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Andreas P. Schnyder

Publications and source records attributed to Andreas P. Schnyder.

At least 19 recordsLinked to original sources

Robust realization of spin-polarized specular Andreev reflection in V$_2$O-based altermagnets

We theoretically investigate charge transport in a junction between a conventional superconductor and a V$_2$O-based altermagnet exhibiting distinctive spin-split quasi-one-dimensional Fermi surfaces. The altermagnet is described by a microscopically motivated seven-basis-state model with six-orbital characters that incorporates sublattice degrees of freedom associated with both V and O sites. Based on calculations performed under various boundary conditions, we demonstrate the robust emergence of specular Andreev reflection with a distinctive spin polarization. Furthermore, we propose an efficient multiterminal setup to detect this specular Andreev reflection through nonlocal conductance measurements. Our results establish V$_2$O-based altermagnets as a promising platform for realizing spin-resolved Cooper pair splitting, which is essential for generating energy-entangled electron pairs.

cond-mat.supr-con

Competing Interlayer Loop Currents and Superconductivity in the Bilayer $t$-$J_\perp$-$V$ Model

The recent discovery of high-$T_c$ superconductivity in pressurized and thin-film bilayer nickelates, featuring a strong interlayer exchange coupling, and their potential similarities with cuprate superconductors, has made this a very active topic in condensed matter physics. In the present paper we study the strongly correlated one-orbital ($d_{x^2-y^2}$) bilayer $t$-$J_\perp$-$V$ model for nickelates, where $V$ denotes the Coulomb interactions, using a controlled large-$N$ expansion at and beyond the mean-field level. Focusing on the out-of-plane spin exchange interaction ($J_\perp$), we find that it triggers both out-of-plane $s$-wave superconductivity and an out-of-plane bond-order phase ($z$-BOP) instability. The $z$-BOP gives rise to a complex $z$-axis hopping dominated by its imaginary component, which drives out-of-plane currents and induces in-plane ones, spontaneously forming on the vertical plaquettes a loop-current state that breaks time-reversal symmetry. Competition between this loop-current phase and superconductivity yields a dome-shaped superconducting region, with optimal superconductivity occurring near the $z$-BOP quantum critical point. The resulting phase diagram features a pure loop-current region, a low-doping coexistence phase, a pure superconducting state at higher doping, and a correlated metallic state.

cond-mat.str-el

Engineering Dirac interface states

We develop a low-energy theory of interface states in anisotropic multivalley Dirac systems whose masses and kinetic parameters are allowed to vary across an interface. For sharp interfaces, current-conserving matching conditions yield analytic expressions for the existence, localization and dispersion of the bound states. We show that the interface velocity is determined by the weighted tangential kinetic terms on the two sides of the seam. Their cancellation can suppress the linear velocity and generate an interface band that is flat to leading order near the projected Dirac point. For the special antisymmetric configuration in which both the Dirac mass and the tangential kinetic coefficient reverse sign with unchanged magnitude, the transparent sharp-interface solution is exactly dispersionless for all conserved momenta within the linear Dirac theory, while the surrounding bulk bands remain dispersive. We extend the theory to smooth interfaces, where the modified bound-state envelope changes the linear interface velocity through a spatial average of the tangential kinetic coefficient. We also investigate quadratic corrections in the kinetic \(σ_x\) and \(σ_y\) channels. To first order in their coefficients and through linear order in the interface momentum, these terms shift the interface-state energy but produce no additional correction to the linear velocity. Finally, we combine continuum and lattice models to show how interface modes from distinct valleys hybridize and how the resulting dispersions depend on microscopic interface properties. Our results establish design principles for controlling the dispersion, localization, and hybridization of Dirac interface states. We further examine two graphene-based mass-domain-wall models as experimentally inspired examples of dispersive copropagating and counterpropagating interface states.

