arXiv subjects

Andreas Michels

Publications and source records attributed to Andreas Michels.

At least 19 recordsLinked to original sources

arXiv2026

Polarized neutron scattering as a probe for vortex-type spin correlations in iron oxide multicore assemblies

We report an experimental investigation of the magnetic microstructure of iron oxide multicore assemblies by means of polarized small-angle neutron scattering (SANS). Guided by a recently developed analytical theory for vortex-state magnetic nanoparticles, we provide a quantitative comparison between the measured and calculated cross sections, revealing signatures that are consistent with vortex-type magnetization configurations at low applied magnetic fields. In particular, the field evolution and the characteristic isotropic ring-type feature of the spin-flip scattering intensity at intermediate momentum transfers are in line with the formation of flux-closure states. The latter are stabilized by the interplay of exchange, Zeeman, and magnetostatic energies. The methodology allows for a statistically significant characterization of vortex states in densely packed nanoparticle systems, thereby complementing surface-sensitive techniques that are commonly limited to the observation of spin structures in individual particles.

cond-mat.mes-hall↗

arXiv2026

Angular anisotropy landscape of vortex ensembles in polarized small-angle neutron scattering

We present a symmetry-resolved classification of two-dimensional spin-flip small-angle neutron scattering (SANS) patterns arising from dilute ensembles of spherical nanoparticles hosting magnetic vortex states. Based on a linear vortex ansatz with an axially symmetric distribution of vortex axes and the corresponding analytical expression for the orientationally averaged spin-flip SANS cross section, we show that the angular scattering patterns organize into four distinct symmetry regimes: a four-fold anisotropy corresponding to coherent field-aligned magnetization, vertical and horizontal two-fold anisotropies associated with aligned and isotropically distributed vortex ensembles, and an isotropic ring-like condition separating the two two-fold regimes. The corresponding symmetry boundaries are obtained analytically and define a compact symmetry landscape in the parameter space of vortex amplitude and vortex-axis distribution width. Comparison with a nonlinear vortex profile shows that these symmetry regions are robust with respect to the detailed radial structure of the vortex core. The angular anisotropies are therefore governed primarily by rotational symmetry and by the statistical distribution of vortex axes, providing a compact and model-transparent classification framework of experimental polarized SANS data.

cond-mat.mes-hall↗

arXiv2026

Nanoscale mapping of internal magnetization dynamics reveals how disorder shapes heat generation in magnetic particle hyperthermia

Magnetic particle hyperthermia relies on the efficient conversion of magnetic field energy into heat in biomedical applications, yet the microscopic mechanisms governing heat generation within individual particles remain poorly understood. In this study, AC magnetometry experiments are combined with dynamic micromagnetic simulations to connect microstructural features, magnetization dynamics, and macroscopic heat dissipation. Beyond macroscopic heating metrics, the heat generation is resolved at the intra-particle level, uncovering a heterogeneous landscape of localized ''hot spots'' with nanometer spatial and nanosecond temporal resolution. The results demonstrate that grain size acts as a key experimentally tunable parameter, balancing anisotropy disorder and pinning strength, thereby controlling both the magnitude and spatio-temporal distribution of heat release within the particle. In particular, nanoflower architectures composed by larger grains deliver larger heat generation, while the smaller grains offer a deeper intra-particle pinning landscape, which effectively redistributes the heat generation over extended time windows. Together, our results provide a mechanistic framework linking nanoparticle microstructure to magnetic heating and establish design principles for optimizing nanoflowers as magnetic hyperthermia transducers.

cond-mat.mes-hall↗

arXiv2026

NuMagSANS: a GPU-accelerated open-source software package for the generic computation of nuclear and magnetic small-angle neutron scattering observables of complex systems

