arXiv subjects

Andrei Manolescu

Publications and source records attributed to Andrei Manolescu.

At least 19 recordsLinked to original sources

arXiv2026

Driven square lattice of quantum dots in a magnetic field coupled to a cylindrical FIR-photon cavity

We present a comprehensive computational study of driven quantum dot arrays in a square lattice configuration, subject to an external magnetic field and coupled to a cylindrical far-infrared photon cavity. The driving is introduced through a harmonic modulation of the full electron-photon interaction, therefore including both paramagnetic and diamagnetic contributions. The electron-electron Coulomb interactions are treated within density functional theory, while the electron-photon coupling is modeled using a many-body configuration interaction approach at each iteration of the density functional. By exploiting the unique properties of the cylindrical TE$_{011}$ cavity mode, we demonstrate selective enhancement of diamagnetic two-photon transitions. Our results reveal that the effectiveness of harmonic modulation of the electron-photon interaction is strongly dependent on both the driving frequency and the electron occupation number per dot. When the driving frequency approaches twice the cavity photon frequency, the system exhibits resonant behavior characterized by efficient photon pumping, occupation of higher-order photon replicas, and activation of collective radial Coulomb breathing modes. These findings establish a controllable mechanism for manipulating photon states in coupled quantum dot-cavity systems and provide insights into the interplay among harmonic modulation, photonic excitations, magnetic confinement, and many-body electron correlations in dimensionally reduced nanostructures.

cond-mat.mes-hall↗

arXiv2026

Role of quantum confinement in semiconductor-superconductor core-shell nanowires

This work is motivated by the experimentally observed coherence of the supercurrent in semiconductor nanowires covered by a half-shell metallic superconductor, which leads to flux dependent supercurrent oscillations with period h/2e, as expected for a tubular superconductor, i.e. Little-Parks oscillations. We perform microscopic model calculations and compare the results for full and half metallic shells. We use an effective Hamiltonian derived from the Green's function of the proximitized semiconductor nanowire, where the presence of the superconductor is represented by a self energy. Furthermore, we incorporate the electrostatic band-bending at the metal-semiconductor interface as a rectangular narrow quantum well on the semiconductor side. The properties of the eigenstates of the effective Hamiltonian are determined by the spatial profile of the corresponding transverse modes in the normal state. For half-shell wires, transverse modes with high-enough energy expand outside the interface quantum well and generate eigenstates with mixed electron-hole character that surround the entire circumference of the nanowire, similar to eigenstates of the full-shell system. We identify these states as being responsible for the observed Little-Parks effect.

cond-mat.mes-hall↗

arXiv2026

Interplay between Aharonov-Bohm and Altshuler-Aronov-Spivak oscillations in phase-pure GaAs/InAs core/shell nanowires of different lengths

In GaAs/InAs core/shell nanowires, comprising a tubular conducting shell, interference phenomena observed under an axial field and originating from closed-loop states encircling the insulating core, provide an ideal platform for superconducting quantum devices that utilize effects such as Aharonov--Bohm or Altshuler--Aronov--Spivak-type conductance oscillations. Both effects are different in nature with respect to phase rigidity because of interference of non-time-reversed or time-reversed paths, respectively. Since their occurrence is largely governed by averaging effects, which depend on sample dimensions and the transport regime, we present a systematic study of flux-periodic oscillations of phase-pure zinc-blende GaAs/InAs core/shell nanowires as a function of gate voltage for samples with different contact separation lengths. Our analysis shows that with increasing contact separation length, averaging effects result in gradual reduction of $h/e$-periodic Aharonov--Bohm-type oscillations, while the $h/2e$-periodic Altshuler--Aronov--Spivak oscillations and its $h/4e$-periodic higher harmonics are enhanced. The additional phase rigidity seen in the $h/3e$-periodic oscillations is attributed to phase rigidity propagating from the neighbouring lower harmonics. Our tight-binding transport simulations on nanowires of different lengths which contain only a few scattering centers confirm the experimental observations regarding the different harmonics and their phase rigidity. Together, our experimental and simulation findings indicate quasi-ballistic transport with persistent Aharonov--Bohm-, and phase-rigid Altshuler--Aronov--Spivak-type oscillations despite few scattering centers.

