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Andreas Reiserer

Publications and source records attributed to Andreas Reiserer.

At least 19 recordsLinked to original sources

Quantum memory on a nanophotonic silicon chip

Integrated photonic circuits offer great promise for quantum technologies. However, due to the rapid propagation of light, many envisioned applications require efficient on-chip quantum memories with a programmable delay, compact footprint, and high fidelity. Implementing this based on standard semiconductor processing technology is an outstanding challenge. Here, we realize such memories using erbium-doped silicon waveguides, fabricated as part of a multi-wafer project by a nanophotonic foundry. We demonstrate light storage with a $44.2(9)\ \text{MHz}$ bandwidth and a programmable delay exceeding $1\ \mu \text{s}$ in a device with a footprint of only $1.5\times 10^{-2}\ \text{mm}^2$, outperforming on-chip delay lines by many orders of magnitude. The phase of the read-out light field is preserved with a visibility of $91.3(30)\ \%$. The efficiency of $1.89(28)\times 10^{-8}$ can be improved in future devices through resonator enhancement and higher dopant concentrations. With this, the demonstrated approach will pave the way towards applications in photonic quantum computing based on scalable silicon processing technology.

quant-ph

Cavity-enhanced optical readout and control of nuclear spin qubits

Their exceptional coherence makes nuclear spins in solids a prime candidate for quantum memories in quantum networks and repeaters. Still, the direct all-optical initialization, coherent control, and readout of individual nuclear spin qubits have been an outstanding challenge. Here, this is achieved by embedding 167-Er dopants in yttrium orthosilicate in a cryogenic Fabry-Perot cavity, whose linewidth of 65 MHz is much smaller than the 0.9 GHz separation of neighboring hyperfine levels. Frequency-selective emission enhancement thus enables a single-shot readout fidelity of 91(2)%. Furthermore, a large magnetic field freezes paramagnetic impurities, leading to coherence times exceeding 0.2 s. The combination of nuclear-spin qubits with frequency-multiplexed addressing and lifetime-limited photon emission in the minimal-loss telecommunications C-band establishes 167-Er as a leading platform for long-range, fiber-based quantum networks.

quant-ph

Single-photon emitters and spin-photon interfaces in silicon

Single photons enable the distribution of quantum information over large distances and thus play a major role in quantum technologies such as communication and computing. Solid-state emitters are practical and efficient sources of single photons that can be manufactured in large numbers. When combined with a spin, the resulting spin-photon interfaces can store quantum states for extended periods and serve as the basis for quantum networks and repeaters. Among the many host materials explored over the past few decades, silicon stands out for its advanced nanofabrication, the maturity of its integrated photonics and microelectronics, and its high isotopic purity, which leads to exceptionally long spin coherence. These properties position silicon single-photon emitters and spin-photon interfaces among the most promising hardware platforms for implementing quantum networks and distributed quantum information processors. This review summarizes the current state of the art and open challenges towards coherent single-photon sources and scalable spin-photon interfaces based on color centers and erbium dopants in nanophotonic silicon structures.

quant-ph

Spectral stability of cavity-enhanced single-photon emitters in silicon

The unrivaled maturity of its nanofabrication makes silicon a promising hardware platform for quantum information processing. To this end, efficient single-photon sources and spin-photon interfaces have been implemented by integrating color centers or erbium dopants into nanophotonic resonators. However, the optical emission frequencies in this approach are subject to temporal fluctuations on both long and short timescales, which hinders the development of quantum applications. Here, we investigate this limitation and demonstrate that it can be alleviated by integrating the emitters into Fabry-Perot instead of nanophotonic resonators. Their larger optical mode volume enables both increasing the distance to crystal surfaces and operating at a lower dopant concentration, which reduces implantation-induced crystal damage and interactions between emitters. As a result, we observe a fivefold reduction of the spectral diffusion linewidth down to 4.0(2) MHz. Calculations and experimental investigations of isotopically purified 28-Si crystals suggest that the remaining spectral instability is caused by laser-induced electric-field fluctuations. In direct comparison with a nanophotonic device, the instability is significantly reduced at the same intracavity power, enabling a tenfold increase of the optical coherence time up to 20(1) microseconds. These findings represent a key step towards spectrally stable spin-photon interfaces in silicon and their potential applications in quantum networking and distributed quantum information processing.

