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Andriy H. Nevidomskyy

Publications and source records attributed to Andriy H. Nevidomskyy.

At least 19 recordsLinked to original sources

Spontaneously Broken Non-Invertible Symmetries in Transverse-Field Ising Qudit Chains

Recent developments have revealed that symmetries need not form a group, but instead can be non-invertible. Here we use analytical arguments and numerical evidence to illuminate how spontaneous symmetry breaking of a non-invertible symmetry is similar yet distinct from ordinary, invertible, symmetry breaking. We consider one-dimensional chains of group-valued qudits, whose local Hilbert space is spanned by elements of a finite group $G$ (reducing to ordinary qubits when $G=\mathbb{Z}_2$). We construct Ising-type transverse-field Hamiltonians with Rep($G$) symmetry whose generators multiply according to the tensor product of irreducible representations (irreps) of the group $G$. For non-Abelian $G$, the symmetry is non-invertible. In the symmetry broken phase there is one ground state per irrep on a closed chain. The symmetry breaking can be detected by local order parameters but, unlike the invertible case, different ground states have distinct entanglement patterns. We show that for each irrep of dimension greater than one the corresponding ground state exhibits string order, entanglement spectrum degeneracies, and has gapless edge modes on an open chain -- features usually associated with symmetry-protected topological order. Consequently, domain wall excitations behave as one-dimensional non-Abelian anyons with non-trivial internal Hilbert spaces and fusion rules. Our work identifies properties of non-invertible symmetry breaking that existing quantum hardware can probe.

cond-mat.str-el

Generalized Wigner theorem for non-invertible symmetries

We establish the conditions under which a conservation law associated with a non-invertible operator may be realized as a symmetry in quantum physics. As established by Wigner, all quantum symmetries must be represented by either unitary or antiunitary transformations. Relinquishing an implicit assumption of invertibility, we demonstrate that the fundamental invariance of quantum transition probabilities under the application of symmetries mandates that all non-invertible symmetries may only correspond to {\it projective} unitary or antiunitary transformations, i.e., {\it partial isometries}. This extends the notion of physical states beyond conventional rays in Hilbert space to equivalence classes in an {\it extended, gauged Hilbert space}, thereby broadening the traditional understanding of symmetry transformations in quantum theory. Our generalized theorem applies irrespective of the origin of the (non)invertible symmetry, holds in arbitrary spatial dimensions, and is independent of the Hamiltonian or action. We explore its physical consequences and, using simple model systems, illustrate how the distinction between invertible and non-invertible symmetries can sometimes be tied to the choice of boundary conditions.

quant-ph

Algebraic Fusion in a (2+1)-dimensional Lattice Model with Generalized Symmetries

The notion of quantum symmetry has recently been extended to include reduced-dimensional transformations and algebraic structures beyond groups. Such generalized symmetries lead to exotic phases of matter and excitations that defy Landau's original paradigm. Here, we develop an algebraic framework for systematically deriving the fusion rules of topological defects in higher-dimensional lattice systems with non-invertible generalized symmetries, and focus on a (2+1)-dimensional quantum Ising plaquette model as a concrete illustration. We show that bond-algebraic automorphisms, when combined with the so-called half-gauging procedure, reveal the structure of the non-invertible duality symmetry operators, which can be explicitly represented as a sequential quantum circuit. The resulting duality defects are constrained by the model's rigid higher symmetries (lower-dimensional subsystem symmetries), leading to restricted mobility. We establish the fusion algebra of these defects. Finally, in constructing the non-invertible duality transformation, we explicitly verify that it acts as a partial isometry on the physical Hilbert space, thereby satisfying a recent generalization of Wigner's theorem applicable to non-invertible symmetries.

quant-ph

Web of Non-invertible Dualities for (2+1) Dimensional Models with Subsystem Symmetries