cond-mat.mtrl-sci

Quantum Geometric Origin of the Intrinsic Nonlinear Hall Effect

We decompose the intrinsic second-order nonlinear Hall effect (NLHE) of a generic multiband system into its quantum-geometric contributions within a fully quantum-mechanical, projector-based formalism. By expanding the nonlinear conductivity in powers of the quasiparticle lifetime $τ$, we recover the established Berry curvature dipole at order $τ$ and clarify discrepancies in previous literature concerning the (interband) quantum metric dipole (or Berry curvature polarizability) contribution at order $τ^0\textrm{.}$ Crucially, our method reveals an additional contribution at order $τ^0$, determined by the {\it intraband} quantum metric dipole (intraQMD), arising from additional virtual interband transitions captured within the fully quantum-mechanical treatment. The intraQMD contribution is generically nonzero in systems with broken time-reversal symmetry and can be distinguished from other geometric contributions by symmetry. Analytical results for low-energy models of topological band crossings, which are hotspots of quantum geometry, demonstrate how band topology influences each contribution. In particular, the intraQMD contribution is especially large in gapped Dirac cones in antiferromagnets. Through a comprehensive symmetry classification of all magnetic space groups, we identify several candidate materials that are expected to exhibit large intrinsic NLHE, including the topological antiferromagnets Yb$_3$Pt$_4$, CuMnAs, and CoNb$_3$S$_6$, as well as the nodal-plane material MnNb$_3$S$_6$.

cond-mat.mes-hall

Raman response in superconducting multiorbital systems with application to nickelates

The recent discovery of high-$T_c$ superconductivity in pressurized and thin film nickelates is nowadays one of the most relevant and active topics in solid-state physics. The origin of superconductivity together with the relevance of multiorbital physics are highly discussed issues in this field. Knowledge of the size of the gap and its symmetry is of fundamental interest to uncover the superconducting mechanism at play in the nickelates. Electronic Raman scattering is a powerful tool to investigate the main characteristics of the gap. Here, we investigate the Raman response in the superconducting phase for three different models: Two-orbital models, including $d_{x^2-y^2}$ and $d_{z^2}$ orbitals, with one and two layers; as well as a bilayer model with the $d_{x^2-y^2}$ orbital as the only active one. For each of these models, we consider different pairing symmetries and determine their characteristic fingerprints in the Raman response. For the two-orbital models, we perform full multiorbital calculations including interorbital and intraorbital scattering, and compare the results with those obtained using the additive Raman response where each band is considered separately. Our results should be useful for discussing the minimal model for superconductivity and its pairing symmetry in nickelates. The obtained results and discussions, as well as the presented formalism, are also of general interest for other multiorbital systems.

cond-mat.supr-con

Detecting pairing symmetry of bilayer nickelates using electronic Raman scattering

The recent discovery of high-temperature superconductivity in both bulk and thin-film bilayer nickelates La$_3$Ni$_2$O$_7$ has garnered significant attention. However, the corresponding pairing symmetry remains debated in both experiments and theoretical studies due to conflicting experimental evidence from bulk and thin-film materials. In this work, we examine the electronic Raman response across different channels for various pairing symmetries within a two-orbital bilayer model. By comparing Raman susceptibilities obtained from multiorbital and band-additive approaches, we demonstrate that Raman response can distinguish between different pairing symmetries and identify pocket-dependent gap amplitudes for both fully gapped and nodal superconducting states. Specifically, the nodal $d_{x^2-y^2}/d_{xy}$-wave pairing exhibits robust low-energy power-law behavior, distinct from a fully gapped pairing. Additionally, for the $s_{\pm}$-wave pairing, the detailed gap anisotropy on the $β$ pocket can be determined. Possible experimental implications are also discussed. Our results highlight the crucial role of multiorbital effects in shaping the Raman spectra and establish electronic Raman scattering as a powerful and symmetry-resolved probe for determining the superconducting gap in unconventional superconductors.

cond-mat.supr-con

Suppression of Spectral Gap and Flat Bands on a Cuprate Superconductor Side-Surface

