arXiv subjects

Andrzej Wiśniewski

Publications and source records attributed to Andrzej Wiśniewski.

7 recordsLinked to original sources

arXiv2026

Far-field terahertz spectroscopy across the charge-density-wave transition in 2H-NbSe$_2$

Charge-density-wave (CDW) formation in 2H-NbSe$_2$ modifies the low-energy electronic structure and gives rise to collective excitations coupled to the lattice. Here, we investigate bulk 2H-NbSe$_2$ single crystals using far-field terahertz time-domain spectroscopy (THz-TDS) in reflection geometry across the CDW transition at $T_{\mathrm{CDW}} \approx 33$~K. Below $T_{\mathrm{CDW}}$, the THz response shows a pronounced high-frequency feature near 1.5~THz together with longer-lived sub-THz oscillations. Both responses progressively weaken upon warming and are strongly suppressed across the CDW transition, supporting their association with the CDW state. Using time-dependent Ginzburg--Landau simulations, we reproduce the main features of the experimental THz response, associating the high-frequency response mainly with CDW amplitude dynamics and the sub-THz response with defect-pinned phase dynamics. The $\sim1.5$~THz feature lies close to the frequency range reported for the Raman CDW amplitude mode, while coupling to lattice degrees of freedom may also influence its spectral position. We also performed complementary angle-resolved photoemission spectroscopy measurements, which reveal momentum-selective redistribution of near-Fermi-level spectral weight across the transition. Together, these results show that far-field THz spectroscopy provides a sensitive probe of collective CDW dynamics in bulk 2H-NbSe$_2$.

cond-mat.mtrl-sci↗

arXiv2024

Copper doping effects on the superconducting properties of Sm-based oxypnictides

A systematic investigation has been performed by synthesis and comprehensive characterization of a series of SmFe1-xCuxAsO0.8F0.2 bulks (x = 0 to 0.2). These samples are well characterized by structural, Raman spectroscopy, microstructural, transport, magnetic measurements, and supplementary calculations within density functional theory (DFT). The parent compound, SmFeAsO0.8F0.2 (Sm1111), exhibits a superconducting transition temperature (Tc) of approximately 54 K. The lattice volume (V) is increased with Cu substitution (x) without observing any impurity phase related to copper, which confirms the successful incorporation of Cu at Fe sites in the superconducting FeAs layers. These analyses are also well in agreement with Raman spectroscopy measurements and relevant DFT results. The superconducting transition is decreased systematically with copper doping and completely suppressed for 7% Cu-doped Sm1111 (x = 0.07). A large amount of Cu substitution (x greater than 0.07) has demonstrated the metal to insulate transition in the low-temperature range, and no impurity phase was observed even at high Cu doping levels (x = 0.2). The calculated critical current density of the parent sample is suppressed with copper substitution, suggesting the reduced pinning centers, sample density, and grain connections, as confirmed by the microstructural analysis. Our studies suggest that the substitution of Cu in the superconducting FeAs layer, resulting the enlargement of the lattice volume, is a source of strong disorder scattering, leading to the suppression of Tc and the emergence of metal-to-insulator, unlike the more successful carrier doping by nickel (Ni) or cobalt (Co), as previously reported.

cond-mat.supr-con↗

arXiv2024

Effect of impurity phase and high-pressure synthesis on the superconducting properties of CaKFe4As4

AeAFe4As4 (Ae = Ca, A = K; 1144) having a transition temperature of 35 K is a stoichiometric family of iron-based superconductors (FBS). Here, we present a detailed study of a high-pressure synthesis of CaKFe4As4 bulks to investigate the impact of these conditions on the superconducting properties of the 1144 family. Additionally, these samples are also prepared by conventional synthesis method at ambient pressure (CSP) and studied the influence of impurities on the superconducting properties of CaKFe4As4. Structural, microstructural, transport and magnetization measurements have been performed to reach the final conclusions. Interestingly, the high-pressure synthesis of the parent CaKFe4As4 compound enhances the transition temperature (Tc) by 2 K and the critical current density (Jc) by one order of magnitude in the whole magnetic field range of 9 T than that of the 1144 bulks prepared by CSP. It suggests the improvement of the pinning centers and grain connections by the high-pressure synthesis approach. Interestingly, our results depict the superconducting onset transition temperature (Tconset) of this stoichiometric 1144 family is robust with the presence of the common 122 (CaFe2As2 or KFe2As2) impurity phases, which is a different behavior compared to other FBS families. However, these impurity phases reduce the grain connections and lead to the phase separation during the formation of the superconducting (1144) phase.

cond-mat.supr-con↗

arXiv2023

Optimization of Synthesis Parameters and Superconducting Properties of GdFeAsO1-xFx