cond-mat.mes-hall↗

arXiv2026

Spin-orbit interaction in core-shell semiconductor-metal nanowires

We study theoretically the spin-orbit interaction of electrons confined in a tubular semiconductor nanowire, between an inner semiconductor core and an outer metallic extra shell. A band off-offset potential is present at the inner semiconductor-semiconductor interface and a more complex potential barrier at the outer metal-semiconductor contact. The cross section of the nanowire has a hexagonal geometry. We use a model derived from the k-dot-p method, and discuss the effects of the interface potentials on the strength of the spin-orbit coupling and on the localization of the wave functions within the semiconductor shell

cond-mat.mes-hall↗

arXiv2026

Transit-time oscillations in nanoscale vacuum diode with a pure resistive load

We examine the Ramo current in a nanoscale planar vacuum diode undergoing field emission in the presence of a DC voltage supply and an external resistor. We describe a simple mechanism for generating persistent current oscillations in the diode due to the voltage drop across the external resistor (beam loading) which reduces the total field and inhibits the emission. The amplitude and the frequency, which is in the THz domain, depend on the operating parameters of the diode. Molecular dynamics simulations are used to find the characteristics and physical basis of the mechanism, and a simple analytical model is presented, in good agreement with the simulation.

cond-mat.mes-hall↗

arXiv2025

Discrete Electron Emission

Analysis of space-charge effects on electron emission typically makes some assumption of continuity and smoothness, whether this is continuity of charge as in the classical derivation of the Child-Langmuir current, or the mean-field approximation used in particle-in-cell simulations. However, when studying the physics of electron emission and propagation at the mesoscale it becomes necessary to consider the discrete nature of electronic charge to account for the space-charge effect of each individual point charge. In this paper we give an extensive analysis of some previous work on the distribution of electrons under space-charge limited conditions. We examine the spacing of electrons as they are emitted from a planar surface, We present simplified models for analysis of such conditions to derive scaling laws for emission and compare them to computer simulations.

physics.acc-ph↗

arXiv2025

Signatures of broken symmetries in the excitations of a periodic 2DEG coupled to a cylindrical photon cavity

In a two-dimensional electron gas (2DEG) in a periodic lateral superlattice subjected to an external homogeneous magnetic field and in a cylindrical far-infrared photon cavity we search for effects of broken symmetries: Static ones, stemming from the unit cell of the system, and the external magnetic field together with the dynamic ones caused by the vector potential of the cavity promoting magnetic types of transitions, and the chirality of the excitation pulse. The Coulomb interaction of the electrons is described within density functional theory, but the electron-photon interactions are handled by a configuration interaction formalism within each step of the density functional approach, both for the static and the dynamic system. In the dynamical calculations we observe weak chiral effects that change character as the strength of the electron-photon interaction and the external magnetic field are increased. From the analysis of the chiral effects we identify an important connection of the para- and diamagnetic electron-photon interactions that promotes the diamagnetic interaction in the present system when the interaction strength is increased. Furthermore, the asymmetric potential in the unit cell of the square array activates collective oscillation modes that are not present in the system when the unit cell has a higher symmetry.

cond-mat.mes-hall↗

arXiv2025

Spin-orbit interaction in tubular prismatic nanowires

We theoretically study the spin-orbit interaction in the outer regions of core-shell nanowires that can act as tubular, prismatic conductors. The polygonal cross section of these wires induces non-uniform electron localization along the wire perimeter. In particular, low-energy electrons accumulate in the corner regions, and in the case of narrow shells, conductive channels form along the sharp edges. In contrast, higher-energy electrons are shifted toward the facets. These two groups of states may be separated by large energy gaps, which can exceed the room-temperature energy in the case of triangular geometries. We compare the impact of spin-orbit interaction on the corner and side states of hexagonal and triangular shells grown on hexagonal cores as well as on triangular shells grown on triangular cores. We find that the spin-orbit splitting, and thus the degeneracy of energy states at finite wave vectors, strongly depend on the tube's geometry. We demonstrate that the weak spin-orbit coupling observed in clean wires can be significantly enhanced if the intermixing of core and shell materials takes place. Moreover, we show that the energy spectrum in the presence of spin-orbit interaction allows for estimating the interaction between states and shows that triangular shells can act as three independent wires in the low-energy regime, while they behave as interacting systems at higher-energy ranges.

cond-mat.mes-hall↗

arXiv2025

Spin-orbit interaction in square core-shell nanowires

We theoretically investigate the spin-orbit interaction of electrons confined in the outer regions of square core-shell nanowires. The polygonal cross section leads to the accumulation of low-energy electrons in the corners and the formation of a significant energy gap that separates these corner-localized states from higher-energy states localized along the sides. We show that the low-energy states behave like the states of independent quantum wires, while the higher-energy states exhibit features characteristic of coupled wires.

cond-mat.mes-hall↗

arXiv2025

Aharonov-Bohm and Altshuler-Aronov-Spivak oscillations in the quasi-ballistic regime in phase-pure GaAs/InAs core/shell nanowires