Side surfaces of cuprate superconductors are expected to display a suppressed $d$-wave order parameter and zero-energy topological flat bands with a large density of states, making them susceptible to symmetry broken orders. Yet such surfaces have never been investigated with momentum-resolved, surface-sensitive probes, because high-temperature superconductors rarely cleave along them. Using focused-ion-beam milling to define a controlled breaking point, we expose pristine (110) side surfaces of overdoped La$_{2-x}$Sr$_x$CuO$_4$ ($x=0.22$) suitable for angle-resolved photoemission. We observe the suppression of the superconducting spectral gap within our energy resolution ($\sim 4~\mathrm{meV}$), and surprisingly, the expected zero-energy flat band peak is also suppressed, despite the high topographic quality of the surface. Self-consistent Bogoliubov--de~Gennes calculations show that the measured geometric roughness of the cleaved surface is too weak to eliminate these modes. The calculations further demonstrate that bulk inhomogeneities characteristic of high-temperature superconductors, modelled as moderate Anderson-type disorder, can broaden the flat-band states beyond detectability. Our results provide the first momentum-resolved view of the electronic structure on a cuprate side surface and reveal disorder as the key factor currently preventing appearance of flat bands and their associated correlated orders.

cond-mat.supr-con

Comparative Raman study of Ruddlesden-Popper nickelates and the monolayer-trilayer polymorph

Ruddlesden-Popper (RP) nickelates have attracted intense interest following the discovery of superconductivity in several members of the series, including bilayer (BL) La$_3$Ni$_2$O$_7$, trilayer (TL) La$_4$Ni$_3$O$_{10}$, and structural polymorphs composed of monolayer-bilayer or monolayer-trilayer (ML-TL) units. However, an inherent propensity of the RP series to form intergrown phases during single-crystal synthesis, together with spatial variations in oxygen stoichiometry, has complicated the determination of their intrinsic material properties. As a consequence, conflicting reports have emerged on both their electronic phase transitions and lattice dynamics. In this work, we perform a comparative study of the phononic and electronic Raman responses of high-quality ML-TL single crystals and contrast them with those of other RP nickelates, using samples with optimized oxygen content. We establish several Raman spectral features that enable unambiguous phase identification across the series. Moreover, we uncover characteristics in the phononic and electronic Raman response of ML-TL that are not reflected in the pure ML and TL compounds. We attribute these differences to a distinctive electronic structure arising from self-doping and confinement effects induced by the ML unit within the ML-TL lattice architecture.

cond-mat.str-el

Quantum geometry and low-frequency optical conductivity of nodal planes

Nodal planes, two-dimensional symmetry-enforced band crossings, can carry a topological charge, similar to Weyl points. While the transport properties of Weyl points are well understood, those of nodal planes remain largely unexplored. These properties are influenced not only by the Berry curvature, but also by other quantum geometric quantities. In this work we study the quantum geometry - specifically the Berry curvature and quantum metric - and the linear optical conductivity of topological nodal planes. We introduce a low-energy model and investigate its low-frequency optical responses to determine the unique signatures of nodal planes. By comparing these findings to the optical response in a tight-binding model with a topological nodal plane, we observe consistent low-frequency behavior with a cubic power law. This paves the way for the experimental detection of nodal planes through optical conductivity measurements for which we suggest suitable materials, most promisingly the material group $X$Mo$_3$S$_3$ ($X$ = Rb, K, Cs).

cond-mat.mes-hall

Exotic superconducting states in altermagnets

The interplay between magnetism and superconductivity is one of the central topics of condensed matter physics, which has recently been put into new light by the discovery of altermagnets. Here, we study this interplay from a fundamental symmetry perspective using irreducible co-representations of the altermagnetic spin-point groups. We construct and tabulate all symmetry-allowed pairing functions for altermagnets, which uncovers numerous exotic pairing states. We focus on three of them, namely: (i) a non-unitary superconductor with different spatial anisotropies for the spin-up and spin-down condensates, (ii) a half-and-half metal-superconductor where only electrons with one of the two spin components form Cooper pairs, and (iii) a spin chiral superconductor with spin-polarized edge states. Interestingly, the first of these three superconductors exhibits an unusual fractional ac Josephson current for only one of the two spin polarizations. We present phenomenological Ginzburg-Landau theories for these unconventional superconductors and show that they correspond to stable minima of the free energies. We examine their topological properties, study the effects of small spin-orbit coupling, consider possible material examples, and investigate their topological responses.

cond-mat.supr-con

Out-of-plane bond-order phase, superconductivity, and their competition in the $t$-$J_\parallel$-$J_\perp$ model: Possible implications for bilayer nickelates

