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Andrey Varykhalov

Publications and source records attributed to Andrey Varykhalov.

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Emergence of high-mobility carriers in topological kagome bad metal Mn$_3$Sn by intense photoexcitation

Kagome-lattice materials offer novel playgrounds of exploring topologically nontrivial states of electrons under influence of many-body interactions. A noncollinear kagome antiferromagnet Mn$_3$Sn has attracted particular interest for application in spintronics owing to the large anomalous Hall effect related to the Weyl dispersion near the Fermi energy. In addition, strong electronic correlation suggesting the Kondo physics has also been implied. However, the effect of correlation on the band topology and their interplay remains elusive. Here, we investigate nonequilibrium Hall transport in a photoexcited Mn$_3$Sn using time-resolved terahertz Faraday rotation spectroscopy. In equilibrium, Mn$_3$Sn is a bad metal close to the Mott-Ioffe-Regal limit with low carrier mobility, and thus only the anomalous Hall effect is discerned. By contrast, intense photoexcitation beyond an approximate threshold gives rise to a clear cyclotron resonance, namely the normal Hall effect, indicating the emergence of unusual carriers with 50 times lighter effective mass and 40 times less scattering. The lifetime of high-mobility carriers as long as a few tens of picoseconds and a threshold-like behavior for the pump fluence are hardly explained by contribution of photoexcited hot carriers. Instead, the emergence of unusual carriers may be accounted for by dielectric screening of the on-site Coulomb interaction by high-density delocalized photocarriers. A possible role of electronic correlation in equilibrium transport in Mn$_3$Sn beyond the single-particle picture is discussed.

cond-mat.str-el

Fermi surface tomography

Fermi surfaces, three-dimensional (3D) abstract interfaces that define the occupied energies of electrons in a solid, are important for characterizing and predicting the thermal, electrical, magnetic, and optical properties of crystalline metals and semiconductors [1]. Angle-resolved photoemission spectroscopy (ARPES) is the only technique directly probing the Fermi surface by measuring the Fermi momenta (kF) from energy and angular distribution of photoelectrons dislodged by monochromatic light [2]. Existing electron analyzers are able to determine a number of kF-vectors simultaneously, but current technical limitations prohibit a direct high-resolution 3D Fermi surface mapping. As a result, no such datasets exist, strongly limiting our knowledge about the Fermi surfaces and restricting a detailed comparison with the widely available nowadays calculated 3D Fermi surfaces. Here we show that using a simpler instrumentation, based on the Fourier electron optics combined with a retardation field of the detector, it is possible to perform 3D-mapping within a very short time interval and with very high resolution. We present the first detailed experimental 3D Fermi surface recorded in the full Brillouin zone along the kz-direction as well as other experimental results featuring multiple advantages of our technique. In combination with various light sources, including synchrotron radiation, our methodology and instrumentation offer new opportunities for high-resolution ARPES in the physical and life sciences.

cond-mat.mtrl-sci