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Andreas T. Güntner

Publications and source records attributed to Andreas T. Güntner.

2 recordsLinked to original sources

Odour sensing in turbulent plumes with high-speed electronic nose and non-invasive ground truth

Chemical sensing in real-world environments requires resolving rapidly fluctuating and spatially heterogeneous concentration fields. However, these dynamics are strongly distorted by widely used, low-cost metal-oxide (MOx) gas sensors, whose thermal and surface-kinetic response acts as a low-pass filter on the underlying concentration signal. Quantifying and compensating for these effects remains challenging, largely due to the lack of benchmark datasets that simultaneously capture the spatiotemporal structure of turbulent odour fields and the time-resolved response of point sensors. Here, we present a dataset combining planar laser-induced fluorescence (PLIF) measurements of an acetone tracer plume with synchronised recordings from a custom, kilohertz-rate microelectromechanical (MEMS) MOx electronic nose deployed in a laboratory wind tunnel. The PLIF system provides quantitative, two-dimensional concentration fields at high spatial and temporal resolution, while the co-located e-nose records film resistance, heater currents, and environmental parameters with aligned timestamps. The dataset enables quantitative assessment of sensor dynamics, development and benchmarking of reconstruction and deconvolution algorithms, and data-driven modelling of plume structure. All recordings, metadata, calibration files, and example analysis scripts are released in open, platform-independent formats. Together, these provide a valuable reference for researchers working in odour-guided robotics, environmental monitoring, computational fluid dynamics, and neuromorphic sensing, supporting the design and evaluation of high-speed odour-sensing systems.

eess.SP↗

Porous metal nitride film synthesis without template

Metal nitrides possess exceptional catalytic, electronic and physical properties making them widely used in (opto-)electronics and as hard coatings. When used as films in surface-active applications, however, their performance remains limited by poor mass transfer and reduced accessibility of reactive sites. This is associated to compact film architecture yielded by conventional deposition techniques (e.g., 16-26% for sputtered W$_2$N). Here, we demonstrate a template-free method for the design of highly porous (porosity > 84%) metal nitride films with high compositional versatility, as demonstrated for Cu3N, W2N, MoNx and TiN. These are obtained by exploiting the self-assembly of fractal-like metal oxide agglomerates during deposition from aerosols followed by their dry nitridation. In case of Cu$_3$N, monocristalline oxide nanoparticles were converted to polycrystalline nitrides during nitridation, as traced by X-ray diffraction and electron microscopy. Such films feature consistently lower resistances than their metal oxide counterparts, as well as high reactivity and mass transfer. This is exploited exemplarily for molecular sensing of NO$_2$ at only 75$^\circ$C temperature, leading to up to a five-fold higher response with faster response time over more compact spin-coated films for. As a result, our approach overcomes critical mass transfer performance limitations of metal nitride films that are also relevant for other applications like electrocatalysis and energy storage.

physics.app-ph↗