Almost four decades of intense research have been invested to study the physics of high-T$_c$ cuprate superconductors. The recent discovery of high-T$_c$ superconductivity in pressurized bilayer nickelates and its potential similarities with cuprate superconductors may open a new window to understand this long-standing problem. We have studied the proposed bilayer $t$-$J_\parallel$-$J_\perp$ model [where $J_\parallel$ ($J_\perp$) is the in-plane (out-of-plane) magnetic exchange] in a large-$N$ approach on the basis of the path integral representation for Hubbard operators, which allows to obtain results at mean-field and beyond mean-field level. We find that $J_\perp$ is a candidate for triggering high superconducting $T_c$ values at quarter filling (hole doping $δ=0.5$) of the $d_{x^2-y^2}$ orbitals. Beyond mean-field level, we find a new phase, an out-of-plane bond-order phase (z-BOP), triggered also by $J_\perp$. z-BOP develops below a critical temperature which decreases with increasing doping and vanishes at a quantum critical point below quarter filling. The occurrence of this phase and its competition with superconductivity leads to a superconducting dome-shaped behavior as a function of doping and as a function of $J_\perp$. Qualitative comparisons with the physics of cuprates and the recent literature on the new pressurized nickelates are given along the paper.

cond-mat.supr-con

Oscillating-charged Andreev Bound States and Their Appearance in UTe$_2$

Surface Andreev bound states, including Majorana bound states in topological superconductors, are typically charge neutral. In this work, we demonstrate the emergence of unconventional charged Andreev bound states in a superconductor with a sublattice degree of freedom, where the sign of charge density of the Andreev bound states oscillates between the two sublattices. The oscillating-charged Andreev bound states lead to a complete breakdown of the proportionality among the electron part of the spectral function, the local density of states, and the tunneling conductance spectrum for energies below the superconducting gap. We also discuss the possible occurrence of these Andreev bound states in UTe$_2$ and locally noncentrosymmetric superconductors.

cond-mat.supr-con

Spin-polarized Specular Andreev Reflections in Altermagnets

We show theoretically that specular Andreev reflection occurs stably at altermagnet--superconductor interfaces, which is a phenomenon that has previously been predicted only in a limited range of materials, such as Dirac/Weyl materials with fine-tuned chemical potentials. Furthermore, the characteristic spin-split bands of the altermagnet lead to a distinctive spin polarization in the specular Andreev reflections. By utilizing this feature, we propose a device that integrates the functions of both a Cooper pair splitter and a spin beam splitter, thereby creating energy-entangled electron pairs. The positive nonlocal conductance and the positive noise cross-correlation are unambiguous signatures of specular Andreev reflections in the proposed device.

cond-mat.supr-con

Weak $\mathbb{Z}_2$ Supertopology

Crystal symmetries can enforce all bands of a material to be topological, a property that is commonly referred to as ``supertopology". Here, we determine the symmetry-enforced $\mathbb{Z}_2$ supertopologies of non-magnetic centrosymmetric materials with weak and strong spin-orbit coupling (SOC). For weak (i.e., negligible) SOC, crystal symmetries can enforce Dirac nodal lines protected by a $π$-Berry phase, while for strong SOC, crystal symmetries can give rise to nontrival weak $\mathbb{Z}_2$ topologies in 2D subplanes of the 3D Brillouin zone. We catalogue all centrosymmetric space groups whose symmetries enforce these $\mathbb{Z}_2$ supertopologies. Suitable material realizations are identified and experimental signatures of the supertopologies, such as quantum spin Hall states, are being discussed.