The realization of various qubit systems based on high-quality hybrid superconducting quantum devices, is often achieved using semiconductor nanowires. For such hybrid devices, a good coupling between the superconductor and the conducting states in the semiconductor wire is crucial. GaAs/InAs core/shell nanowires with an insulating core, and a conductive InAs shell fulfill this requirement, since the electronic states are strongly confined near the surface. However, maintaining a good crystal quality in the conducting shell is a challenge for this type of nanowire. In this work, we present phase-pure zincblende GaAs/InAs core/shell nanowires and analyze their low-temperature magnetotransport properties. We observe pronounced magnetic flux quantum periodic oscillations, which can be attributed to a combination of Aharonov-Bohm and Altshuler-Aronov-Spivak oscillations. From the gate and temperature dependence of the conductance oscillations, as well as from supporting theoretical transport calculations, we conclude that the conducting states in the shell are in the quasi-ballistic transport regime, with few scattering centers, but nevertheless leading to an Altshuler-Aronov-Spivak correction that dominates at small magnetic field strengths. Our results demonstrate that phase-pure zincblende GaAs/InAs core/shell nanowires represent a very promising alternative semiconductor nanowire-based platform for hybrid quantum devices.

cond-mat.mes-hall↗

arXiv2024

Spin-phase transition in an array of quantum rings controlled by cavity photons

We model a spin-phase transition in a two-dimensional square array, or a lateral superlattice, of quantum rings in an external perpendicular homogeneous magnetic field. The electron system is placed in a circular cylindrical far-infrared photon cavity with a single circularly symmetric photon mode. Our numerical results reveal that the spin ordering of the two-dimensional electron gas in each quantum ring can be influenced or controlled by the electron-photon coupling strength and the energy of the photons. The Coulomb interaction between the electrons is described by a spin-density functional approach, but the para- and the diamagnetic electron-photon interactions are modeled via a configuration interaction formalism in a truncated many-body Fock-space, which is updated in each iteration step of the density functional approach. In the absence of external electromagnetic pulses this spin-phase transition is replicated in the orbital magnetization of the rings. The spin-phase transition can be suppressed by a strong electron-photon interaction. In addition, fluctuations in the spin configuration are found in dynamical calculations, where the system is excited by a time-dependent scheme specially fit for emphasizing the diamagnetic electron-photon interaction.

cond-mat.mes-hall↗

arXiv2024

The tuning of para- and diamagnetic cavity photon excitations in a square array of quantum dots in a magnetic field

We employ a ``real-time'' excitation scheme to calculate the excitation spectra of a two-dimensional electron system in a square array of quantum dots placed in a circular cylindrical far-infrared photon cavity subjected to a perpendicular homogeneous external magnetic field. The Coulomb interaction of the electrons is handled via spin density functional theory and the para- and the diamagnetic parts of the electron-photon coupling are updated according to a configuration interaction method in each iteration of the density functional calculation. The results show that an excitation scheme built on using the symmetry of the lateral square superlattice of the dots and the cylindrical cavity produces both para- and diamagnetic resonance peaks with oscillator strengths that can be steered by the excitation pulse parameters. The excitation method breaks the conditions for the generalized Kohn theorem and allows for insight into the subband structure of the electron system and can be used both in and outside the linear response regime.

cond-mat.mes-hall↗

arXiv2024

Impact of interface defects on the band alignment and performance of TiO$_2$/MAPI/Cu$_2$O perovskite solar cells

Optimizing the interfaces in perovskite solar cells (PSCs) is essential for enhancing their performance, improving their stability, and making them commercially viable for large-scale deployment in solar energy harvesting applications. Point defects, like vacancies, have a dual role, as they can inherently provide a proper doping, but they can also reduce the collected current by trap-assisted recombination. Moreover, they can play an active role in ion migration and degradation. Using ab initio density functional theory (DFT) calculations we investigate the changes in the band alignment induced by interfacial vacancy defects in a TiO$_2$/MAPI/Cu$_2$O based PSC. Depending on the type of the vacancy (Ti, Cu, O, Pb, I) in the oxide and perovskite materials, additional doping is superimposed on the already existing background. Their effect on the performance of the PSCs becomes visible, as shown by SCAPS simulations. The most significant impact is observed for $p$ type doping of TiO$_2$ and $n$ type doping of Cu$_2$O, while the effective doping of the perovskite layer affects one of the two interfaces. We discuss these results based on modifications of the band structure near the active interfaces and provide further insights concerning the optimization of electron and hole collection.

cond-mat.mtrl-sci↗

arXiv2024

Electron transporting bilayers for perovskite solar cells: spray coating deposition of c-TiO2/m-SnO2-quantum dots