We extend non-invertible duality concepts from one-dimensional systems to two spatial dimensions by constructing a web of non-invertible dualities for lattice models with subsystem symmetries. For the $\mathbb{Z}_2 \times \mathbb{Z}_2$ subsystem symmetry on the square lattice, we build two complementary dualities: a map that sends spontaneous subsystem symmetry-broken (SSSB) phases to the trivial phase (the analogue of the Kramers-Wannier (KW) duality in 1+1D), and a generalized subsystem Kennedy-Tasaki (KT) transformation that maps SSSB phases to subsystem symmetry-protected topological (SSPT) phases while leaving the trivial phase invariant. These dualities are boundary-sensitive. On open lattices, both subsystem KW and KT transformations act as unitary, invertible operators. In particular, the KT map not only matches the bulk Hamiltonians of the dual phases but also carries the spontaneous ground-state degeneracy of the SSSB phase onto the protected boundary degeneracy of the SSPT phase. On closed manifolds, however, both maps become intrinsically non-unitary and non-invertible when restricted to the original Hilbert space. We demonstrate this non-invertibility via ground-state degeneracy matching (in two copies of the Xu-Moore/Ising-plaquette model), analysis of symmetry-twist sectors mapping, and the fusion algebra of the duality operator. Enlarging the Hilbert space to include twisted sectors allows the subsystem KW map to be formulated as a projective unitary preserving quantum transition probabilities, consistent with generalized Wigner-theorem-based constructions. We also show that the KT map faithfully transmits the algebraic content of bulk and edge invariants diagnosing strong SSPT order: although strictly local SSPT repair operators map to highly nonlocal objects in the dual SSSB phase, the essential commutation algebra and the bulk-edge correspondence remain intact.

cond-mat.str-el

Stabilizing Fractional Chern States in Twisted MoTe2: Multi-band Correlations via Non-perturbative Renormalization Group

The observation of fraction quantum Hall states in twisted MoTe2 has sparked a lof of interest in this phenomenon. Most theoretical works to date rely on the brute-force exact diagonalization which is limited to the one partially occupied band. In this work, we present strong evidence that the effect of higher lying bands cannot be ignored due to strong interband interactions. To tackle these effects, we introduce a non-perturbative driven similarity renormalization group (DSRG) method, originally developed for problems in quantum chemistry. We apply this methodology to twisted MoTe2 at fractional hole fillings of ν = 1/3 and 2/3 across a spectrum of twist angles. Our results show that at ν = 1/3, the many-body excitation energy gaps are substantially reduced compared to the one-band treatment. For ν = 2/3, we find that the dynamic correlations stemming from interband interactions stabilize fractional Chern insulating phases at larger twist angles, consistent with the experimental findings. By examining the correlated orbitals and their single-particle topological features, we demonstrate that this stabilization at higher twist angles arises predominantly from the dynamic correlations, rather than conditions on the single-particle quantum geometric tensor.

cond-mat.str-el

Particle-hole asymmetric phases in doped twisted bilayer graphene

Despite much theoretical work, developing a comprehensive ab initio model for twisted bilayer graphene (TBG) has proven challenging due to the inherent trade-off between accurately describing the band structure and incorporating the interactions within the Hamiltonian, particularly given the topological obstruction -- so-called fragile topology -- to the description of the model in terms of localized symmetric Wannier functions within the flat band manifold. Here, we circumvent this obstruction by using an extended 8-orbital model, for which localized Wannier orbitals have been formulated by Carr et al. [1]. We constructed an extended multi-orbital Hubbard model, and performed Hartree-Fock (HF) calculations to explore its phase diagram across commensurate fillings from -3 to 3. We found several nearly-degenerate insulating states at charge neutrality, all of which exhibit orbital orders. Crucially, TBG near magic angle is known to be particle-hole asymmetric, which is naturally captured by the single-particle band structure of our model and is reflected in the distinction between the symmetry broken states obtained at electron and hole dopings away from the charge neutral point. At filling -1 and +2, quantum anomalous hall states are obtained, while for the rest of the integer fillings away from charge neutrality, we found the system to realize metallic states with various orbital, valley and spin orderings. We also observed that most of the Hartree--Fock ground states exhibit a generalized valley Hund's-like rule, resulting in valley polarization. Importantly, we show that the incorporation of the intra-valley and inter-valley exchange interactions is crucial to properly stabilize the ordered symmetry-broken states. In agreement with experiments, we find significant particle-hole asymmetry, which underscores the importance of using particle-hole asymmetric models.

cond-mat.str-el

Dipolar-octupolar correlations and hierarchy of exchange interactions in Ce$_2$Hf$_2$O$_7$

