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Andrius Baltuska

Publications and source records attributed to Andrius Baltuska.

10 recordsLinked to original sources
arXiv2024

One-dimensional mapping of femtosecond laser filaments using coherent microwave scattering

This paper reports on the use of coherent microwave scattering (CMS) for spatially resolved electron number density measurements of elongated plasma structures induced at mid-IR femtosecond filamentation in air. The presented studies comprise one-dimensional mapping of laser filaments induced via 3.9 um, 127.3 fs laser pulses at output energies up to 15 mJ. The axial electron number density was measured to be invariant (about 2x10$^{15}$ cm$^{-3}$) along the entire filament length and for all tested laser pulse energies 5-15 mJ, and the corresponding laser intensity in the middle portion of the filament was estimated to be nearly constant for 5-15 mJ pulse energies (about 30-40 TW/cm$^2$). These fundings support that intensity clamping conditions were achieved in the experiments. The proposed approach enables capabilities that are currently unavailable to perform absolute and longitudinally resolved measurements of electron number density in laser filaments and to precisely characterize conditions associated with self-focusing and intensity clamping.

physics.plasm-ph↗
arXiv2023

Analysis of High-Contrast All-Optical Dual Wavelength Switching in Asymmetric Dual-Core Fibers

We systematically present experimental and theoretical results for the dual-wavelength switching of 1560 nm, 75 fs signal pulses (SPs) driven by 1030 nm, 270 fs control pulses (CPs) in a dual-core fiber (DCF). We demonstrate a switching contrast of 31.9 dB, corresponding to a propagation distance of 14 mm, achieved by launching temporally synchronized SP-CP pairs into the fast core of the DCF with moderate inter-core asymmetry. Our analysis employs a system of three coupled propagation equations to identify the compensation of the asymmetry by nonlinearity as the physical mechanism behind the efficient switching performance.

physics.optics↗
arXiv2022

Rapid-scan nonlinear time-resolved spectroscopy over arbitrary delay intervals

Femtosecond dual-comb lasers have revolutionized linear Fourier-domain spectroscopy by offering a rapid motion-free, precise and accurate measurement mode with easy registration of the combs beat note in the RF domain. Extensions of this technique found already application for nonlinear time-resolved spectroscopy within the energy limit available from sources operating at the full oscillator repetition rate. Here, we present a technique based on time filtering of femtosecond frequency combs by pulse gating in a laser amplifier. This gives the required boost to the pulse energy and provides the flexibility to engineer pairs of arbitrarily delayed wavelength-tunable pulses for pump-probe techniques. Using a dual-channel millijoule amplifier, we demonstrate programmable generation of both extremely short, fs, and extremely long (>ns) interpulse delays. A predetermined arbitrarily chosen interpulse delay can be directly realized in each successive amplifier shot, eliminating the massive waiting time required to alter the delay setting by means of an optomechanical line or an asynchronous scan of two free-running oscillators. We confirm the versatility of this delay generation method by measuring chi^(2) cross-correlation and chi^(3) multicomponent population recovery kinetics.

physics.optics↗
arXiv2022

Ionization rate and plasma dynamics at 3.9 micron femtosecond photoionization of air

The introduction of mid-IR optical parametric chirped pulse amplifiers (OPCPAs) has catalyzed interest in multi-millijoule, infrared femtosecond pulse-based filamentation. As tunneling ionization is a fundamental first stage in these high-intensity laser-matter interactions, characterizing the process is critical to understand derivative topical studies on femtosecond filamentation and self-focusing. Here, we report constructive-elastic microwave scattering-based measurements of total electron count, electron number densities, and photoionization rates generated by 3.9 micron femtosecond mid-infrared tunneling ionization of atmospheric air. Consequently, we determine photoionization rates in the range of 5.0x10$^{8}$-6.1x10$^{9}$ s$^{-1}$ for radiation intensities 1.3x10$^{13}$-1.9x10$^{14}$ W/cm$^{2}$, respectively. The proposed approach paves the wave to precisely tabulate photoionization rates in mid-IR for broad range of intensities and gas types and to study plasma dynamics at mid-IR filamentation.