Herein we present a comparative study among different mesoporous electron transporter layers (ETLs), namely nanometric m-TiO2, m-SnO2 and m-SnO2 quantum dots (QDs), deposited by spray coating method. The experimental data correlated with the photovoltaic parameters indicate that the SnO2 mesoporous layer obtained from the spray deposition of the in-house prepared QDs solution is the best candidate between the three used mesoporous ETLs. The use of the in-house prepared SnO2 QDs solution presents smaller agglomerates composed of 3 nm NPs resulting in the formation of a thinner, more uniform, and compact mesoporous ETL, compared with the other two ETL solutions. The formamidinium-methylamonium-potassium (FAMA@10K) perovskite deposited on this m-SnO2 QDs ETL presents a lower RMS, more uniformity and, a higher amount of PbI2. Interestingly, this higher concentration for PbI2 seems to enhance the performance of the perovskite solar cells (PSC), compared to the other two mesoporous ETLs. Our work reveals that SnO2 QDs solution can be easily produced in the laboratory and it is more suited for the deposition of the mesoporous ETL when choosing a FAMA@10K configuration perovskite solar cell with power conversion efficiency (PCE) higher than 10%.

physics.app-ph↗

arXiv2024

Optimal field-free magnetization switching via spin-orbit torque on the surface of a topological insulator

We present an optimal field-free protocol for current-induced switching of a perpendicularly magnetized ferromagnetic insulator nanoelement on the surface of a topological insulator. The time dependence of in-plane components of the surface current, which drives the magnetization reversal via the Dirac spin-orbit torque with minimal Joule heating, is derived analytically as a function of the switching time and material properties. Our analysis identifies that energy-efficient switching is achieved for vanishing damping-like torque. The optimal reversal time that balances switching speed and energy efficiency is determined. When we compare topological insulators to heavy-metal systems, we find similar switching costs for the optimal ratio between the spin-orbit torque coefficients. However, topological insulators offer the advantage of tunable material properties. Finally, we propose a robust and efficient simplified switching protocol using a down-chirped rotating current pulse, tailored to realistic ferromagnetic/topological insulator systems.

cond-mat.mes-hall↗

arXiv2024

Anisotropic transport properties in prismatic topological insulator nanowires

The surface of a three dimensional topological insulator (TI) hosts surface states whose properties are determined by a Dirac-like equation. The electronic system on the surface of TI nanowires with polygonal cross-sectional shape adopts the corresponding polygonal shape. In a constant transverse magnetic field, such an electronic system exhibits rich properties as different facets of the polygon experience different values of the magnetic field due to the changing magnetic field projection between facets. We investigate the energy spectrum and transport properties of nanowires where we consider three different polygonal shapes, all showing distinct properties visible in the energy spectrum and transport properties. Here we propose that the wire conductance can be used to differentiate between cross-sectional shapes of the nanowire by rotating the magnetic field around the wire. Distinguishing between the different shapes also works in the presence of impurities as long as conductance steps are discernible, thus revealing the sub-band structure.

cond-mat.mes-hall↗

arXiv2024

Magneto-optical properties of a quantum dot array interacting with a far-infrared photon mode of a cylindrical cavity

We model the equilibrium properties of a two-dimensional electron gas in a square lateral superlattice of quantum dots in a GaAs heterostructure subject to an external homogeneous perpendicular magnetic field and a far-infrared circular cylindrical photon cavity with one quantized mode, the TE011 mode. In a truncated linear basis constructed by a tensor product of the single-electron states of the noninteracting system and the eigenstates of the photon number operator, a local spin density approximation of density functional theory is used to compute the electron-photon states of the two-dimensional electron gas in the cavity. The common spatial symmetry of the vector fields for the external magnetic field and the cavity photon field in the long wavelength approximation enhances higher order magnetic single- and multi-photon processes for both the para- and the diamagnetic electron-photon interactions. The electron-photon coupling introduces explicit photon replicas into the bandstructure and all subbands gain a photon content, constant for each subband, that can deviate from an integer value as the coupling is increased or the photon energy is varied. The subbands show a complex Rabi anticrossing behavior when the photon energy and the coupling bring subbands into resonances. The complicated energy subband structure leads to photon density variations in reciprocal space when resonances occur in the spectrum. The electron-photon coupling polarizes the charge density and tends to reduce the Coulomb exchange effects as the coupling strength increases.

cond-mat.mes-hall↗

arXiv2023

Flux-periodic oscillations in proximitized core-shell nanowires

Flux-periodic oscillations of the superconducting gap in proximitized core-shell nanowires are explored. Periodicity of oscillations in the energy spectrum of a cylindrical nanowire is compared with nanowires having hexagonal and square cross-section geometry, along with the effects of Zeeman and Rashba spin-orbit interaction. A transition between h/e and h/2e periodicity is found and shown to be dependent on the chemical potential, with correspondence to degeneracy points of the angular momentum quantum number. For a thin shell of a square nanowire, solely h/e periodicity is found in the infinite wire spectrum and shown to result from energy separation between the lowest groups of excited states.

cond-mat.mes-hall↗