We present NuMagSANS, a GPU-accelerated software package for calculating nuclear and magnetic small-angle neutron scattering (SANS) cross sections and correlation functions. The program allows users to import position-dependent nuclear density and magnetization data, providing a large flexibility for analyzing the scattering signatures of complex systems, particularly magnetic materials. Full rotational control of the sample is supported, allowing a comprehensive exploration of angular-dependent scattering features. NuMagSANS includes a versatile library of approximately 100 response functions that encompass two-dimensional SANS cross sections, correlation functions, and azimuthally averaged quantities. These capabilities allow users to gain detailed insight into the structural and magnetic characteristics of their samples. GPU acceleration ensures rapid computations, even for large data sets, making NuMagSANS a powerful and efficient tool for advanced SANS analysis.

cond-mat.mtrl-sci↗

arXiv2026

Minimal model for vortex nucleation and reversal in spherical magnetic nanoparticles

Magnetic nanoparticles beyond the single-domain limit often develop vortex-like magnetization textures arising from the competition between exchange and magnetostatic energies. While such states are routinely studied using micromagnetic simulations, transparent analytical descriptions of vortex-mediated hysteresis and nucleation remain scarce. Here, we develop a semi-analytical minimal framework for vortex states in spherical magnetic nanoparticles. Guided by micromagnetic simulations, we introduce a parametrized vortex magnetization Ansatz based on hyperbolic functions that continuously interpolates between uniform and vortex states. In this way, we achieve a complexity reduction leading to a minimal Hamiltonian, which enables the efficient computation of magnetization curves and provides insight into vortex-mediated magnetization reversal. As an application, we derive analytical estimates for the critical vortex nucleation radius and field, recovering the functional form of Brown's classic result and extending it within a variational framework.

cond-mat.mtrl-sci↗

arXiv2025

Regularized Micromagnetic Theory for Bloch Points

Magnetic singularities known as Bloch points (BPs) present a fundamental challenge for micromagnetic theory, which is based on the assumption of a fixed magnetization vector length. Due to the divergence of the effective field at a BP, classical micromagnetics fails to adequately describe BP dynamics. To address this issue, we propose a regularized micromagnetic model in which the magnetization vector can vary in length but not exceed a threshold value. More specifically, the magnetization is treated as an order parameter constrained to a S3-sphere. This constraint respects fundamental properties of local spin expectation values in quantum systems. We derive the corresponding regularized Landau-Lifshitz-Gilbert equation and the analogue of the Thiele equation describing the steady motion of spin textures under various external stimuli. We demonstrate the applicability of our theory by modeling the dynamics of several magnetic textures containing BPs, including domain walls in nanowires, chiral bobbers, and magnetic dipolar strings. The presented results extend micromagnetic theory by incorporating a regularized description of BP dynamics.

cond-mat.mes-hall↗

arXiv2025

Micromagnetic structure of oxidized magnetite nanoparticles: sharp structural versus diffuse magnetic interface

The oxidation of magnetite to maghemite is a naturally occurring process that leads to the degradation of the magnetic properties of magnetite nanoparticles. Despite being systematically observed with traditional macroscopic magnetization measurement techniques, a detailed understanding of this process at the microscale is still missing. In this study, we track the evolution of the magnetic structure of magnetite nanoparticles during their oxidation to maghemite through numerical micromagnetic simulations. To capture realistic interparticle effects, we incorporate dipolar interactions by modeling the nanoparticles arranged in chains. Our computational results are benchmarked against experimental data from magnetotactic bacteria, studied over a time scale of years. To resolve the magnetization at the interface between both oxide phases, we propose spin-polarized small-angle neutron scattering (SANS), an experimental technique capable of probing magnetization textures at nanometer length scales. By analyzing the pair-distance distribution function extracted from SANS, we identify distinct signatures of magnetic disorder. Specifically, our findings suggest that the magnetization from the non-oxidized core region varies smoothly across the (structurally sharp) interface into the oxidized shell. The existence of such a diffuse magnetic interface may account for the superior magnetic properties of partially oxidized magnetite nanoparticles compared to fully converted maghemite samples.

