arXiv subjects

Andreas Knorr

Publications and source records attributed to Andreas Knorr.

At least 91 records · Page 5Linked to original sources

arXiv2019

Comparison between continuous- and discrete-mode coherent feedback for the Jaynes-Cummings model

Using the example of the Jaynes-Cummings model, we present a comparison between time-delayed coherent feedback mediated by reservoirs with continuous and discrete mode structures and work out their qualitative differences. In contrast to the discrete-mode case, the continuous-mode case results in the well-known single-delay dynamics which can, e.g., stabilize Rabi oscillations. The discrete-mode case, however, shows population trapping, not present in the continuous-mode model. Given these differences, we discuss the cavity output spectra and show how these characteristic properties are spectrally identifiable. This work demonstrates the fundamental difference between the continuous-mode case, which represents a truly dissipative mechanism, and the discrete-mode case that is in principle based on a coherent excitation exchange process.

quant-ph↗

arXiv2019

Quantum Pyragas control: Selective-control of individual photon probabilities

Pyragas control allows to stabilize unstable states in applied nonlinear science. We propose to apply a quantum version of the Pyragas protocol to control individual photon-probabilities in an otherwise only globally accessible photon-probability distribution of a quantum light emitter. The versatility of quantum Pyragas control is demonstrated for the case of a two-level emitter in a pulsed laser-driven half cavity. We show that one- and two-photon events respond in a qualitatively different way to the half-cavity induced feedback signal. One-photon events are either enhanced or suppressed, depending on the choice of parameters. In contrast, two-photon events undergo exclusively an enhancement up to $50\%$ for the chosen pulse areas. We hereby propose an implementation of quantum Pyragas control via a time-delayed feedback setup.

quant-ph↗

arXiv2018

Carrier dynamics in graphene: ultrafast many-particle phenomena

Graphene is an ideal material to study fundamental Coulomb- and phonon-induced carrier scattering processes. Its remarkable gapless and linear band structure opens up new carrier relaxation channels. In particular, Auger scattering bridging the valence and the conduction band changes the number of charge carriers and gives rise to a significant carrier multiplication - an ultrafast many-particle phenomenon that is promising for the design of highly efficient photodetectors. Furthermore, the vanishing density of states at the Dirac point combined with ultrafast phonon-induced intraband scattering results in an accumulation of carriers and a population inversion suggesting the design of graphene-based terahertz lasers. Here, we review our work on the ultrafast carrier dynamics in graphene and Landau-quantized graphene is presented providing a microscopic view on the appearance of carrier multiplication and population inversion.

cond-mat.mes-hall↗

arXiv2018

Stabilizing quantum coherence against pure dephasing in the presence of quantum feedback at finite temperature

A general formalism to describe the dynamics of quantum emitters in structured reservoirs is introduced. As an application, we investigate the optical coherence of an atom-like emitter diagonally coupled via a link-boson to a structured bosonic reservoir and obtain unconventional dephasing dynamics due to non-Markovian quantum feedback for different temperatures. For a two-level emitter embedded in a phonon cavity preservation of finite coherence is predicted up to room temperature.

quant-ph↗

arXiv2018

Optical fingerprint of non-covalently functionalized transition metal dichalcogenides

Atomically thin transition metal dichalcogenides (TMDs) hold promising potential for applications in optoelectronics. Due to their direct band gap and the extraordinarily strong Coulomb interaction, TMDs exhibit efficient light-matter coupling and tightly bound excitons. Moreover, large spin orbit coupling in combination with circular dichroism allows for spin and valley selective optical excitation. As atomically thin materials, they are very sensitive to changes in the surrounding environment. This motivates a functionalization approach, where external molecules are adsorbed to the materials surface to tailor its optical properties. Here, we apply the density matrix theory to investigate the potential of non-covalently functionalized TMDs. Considering exemplary spiropyran molecules with a strong dipole moment, we predict spectral redshifts and the appearance of an additional side peak in the absorption spectrum of functionalized TMDs. We show that the molecular characteristics, e.g. coverage, orientation and dipole moment, crucially influence the optical properties of TMDs, leaving a unique optical fingerprint in the absorption spectrum. Furthermore, we find that the molecular dipole moments open a channel for coherent intervalley coupling between the high-symmetry K and K' points which may open new possibilities for spin-valleytronics application.

