SearcharxivSearch

arXiv subjects

Andrew J. Millis

Publications and source records attributed to Andrew J. Millis.

At least 19 recordsLinked to original sources

Non-uniform quantum geometry stabilizes generalized Wigner crystals

Moiré materials host fractional Chern insulators and electron crystals in close proximity, but the mechanism selecting between them remains an open question. We address this competition in Chern bands with ideal but momentum-dependent quantum geometry -- Aharonov-Casher bands. We present an ansatz wave function for generalized Wigner crystals and, by comparing its energy to that of the competing Laughlin-like state, map out the phase diagram at filling fraction $ν=1/m$ as a function of the degree of geometric non-uniformity. Our work identifies quantum geometry-controlled zero point fluctuations of the charge density of the generalized Wigner crystal as the mechanism controlling its relative stability, implying a kind of quantum Lindemann criterion for the crystal-liquid phase boundary.

cond-mat.str-el

Probing Impurity Quantum Criticality with Entanglement Witnesses

Entanglement is a defining feature of quantum mechanics, and its relation to quantum criticality is of considerable current interest. Here we show that measurable spin and charge fluctuations provide an entanglement witness of quantum criticality in the two-impurity Kondo model, which has experimental realizations in terms of coupled quantum dots and magnetic impurities added to surfaces. We use density-matrix renormalization group and numerical renormalization group calculations to resolve the non-Fermi-liquid critical point separating two independently Kondo-screened impurities from an inter-impurity singlet and interpret it as a change in the dominant entanglement partner of each local moment: from entanglement of the local moment with an extended set of conduction-electron degrees of freedom to entanglement with the other impurity. This reorganization is accompanied by a singular response of the impurity-bath entanglement and the inter-impurity susceptibility. We show how the same structure is encoded in the quantum Fisher information of collective spin and charge operators at zero and finite temperatures, connecting the entanglement picture to experimentally accessible dynamical response functions. Our results establish impurity systems as controlled settings in which quantum-critical entanglement can be detected through measurable correlations, and provide further insight into the possibility of understanding heavy-fermion physics in terms of entanglement.

cond-mat.str-el

Beyond mean-field dynamics of the Dicke model with non-Markovian dephasing

We present a density matrix-based time dependent projection operator formalism to calculate the beyond mean-field dynamics of systems with non-Markovian local baths and one-to-all interactions. Such models encapsulate the physics of condensed phase systems immersed in optical cavities. We use this method, combined with tensor network influence functionals, to study the dynamics of the Dicke model coupled to non-Markovian local dephasing baths at zero temperature, which has a superradiant phase transition in the mean-field limit. The method corrects a spurious initial state dependence found in the mean-field dynamics and describes the emergence of new time scales which are absent in the mean-field dynamics. Our formalism, based on density matrices, is applicable to other quantum optical systems with one-to-all interactions at finite temperatures.

quant-ph

Self-consistent GW theory for superconductivity in SrTiO3 models

Superconductivity in doped SrTiO$_3$ occurs over a wide range of carrier densities, including those for which the Fermi energy is below the polar longitudinal optical phonon scale. In this regime, the assumptions underpinning conventional implementations of Migdal-Eliashberg theory, including frequency cutoffs at the phonon scale and a Coulomb pseudopotential $μ^\ast$, are not valid. We solve the finite-temperature $GW$ equations with full momentum and frequency dependence, without cutoffs or $μ^\ast$, for polar one-band models of SrTiO$_3$, using effective masses and three-phonon dielectric functions parameterized from ab initio calculations. Comparing different self-consistency levels, namely $G_0W_0$, $GW_0$, and fully self-consistent $GW$, we find that the one-shot ($G_0W_0$) kernel overestimates the pairing-onset temperature by one to two orders of magnitude. The dominant suppression comes from replacing $G_0$ by $G$, thereby incorporating the phonon renormalization factor in the electron Green function. Using the self-consistently computed interaction $W$ further lowers and narrows the pairing-onset dome. In the dilute limit, our calculations identify the pairing channel as the Fröhlich phonon interaction screened by the incipient ferroelectricity of the material, with plasmonic and electronic screening effects negligible. The numerical solution of the full equations reveals a pairing-onset scale that remains non-zero as the density tends to zero, whereas Fermi-surface projection or Fermi-energy frequency truncation removes it. This work highlights the relevance of incipient ferroelectricity, the importance of self-consistency, and the need for a full momentum- and frequency-dependent treatment in modeling superconductivity in SrTiO$_3$-like doped polar semiconductors.