cond-mat.mes-hall↗

arXiv2025

Scaling in Magnetic Neutron Scattering

We report the discovery of scaling in the mesoscale magnetic microstructure of bulk ferromagnets. Supported by analytical micromagnetic theory, we introduce the field-dependent scaling length $l_{\mathrm{C}}(H)$, which describes the characteristic long-wavelength magnetization fluctuations that are caused by microstructural defects by means of magnetoelastic and magnetocrystalline anisotropy. The scaling length $l_{\mathrm{C}}$ is identified to consist of the micromagnetic exchange length of the field $l_{\mathrm{H}}$, which depends on the magnetic interactions, and a field-independent contribution that reflects the properties of the magnetic anisotropy field and the magnetostatic fluctuations. The latter finding is rooted in the convolution relationship between the grain microstructure and micromagnetic response functions. We validated the scaling property by analyzing experimental data for the magnetic neutron scattering cross section. When plotted as a function of the dimensionless scaled scattering vector $\mathfrak{q}(H) = q \, l_{\mathrm{C}}(H)$, the field-dependent amplitude-scaled neutron data of nanocrystalline Co and a Nd-Fe-B-based nanocomposite collapse onto a single master curve, demonstrating universal behavior. The scaling length $l_{\mathrm{C}}$ provides a framework for analyzing the field-dependent neutron scattering cross section, highlighting the existence of critical length scales that govern the mesoscale microstructure of magnetic materials.

cond-mat.mes-hall↗

arXiv2025

Skyrmionic Schr\"odinger cat states in monoaxial chiral magnets

We study the low-energy excitation spectra of a spin-1/2 quantum Heisenberg model with a monoaxial Dzyaloshinskii-Moriya interaction. Using the density matrix renormalization group method, our analysis reveals a degeneracy between skyrmion and antiskyrmion states, enabling the formation of a mesoscopic Schr\"odinger cat state - a quantum superposition of these topologically distinct textures. To characterize this nontrivial state, we compute two-point spin correlation functions, highlighting signatures accessible via neutron scattering experiments. Furthermore, we demonstrate that applying a magnetic field gradient induces a coherent time evolution of the cat state, offering a controllable mechanism for its manipulation. These findings provide a framework for the detection of skyrmionic Schr\"odinger cat states in quantum magnets.

cond-mat.mes-hall↗

arXiv2025

Stability and Nucleation of Dipole Strings in Uniaxial Chiral Magnets

We report on the stability of the magnetic dipole string (DS), a three-dimensional magnetic texture formed by two coupled Bloch points with opposite topological charges, separated by an equilibrium distance. Previous studies demonstrated the stability of such configurations through geometric confinement or coupling with local perturbations in the magnetization field, such as skyrmion strings or dislocations in helical modulations. Here, we show that, in uniaxial chiral magnets, an isolated DS remains stable in an unperturbed vacuum, thus representing a true three-dimensional soliton. The phase diagram illustrates the stability of the DS embedded in the conical or helical phases across a broad range of material parameters and external magnetic fields. Using the geodesic nudged elastic band method applied to a regularized micromagnetic model, we demonstrate that isolated DSs are protected from collapse by an energy barrier. Stochastic spin-lattice simulations demonstrate that DSs can spontaneously nucleate during in-field annealing. This work aims to stimulate the experimental observation of DSs and further exploration of uniaxial chiral magnets.

cond-mat.mes-hall↗

arXiv2024

Quantum and classical magnetic Bloch points

A Bloch point represents a three-dimensional hedgehog singularity of a magnetic vector field in which the magnetization vanishes. However, standard micromagnetic theory, developed for magnetic moments of fixed lengths, lacks full applicability in studying such singularities. To address this gap, we study a Bloch point in a quantum Heisenberg model for the case of spin-1/2 particles. Performing an exact diagonalization of the Hamiltonian as well as using density matrix renormalization group techniques, we obtain the ground state, which can be used to recover the corresponding magnetization profile. Our findings demonstrate a variation of the spin length in the quantum model, leading smoothly to zero magnetization at the Bloch point. Our results indicate the necessity of generalizing the classical micromagnetic model by adding the third degree of freedom of the spins: the ability to change its length. To this end, we introduce the micromagnetic $\mathbb{S}_{3}$-model, which enables the description of magnets with and without Bloch point singularities.

cond-mat.str-el↗

arXiv2024

Magnetic microstructure of nanocrystalline Fe-Nb-B alloys as seen by small-angle neutron and X-ray scattering