REFeAsO (RE1111; RE: rare earth) belongs to the 1111 family of iron-based superconductors (FBS), which illustrates the enhancement of the superconducting transition (Tc) with smaller radii of RE. However, the synthesis of the 1111 phase with a heavy rare-earth is always challenging. In this paper, we report the optimization of the growth and superconducting properties of F-doped GdFeAsO1-xFx bulks by preparing the samples in a wide temperature range (700-1100°C) at ambient pressure. The optimized synthesis parameters are concluded based on structural, microstructural, transport, and magnetic measurements. These findings suggest that the optimal conditions for preparing F-doped Gd1111 bulks involve a two-step process at 900°C for 61 hours at ambient pressure, which is lower than previously reported. The optimized samples have revealed the superconducting transition temperature (Tconset) of 43 K for GdFeAsO0.83F0.17. The first-time reported critical current Jc value for this Gd1111 is observed of the order of 10^3 (A/cm^2) at 0 T and 5 K. Our investigation also concluded that highly pure precursors, particularly gadolinium metal, are required to achieve the superconducting properties of F-doped Gd1111. A high growth pressure of 1 GPa reduces the superconducting properties of F-doped Gd1111.

cond-mat.supr-con↗

arXiv2023

Cometal addition effect on superconducting properties and granular behaviours of polycrystalline FeSe0.5Te0.5

The enhanced performance of superconducting FeSe0.5Te0.5 materials with added microsized Pb and Sn particles is presented. A series of Pb and Sn added FeSe0.5Te0.5 (FeSe0.5Te0.5 + xPb + ySn; x = y = 0-0.1) bulks are fabricated by solid-state reaction method and characterized through various measurements. A very small amount of Sn and Pb additions enhance the transition temperature (Tconset) of pure FeSe0.5Te0.5 by 1 K, sharpening the superconducting transition and improving the metallic nature in the normal state, whereas larger metal additions reduce Tconset by broadening the superconducting transition. Microstructural analysis and transport studies suggest that at x=y>0.02, Pb and Sn additions enhance the impurity phases, reduce the coupling between grains, and suppress the superconducting percolation, leading to a broad transition. FeSe0.5Te0.5 samples with 2wt% of cometal additions show the best performance with their critical current density, Jc, and the pinning force, Fp, which might be attributable to providing effective flux pinning centres. Our study shows that the inclusion of a relatively small amount of Pb and Sn works effectively for the enhancement of superconducting properties with an improvement of intergrain connections as well as better phase uniformity.

cond-mat.supr-con↗

arXiv2023

High-pressure synthesis and the enhancement of the superconducting properties of FeSe0.5Te0.5

A series of FeSe0.5Te0.5 bulk samples have been prepared through the high gas pressure and high-temperature synthesis (HP-HTS) method to optimize the growth conditions, for the first time and investigated for their superconducting properties using structural, microstructure, transport, and magnetic measurements to reach the final conclusions. Ex-situ and in-situ processes are used to prepare bulk samples under a range of growth pressures using Ta-tube and without Tatube. The parent compound synthesized by convenient synthesis method at ambient pressure (CSP) exhibits a superconducting transition temperature of 14.8 K. Our data demonstrate that the prepared FeSe0.5Te0.5 sealed in a Ta-tube is of better quality than the samples without a Ta-tube, and the optimum growth conditions (500 MPa, 600°C for 1 h) are favourable for the development of the tetragonal FeSe0.5Te0.5 phase. The optimum bulk FeSe0.5Te0.5 depicts a higher transition temperature of 17.3 K and a high critical current density of the order of >10^4 A/cm^2 at 0 T, which is improved over the entire magnetic field range and almost twice higher than the parent compound prepared through CSP. Our studies confirm that the high-pressure synthesis method is a highly efficient way to improve the superconducting transition, grain connectivity, sample density, and also pinning properties of a superconductor.

cond-mat.supr-con↗

arXiv2022

Topological Lifshitz transition in Weyl semimetal NbP decorated with heavy elements

Studies of the Fermi surface modification after in-situ covering NbP semimetal with heavy elements Pb and Nb ultrathin layers were performed by means of angle-resolved photoemission spectroscopy (ARPES). First, the electronic structure was investigated for pristine single crystals with two possible terminations (P and Nb) of the (0 0 1) surface. The nature of the electronic states of these two cleaving planes is different: P-terminated surface shows spoon and bow tie shaped fingerprints, whereas these shapes are not present in Nb-terminated surfaces. ARPES studies show that even 1 monolayer (ML) of Pb causes topological quantum Lifshitz transition (TQLT) in P- and Nb-terminated surfaces. Deposited Pb 5d electrons have wide extended atomic orbitals which leads to strong hybridization with Pb-terminated surface and a corresponding shift in the Fermi energy. Nb has less capability to perturb the system than Pb because Nb has weaker spin-orbit coupling than Pb. Nb-terminated surface subjected to surface decoration with approximately 1.3 ML of Nb shows no dramatic modification in the Fermi surface. In the case of Nb decorated P-terminated surface, deposition of approximately 1 ML modifies the electronic structure of NbP and it is on the verge of TQLT. Despite the strong spin-orbit and strong hybridization of the heavy elements on the surface, it is possible to observe the TQLT of the surface states thanks to the robustness of the bulk topology.

cond-mat.mtrl-sci↗