arXiv subjects

Andreas D. Wieck

Publications and source records attributed to Andreas D. Wieck.

At least 19 recordsLinked to original sources

arXiv2026

Active control of THz plasmon propagation in a one-dimensional electronic waveguide

Quantum nanoelectronics is pushing towards ever higher operating frequencies in order to realise quantum technologies capable of processing information at unprecedented speeds. A particularly promising direction is the development of flying electron qubits, which offer the prospect of quantum operations on picosecond timescales. Achieving in-flight quantum control in this regime would establish a fundamentally new paradigm for studying quantum entanglement and enable a novel form of quantum information processing based on propagating electronic wavepackets. Here we report a first step towards this goal by injecting ultrashort electron wavepackets into an engineered quantum nanoelectronic device. We demonstrate active control over the propagation speed of an electron wavepacket with a temporal duration as short as 4 ps in a quasi-one-dimensional electron waveguide with a length ranging from 10 $\mathrmμ$m to 40 $\mathrmμ$m. This advance provides a key building block for ultrafast quantum operations using flying electrons. Beyond its technological implications, our approach offers a platform for exploring the intrinsic dynamical processes that govern quantum transport and coherence in nanoscale electronic systems.

cond-mat.mes-hall↗

arXiv2026

Robust biexciton preparation for entangled photon-pair generation by single-shot Floquet driving

Quantum emitters driven by resonant two-photon excitation are a leading source for deterministically generated entangled photon pairs, essential for scalable photonic quantum technologies. However, conventional excitation schemes pose various constraints, limiting their scalability and practicability. Here, we demonstrate how biexciton preparation schemes with significantly improved robustness and reduced experimental demands can be identified using a novel design principle: ultrafast single-shot Floquet driving. This is achieved by employing two strongly and symmetrically detuned dichromatic pulses, whose superposition generates a stroboscopic Hamiltonian that enables direct coupling between ground and biexciton states. Moreover, a pulse delay serves as a tuning knob, introducing an effective magnetic field making biexciton preparation particularly robust. Experimentally, we achieve a biexciton occupation exceeding 96% and preserve photon-pair entanglement with a fidelity of 93.4%. Our work opens avenues for designing a class of quantum control protocols with superior performance across diverse quantum emitters and qubit platforms.

quant-ph↗

arXiv2026

Real-time dynamics of triplet-resonant tunneling driven by nonequilibrium phonons

Driven nonequilibrium systems can host emergent functionalities beyond equilibrium, but real-time access to excited-state dynamics remains limited. Here we report real-time measurements of phonon-driven charge and spin dynamics in excited states of a double quantum dot. Under phonon irradiation, resonant inter-dot tunneling emerges at triplet resonance. Time-resolved charge sensing reveals that the resonant inter-dot tunneling is strongly modified by spin blockade. For weaker inter-dot coupling, the nonequilibrium phonon environment generates a unidirectional transport cycle along the phonon density gradient.

cond-mat.mes-hall↗

arXiv2026

Spectral shadows of a single GaAs quantum dot

Semiconductor quantum dots are a promising platform for generating single and entangled photons.Still, their use is limited even in the most advanced structures by changes in the charge state of the quantum dot and its environment. Here, we present detailed time-resolved resonance fluorescence measurements on a single charge-tunable GaAs quantum dot, shedding new light on the spectral shadows invoked by the complex impurity environment. Detuning-dependent measurements reveal the existence of multiple Stark-shifted resonances, which are associated with rare spectral jumps smaller than the homogeneous linewidth and, therefore, typically concealed in the measurement noise. We observe similar environmentally induced Stark shifts for both the neutral exciton and negatively charged trion transitions, while the positively and doubly negatively charged trions exhibit significant differences. Our investigation quantifies the underlying impurity charge dynamics over a range from well below milliseconds to seconds, revealing that the hole occupation of the positively charged trion transition is constrained by rapid hole loss and slow hole recapture dynamics. Utilizing a second non-resonant laser, we increase the hole occupancy by over an order of magnitude and identify both a prolonged hole residence time and an enhanced hole tunneling rate into the quantum dot. These findings are supported by complementary spin noise spectroscopy measurements, which offer a significantly higher bandwidth compared to the time-resolved resonance fluorescence measurements.

