arXiv subjects

Andreas Isacsson

Publications and source records attributed to Andreas Isacsson.

25 records · Page 2Linked to original sources

arXiv2014

Scattering of flexural acoustic phonons at grain boundaries in graphene

We investigate the scattering of long-wavelength flexural phonons against grain boundaries in graphene using molecular dynamics simulations. Three symmetric tilt grain boundaires are considered: one with a misorientation angle of $17.9^\circ$ displaying an out-of-plane buckling 1.5 nm high and 5 nm wide, one with a misorientation angle of $9.4^\circ$ and an out-of-plane buckling 0.6 nm high and 1.7 nm wide, and one with a misorientation angle of $32.2^\circ$ and no out-of-plane buckling. At the flat grain boundary, the phonon transmission exceeds 95 % for wavelengths above 1 nm. The buckled boundaries have a substantially lower transmission in this wavelength range, with a minimum transmission of 20 % for the $17.9^\circ$ boundary and 40 % for the $9.4^\circ$ boundary. At the buckled boundaries, coupling between flexural and longitudinal phonon modes is also observed. The results indicate that scattering of long-wavelength flexural phonons at grain boundaries in graphene is mainly due to out-of-plane buckling. A continuum mechanical model of the scattering process has been developed, providing a deeper understanding of the scattering process as well as a way to calculate the effect of a grain boundary on long-wavelength flexural phonons based on the buckling size.

cond-mat.mtrl-sci↗

arXiv2014

FPU physics with nanomechanical graphene resonators: intrinsic relaxation and thermalization from flexural mode coupling

Thermalization in nonlinear systems is a central concept in statistical mechanics and has been extensively studied theoretically since the seminal work of Fermi, Pasta and Ulam (FPU). Using molecular dynamics and continuum modeling of a ring-down setup, we show that thermalization due to nonlinear mode coupling intrinsically limits the quality factor of nanomechanical graphene drums and turns them into potential test beds for FPU physics. We find the thermalization rate $Γ$ to be independent of radius and scaling as $Γ\sim T^*/ε_{\rm pre}^2$, where $T^*$ and $ε_{\rm pre}$ are effective resonator temperature and prestrain.

cond-mat.mes-hall↗

arXiv2013

Nonlinear-dissipation-induced Entanglement of Coupled Nonlinear Oscillators

The quantum dynamics of two weakly coupled nonlinear oscillators is analytically and numerically investigated in the context of nonlinear dissipation. The latter facilitates the creation and preservation of non-classical steady states. Starting from a microscopic description of two oscillators individually interacting with their dissipative environments, it is found that in addition to energy relaxation, dephasing arises due to the mutual coupling. Using the negativity as an entanglement measure, it is shown that the coupling entangles the oscillators in the long-time limit. For finite temperatures, entanglement sudden death and rebirth are observed.

quant-ph↗

arXiv2013

Multi-phonon relaxation and generation of quantum states in a nonlinear mechanical oscillator

The dissipative quantum dynamics of an anharmonic oscillator is investigated theoretically in the context of carbon-based nano-mechanical systems. In the short-time limit, it is known that macroscopic superposition states appear for such oscillators. In the long-time limit, single and multi-phonon dissipation lead to decoherence of the non-classical states. However, at zero temperature, as a result of two-phonon losses the quantum oscillator eventually evolves into a non-classical steady state. The relaxation of this state due to thermal excitations and one-phonon losses is numerically and analytically studied. The possibility of verifying the occurrence of the non-classical state is investigated and signatures of the quantum features arising in a ring-down setup are presented. The feasibility of the verification scheme is discussed in the context of quantum nano-mechanical systems.

cond-mat.mes-hall↗

arXiv2012

Nonlinear Damping in Graphene Resonators

Based on a continuum mechanical model for single-layer graphene we propose and analyze a microscopic mechanism for dissipation in nanoelectromechanical graphene resonators. We find that coupling between flexural modes and in-plane phonons leads to linear and nonlinear damping of out-of-plane vibrations. By tuning external parameters such as bias and ac voltages, one can cross over from a linear to a nonlinear-damping dominated regime. We discuss the behavior of the effective quality factor in this context.

cond-mat.mes-hall↗

arXiv2012

Determination of the Bending Rigidity of Graphene via Electrostatic Actuation of Buckled Membranes

The small mass and atomic-scale thickness of graphene membranes make them highly suitable for nanoelectromechanical devices such as e.g. mass sensors, high frequency resonators or memory elements. Although only atomically thick, many of the mechanical properties of graphene membranes can be described by classical continuum mechanics. An important parameter for predicting the performance and linearity of graphene nanoelectromechanical devices as well as for describing ripple formation and other properties such as electron scattering mechanisms, is the bending rigidity, κ. In spite of the importance of this parameter it has so far only been estimated indirectly for monolayer graphene from the phonon spectrum of graphite, estimated from AFM measurements or predicted from ab initio calculations or bond-order potential models. Here, we employ a new approach to the experimental determination of κ by exploiting the snap-through instability in pre-buckled graphene membranes. We demonstrate the reproducible fabrication of convex buckled graphene membranes by controlling the thermal stress during the fabrication procedure and show the abrupt switching from convex to concave geometry that occurs when electrostatic pressure is applied via an underlying gate electrode. The bending rigidity of bilayer graphene membranes under ambient conditions was determined to be $35.5^{+20}_{-15}$ eV. Monolayers have significantly lower κ than bilayers.

cond-mat.mtrl-sci↗

arXiv2008

Continuum elastic modeling of graphene resonators

Starting from an atomistic approach we have derived a hierarchy of successively more simplified continuum elasticity descriptions for modeling the mechanical properties of suspended graphene sheets. The descriptions are validated by applying them to square graphene-based resonators with clamped edges and studying numerically their mechanical responses. Both static and dynamic responses are treated. We find that already for deflections of the order of 0.5Å a theory that correctly accounts for nonlinearities is necessary and that for many purposes a set of coupled Duffing-type equations may be used to accurately describe the dynamics of graphene membranes.

cond-mat.other↗