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Andreas Thies

Publications and source records attributed to Andreas Thies.

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Emergence of Propagating Exciton-Polaritons in Hybrid Waveguide-van der Waals Heterostructures

Integrating few-layer materials into photonic circuits is a promising concept for novel on-chip photonic applications. We incorporate transition metal dichalcogenides (TMDs) with femtosecond-laser-written surface waveguides, which are embedded in fused silica chips. Our novel low-temperature optical spectroscopy setup enables coupling to the waveguide and simultaneous focus from the top to the TMD layer for a distinct excitation and collection of micro-photoluminescence ($\mu$PL) signals in several measurement geometries. Along these lines, we observe spectral changes of the A exciton for encapsulated TMD monolayers when capturing the $\mu$PL signal propagating through the waveguide. Depending on the thickness of the encapsulation with hexagonal boron nitride (hBN), these changes manifest as energetic redshifts of the A exciton, or even a splitting of the A exciton into two components. We attribute this behavior to strong coupling of the waveguide mode and the exciton in the sample, giving rise to the formation of propagating exciton-polaritons. Our interpretation is supported by calculations for a simplified model of a slab waveguide in the vicinity of an exciton by using the transfer matrix method. Having proven to be a highly adaptable framework for the study of propagating polaritons, our experimental platform likewise holds great promise for harnessing the unique properties of exciton-polaristons in integrated photonic circuits.

cond-mat.mes-hall

Quantum Electrometer for Time-Resolved Material Science at the Atomic Lattice Scale

The detection of individual charges plays a crucial role in fundamental material science and the advancement of classical and quantum high-performance technologies that operate with low noise. However, resolving charges at the lattice scale in a time-resolved manner has not been achieved so far. Here, we present the development of an electrometer with 60 ns acquisition steps, leveraging on the spectroscopy of an optically-active spin defect embedded in a solid-state material with a non-linear Stark response. By applying our approach to diamond, a widely used platform for quantum technology applications, we can distinguish the distinct charge traps at the lattice scale, quantify their impact on transport dynamics and noise generation, analyze relevant material properties, and develop strategies for material optimization.

physics.app-ph

Telecom-Band SPDC in AlGaAs-on-Insulator Waveguides

Widespread commercial adoption of telecom-band quantum-key-distribution (QKD) will require fully integrated, room-temperature transmitters. Implementing highly efficient spontaneous parametric down-conversion (SPDC) on a platform that offers co-integration of the pump laser has been an outstanding challenge. Here, using such a platform based on AlGaAs-on-insulator waveguides, we report telecom-band SPDC (and second harmonic generation) with exceedingly large efficiencies of 26 GHz generated pairs/mW over a 7 THz bandwidth, which would saturate the usable photon-flux for a 70-channel wavelength-multiplexed QKD-system at merely 1.6 mW of pump laser power.

quant-ph

Optical probing of phononic properties of a tin-vacancy color center in diamond

The coherence characteristics of a tin-vacancy color center (SnV) in diamond are investigated through optical means, including linewidth broadening effects and coherent population trapping (CPT) between the ground state orbital levels. Spectral analysis is required as due to the large spin-orbit splitting of the orbital ground states, thermalization between the ground states occurs at rates that are impractical to measure directly in the time domain. First, by implementing a temperature-dependent linewidth broadening measurement, including the challenging-to-measure D transition, phononic coupling coefficients are determined. These measurements are performed on an emitter with a lifetime-limited linewidth and atom-like properties, making the measurement representative for high-quality SnVs. Next, a CPT-type experiment is carried out to independently analyze thermal decoherence processes at 4 K. The spectral information is transformed into its conjugate variable time, providing picosecond resolution and revealing an orbital depolarization timescale of ${\sim30{\rm~ps}}$. Consequences of the investigated dynamics are then used to estimate spin dephasing times limited by thermal effects.

quant-ph

On-Chip Integration of Single Solid-State Quantum Emitters with a SiO$_2$ Photonic Platform

One important building block for future integrated nanophotonic devices is the scalable on-chip interfacing of single photon emitters and quantum memories with single optical modes. Here we present the deterministic integration of a single solid-state qubit, the nitrogen-vacancy (NV) center, with a photonic platform consisting exclusively of SiO$_2$ grown thermally on a Si substrate. The platform stands out by its ultra-low fluorescence and the ability to produce various passive structures such as high-Q microresonators and mode-size converters. By numerical analysis an optimal structure for the efficient coupling of a dipole emitter to the guided mode could be determined. Experimentally, the integration of a preselected NV emitter was performed with an atomic force microscope and the on-chip excitation of the quantum emitter as well as the coupling of single photons to the guided mode of the integrated structure could be demonstrated. Our approach shows the potential of this platform as a robust nanoscale interface of on-chip photonic structures with solid-state qubits.

physics.optics