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arXiv2026

Near transform-limited single photons from rapid-thermal annealed quantum dots

Single-photon emitters are essential components for quantum communication systems, enabling applications such as secure quantum key distribution and the long-term vision of a quantum internet. Among various candidates, self-assembled InAs/GaAs quantum dots (QDs) remain highly promising due to their ability to emit coherent and indistinguishable photons, as well as their compatibility with photonic integration. In this work, we investigate the impact of post-growth rapid thermal annealing (RTA) on the quantum optical properties of single self-assembled QDs embedded in a p-i-n diode structure. The annealing process induces a controlled blueshift of the emission wavelength by promoting Ga in-diffusion and intermixing. Using resonance fluorescence measurements at cryogenic temperatures (4.2 K), we investigate the single-photon statistics, the emission linewidths, and coherence time $T_2$ of the emitted photons. Our results show that, despite the high annealing temperature of $760^\circ$C, the process does not degrade the optical quality of the quantum dots strongly. Instead, we observe single-photon emission with near transform-limited linewidths, where the dephasing time $T_2$ is only a factor 1.5 above the Fourier-limit $T_2=2T_1$. These findings demonstrate that rapid thermal annealing (RTA) serves as an effective tuning method that preserves the key single-photon emission properties and may help reduce undesirable effects such as non-radiative Auger recombination in quantum photonic applications.

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arXiv2026

Exciton-resonant detection of high-frequency surface acoustic waves from subwavelength metal gratings

We report on all-optical generation and detection of high-frequency (up to about 30 GHz) surface acoustic waves (SAWs) in GaAs/AlGaAs heterostructures with short-period Au gratings on top. A highly sensitive method for SAW detection is demonstrated using a polarization-resolved pump-probe technique that exploits the narrow exciton resonance in high-quality GaAs. The elastic strain of the SAW modulates the exciton energy in the time domain. As a result, even a small deformation produces a noticeable change in the dielectric function at the detection wavelength leading to an order of magnitude increase in the detection sensitivity as compared to off-resonant conditions. A theoretical model is developed that considers two detection schemes: one accounting for probe light diffraction and one corresponding to a non-diffractive situation.

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arXiv2025

Exchange interaction in gate-defined quantum dots beyond the Hubbard model

A quantitative description of the exchange interaction in quantum dots is relevant for modeling gate operations of spin qubits. By measuring the amplitude and frequency of exchange-driven qubit state oscillations, we measure the detuning dependence of the exchange coupling in a GaAs double quantum dot over three orders of magnitude. Both 1D and 3D full configuration interaction simulations can replicate the observed behavior. Extending a Hubbard model by including excited states increases the range of detuning where it provides a good fit, thus elucidating the underlying physics.

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arXiv2025

Eigenstate control of plasmon wavepackets with electron-channel blockade

Coherent manipulation of plasmon wavepackets in solid-state systems is crucial for advancing nanoscale electronic devices, offering a unique platform for quantum information processing based on propagating quantum bits. Controlling the eigenstate of plasmon wavepackets is essential, as it determines its propagation speed and hence the number of quantum operations that can be performed during its flight-time through a quantum system. When plasmon wavepackets are generated by short voltage pulses and transmitted through nanoscale devices, they distribute among multiple electron conduction channels via Coulomb interactions, a phenomenon known as charge fractionalisation. This spreading complicates plasmon manipulation in quantum circuits and makes precise control of the eigenstates of plasmon wavepackets challenging. Using a cavity, we demonstrate the ability to isolate and select electron conduction channels contributing to plasmon excitation, thus enabling precise control of plasmon eigenstate. Specifically, we observe an electron-channel blockade effect, where charge fractionalisation into cavity-confined channels is suppressed due to the plasmon's narrow energy distribution, enabling more stable and predictable plasmonic circuits. This technique provides a versatile tool for designing plasmonic circuits, offering the ability to tailor plasmon speed through local parameters, minimise unwanted plasmon excitation in adjacent circuits, and enable the precise selection of electron-channel plasmon eigenstates in quantum interferometers.