High-resolution neutron spectroscopy on Ce$_2$Hf$_2$O$_7$ reveals a correlated state characterized by distinct dipolar scattering signals -- quasi-elastic and inelastic contributions consistent with `photon' and `spinon' excitations in quantum spin ice. These signals coexist with weak octupolar scattering. Fits of thermodynamic data using numerical methods indicate a dominant octupolar exchange, $J_{x}$ or $J_{y}$, with substantial dipolar $J_{z}$ and minute dipole-octupole $J_{xz}$ couplings. The $J_{xz}$ value is corroborated by an independent fit of the neutron scattering amplitude balance between dipolar and octupolar `photon' contributions, highlighting its importance to understand neutron scattering results in this family. Ce$_2$Hf$_2$O$_7$ enriches the landscape of dipole-octupole pyrochlore physics, and reveals a `quantum multipolar liquid' where hybrid correlations involve multiple terms in moment series expansion, opening questions on their intertwining and hierarchy in quantum phases.

cond-mat.str-el

Simulating Spin Dynamics of Supersolid States in a Quantum Ising Magnet

Motivated by a recent experimental study on the quantum Ising magnet $\text{K}_2\text{Co}(\text{SeO}_3)_2$ that presented spectroscopic evidence of zero-field supersolidity (Chen et al., arXiv:2402.15869), we simulate the excitation spectrum of the corresponding microscopic $XXZ$ model for the compound, using the recently developed excitation ansatz for infinite projected entangled-pair states. We map out the ground state phase diagram and compute the dynamical spin structure factors across a range of magnetic field strengths, focusing especially on the two supersolid phases found near zero and saturation fields. Our simulated excitation spectra for the zero-field supersolid "Y" phase are in excellent agreement with the experimental data - recovering the low-energy branches and integer quantized excited energy levels $ω_n=nJ_{zz}$. Furthermore, we demonstrate the nonlocal multi-spin-flip features for modes at $ω_2$, indicative of their multi-magnon nature. Additionally, we identify characteristics of the high-field supersolid "$Ψ$" phase in the simulated spectra, which should be compared with future experimental results.

cond-mat.str-el

High-Field Superconducting Halo in UTe$_2$

Heavy fermion UTe$_2$ is a promising candidate for topological superconductivity that also exhibits multiple high-field superconducting phases. The SC$_{\rm{FP}}$ phase has only been observed in off-axis magnetic fields in the $bc$ plane at fields greater than 40 teslas, a striking scale given its critical temperature of only 2 kelvins. Here, we extend measurements of this unique superconducting state outside of the $bc$ plane and reveal its core structure. The SC$_{\rm{FP}}$ phase is not confined to fields in the $bc$ plane and in fact wraps around the $b$ axis in a halo-like fashion. In other words, this superconducting state, which exists in fields above 73 teslas, is stabilized by a field component perpendicular to the magnetic easy axis. These remarkable field scales further underscore UTe$_2$'s unique magnetophilic superconducting tendencies and suggest an underlying pairing mechanism that is qualitatively distinct from known theories for field-enhanced superconductivity. Phenomenological modeling points to a two-component, non-unitary spin triplet order parameter with finite orbital momentum of the Cooper pairs as a natural explanation for the field-angle dependence of the upper critical field of the SC$_{\rm{FP}}$ phase.

cond-mat.supr-con

Thermodynamics of the dipole-octupole pyrochlore magnet Ce$_2$Hf$_2$O$_{7}$ in applied magnetic fields

The recently discovered dipole-octupole pyrochlore magnet Ce$_2$Hf$_2$O$_7$ is a promising three-dimensional quantum spin liquid candidate which shows no signs of ordering at low temperature. The low energy effective pseudospin-1/2 description in a magnetic field is characterized by the XYZ Hamiltonian and a Zeeman term where the dipolar local $z$-component of the pseudospin couples to the local $z$-component of the applied magnetic field, while the local $x$- and $y$-components of the pseudospin remain decoupled as a consequence of their octupolar character. Using effective Hamiltonian parameters determined in V. Poree et al., arXiv:2305.08261 (2023), remarkable experimental features can be reproduced, as for instance the specific heat and magnetization data as well as the continuum of states seen in neutron scattering. Here we investigate the thermodynamic response to magnetic fields applied along the global [110] direction using specific heat measurements and fits using numerical methods, and solve the corresponding magnetic structure using neutron diffraction. Specific heat data in moderate fields are reproduced well, however, at high fields the agreement is not satisfactory. We especially observe a two-step release of entropy, a finding that demands a review of both theory and experiment. We address it within the framework of three possible scenarios, including an analysis of the crystal field Hamiltonian not restricted to the two-dimensional single-ion doublet subspace. We conclusively rule out two of these scenarios and find qualitative agreement with a simple model of field misalignment with respect to the crystalline direction. We discuss the implications of our findings for [111] applied fields and for future experiments on Ce$_2$Hf$_2$O$_7$ and its sister compounds.