physics.plasm-ph↗
arXiv2022

A stochastic nonlinear model of the dynamics of actively Q-switched lasers

In this paper, we present a novel stochastic and spatially lumped multi-mode model to describe the nonlinear dynamics of actively Q-switched lasers and random perturbations due to amplified spontaneous emission. This model will serve as a basis for the design of (nonlinear) control and estimation strategies and thus a high value is set on its computational efficiency. Therefore, a common traveling-wave model is chosen as a starting point and a number of model-order reduction steps are performed. As a result, a set of nonlinear ordinary differential equations for the dynamic behavior of the laser during a switching cycle is obtained. A semi-analytic solution of these differential equations yields expressions for the population inversion after a switching cycle and for the output energy, which are then used to formulate a nonlinear discrete-time model for the pulse-to-pulse dynamics. Simulation studies including models with different levels of complexity and first experimental results demonstrate the feasibility of the proposed approach.

physics.optics↗
arXiv2020

Solitary beam propagation in a nonlinear optical resonator enables high-efficiency pulse compression and mode self-cleaning

Generating intense ultrashort pulses with high-quality spatial modes is crucial for ultrafast and strong-field science. This can be accomplished by controlling propagation of femtosecond pulses under the influence of Kerr nonlinearity and achieving stable propagation with high intensity. In this work, we propose that the generation of spatial solitons in periodic layered Kerr media can provide an optimum condition for supercontinuum generation and pulse compression using multiple thin plates. With both the experimental and theoretical investigations, we successfully identify these solitary modes and reveal a universal relationship between the beam size and the critical nonlinear phase. Space-time coupling is shown to strongly influence the spectral, spatial and temporal profiles of femtosecond pulses. Taking advantage of the unique characters of these solitary modes, we demonstrate single-stage supercontinuum generation and compression of femtosecond pulses from initially 170 fs down to 22 fs with an efficiency ~90%. We also provide evidence of efficient mode self-cleaning which suggests rich spatial-temporal self-organization processes of laser beams in a nonlinear resonator.

physics.optics↗
arXiv2019

Zero-energy proton dissociation of H$_2^+$ through stimulated Raman scattering

We show that (near-)zero energy proton emission from H$_2^+$ in strong two-color and broadband laser fields is dominated by a stimulated Raman scattering process taking place on the electronic ground state. It is furthermore shown that in the (near-)zero energy region the asymmetry in proton ejection induced by asymmetric laser fields is due to the interplay of several processes, rather than only pathway interferences, with vibrational trapping (or bond-hardening) taking a key role.

physics.chem-ph↗
arXiv2018

Bismuth Ferrite Dielectric Nanoparticles Excited at Telecom Wavelengths as Multicolor Sources by Second, Third, and Fourth Harmonic Generation

We demonstrate the simultaneous generation of second, third, and fourth harmonic from a single dielectric Bismuth Ferrite nanoparticle excited by a telecom fiber laser at 1560 nm. We first characterize the signals associated with different nonlinear orders in terms of spectrum, excitation intensity dependence, and relative signal strengths. Successively, on the basis of the polarization-resolved emission curves of the three harmonics, we discuss the interplay of susceptibility tensor components at the different orders and we show how polarization can be used as an optical handle to control the relative frequency conversion properties.

physics.optics↗
arXiv2018

Filamentation of Mid-IR pulses in ambient air in the vicinity of molecular resonances

Properties of filaments ignited by multi-millijoule, 90-fs mid-IR pulses centered at 3.9 μm are examined experimentally by monitoring plasma density and losses as well as spectral dynamics and beam profile evolution at different focusing strengths. By softening the focusing from strong (f=0.25 m) to loose (f=7 m) we observe a shift from plasma assisted filamentation to filaments with low plasma density. In the latter case, filamentation manifests itself by beam self-symmetrization and spatial self-channeling. Spectral dynamics in the case of loose focusing is dominated by the non-linear Raman frequency downshift, which leads to the overlap with the CO2 resonance in the vicinity of 4.2 μm. The dynamic CO2 absorption in the case of 3.9-μm filaments with their low plasma content is the main mechanism of energy losses and either alone or together with other nonlinear processes contributes to the arrest of intensity.

physics.optics↗