cond-mat.supr-con

Nonequilibrium orders in parametrically driven field theories

Driving quantum materials with coherent light has proven a powerful platform to realize a plethora of interesting phases and transitions, ranging from ferroelectricity to superconductivity and limit cycles in pumped magnonics. In this paper we develop the field theoretical framework to describe nonequilibrium phases that emerge in systems pumped by rapid parametric drives. We consider paradigmatic O(N) models that describe the long-wavelength fluctuations of ordering fields in many condensed matter set ups. We show that rapid parametric driving of these models can induce an effective pump mechanism in the long wavelength regime through nonlinear scattering. This induces a nonequilibrium transition into a time-crystalline phase.

cond-mat.stat-mech

Spinless charged excitation at the interface between a conventional topological insulator and a topological Mott insulator

We investigate the interface separating two topologically distinct insulating phases of matter using extensive density-matrix renormalization group calculations to study the triangular-lattice Hofstadter-Hubbard model with a spatially varying interaction strength, chosen to realize both integer quantum Hall and chiral spin liquid states in different spatial regions. We find that the integer quantum Hall-chiral spin liquid interface hosts a spinless charged excitation that is bound to the interface. This mode at the interface is identified through charge and spin pumping, and by direct calculations of low-lying excited states. We also characterize bulk excitations in both phases, finding evidence for fractionalization in the chiral spin liquid and for spin-triplet exciton formation in the integer quantum Hall phase.

cond-mat.str-el

Cavity-enhanced superconducting response in an underdoped cuprate

Superconductors carry electrical current without resistance when paired electrons condense into a coherent macroscopic quantum state. In underdoped cuprates, evidence suggests that pairing-related correlations and superconducting fluctuations can survive above the temperature at which global coherence is lost, pointing to phase fluctuations as a key limitation on superconductivity in this regime. Motivated by recent demonstrations of cavity-modified collective states in quantum materials, we investigate whether superconducting coherence can be stabilized by engineering the electromagnetic environment of the superconductor. We study an underdoped YBa$_2$Cu$_3$O$_{7-δ}$ thin film in a tunable terahertz cavity formed with a semi-transparent gold mirror. From temperature-dependent terahertz transmission measurements, we find that the cavity enhances the superconducting response below the critical temperature, with an increase of the inferred superfluid weight. The effect becomes more pronounced at smaller cavity lengths and is accompanied by an upward shift of the superconducting onset temperature. Calculations based on a cavity-coupled model for phase-fluctuating superconductors capture these trends and support an interpretation in terms of cavity-enhanced phase stiffness. These results showcase the potential of cavity engineering for designing emergent functionalities in correlated systems.

cond-mat.supr-con

Electron-phonon coupling in correlated materials: insights from the Hubbard-Holstein model

Dynamical mean-field theory computations of the electron self energy of the Hubbard-Holstein model as a function of electron-phonon and electron-electron interactions are analyzed to gain insight into the dependence of electron-phonon couplings on correlation strength in quantum materials. We find that the electron-phonon interaction is strongly suppressed by electronic correlations, while electron-electron correlation effects at Fermi liquid scales are only weakly modified by coupling to phonons, with phonon-induced modifications most evident at high frequencies on the order of the electronic bandwidth. Implications for beyond-density functional theories of the electron-phonon interaction are discussed.

cond-mat.str-el

Squeezing dynamical singlets in bilayer nickelates

We present realistic calculations within the density functional plus cluster dynamical mean-field formalism indicating that the physics of the the bilayer Ruddlesden-Popper nickelates is to a significant extent controlled by interlayer "dynamical singlets'' which are formed from the $3z^{2}-r^{2}$ orbitals singly occupied by electrons and are hybridized with itinerant planar $x^{2}-y^{2}$ orbitals. The hybridization is found to respond differently to hydrostatic pressure and to epitaxial strain, capturing the experimentally observed dichotomy between bulk single crystals and epitaxial thin films and reproducing several experimental results including angle-resolved photoemission and transport measurements.

cond-mat.str-el

On-demand steering of hyperbolic chiral polaritons

Control of light polarization and propagation in sub-wavelength architectures is foundational to nanophotonic technologies. A frontier direction is to leverage strong optical spin-orbit interactions to realize polarization-selective light steering, known as the photonic spin Hall effect. In this context, hyperbolic plasmon polaritons (HPPs) are of particular interest as they offer large optical spin-orbit coupling from strong confinement and dielectric anisotropy, as well as ray-like propagation. Despite theoretical predictions, however, the hyperbolic spin Hall effect in natural materials has remained elusive. Here, we demonstrate the hyperbolic spin Hall effect in the visible and near-infrared range in the natural hyperbolic van der Waals metal MoOCl2. Enabling this discovery is a novel far-field pump-probe microscope that facilitates the launching and imaging of HPPs with exceptional sensitivity through interference with a high-momentum reference field. This approach preserves excellent control over light polarization, overcoming a key barrier to polarization-selective interrogation of hyperbolic materials. We show that both hyperbolic and surface plasmons in MoOCl2 display chiral fields, and that their propagation direction can be completely switched upon light helicity reversal. Our results demonstrate on-demand steering of chiral plasmons, firmly establishing natural hyperbolic materials as ideal components for reconfigurable nanophotonics and chiral light-matter coupling.