cond-mat.mtrl-sci

Tunable Octdong and Spindle-Torus Fermi Surfaces in Kramers Nodal Line Metals

It has recently been proposed that all achiral non-centrosymmetric crystals host so-called Kramers nodal lines, which are doubly degenerate band crossings connecting time-reversal invariant momenta in the Brillouin zone that arise due to spin-orbit coupling. When Kramers nodal lines intersect the Fermi level, they form exotic three-dimensional Fermi surfaces which is certain configurations can be fully described by two-dimensional massless Dirac fermions. These Fermi surfaces are predicted to realize a quantized optical conductivity with multiple quantized levels a large light- and field-induced anomalous Hall effect. However, until now, no Kramers nodal line metal with such unconventional Fermi surfaces has been experimentally observed. Here, we extend the search for Kramers nodal line metals beyond the previously considered case in which the Fermi surfaces enclose a single time-reversal invariant momentum. Using angle-resolved photoelectron spectroscopy measurements and ab-initio calculations, we present evidence that the 3R polytypes of TaS$_2$ and NbS$_2$ are Kramers nodal line metals with open Octdong and Spindle-torus Fermi surfaces, respectively. We show that by reducing the band filling, a transition between these two configurations can be observed. Moreover, our data suggests a naturally occurring size quantization effect of inclusions of 3R-TaS$_2$ in commercially available 2H-TaS$_2$ crystals, which could enable the observation of quantized optical conductivity. Finally, since the open Fermi-surfaces encircle two time-reversal invariant momenta each, we predict a phase transition from a Kramers nodal line metal to a conventional metal by strain or uniaxial pressure. Our work establishes the 3R phase of metallic transition metal dichalcogenides as a tunable platform to explore new phenomena expected from exotic Fermi surfaces in Kramers nodal line metals.

cond-mat.mtrl-sci

Noise-to-current ratio divergence as a fingerprint of dispersing Majorana edge modes

The definitive detection of Majorana modes in topological superconductors is a key issue in condensed matter physics. Here we propose a smoking-gun experiment for the detection of one-dimensional dispersing Majorana edge modes, based on theoretical results for multi-terminal transport in a setup consisting of two normal metal leads and a topological superconductor. In the proposed device, the unpaired nature of the Majorana edge modes inherently leads to the absence of the charge current in the linear response regime, while the current fluctuation remains significant. Therefore, the divergence in the noise-to-current ratio serves as unambiguous evidence for the presence of the dispersing Majorana edge modes. We reach this conclusion analytically, without relying on any specific model of topological superconductors. In addition, using tight-binding models of topological-insulator-based topological superconductors, we numerically verify the predicted divergent noise-to-current ratio. We also discuss the application of our proposal to the CoSi$_2$/TiSi$_2$ heterostructure and the iron-based superconductor FeTe$_{1-x}$Se$_x$.

cond-mat.supr-con

Callan-Rubakov effects in topological insulators

The Callan-Rubakov effect describes monopole-catalyzed proton decay. While this effect is fundamental for quantum field theories, its experimental observation has remained far from reality. Here, we reveal a similar, but experimentally reachable, defect-catalysis of the quantum anomaly in topological materials. In particular, surface Dirac fermions on topological insulators develop a distinct localized state at the position of dislocations or $π$-fluxes, which mediates spin-flip time-reversal breaking scattering or absorption of electrons. Despite the Hermiticity of topological insulators, a non-Hermitian topological number guarantees the robust existence of the localized state. Our finding implies that non-magnetic defects may behave like magnetic impurities on surfaces of topological insulators. Using the K-theory classification, we generalize this condensed-matter version of the Callan-Rubakov effect to other classes of topological materials.

cond-mat.mes-hall

Fate of Bosonic Topological Edge Modes in the Presence of Many-Body Interactions

Many magnetic materials are predicted to exhibit bosonic topological edge modes in their excitation spectra, because of the nontrivial topology of their magnon, triplon, or other quasi-particle band structures. However, there is a discrepancy between theory prediction and experimental observation, which suggests some underlying mechanism that intrinsically suppresses the expected experimental signatures, like the thermal Hall current. Many-body interactions that are not accounted for in the non-interacting quasi-particle picture are most often identified as the reason for the absence of the topological edge modes. Here we report persistent bosonic edge modes at the boundaries of a ladder quantum paramagnet with gapped triplon excitations in the presence of the full many-body interaction. We use tensor network methods to resolve topological edge modes in the time-dependent spin-spin correlations and the dynamical structure factor, which is directly accessible experimentally. We further show that signatures of these edge modes survive even when the non-interacting quasi-particle theory breaks down, discuss the topological phase diagram of the model, demonstrate the fractionalization of its low-lying excitations, and propose potential material candidates.

cond-mat.str-el