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arXiv2025

High fidelity flopping-mode single spin operation with tuning inter-dot orbital levels

Fast spin manipulation and long spin coherence time in quantum dots are essential features for high fidelity semiconductor spin qubits. However, generally it has not been well established how to optimize these two properties simultaneously, because these two properties are usually not independent from each other. Therefore, the scheme for high fidelity operation by simultaneous tuning Rabi frequency and coherence time, which does not rely on the material-dependent strong spin-orbit interaction and the local magnetic field gradient limiting their scalability, are strongly demanded. Here, we demonstrate an approach to achieve high-fidelity spin control by tuning inter-dot spin-orbit coupling in a GaAs triple quantum dot (TQD), where the third dot provides precise control over orbital energy levels. In an electrically stable charge state with optimized tunnel coupling, we achieve Rabi frequencies exceeding 100 MHz while maintaining coherence through proper tuning of the inter-dot orbital levels of the TQD. By implementing a machine learning-based feedback control that efficiently estimates qubit frequency using past measurement data, we characterize and mitigate the impact of low frequency noise on qubit coherence with minimal measurement overhead. Finally, we demonstrate a $π$/2 gate fidelity of 99.7\% with a gate time of 4 ns through randomized benchmarking, even in a GaAs quantum dot device where electron spin coherence is typically limited by strong hyperfine interaction with nuclear spins. Our approach provides a scalable strategy for high-fidelity spin control in semiconductor quantum dot arrays by utilizing device-specific parameters rather than relying on material properties or external field gradients.

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arXiv2025

Enhancement of Indistinguishable Photon Emission from a GaAs Quantum Dot via Charge Noise Suppression

The generation of indistinguishable single photons is a fundamental requirement for future quantum technologies, particularly in quantum repeater networks and for distributed quantum computing based on entanglement distribution. However, spectral jitter, often induced by charge noise in epitaxial quantum dots, leads to exciton dephasing, thereby limiting their practical usage in quantum applications. We present a straightforward approach to mitigate charge noise-induced decoherence in droplet-etched GaAs quantum dots embedded in an n-i-p diode structure and integrated deterministically into an electrically contacted circular Bragg grating resonator for emission enhancement. The quantum device allows for the stabilization of the charge environment by applying an external electrical field while producing a photon extraction efficiency of approximately (37 +- 2)%. Hong-Ou-Mandel two-photon interference measurements reveal a strong voltage dependence of the exciton dephasing time and interference visibility on the applied bias in excellent agreement with our theoretical predictions. Notably, the reduction in visibility from a maximum, charge-stabilized corrected value of 97 percent at the optimum bias point follows an inverse square dependence (proportional to 1/I^2) with increasing diode current (I) in forward direction. Under a quasi-resonant excitation scheme, we achieve a maximum exciton dephasing time (T2*) of approximately (6.8 +-0.5) ns, reaching nearly the Fourier limit (T2 = 2T1) without the need for complex echo schemes like Ramsey or Carr-Purcell-Meiboom-Gill sequences. These findings are consistent with theoretical predictions from rate equation modeling and quantum optical analysis as well as voltage-dependent linewidth measurements, demonstrating optimized electrical control of exciton dephasing.

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arXiv2025

Towards quantitative understanding of quantum dot ensemble capacitance-voltage spectroscopy

Inhomogeneous ensembles of quantum dots (QDs) coupled to a charge reservoir are widely studied by using, e.g., electrical methods like capacitance-voltage spectroscopy. We present experimental measurements of the QD capacitance as a function of varying parameters such as ac frequency and bath temperature. The experiment reveals distinct shifts in the position of the capacitance peaks. While temperature-induced shifts have been explained by previous models, the observation of frequency-dependent shifts has not been explained so far. Given that existing models fall short in explaining these phenomena, we propose a refined theoretical model based on a master equation approach which incorporates energy-dependent tunneling effects. This approach successfully reproduces the experimental data. We highlight the critical role of energy-dependent tunneling in two distinct regimes: at low temperatures, ensemble effects arising from energy-level dispersion in differently sized QDs dominate the spectral response; at high temperatures and frequencies, we observe a peak shift of a different nature, which is best described by optimizing the conjoint probability of successive in- and out-tunneling events. Our findings contribute to a deeper understanding of tunnel processes and the physical properties of QD ensembles coupled to a common reservoir, with implications for their development in applications such as single-photon sources and spin qubits.