cond-mat.mtrl-sci↗

arXiv2017

Theory of excitation transfer between two-dimensional semiconductor and molecular layers

The geometry-dependent energy transfer rate from an electrically pumped inorganic semiconductor quantum well into an organic molecular layer is studied theoretically. We focus on Förster-type nonradiative excitation transfer between the organic and inorganic layer and include quasi-momentum conservation and intermolecular coupling between the molecules in the organic film. (Transition) partial charges calculated from density-functional theory are used to calculate the coupling elements. The partial charges describe the spatial charge distribution and go beyond the common dipole-dipole interaction. We find that the transfer rates are highly sensitive to variations in the geometry of the hybrid inorganic/organic system. For instance, the transfer efficiency is improved by orders of magnitude by tuning the relative orientation and positioning of the molecules. Also, the operating regime is identified where in-scattering dominates over unwanted back-scattering from the molecular layer into the substrate.

cond-mat.mes-hall↗

arXiv2017

Phonon Sidebands in Transition Metal Dichalcogenides

Excitons dominate the optical properties of monolayer transition metal dichalcogenides (TMDs). Besides optically accessible bright exciton states, TMDs exhibit also a multitude of optically forbidden dark excitons. Here, we show that efficient exciton-phonon scattering couples bright and dark states and gives rise to an asymmetric excitonic line shape. The observed asymmetry can be traced back to phonon-induced sidebands that are accompanied by a polaron redshift. We present a joint theory-experiment study investigating the microscopic origin of these sidebands in different TMD materials taking into account intra- and intervalley scattering channels opened by optical and acoustic phonons. The gained insights contribute to a better understanding of the optical fingerprint of these technologically promising nanomaterials.

cond-mat.mes-hall↗

arXiv2017

Correlations of cascaded photons: An analytical study in the two-photon Mollow regime

Mollow physics in the two-photon regime shows interesting features such as path-controlled time-reordering of photon pairs without the need to delay them. Here, we calculate analytically the two-photon correlations $ g^{(2)}(τ)$, essential to discuss and study such phenomena in the resonant-driven dressed-state regime. It is shown that there exists upper and lower bounds of the $ g^{(2)}(τ)-$ function for certain spectrally-selected photon pairs. Recent reported experiments agree with the presented theory and thereby it is shown that the resonant-driven four-level system is an interesting source for steerable quantum light in quantum cascade setups. We furthermore discuss the unlikeliness to observe antibunching for the delay time $ τ=0 $ in the exciton-biexciton correlation functions in such experiments, since antibunching stems from a coherent and in-phase superposition of different photon emission events. Due to the occuring laser photon scattering, this coherent superposition state is easily disturbed and leads to correlation functions of $ g^{(2)}(0)=1$.

quant-ph↗

arXiv2017

Dark excitons in transition metal dichalcogenides

Monolayer transition metal dichalcogenides (TMDs) exhibit a remarkably strong Coulomb interaction that manifests in tightly bound excitons. Due to the complex electronic band structure exhibiting several spin-split valleys in the conduction and valence band, dark excitonic states can be formed. They are inaccessibly by light due to the required spin-flip and/or momentum transfer. The relative position of these dark states with respect to the optically accessible bright excitons has a crucial impact on the emission efficiency of these materials and thus on their technological potential. Based on the solution of the Wannier equation, we present the excitonic landscape of the most studied TMD materials including the spectral position of momentum- and spin-forbidden excitonic states. We show that the knowledge of the electronic dispersion does not allow to conclude about the nature of the material's band gap, since excitonic effects can give rise to significant changes. Furthermore, we reveal that an exponentially reduced photoluminescence yield does not necessarily reflect a transition from a direct to a non-direct gap material, but can be ascribed in most cases to a change of the relative spectral distance between bright and dark excitonic states.