cond-mat.mtrl-sci

Neural-Network Quantum Embedding Solvers for Correlated Materials

Quantum impurity solvers are the computational bottleneck of quantum embedding approaches to correlated materials, such as dynamical mean-field theory (DMFT). We show that neural networks trained on synthetic, material-agnostic data learn the impurity mapping from hybridization functions and local interactions to Green's functions with quantitative accuracy for both model systems and real materials, providing fast solvers for single- and multi-orbital models. Benchmarks against numerically controlled quantum Monte Carlo show that the method reproduces the Mott transition, multi-orbital phase diagrams of Hubbard-Kanamori models, and the electronic properties of SrVO$_3$ and SrMnO$_3$. The learned solvers achieve orders-of-magnitude speedup and can initialize controlled calculations, dramatically accelerating DMFT while preserving accuracy.

cond-mat.str-el

From One to Two Dimensions: Magnetic Phases in Weakly Coupled Spin Ladders

A large variety of materials can be approximately described by means of spin-1/2 Heisenberg ladders. Here, the Density Matrix Renormalization Group (DMRG) algorithm together with a previously established numerical self-consistent mean-field approximation is used to investigate the magnetic properties of spin ladders coupled in a second dimension. The full ground state phase diagram including spin-gapped, antiferromagnetic, ferrimagnetic and fully polarized phases is presented as a function of interladder and intraladder coupling and magnetic field. Measurement of the dependence of magnetization on applied magnetic field is shown to enable location of a material on the phase diagram and determination of the Hamiltonian parameters. These results provide a practical route toward identifying and characterizing magnetic materials composed of coupled spin ladders.

cond-mat.str-el

Dynamical instability in a Floquet-Driven Dissipative System

We analyse the magnon spectrum and distribution function of the antiferromagnetic phase of the Floquet-driven Hubbard model. Above a critical drive strength, we find a dynamical instability, resulting from a change in sign of the magnon damping at a non-zero wavevector. The change in sign means that infinitesimal fluctuations grow with time, corresponding to an instability of the driven state. Implications for the nonequilibrium distribution function and the strong drive nonlinear dynamics are discussed.

cond-mat.str-el

Angle evolution of the superconducting phase diagram in twisted bilayer WSe2

Recent observations of superconductivity in twisted bilayer WSe$_2$ have extended the family of moiré superconductors beyond twisted graphene. In WSe$_2$ two different twist angles were studied, 3.65° and 5.0°, and two seemingly distinct superconducting phase diagrams were reported, raising the question of whether the superconducting phases in the two devices share a similar origin. Here we address the question by experimentally mapping the evolution of the phase diagram across devices with twist angles spanning the range defined by the initial reports, and comparing the results to twist angle-dependent theory. We find that the superconducting state evolves smoothly with twist angle and at all twist angles is proximal to a Fermi surface reconstruction with, presumably, antiferromagnetic ordering, but is neither necessarily tied to the Van Hove singularity, nor to the half band insulator. Our results connect the previously distinct phase diagrams at 3.65° and 5°, and offer new insight into the origin of the superconductivity in this system and its evolution as the correlation strength increases. More broadly, the smooth phase diagram evolution, repeatability between different devices, and dynamic gate tunability within each device, establish twisted transition metal dichalcogenides as a unique platform for the study of correlated phases as the ratio of interaction strength to bandwidth is varied.

cond-mat.mes-hall

Higher Chern bands in helical homotrilayer transition metal dichalcogenides

We propose helically twisted homotrilayer transition metal dichalcogenides as a platform for realizing correlated topological phases of matter with higher and tunable Chern numbers. We show that a clear separation of scales emerges for small twist angles, allowing us to derive a low-energy continuum model that captures the physics within moiré-scale domains. We identify regimes of twist angle and displacement field for which the highest-lying hole band is isolated from other bands and is topological with $K$-valley Chern number $C=-2$. We demonstrate that varying the displacement field can induce a transition from $C=-2$ to $C=-1$, as well as from a topologically trivial band to a $C=-1$ band. We derive an effective tight-binding description for a high-symmetry stacking domain which is valid for a wide range of twist angles, and we show that the $C=-2$ band can remain stable at filling fraction $ν=-1$ in the presence of interactions in Hartree-Fock calculations.

