiv2021

Characterizing four-body indistinguishability via symmetries

We show how to characterize the indistinguishability of up to four identical, bosonic or fermionic particles, which are rendered partially distinguishable through their internal degrees of freedom prepared in mixed states. This is accomplished via their counting statistics when subjected to a highly symmetric unitary acting upon their external (i.e., dynamical) degrees of freedom. For pure internal states, we further extract information on the particles' collective phases, which ultimately allows for an experimental reconstruction of the full many-particle density operator up to complex conjugation.

quant-ph↗

arXiv2021

Wave-particle duality of many-body quantum states

We formulate a general theory of wave-particle duality for many-body quantum states, which quantifies how wave- and particle-like properties balance each other. Much as in the well-understood single-particle case, which-way information -- here on the level of many-particle paths -- lends particle-character, while interference -- here due to coherent superpositions of many-particle amplitudes -- indicates wave-like properties. We analyze how many-particle which-way information, continuously tunable by the level of distinguishability of fermionic or bosonic, identical and possibly interacting particles, constrains interference contributions to many-particle observables and thus controls the quantum-to-classical transition in many-particle quantum systems. The versatility of our theoretical framework is illustrated for Hong-Ou-Mandel- and Bose-Hubbard-like exemplary settings.

quant-ph↗

arXiv2021

Pulse area dependence of multiple quantum coherence signals in dilute thermal gases

In the general framework of open quantum systems, we assess the impact of the pulse area on single and double quantum coherence (1QC and 2QC) signals extracted from fluorescence emitted by dilute thermal gases. We show that 1QC and 2QC signals are periodic functions of the pulse area, with distinctive features which reflect the particles' interactions via photon exchange, the polarizations of the laser pulses, and the observation direction.

quant-ph↗

arXiv2021

Optimization of selective two-photon absorption in cavity polaritons

We investigate optimal states of photon pairs to excite a target transition in a multilevel quantum system. With the help of coherent control theory for two-photon absorption with quantum light, we infer the maximal population achievable by optimal entangled vs. separable states of light. Interference between excitation pathways, as well as the presence of nearby states, may hamper the selective excitation of a particular target state, but we show that quantum correlations can help to overcome this problem, and enhance the achievable "selectivity" between two energy levels, i.e. the relative difference in population transferred into each of them. We find that the added value of optimal entangled states of light increases with broadening linewidths of the target states.

quant-ph↗