cond-mat.str-el

Fractional matter coupled to the emergent gauge field in a quantum spin ice

Electronic spins can form long-range entangled phases of condensed matter named quantum spin liquids. Their existence is conceptualized in models of two- or three-dimensional frustrated magnets that evade symmetry-breaking order down to zero temperature. Quantum spin ice (QSI) is a theoretically well-established example described by an emergent quantum electrodynamics, with excitations behaving like photon and matter quasiparticles. The latter are fractionally charged and equivalent to the `spinons' emerging from coherent phases of singlets in one dimension, where clear experimental proofs of fractionalization exist. However, in frustrated magnets it remains difficult to establish consensual evidence for quantum spin liquid ground states and their fractional excitations. Here, we use backscattering neutron spectroscopy to achieve extremely high resolution of the time-dependent magnetic response of the candidate QSI material Ce$_2$Sn$_2$O$_7$. We find a gapped spectrum featuring a threshold and peaks that match theories for pair production and propagation of fractional matter excitations (spinons) strongly coupled to a background gauge field. The multiple peaks are a specific signature of the $π$-flux phase of QSI, providing spectroscopic evidence for fractionalization in a three-dimensional quantum spin liquid.

cond-mat.str-el

Strange-metal behavior without fine-tuning in PrV2Al20

Strange-metal behavior observed in the praseodymium-based heavy-fermion material PrV2Al20 has been tentatively interpreted in the framework of proximity to a quantum critical point (QCP) associated with quadrupolar ordering. Here, we demonstrate that an alternative, natural explanation exists without invoking a QCP, in terms of the unconventional nature of the quadrupolar Kondo effect taking place in non-Kramers ions. Using a combination of ab initio density-functional theory calculations and analytical arguments, we construct a periodic Anderson model with realistic parameters to describe PrV2Al20. We solve the model using dynamical mean-field theory preserving the model symmetries and demonstrate the non-Fermi liquid strange-metal behavior stemming from the two-channel nature of the quadrupolar Kondo effect. Our calculations provide an explanation for the puzzling temperature dependence in the magnetic susceptibility, and provide a basis for analyzing future photoemission experiments.

cond-mat.str-el

Experimentally tunable QED in dipolar-octupolar quantum spin ice

We propose a readily achievable experimental setting where an external magnetic field is used to tune the emergent quantum electrodynamics (eQED) of dipolar-octupolar quantum spin ice (DO-QSI). In $U(1)_π$ DO-QSI -- the proposed ground state of QSI candidates Ce$_2$Zr$_2$O$_7$, Ce$_2$Sn$_2$O$_7$ and Ce$_2$Hf$_2$O$_7$ -- we show that the field can be used to control the emergent speed of light (and, consequently, the emergent fine structure constant). Depending on the field's alignment with the crystal, one may induce different speeds for the two polarizations of the emergent photons, in a fascinating analogue of the electro-optic Kerr effect. In $U(1)_0$ DO-QSI -- yet to be uncovered experimentally -- we find a number of unusual field-induced transitions, including a transition between $0$- and $π$-flux QSI phases, as well as phases with frustrated flux configurations. We discuss experimental signatures of these effects in the spinon excitation spectrum, which can be readily accessed for instance in inelastic neutron scattering measurements. Our proposal opens the gate to a plethora of experimentally accessible, engineerable eQED phenomena in the emergent universes of quantum spin ice.

cond-mat.str-el

Realizing fracton order from long-range quantum entanglement in programmable Rydberg atom arrays

Storing quantum information, unlike information in a classical computer, requires battling quantum decoherence, which results in a loss of information over time. To achieve error-resistant quantum memory, one would like to store the information in a quantum superposition of degenerate states engineered in such a way that local sources of noise cannot change one state into another, thus preventing quantum decoherence. One promising concept is that of fracton order -- a phase of matter with a large ground state degeneracy that grows subextensively with the system size. Unfortunately, the models realizing fractons are not friendly to experimental implementations as they require unnatural interactions between a substantial number (of the order of ten) of qubits. We demonstrate how this limitation can be circumvented by leveraging the long-range quantum entanglement created using only pairwise interactions between the code and ancilla qubits, realizable in programmable tweezer arrays of Rydberg atoms. We show that this platform also allows to detect and correct certain types of errors en route to the goal of true error-resistant quantum memory.