quant-ph

Inhibited radiative decay enhances single-photon emitters

Quantum networks and modular quantum computers require efficient spin-photon interfaces, often realized using optical resonators that enhance radiative decay on a desired transition. However, this requires small mode volumes and high quality factors, which limits multiplexing capacity and demands precise frequency tuning. Here, we demonstrate an alternative approach that circumvents these bottlenecks for upscaling. Using a W1 silicon photonic crystal waveguide with a tailored photonic bandgap, we selectively inhibit unwanted decay pathways, thereby redirecting emission to the desired transition. This enables efficient photon collection over a large frequency range, allowing the resolution and individual addressing of tens of erbium dopants. Their lifetimes are preserved, or even increased, compared to bulk material. The extended mode volume of the devices enables the use of lower dopant concentrations, thereby improving emitter coherence. Our approach can be combined with Purcell enhancement and applied to other spin-qubit platforms, opening intriguing perspectives for photonic quantum technologies.

quant-ph

Cavity-enhanced spectroscopy of individual nuclear spins in a dense bath

Echo-based spectroscopy of the superhyperfine interaction of an electronic spin with nuclear spins in its surroundings enables detailed insights into the microscopic magnetic environment of spins in solids. Still, it is an outstanding challenge to resolve individual nuclear spins in a dense bath, in which many of them exhibit a comparable coupling strength. This simultaneously requires a high spectral resolution and a large signal-to-noise ratio. However, when probing spin ensembles, dipolar interactions between the dopants can lead to a concentration-dependent trade-off between resolution and signal. Here, we fully eliminate this limitation of previous optical-echo-envelope-modulation spectroscopy experiments by integrating the emitters into a high-finesse resonator, which allows for strong optical echoes even at very low concentrations. To demonstrate its potential, the technique is applied to erbium dopants in yttrium-orthosilicate (Er:YSO). Achieving an unprecedented spectral resolution enables precise measurements of the superhyperfine interaction with four of the Y nuclear spins densely surrounding each emitter. The achieved boost of the signal, enabled by the resonator, allows for extending the approach to the lowest concentration possible -- to the level of single dopants, thereby providing a tool for detecting and studying individual nuclear spins. Thus, our technique paves the way for an improved understanding of dense nuclear spin baths in solids.

quant-ph

Luminescence thermometry based on photon emitters in nanophotonic silicon waveguides

The reliable measurement and accurate control of the temperature within nanophotonic devices is a key prerequisite for their application in both classical and quantum technologies. Established approaches use sensors that are attached in proximity to the components, which only offers a limited spatial resolution and thus impedes the measurement of local heating effects. Here, we therefore study an alternative temperature sensing technique that is based on measuring the luminescence of erbium emitters directly integrated into nanophotonic silicon waveguides. To cover the entire temperature range from 295 K to 2 K, we investigate two different approaches: The thermal activation of non-radiative decay channels for temperatures above 200 K and the thermal depopulation of spin- and crystal field levels at lower temperatures. The achieved sensitivity is 0.22(4) %/K at room temperature and increases up to 420(50) %/K at approximately 2 K. Within a few-minute measurement interval, we thus achieve a measurement precision that ranges from 0.04(1) K at the lowest studied temperature to 6(1) K at ambient conditions. In the future, the measurement time can be further reduced by optimizing the excitation pulse sequence and the fiber-to-chip coupling efficiency. Combining this with spatially selective implantation promises precise thermometry from ambient to cryogenic temperatures with a spatial resolution down to a few nanometers.

quant-ph

Characterization of the spin and crystal field Hamiltonian of erbium dopants in silicon

The integration of coherent emitters into low-loss photonic circuits is a key technology for quantum networking. In this context, nanophotonic silicon devices implanted with erbium are a promising hardware platform that combines advanced wafer-scale nanofabrication technology with coherent emission in the minimal-loss band of optical fibers. Recent studies have reported two distinct sites in the silicon lattice in which erbium can be reproducibly integrated with particularly promising properties. Here, for an in-depth analysis of these sites, resonant fluorescence spectroscopy is performed on a nanophotonic waveguide in magnetic fields applied along different orientations. In this way, the site symmetry is determined, the spin Hamiltonian is reconstructed and a partial fit of the crystal field Hamiltonian is performed. The obtained quantitative description of the magnetic interaction allows the optimization of Zeeman splittings, optical branching ratios or microwave driving to the needs of future experiments. Beyond that, the derived site symmetry constrains the location of the erbium dopant in the silicon unit cell. This is a key step towards a detailed microscopic understanding of the erbium sites, which may help to improve the integration yield, thus paving the way to efficient nanophotonic quantum memories based on the Er:Si platform.