We have investigated the magnetic microstructure of two-phase Fe-Nb-B~based Nanoperm alloys using unpolarized small-angle neutron scattering (SANS) and small-angle X-ray scattering (SAXS). Our SANS analysis reveals a significantly large magnetic scattering contribution due to spin misalignment, primarily originating from the substantial jump in the longitudinal magnetization at the interfaces between the particles and the matrix. The magnetic scattering exhibits an angular anisotropy that resembles a clover-leaf-type pattern, consistent with the predictions of micromagnetic SANS theory. Analysis of the one-dimensional SANS data yields values for the exchange-stiffness constant and the average anisotropy and magnetostatic fields. The micromagnetic correlation lengths for all three samples exhibit a similar field variation with sizes ranging between about 10-35 nm. We also find that the nuclear and magnetic residual scattering component of the SANS cross section exhibits a similar $q$ dependency as the SAXS data. These findings further validate the applicability of the micromagnetic SANS theory, and the mesoscopic information obtained is important for the advancement of the soft magnetic properties of this class of material.

cond-mat.mtrl-sci↗

arXiv2024

Small-angle neutron scattering signatures of magnetic hopfions

Magnetic hopfions are three-dimensional localized magnetic topological solitons which can exist in the bulk of magnetic materials. Based on a Ritz model for magnetic hopfions in a chiral magnet, the unpolarized magnetic small-angle neutron scattering (SANS) cross section, the spin-flip scattering cross section, and the chiral function (characterizing the imbalance between the two spin-flip scattering amplitudes) are computed here analytically; while the real-space correlation function is obtained numerically. Features of these functions, specific to magnetic hopfions, are discussed. Our results enable the SANS method to be used for the detection of magnetic hopfions.

cond-mat.mes-hall↗

arXiv2024

Framework for Polarized Magnetic Neutron Scattering from Nanoparticle Assemblies with Vortex-Type Spin Textures

Within the framework of the recently introduced multi-nanoparticle power-series expansion method for the polarized small-angle neutron scattering (SANS) cross section, we present analytical expressions for the polarized SANS observables arising from dilute nanoparticle assemblies with antisymmetric vortex-type spin structures. We establish connections between the magnetic correlation coefficients and the magnetic field-dependent vortex-axes distribution function, which is related to the random orientations of the magnetocrystalline anisotropy axes of the nanoparticles. Our analytical results are validated through a comparative analysis with micromagnetic simulations. This framework contributes to a comprehensive understanding of polarized magnetic neutron scattering from spherical nanoparticle systems exhibiting vortex-type spin structures.

cond-mat.mtrl-sci↗

arXiv2024

Neutron-scattering signature of the Dzyaloshinskii-Moriya interaction in nanoparticles

The antisymmetric Dzyaloshinkii-Moriya interaction (DMI) arises in systems with broken inversion symmetry and strong spin-orbit coupling. In conjunction with the isotropic and symmetric exchange interaction, magnetic anisotropy, the dipolar interaction, and an externally applied magnetic field, the DMI supports and stabilizes the formation of various kinds of complex mesoscale magnetization configurations, such as helices, spin spirals, skyrmions, or hopfions. A question of importance in this context addresses the neutron-scattering signature of the DMI, in particular in nanoparticle assemblies, where the related magnetic scattering signal is diffuse in character and not of the single-crystal diffraction-peak-type, as it is e.g.\ seen in the B20 compounds. Using micromagnetic simulations we study the effect of the DMI in spherical FeGe nanoparticles on the randomly-averaged magnetic neutron scattering observables, more specifically on the spin-flip small-angle neutron scattering cross section, the related chiral function, and the pair-distance distribution function. Within the studied parameter space for the particle size ($60 \, \mathrm{nm} \leq L \leq 200 \, \mathrm{nm}$) and the applied magnetic field ($-1 \, \mathrm{T} \leq μ_0 H_0 \leq 1 \, \mathrm{T}$), we find that the chiral function is only nonzero when the DMI is taken into account in the simulations. This result is discussed within the context of the symmetry properties of the magnetization Fourier components and of the involved energies under space inversion. Finally, for small applied magnetic fields, we provide an easy-to-implement analytical correlation function for the DMI-induced spin modulations (with wave vector $k_{\mathrm{d}}$). The corresponding randomly-averaged spin-flip SANS cross section reproduces the main features found in the numerical simulations.