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arXiv2025

Optical and magnetic response by design in GaAs quantum dots

Quantum networking technologies use spin qubits and their interface to single photons as core components of a network node. This necessitates the ability to co-design the magnetic- and optical-dipole response of a quantum system. These properties are notoriously difficult to design in many solid-state systems, where spin-orbit coupling and the crystalline environment for each qubit create inhomogeneity of electronic g-factors and optically active states. Here, we show that GaAs quantum dots (QDs) obtained via the quasi-strain-free local droplet etching epitaxy growth method provide spin and optical properties predictable from assuming the highest possible QD symmetry. Our measurements of electron and hole g-tensors and of transition dipole moment orientations for charged excitons agree with our predictions from a multiband k.p simulation constrained only by a single atomic-force-microscopy reconstruction of QD morphology. This agreement is verified across multiple wavelength-specific growth runs at different facilities within the range of 730 nm to 790 nm for the exciton emission. Remarkably, our measurements and simulations track the in-plane electron g-factors through a zero-crossing from -0.1 to 0.3 and linear optical dipole moment orientations fully determined by an external magnetic field. The robustness of our results demonstrates the capability to design - prior to growth - the properties of a spin qubit and its tunable optical interface best adapted to a target magnetic and photonic environment with direct application for high-quality spin-photon entanglement.

quant-ph↗

arXiv2025

Electrical control of a Kondo spin screening cloud

Quantitative analysis of quantum many-body systems, consisting of numerous itinerant electrons that interact with localized spins or electrons, is a long-standing issue. The Kondo cloud, a quantum many-body object of conduction electrons that screens a single localized spin, is the building block of such strongly correlated electronic systems. While quantitative analysis of the Kondo cloud associated with a single magnetic impurity is well established for uniform conduction electrons, the fundamental properties of a deformed Kondo cloud influenced by conduction electrons with a modulated density of states remain unsolved. Here we report engineering of the Kondo cloud deformation by confining a part of the cloud into a quantum box called the Kondo box that mimics realistic material systems. We demonstrate quantitative control of the Kondo cloud by developing a way of tuning quantum interference in the box and monitoring the Kondo entanglement. The temperature dependence of the entanglement reveals counterintuitively that the cloud shape is altered mainly outside the box although the quantum interference in the box is tuned. Our work provides a way to simulate various strongly correlated systems by integrating the Kondo cloud, which is not possible in the current theoretical framework.

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arXiv2025

Evidence of Coulomb liquid phase in few-electron droplets

Emergence of universal collective behaviour from interactions within a sufficiently large group of elementary constituents is a fundamental scientific paradigm. In physics, correlations in fluctuating microscopic observables can provide key information about collective states of matter such as deconfined quark-gluon plasma in heavy-ion collisions or expanding quantum degenerate gases. Mesoscopic colliders, through shot-noise measurements, have provided smoking-gun evidence on the nature of exotic electronic excitations such as fractional charges, levitons and anyon statistics. Yet, bridging the gap between two-particle collisions and the emergence of collectivity as the number of interacting particles increases remains a challenging task at the microscopic level. Here we demonstrate all-body correlations in the partitioning of electron droplets containing up to N = 5 electrons, driven by a moving potential well through a Y-junction in a semiconductor device. Analyzing the partitioning data using high-order multivariate cumulants and finite-size scaling towards the thermodynamic limit reveals distinctive fingerprints of a strongly-correlated Coulomb liquid. These fingerprints agree well with a universal limit where the partitioning of a droplet is predicted by a single collective variable. Our electron-droplet collider provides critical insight into the interplay of confinement and interaction effects in small electron systems and highlights a new way to study engineered states of matter.