quant-ph

Field induced non-BEC transitions in frustrated magnets

Frustrated spin-systems have traditionally proven challenging to understand, owing to a scarcity of controlled methods for their analyses. By contrast, under strong magnetic fields, certain aspects of spin systems admit simpler and universal description in terms of hardcore bosons. The bosonic formalism is anchored by the phenomenon of Bose-Einstein condensation (BEC), which has helped explain the behaviors of a wide range of magnetic compounds under applied magnetic fields. Here, we focus on the interplay between frustration and externally applied magnetic field to identify instances where the BEC paradigm is no longer applicable. As a representative example, we consider the antiferromagnetic $J_1 - J_2 - J_3$ model on the square lattice in the presence of a uniform external magnetic field, and demonstrate that the frustration-driven suppression of the Néel order leads to a Lifshitz transition for the hardcore bosons. In the vicinity of the Lifshitz point, the physics becomes unmoored from the BEC paradigm, and the behavior of the system, both at and below the saturation field, is controlled by a Lifshitz multicritical point. We obtain the resultant universal scaling behaviors, and provide strong evidence for the existence of a frustration and magnetic-field driven correlated bosonic liquid state along the entire phase boundary separating the Néel phase from other magnetically ordered states.

cond-mat.str-el

Quantum Simulation of an Extended Dicke Model with a Magnetic Solid

The Dicke model describes the cooperative interaction of an ensemble of two-level atoms with a single-mode photonic field and exhibits a quantum phase transition as a function of light--matter coupling strength. Extending this model by incorporating short-range atom--atom interactions makes the problem intractable but is expected to produce new phases. Here, we simulate such an extended Dicke model using a crystal of ErFeO$_3$, where the role of atoms (photons) is played by Er$^{3+}$ spins (Fe$^{3+}$ magnons). Through magnetocaloric effect and terahertz magnetospectroscopy measurements, we demonstrated the existence of a novel atomically ordered phase in addition to the superradiant and normal phases that are expected from the standard Dicke model. Further, we elucidated the nature of the phase boundaries in the temperature--magnetic-field phase diagram, identifying both first-order and second-order phase transitions. These results lay the foundation for studying multiatomic quantum optics models using well-characterized many-body condensed matter systems.

quant-ph

Two-Step Electronic Response to Magnetic Ordering in a van der Waals Ferromagnet

The two-dimensional (2D) material Cr$_2$Ge$_2$Te$_6$ is a member of the class of insulating van der Waals magnets. Here, using high resolution angle-resolved photoemission spectroscopy in a detailed temperature dependence study, we identify a clear response of the electronic structure to a dimensional crossover in the form of two distinct temperature scales marking onsets of modifications in the electronic structure. Specifically, we observe Te $p$-orbital-dominated bands to undergo changes at the Curie transition temperature T$_C$ while the Cr $d$-orbital-dominated bands begin evolving at a higher temperature scale. Combined with neutron scattering, density functional theory calculations, and Monte Carlo simulations, we find that the electronic system can be consistently understood to respond sequentially to the distinct temperatures at which in-plane and out-of-plane spin correlations exceed a characteristic length scale. Our findings reveal the sensitivity of the orbital-selective electronic structure for probing the dynamical evolution of local moment correlations in vdW insulating magnets.

cond-mat.str-el

Classification of Classical Spin Liquids: Topological Quantum Chemistry and Crystalline Symmetry

Frustrated magnetic systems can host highly interesting phases known as classical spin liquids (CSLs), which feature {extensive} ground state degeneracy and lack long-range magnetic order. Recently, Yan and Benton et al. proposed a classification scheme of CSLs in the large-$\mathcal{N}$ (soft spin) limit [arXiv.2305.00155], [arXiv:2305.19189]. This scheme classifies CSLs into two categories: the algebraic CSLs and the fragile topological CSLs, each with their own correlation properties, low energy effective description, and finer classification frameworks. In this work, we further develop the classification scheme by considering the role of crystalline symmetry. We present a mathematical framework for computing the band representation of the flat bands in the spectrum of these CSLs, which extends beyond the conventional representation analysis. It allows one to determine whether the algebraic CSLs, which features gapless points on their bottom flat bands, are protected by symmetry or not. It also provides more information on the finer classifications of algebraic and fragile topological CSLs. We demonstrate this framework via concrete examples and showcase its power by constructing a pinch-line algebraic CSL protected by symmetry.

cond-mat.str-el