cond-mat.mtrl-sci↗

arXiv2017

Mapping of the dark exciton landscape in transition metal dichalcogenides

Transition metal dichalcogenides (TMDs) exhibit a remarkable exciton physics including optically accessible (bright) as well as spin- and momentum-forbidden (dark) excitonic states. So far the dark exciton landscape has not been revealed leaving in particular the spectral position of momentum-forbidden dark states completely unclear. This has a significant impact on the technological application potential of TMDs, since the nature of the energetically lowest state determines, if the material is a direct-gap semiconductor. Here, we show how dark states can be experimentally revealed by probing the intra-excitonic 1s-2p transition. Distinguishing the optical response shortly after the excitation (< 100$\,$fs) and after the exciton thermalization (> 1$\,$ps) allows us to demonstrate the relative position of bright and dark excitons. We find both in theory and experiment a clear blue-shift in the optical response demonstrating for the first time the transition of bright exciton populations into lower lying momentum- and spin-forbidden dark excitonic states in monolayer WSe$_2$.

cond-mat.mtrl-sci↗

arXiv2017

Superradiant to subradiant phase transition in the open system Dicke model: Dark state cascades

Collectivity in ensembles of atoms gives rise to effects like super- and subradiance. While superradiance is well studied and experimentally accessible, subradiance remains elusive since it is difficult to track experimentally as well as theoretically. Here we present a new type of phase transition in the resonantly driven, open Dicke model that leads to a deterministic generation of subradiant states. At the transition the system switches from a predominantly superradiant to a predominantly subradiant state. Clear experimental signatures for the effect are presented and entanglement properties are discussed. Letting the system relax into the ground state generates a cascade of dark Dicke states, with dark state populations up to unity. Furthermore we introduce a collectivity measure that allows to quantify collective behavior.

quant-ph↗

arXiv2017

Quantum cascade driving: Dissipatively mediated coherences

Quantum cascaded systems offer the possibility to manipulate a target system with the quantum state of a source system. Here, we study in detail the differences between a direct quantum cascade and coherent/incoherent driving for the case of two coupled cavity-QED systems. We discuss qualitative differences between these excitations scenarios, which are particular strong for higher-order photon-photon correlations: $g^{(n)}(0)$ with $ n>2 $. Quantum cascaded systems show a behavior differing from the idealized cases of individual coherent/incoherent driving and allow to produce qualitatively different quantum statistics. Furthermore, the quantum cascaded driving exhibits an interesting mixture of quantum coherent and incoherent excitation dynamics. We develop a measure, where the two regimes intermix and quantify these differences via experimentally accessible higher-order photon correlations.

quant-ph↗

arXiv2017

Path-controlled time reordering of paired photons in a dressed three-level cascade

The two-photon dressing of a "three-level ladder" system, here the ground state, the exciton and the biexciton of a semiconductor quantum dot, leads to new eigenstates and allows one to manipulate the time ordering of the paired photons without unitary post processing. We show that, after spectral post-selection of the single dressed states, the time ordering of the cascaded photons can be removed or conserved. Our joint experimental and theoretical study demonstrates the high potential of a "ladder" system to be a versatile source of orthogonally polarized, bunched or antibunched pairs of photons.

quant-ph↗

arXiv2017

Intensified antibunching via feedback-induced quantum interference

We numerically show that time delayed coherent feedback controls the statistical output characteristics of driven quantum emitters. Quantum feedback allows to enhance or suppress a wide range of classical and nonclassical features of the emitted quantum light. As exemplary quantum system, we use a pumped cavity containing two emitters. By applying phase-selective feedback, we demonstrate that photon antibunching and bunching can be increased in orders of magnitude due to intrinsically and externally controllabe quantum interferences. Our modelling is based on a fully non-Markovian quantum simulation of a structured photon continuum. We show that an approximative method in the Schrödinger picture allows a very good estimate for quantum feedback induced features for low pump rates.

quant-ph↗

arXiv2017

Dark and bright exciton formation, thermalization, and photoluminescence in monolayer transition metal dichalcogenides

