arXiv subjects

Andreas Hohenau

Publications and source records attributed to Andreas Hohenau.

12 recordsLinked to original sources

arXiv2026

Transmissive extreme ultraviolet metagrating

Extreme ultraviolet (EUV) radiation is a key tool for attosecond physics and lithography. However, strong material absorption limits the availability of transmissive optical elements at these wavelengths. Metaoptics exploit geometry to control the wavefront of transmitted light on the nanoscale and, due to their minimal thickness, promise to fill this gap. Here, we demonstrate the first EUV metaoptics for broadband applications: we design, fabricate, and experimentally investigate a blazed transmissive EUV metagrating and compare it with a focused-ion-beam-milled sawtooth-blazed grating serving as an in-situ reference. The metagrating achieves an angular dispersion of 0.04{\deg}/nm with a directionality (the ratio of the +1st and -1st diffraction order efficiency) of up to 5.8. The device shows phase-based operation up to 50 eV photon energy (down to 25 nm vacuum wavelength) and an octave-spanning bandwidth of 25 eV, doubling the previous spectral window addressable by metasurfaces. Comparing both gratings' performance reveals that, when accounting for fabrication constraints, EUV metasurfaces are competitive with free-form optics while offering scalability to large apertures and arbitrary phase profiles. Broadband transmissive operation removes the need for grazing incidence optics, defeating a major source of aberrations, and allows polarization-insensitive spectral analysis, enabling energy-resolved ultrafast spectroscopy in compact experimental configurations.

physics.optics↗

arXiv2024

Photoacoustic microscopy with meta-optics

Recent advances in the miniaturization of optical elements have led to the emergence of novel imaging systems, used for industrial and consumer-based applications. The underlying methods are particularly prevalent in the realms of medical imaging and optical microscopy. Avoiding bulky optical elements can be extremely beneficial to many microscopy modalities, one of which is photoacoustic microscopy. Relying on short, highly focused light pulses that need to be precisely controlled, large and heavy optical elements can often hinder the overall performance of such systems. We propose the utilization of increasingly popular optical elements, so-called meta-optics, in the excitation path of a photoacoustic microscope. The metalenses, which were designed and used for this work, consist of sub-wavelength elements that enable elaborate phase control of incident light and multifunctionality within a single optical element. This allowed us to not only replace common optical elements in the excitation path of the photoacoustic microscope, completely omitting any conventional glass elements, but also to design an adapted lens, increasing the depth of field. With our work, we prove the benefit of meta-optics for photoacoustic microscopy by comparing two different metalenses to a conventional glass lens in simulations as well as experiments. We expect this to be a step into the direction of more advanced meta-optics being utilized in photoacoustic imaging setups.

physics.optics↗

arXiv2022

Transient absorption microscopy setup with multi-ten-kilohertz shot-to-shot subtraction and discrete Fourier analysis

Recording of transient absorption microscopy images requires fast detection of minute optical density changes, which is typically achieved with high-repetition-rate laser sources and lock-in detection. Here, we present a highly flexible and cost-efficient detection scheme based on a conventional photodiode and an USB oscilloscope with MHz bandwidth, that deviates from the commonly used lock-in scheme and achieves benchmark sensitivity. Our scheme combines shot-to-shot evaluation of pump-probe and probe-only measurements, a home-built photodetector circuit optimized for low pulse energies applying low-pass amplification, and a custom evaluation algorithm based on Fourier transformation. Advantages of this approach include abilities to simultaneously monitor multiple frequencies, parallelization of multiple detector channels, and detection of different pulse sequences (e.g., include pump-only). With a 40 kHz repetition-rate laser system powering two non-collinear optical parametric amplifiers for wide tuneability, we demonstrate the 2-D imaging performance of our transient absorption microscope with studies on micro-crystalline molecular thin films.

physics.optics↗

arXiv2017

Fluorescence coupling to plasmonic nanoparticles

The combination of single photon emitters (quantum dots) and tailored metal nanoparticles with defined size and shape allows a detailed study of the interaction between light and matter. The enhanced optical near-field of the nanoparticles can strongly influence the absorption and emission of nearby fluorescent quantum dots. We show that a controlled spatial arrangement enables the analysis and understanding of polarization dependent coupling between a metal nanoparticle and few or single fluorescent quantum dots. Modifications in the fluorescence spectrum and lifetime are analyzed and compare well with simulations.

cond-mat.mes-hall↗

arXiv2012

Influence of surface roughness on the optical properties of plasmonic nanoparticles

For plasmonic nanoparticles, we investigate the influence of surface roughness inherent to top-down fabrication on the optical properties, and find that it has a surprisingly small influence on the position and width of the plasmon peaks. Our experimental observation is supported by simulations based on the boundary element method approach. Using a perturbation approach, suitable for metallic nanoparticles with a moderate degree of surface roughness, we demonstrate that the reason for this lies in motional narrowing where the plasmon averages over the random height fluctuations. Surface roughness in large arrays of identical nanoparticles, such as encountered in the context of metamaterials, is thus expected to not constitute a major roadblock.