quant-ph

Optical single-shot readout of spin qubits in silicon

The digital revolution was enabled by nanostructured devices made from silicon. A similar prominence of this material is anticipated in the upcoming quantum era as the unrivalled maturity of silicon nanofabrication offers unique advantages for integration and up-scaling, while its favorable material properties facilitate quantum memories with hour-long coherence. While small spin-qubit registers have exceeded error-correction thresholds, their connection to large quantum computers is an outstanding challenge. To this end, spin qubits with optical interfaces offer key advantages: they can minimize the heat load and give access to modular quantum computing architectures that eliminate cross-talk and offer a large connectivity via room-temperature photon routing. Here, we implement such an efficient spin-photon interface based on erbium dopants in a nanophotonic resonator. We thus demonstrate optical single-shot readout of a spin in silicon whose coherence exceeds the Purcell-enhanced optical lifetime, paving the way for entangling remote spins via photon interference. As erbium dopants can emit coherent photons in the minimal-loss band of optical fibers, and tens of such qubits can be spectrally multiplexed in each resonator, the demonstrated hardware platform offers unique promise for distributed quantum information processing and the implementation of a quantum internet based on integrated silicon devices.

quant-ph

Spectral Multiplexing of Rare-earth Emitters in a Co-doped Crystalline Membrane

The spectral addressing of many individual rare-earth dopants in optical resonators offers great potential for realizing distributed quantum information processors. To this end, it is required to understand and control the spectral properties of the emitters in micron-scale devices. Here, erbium emitters are investigated in a Fabry-Perot resonator which contains a ten-micrometer-thin membrane of crystalline yttrium orthosilicate that is co-doped with europium. The co-doping allows for tailoring the inhomogeneous distribution of the emitter frequency, which enables high-fidelity spectral multiplexing of more than 360 qubits with Purcell factors exceeding 35. At the same time, the optical coherence is preserved up to 0.62(3) ms under dynamical decoupling. Without decoupling, the coherence still reaches the lifetime limit for the emitters with the strongest Purcell enhancement that leads up to a 110-fold lifetime reduction, down to 0.104(9) ms. Future work may combine this with long-lived nuclear spin memories, which makes the investigated co-doped membranes a promising platform for quantum repeaters and distributed quantum computers.

quant-ph

Erbium emitters in commercially fabricated nanophotonic silicon waveguides

Quantum memories integrated into nanophotonic silicon devices are a promising platform for large quantum networks and scalable photonic quantum computers. In this context, erbium dopants are particularly attractive, as they combine optical transitions in the telecommunications frequency band with the potential for second-long coherence time. Here we show that these emitters can be reliably integrated into commercially fabricated low-loss waveguides. We investigate several integration procedures and obtain ensembles of many emitters with an inhomogeneous broadening of < 2 GHz and a homogeneous linewidth of < 30 kHz. We further observe the splitting of the electronic spin states in a magnetic field up to 9 T that freezes paramagnetic impurities. Our findings are an important step towards long-lived quantum memories that can be fabricated on a wafer-scale using CMOS technology.

quant-ph

Purcell enhancement of single-photon emitters in silicon

Individual spins that are coupled to telecommunication photons offer unique promise for distributed quantum information processing once a coherent and efficient spin-photon interface can be fabricated at scale. We implement such an interface by integrating erbium dopants into a nanophotonic silicon resonator. We achieve spin-resolved excitation of individual emitters with < 0.1 GHz spectral diffusion linewidth. Upon resonant driving, we observe optical Rabi oscillations and single-photon emission with a 78-fold Purcell enhancement. Our results establish a promising new platform for quantum networks.

quant-ph

Cavity-enhanced quantum network nodes

A future quantum network will consist of quantum processors that are connected by quantum channels, just like conventional computers are wired up to form the Internet. In contrast to classical devices, however, the entanglement and non-local correlations available in a quantum-controlled system facilitate novel fundamental tests of quantum theory. In addition, they enable numerous applications in distributed quantum information processing, quantum communication, and precision measurement. While pioneering experiments have demonstrated the entanglement of two quantum nodes separated by up to 1.3 km, and three nodes in the same laboratory, accessing the full potential of quantum networks requires scaling of these prototypes to many more nodes and global distances. This is an outstanding challenge, posing high demands on qubit control fidelity, qubit coherence time, and coupling efficiency between stationary and flying qubits. In this work, I will describe how optical resonators facilitate quantum network nodes that achieve the above-mentioned prerequisites in different physical systems -- trapped atoms, defect centers in wide-bandgap semiconductors, and rare-earth dopants -- by enabling high-fidelity qubit initialization and readout, efficient generation of qubit-photon and remote qubit-qubit entanglement, as well as quantum gates between stationary and flying qubits. These advances open a realistic perspective towards the implementation of global-scale quantum networks in the near future.