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arXiv2025

Electronic interferometry with ultrashort plasmonic pulses

Electronic flying qubits offer an interesting alternative to photonic qubits: electrons propagate slower, hence easier to control in real time, and Coulomb interaction enables direct entanglement between different qubits. Although their coherence time is limited, flying electrons in the form of picosecond plasmonic pulses could be competitive in terms of the number of achievable coherent operations. The key challenge in achieving this critical milestone is the development of a new technology capable of injecting 'on-demand' single-electron wavepackets into quantum devices, with temporal durations comparable to or shorter than the device dimensions. Here, we take a significant step towards achieving this regime in a quantum nanoelectronic system by injecting ultrashort single-electron plasmonic pulses into a 14-micrometer-long Mach-Zehnder interferometer. Our results establish that quantum coherence is robust under the on-demand injection of ultrashort plasmonic pulses, as evidenced by the observation of coherent oscillations in the single-electron regime. Building on this, our results demonstrate for the first time the existence of a new "non-adiabatic" regime that is prominent at high frequencies. This breakthrough highlights the potential of flying qubits as a promising alternative to localised qubit architectures, offering advantages such as a reduced hardware footprint, enhanced connectivity, and scalability for quantum information processing.

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arXiv2024

Semiconductor Circuits for Quantum Computing with Electronic Wave Packets

Standard approaches to quantum computing require significant overhead to correct for errors. The hardware size for conventional quantum processors in solids often increases linearly with the number of physical qubits, such as for transmon qubits in superconducting circuits or electron spin qubits in quantum dot arrays. While photonic circuits based on flying qubits do not suffer from decoherence or lack of potential scalability, they have encountered significant challenges to overcome photon loss in long delay circuits. Here, we propose an alternative approach that utilizes flying electronic wave packets propagating in solid-state quantum semiconductor circuits. Using a novel time-bin architecture for the electronic wave packets, hardware requirements are drastically reduced because qubits can be created on-demand and manipulated with a common hardware element, unlike the localized approach of wiring each qubit individually. The electronic Coulomb interaction enables reliable coupling and readout of qubits. Improving upon previous devices, we realize electronic interference at the level of a single quantized mode that can be used for manipulation of electronic wavepackets. This important landmark lays the foundation for fault-tolerant quantum computing with a compact and scalable architecture based on electron interferometry in semiconductors.

cond-mat.mes-hall↗

arXiv2024

High-fidelity spin readout via the double latching mechanism

Projective measurement of single electron spins, or spin readout, is among the most fundamental technologies for spin-based quantum information processing. Implementing spin readout with both high-fidelity and scalability is indispensable for developing fault-tolerant quantum computers in large-scale spin-qubit arrays. To achieve high fidelity, a latching mechanism is useful. However, the fidelity can be decreased by spin relaxation and charge state leakage, and the scalability is currently challenging. Here, we propose and demonstrate a double-latching high-fidelity spin readout scheme, which suppresses errors via an additional latching process. We experimentally show that the double-latching mechanism provides significantly higher fidelity than the conventional latching mechanism and estimate a potential spin readout fidelity of 99.94% using highly spin-dependent tunnel rates. Due to isolation from error-inducing processes, the double-latching mechanism combined with scalable charge readout is expected to be useful for large-scale spin-qubit arrays while maintaining high fidelity.

cond-mat.mes-hall↗

arXiv2024

All-optical ultrafast arbitrary rotation of hole orbital qubits with direct phase control

Complete quantum control of a stationary quantum bit embedded in a quantum emitter is crucial for photonic quantum information technologies. Recently, the orbital degree of freedom in optically active quantum dots has emerged as a promising candidate. However, the essential ability to perform arbitrary rotations on orbital qubits remains elusive. Here, we demonstrate arbitrary rotation of a hole orbital qubit with direct phase control using picosecond optical pulses. This is achieved by successfully inducing stimulated Raman transitions within $Λ$ systems coupled via radiative Auger processes. The new capability enables direct control of polar and azimuth angles of the Bloch vector without requiring timed precession. Our results establish orbital states in solid-state quantum emitters as a viable resource for applications in high-speed quantum information processing.

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