cond-mat.mes-hall↗

arXiv2023

Signature of surface anisotropy in the spin-flip neutron scattering cross section of spherical nanoparticles: atomistic simulations and analytical theory

We investigate the signature of magnetic surface anisotropy in nanoparticles in their spin-flip neutron scattering cross section. Taking into account the isotropic exchange interaction, an external magnetic field, a uniaxial or cubic magnetic anisotropy for the particle's core, and several models for the surface anisotropy (Néel, conventional, random), we compute the spin-flip small-angle neutron scattering (SANS) cross section from the equilibrium spin structures obtained using the Landau-Lifshitz equation. The sign of the surface anisotropy constant, which is related to the appearance of tangential- or radial-like spin textures, can be distinguished from the momentum-transfer dependence of the spin-flip signal. The data cannot be described by the well-known and often-used analytical expressions for uniformly magnetized spherical or core-shell particles, in particular at remanence or at the coercive field. Based on a second-order polynomial expansion for the magnetization vector field, we develop a novel minimal model for the azimuthally-averaged magnetic SANS cross section. The theoretical expression considers a general magnetization inhomogeneity and is not restricted to the presence of surface anisotropy. It is shown that the model describes very well our simulation data as well as more complex spin patterns such as vortex-like structures. Only seven expansion coefficients and some basis functions are sufficient to describe the scattering behavior of a very large number of atomic spins.

cond-mat.mtrl-sci↗

arXiv2023

Fingerprint of vortex-like flux closure in isotropic Nd-Fe-B bulk magnet

Taking advantage of recent progress in neutron instrumentation and in the understanding of magnetic-field-dependent small-angle neutron scattering, here, we study the three-dimensional magnetization distribution within an isotropic Nd-Fe-B bulk magnet. The magnetic neutron scattering cross section of this system features the so-called spike anisotropy, which points towards the presence of a strong magnetodipolar interaction. This experimental result combined with a damped oscillatory behavior of the corresponding correlation function and recent micromagnetic simulation results on spherical nanoparticles suggest an interpretation of the neutron data in terms of vortex-like flux-closure patterns. The field-dependent correlation length Lc is well reproduced by a phenomenological power-law model. While the experimental neutron data for Lc are described by an exponent close to unity (p = 0.86), the simulation results yield p = 1.70, posing a challenge to theory to include vortex-vortex interaction effects.

cond-mat.mes-hall↗

arXiv2023

Micromagnetics of ferromagnetic/antiferromagnetic nanocomposite materials. Part II: Mesoscopic modeling

In the second part of this publication, we present simulation results for two three-dimensional models of Heusler-type alloys obtained by the mesoscopic micromagnetic approach. In the first model, we simulate the magnetization reversal of a single ferromagnetic (FM) inclusion within a monocrystalline antiferromagnetic (AFM) matrix, revealing the evolution of the complex magnetization distribution within this inclusion when the external field is changed. The main result of this ``monocrystalline'' model is the absence of any hysteretic behavior by the magnetization reversal of the FM inclusion. Hence, this model is unable to reproduce the basic experimental result for the corresponding nanocomposite -- hysteresis in the magnetization reversal of FM inclusions with a vertical shift of the corresponding loops. To explain this latter feature, in the second model we introduce a polycrystalline AFM matrix, with exchange interactions between AFM crystallites and between the FM inclusion and these crystallites. We show that within this model we can not only reproduce the hysteretic character of the remagnetization process, but also achieve a semi-quantitative agreement with the experimentally observed hysteresis loop assuming that the concentration of FM inclusions strongly fluctuates. These findings demonstrate the reliability of our enhanced micromagnetic model and set the basis for its applications in future studies of Heusler alloys and FM/AFM nanocomposites.

cond-mat.mtrl-sci↗