cond-mat.mes-hall

Theory of intervalley-coherent AFM order and topological superconductivity in tWSe$_2$

The recent observation of superconductivity in the vicinity of Fermi surface reconstructed insulating or metallic states has established twisted bilayers of WSe\textsubscript{2} as an exciting platform to study the interplay of strong electron-electron interactions, broken symmetries and topology. In this work, we use a first-principles, material-specific theoretical treatment that is unbiased with respect to electronic instabilities to study the emergence of electronic ordering in twisted WSe\textsubscript{2} driven by gate-screened Coulomb interactions. We construct exponentially localized moiré Wannier orbitals that faithfully capture the bandstructure and topology of the system, project the gate-screened Coulomb interaction onto them and use unbiased functional renormalization group techniques to resolve the momentum and orbital structure of the leading instabilities and the relevant energy scales. We find an interplay between intervalley-coherent antiferromagnetic (IVC-AFM) order and chiral, mixed-parity $d/p$-wave superconductivity for carrier concentrations near a displacement field and twist-angle-tunable van-Hove singularity. Our microscopic approach establishes incommensurate IVC-AFM spin fluctuations as the dominant electronic mechanism driving the formation of superconductivity in $θ= 5.08^{\circ}$ twisted WSe\textsubscript{2} and explains key aspects of recent experiments including the asymmetric density dependence of the spin ordering with respect to the van-Hove line, the single and double-peak structure of the DOS in the ordered (hole-doped) IVC-AFM phase, the emergence of superconductivity as the density is varied across the van-Hove line and the evolution of the displacement field-density phase diagram with twist angles between $3.7^{\circ} \dots 5^{\circ}$.

cond-mat.str-el

Cavity-altered superconductivity

Is it feasible to alter the ground state properties of a material by engineering its electromagnetic environment? Inspired by theoretical predictions, experimental realizations of such cavity-controlled properties without optical excitation are beginning to emerge. Here, we devised and implemented a novel platform to realize cavity-altered materials. Single crystals of hyperbolic van der Waals (vdW) compounds provide a resonant electromagnetic environment with enhanced density of photonic states and prominent mode confinement. We interfaced hexagonal boron nitride (hBN) with the molecular superconductor $κ$-(BEDT-TTF)$_2$Cu[N(CN)$_2$]Br ($κ$-ET). The frequencies of infrared (IR) hyperbolic modes of hBN match the IR-active carbon-carbon stretching molecular resonance of ($κ$-ET) implicated in superconductivity. Nano-optical data supported by first-principles molecular Langevin dynamics simulations confirm the presence of resonant coupling between the hBN hyperbolic cavity modes and the carbon-carbon stretching mode in ($κ$-ET). Meissner effect measurements via magnetic force microscopy demonstrate a strong suppression of superfluid density near the hBN/($κ$-ET) interface. Non-resonant control heterostructures, including RuCl$_3$/($κ$-ET) and hBN/$\text{Bi}_2\text{Sr}_2\text{CaCu}_2\text{O}_{8+x}$, do not display the superfluid suppression. These observations suggest that hBN/($κ$-ET) realizes a cavity-altered superconducting ground state. Our work highlights the potential of dark cavities devoid of external photons for engineering electronic ground state properties of complex quantum materials.

cond-mat.supr-con

Twist-angle evolution of the intervalley-coherent antiferromagnet in twisted WSe$_2$

Recent experimental reports of correlated physics in twisted homobilayer WSe$_2$ have spurred interest in the interplay of electronic interactions and topology in this system. Here, we explore its phase diagram using the Hartree-Fock approximation within a three-orbital Wannier model of the bilayer. Our analysis reveals a dominant intervalley-coherent antiferromagnetic instability, whose stability in the space of twist angle, interaction strength, out-of-plane displacement field, and hole density is primarily set by nesting and commensurability. At large angles or low interaction-to-bandwidth ratios, the instability arises at hole densities above half filling near a van-Hove line where the strong Fermi surface nesting occurs due to the flatness of the band in a region enclosing the van-Hove and $κ$ points. Increasing interaction strength or decreasing the twist angle gradually shifts the ordered phase toward half filling, where the strongest antiferromagnetic order gets pinned due to commensurability effects that enable a full gap opening. The antiferromagnetic order parameter strongly couples to the layer polarization, which makes its transition to the normal state sharp in the strong-coupling limit and carries implications for collective modes. Our Hartree-Fock phase diagram reproduces key aspects of recent experiments and the reconstructed Fermi surfaces and DOS in the antiferromagnetic phase account for subtle transport signatures observed in these studies.

cond-mat.str-el