quant-ph

Spectral multiplexing of telecom emitters with stable transition frequency

In a quantum network, coherent emitters can be entangled over large distances using photonic channels. In solid-state devices, the required efficient light-emitter interface can be implemented by confining the light in nanophotonic structures. However, fluctuating charges and magnetic moments at the nearby interface then lead to spectral instability of the emitters. Here we avoid this limitation when enhancing the photon emission up to 70(12)-fold using a Fabry-Perot resonator with an embedded 19 micrometer thin crystalline membrane, in which we observe around 100 individual erbium emitters. In long-term measurements, they exhibit an exceptional spectral stability of < 0.2 MHz that is limited by the coupling to surrounding nuclear spins. We further implement spectrally multiplexed coherent control and find an optical coherence time of 0.11(1) ms, approaching the lifetime limit of 0.3 ms for the strongest-coupled emitters. Our results constitute an important step towards frequency-multiplexed quantum-network nodes operating directly at a telecommunication wavelength.

quant-ph

Narrow optical transitions in erbium-implanted silicon waveguides

The realization of a scalable architecture for quantum information processing is a major challenge for quantum science. A promising approach is based on emitters in nanostructures that are coupled by light. Here, we show that erbium dopants can be reproducibly integrated at well-defined lattice sites by implantation into pure silicon. We thus achieve a narrow inhomogeneous broadening, less than 1 GHz, strong optical transitions, and an outstanding optical coherence even at temperatures of 8 K, with an upper bound to the homogeneous linewidth of around 10 kHz. Our study thus introduces a promising materials platform for the implementation of on-chip quantum memories, microwave-to-optical conversion, and distributed quantum information processing.

quant-ph

Coherent control in the ground and optically excited state of an ensemble of erbium dopants

Ensembles of erbium dopants can realize quantum memories and frequency converters that operate in the minimal-loss wavelength band of fiber optical communication. Their operation requires the initialization, coherent control and readout of the electronic spin state. In this work, we use a split-ring microwave resonator to demonstrate such control in both the ground and optically excited state. The presented techniques can also be applied to other combinations of dopant and host, and may facilitate the development of new quantum memory protocols and sensing schemes.

quant-ph

Laser stabilization to a cryogenic fiber ring resonator

The frequency stability of lasers is limited by thermal noise in state-of-the-art frequency references. Further improvement requires operation at cryogenic temperature. In this context, we investigate a fiber-based ring resonator. Our system exhibits a first-order temperature-insensitive point around $3.55$ K, much lower than that of crystalline silicon. The observed low sensitivity with respect to vibrations ($<5\cdot{10^{-11}}\,\text{m}^{-1} \text{s}^{2}$), temperature ($-22(1)\cdot{10^{-9}}\,\text{K}^{-2}$) and pressure changes ($4.2(2)\cdot{10^{-11}}\,\text{mbar}^{-2}$) makes our approach promising for future precision experiments.

physics.optics

Coherent and Purcell-enhanced emission from erbium dopants in a cryogenic high-Q resonator

The stability and outstanding coherence of dopants and other atom-like defects in tailored host crystals make them a leading platform for the implementation of distributed quantum information processing and sensing in quantum networks. Albeit the required efficient light-matter coupling can be achieved via the integration into nanoscale resonators, in this approach the proximity of interfaces is detrimental to the coherence of even the least-sensitive emitters. Here, we establish an alternative: By integrating a 19 micrometer thin erbium-doped crystal into a cryogenic Fabry-Perot resonator with a quality factor of nine million, we can demonstrate 59(6)-fold enhancement of the emission rate, corresponding to a two-level Purcell factor of 530(50), while preserving lifetime-limited optical coherence up to 0.54(1) ms. With its emission at the minimal-loss wavelength of optical fibers and its outcoupling efficiency of 46(8) %, our system enables coherent and efficient nodes for long-distance quantum networks.

quant-ph