cond-mat.mes-hall↗

arXiv2012

Analysis of damping-induced phase flips of plasmonic nanowire modes

We launch surface plasmons from one end of a silver nanowire by asymmetric illumination with white light and use plasmon-to-light scattering at the nanowire ends to probe spectroscopically the plasmonic Fabry-Perot wire modes. The spectral positions of the maxima and minima in the scattered intensity from both nanowire ends are found to be either in phase or out-of phase, depending on the nanowire length and the spectral range. This behavior can be explained by a generalized Fabry-Perot model. The turnover-point between the two regimes is sensitive to the surface plasmon round trip losses and thus opens a new possibility for detecting changes of the optical absorption in the nanowire environment.

cond-mat.mes-hall↗

arXiv2012

Plasmonic modes of gold nano-particle arrays on thin gold films

Regular arrays of metal nanoparticles on metal films have tuneable optical resonances that can be applied for surface enhanced Raman scattering or biosensing. With the aim of developing more surface selective geometries we investigate regular gold nanoparticle arrays on 25nm thick gold films, which allow to excite asymmetric surface plasmon modes featuring a much better field confinement compared to the symmetric modes used in conventional surface plasmon resonance setups. By optical extinction spectroscopy we identify the plasmonic modes sustained by our structures. Furthermore, the role of thermal treatment of the metal structures is investigated, revealing the role of modifications in the crystalline structure of gold on the optical properties.

cond-mat.mes-hall↗

arXiv2011

Gold Nanoparticles for Plasmonic Biosensing: The Role of Metal Crystallinity and Nanoscale Roughness

Noble metal nanoparticles show specific optical properties due to the excitation of localized surface plasmons that make them attractive candidates for highly sensitive bionanosensors. The underlying physical principle is either an analyte-induced modification of the dielectric properties of the medium surrounding the nanoparticle or an increase of the excitation and emission rates of an optically active analyte by the resonantly enhanced plasmon field. Either way, besides the nanoparticle geometry the dielectric properties of the metal and nanoscale surface roughness play an important role for the sensing performance. As the underlying principles are however not yet well understood, we aim here at an improved understanding by analyzing the optical characteristics of lithographically fabricated nanoparticles with different crystallinity and roughness parameters. We vary these parameters by thermal annealing and apply a thin gold film as a model system to retrieve modifications in the dielectric function. We investigate, on one hand, extinction spectra that reflect the far-field properties of the plasmonic excitation and, on the other hand, surface-enhanced Raman spectra that serve as a near-field probe. Our results provide improved insight into localized surface plasmons and their application in bionanosensing.

physics.optics↗

arXiv2010

Plasmonic crystal demultiplexer and multiports

Artificially built periodic optical structures in dielectric and metallic media have generated considerable interest due to their potential for optical device miniaturization. In this context plasmonics, i.e., optics based on surface plasmon polaritons (SPPs) offers new exciting prospects. SPPs are hybrid light/electron surface waves at the interface between a dielectric and a metal and as such hold the potential for 2D optical functionality. Indeed, SPP elements as mirrors, splitters and interferometers have been recently demonstrated. However, for plasmonics to qualify at the information technology level requires necessarily the realization of wavelength division (demultiplexing) which constitutes a fundamental ingredient of optical communication. In the following we experimentally demonstrate 2D SPP demultiplexing in the visible spectral range by using photonic crystals for SPPs (plasmonic crystals). In addition, we demonstrate that plasmonic crystal are capable of realizing integrated linear multiports which could constitute building blocks of analog or quantum optical computing.

physics.optics↗

arXiv2010

How to erase surface plasmon fringes

We report the realization of a dual surface plasmon polariton (SPP) microscope based on leakage radiation (LR) analysis. The microscope can either image SPP propagation in the direct space or tin the Fourier space. This particularity allows in turn manipulation of the LR image for a clear separation of different interfering SPP contributions present close to optical nanoelements.

physics.optics↗

arXiv2010

Surface Plasmon Polariton microscope with Parabolic Reflectors

We report the realization of a two--dimensional optical microscope for surface plasmons polaritons (SPPs) based on parabolic Bragg mirrors. These mirrors are built from lithographically fabricated gold nanostructures on gold thin films. We show by direct imaging by leakage radiation microscopy that the magnification power of the SPP microscope follows basic predictions of geometrical optics. Spatial resolution down to the value set by the diffraction limit is demonstrated.

physics.optics↗

arXiv2006

Momentum transfer for momentum transfer-free which-path experiments

We analyze the origin of interference disappearance in which-path double aperture experiments. We show that we can unambiguously define an observable momentum transfer between the quantum particle and the path detector and we prove in particular that the so called ``momentum transfer free'' experiments can be in fact logically interpreted in term of momentum transfer.

quant-ph↗