The remarkably strong Coulomb interaction in atomically thin transition metal dichalcogenides (TMDs) results in an extraordinarily rich many-particle physics including the formation of tightly bound excitons. Besides optically accessible bright excitonic states, these materials also exhibit a variety of dark excitons. Since they can even lie below the bright states, they have a strong influence on the exciton dynamics, lifetimes, and photoluminescence. While very recently, the presence of dark excitonic states has been experimentally demonstrated, the origin of these states, their formation, and dynamics have not been revealed yet. Here, we present a microscopic study shedding light on time- and energy-resolved formation and thermalization of bright and dark intra- and intervalley excitons as well as their impact on the photoluminescence in different TMD materials. We demonstrate that intervalley dark excitons, so far widely overlooked in current literature, play a crucial role in tungsten-based TMDs giving rise to an enhanced photoluminescence and reduced exciton lifetimes at elevated temperatures.

cond-mat.mes-hall↗

arXiv2017

A bright triggered twin-photon source in the solid state

A non-classical light source emitting pairs of identical photons represents a versatile resource of interdisciplinary importance with applications in quantum optics and quantum biology. Emerging research fields, which benefit from such type of quantum light source, include quantum-optical spectroscopy or experiments on photoreceptor cells sensitive to photon statistics. To date, photon twins have mostly been generated using parametric downconversion sources, relying on Poissonian number distributions, or atoms, exhibiting low emission rates. Here, we propose and experimentally demonstrate the efficient, triggered generation of photon twins using the energy-degenerate biexciton-exciton radiative cascade of a single semiconductor quantum dot. Deterministically integrated within a microlens, this nanostructure emits highly-correlated photon pairs, degenerate in energy and polarization, at a rate of up to (234 $\pm$ 4) kHz. Furthermore, we verify a significant degree of photon-indistinguishability and directly observe twin-photon emission by employing photon-number-resolving detectors, which enables the reconstruction of the emitted photon number distribution.

quant-ph↗

arXiv2016

Transition from Jaynes-Cummings to Autler-Townes ladder in a quantum dot-microcavity system

We study experimentally and theoretically a coherently-driven strongly-coupled quantum dot-microcavity system. Our focus is on physics of the unexplored intermediate excitation regime where the resonant laser field dresses a strongly-coupled single exciton-photon (polariton) system resulting in a ladder of laser-dressed Jaynes-Cummings states. In that case both the coupling of the emitter to the confined light field of the microcavity and to the light field of the external laser are equally important, as proved by observation of injection pulling of the polariton branches by an external laser. This intermediate interaction regime is of particular interest since it connects the purely quantum mechanical Jaynes-Cummings ladder and the semi-classical Autler-Townes ladder. Exploring the driving strength-dependence of the mutually coupled system we establish the maximum in the resonance fluorescence signal to be a robust fingerprint of the intermediate regime and observe signatures indicating the laser-dressed Jaynes-Cummings ladder. In order to address the underlying physics we excite the coupled system via the matter component of fermionic nature undergoing saturation - in contrast to commonly used cavity-mediated excitation.

cond-mat.mes-hall↗

arXiv2016

Out of the dark and into the light: towards dark-state based chemical sensors

The rapidly increasing use of sensors throughout different research disciplines and the demand for more efficient devices with less power consumption depends critically on the emergence of new sensor materials and novel sensor concepts. Atomically thin transition metal dichalcogenides have a huge potential for sensor development within a wide range of applications. Their optimal surface-to-volume ratio combined with strong light-matter interaction results in a high sensitivity to changes in their surrounding. Here, we present a novel, highly efficient sensing mechanism to detect molecules based on dark excitons in these materials. We show that the presence of molecules with a dipole moment transforms dark states into bright excitons resulting in an additional pronounced peak in easy accessible optical spectra. This effect exhibits a huge potential for sensor applications, since it offers an unambiguous optical finger print for the detection of molecules - in contrast to common sensing schemes relying on small peak shifts and intensity changes.

cond-mat.mtrl-sci↗