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Andy Chia

Publications and source records attributed to Andy Chia.

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Quantization of nonlinear non-Hamiltonian systems

Several important dynamical systems are in $\mathbb{R}^2$, defined by the pair of differential equations $(x',y')=(f(x,y),g(x,y))$. A question of fundamental importance is how such systems might behave quantum mechanically. In developing quantum theory, Dirac and others realized that classical Hamiltonian systems can be mapped to their quantum counterparts via canonical quantization. The resulting quantum dynamics is always physical, characterized by completely-positive and trace-preserving evolutions in the Schr\"{o}dinger picture. However, whether non-Hamiltonian systems can be quantized systematically while respecting the same physical requirements has remained a long-standing problem. Here we resolve this question when $f(x,y)$ and $g(x,y)$ are arbitrary polynomials. By leveraging open-systems theory, we prove constructively that every polynomial system admits a physical generator of time evolution in the form of a Lindbladian. We call our method cascade quantization, and demonstrate its power by analyzing several paradigmatic examples of nonlinear dynamics such as bifurcations, noise-activated spiking, and Li\'{e}nard systems. In effect, our method can quantize any classical system whose $f(x,y)$ and $g(x,y)$ are analytic with arbitrary precision. More importantly, cascade quantization is exact. This means restrictive system properties usually assumed in the literature to facilitate quantization, such as weak nonlinearity, rotational symmetry, or semiclassical dynamics, can all be dispensed with by cascade quantization. We also highlight the advantages of cascade quantization over existing proposals, by weighing it against examples from the variational paradigm using Lagrangians, as well as non-variational approaches.

quant-ph

Optimal quantum metrology for two-photon absorption

Two-photon absorption (TPA) is a nonlinear optical process with wide-ranging applications from spectroscopy to super-resolution imaging. Despite this, the precise measurement and characterisation of TPA parameters are challenging due to their inherently weak nature. We study the potential of single-mode quantum light to enhance TPA parameter estimation through the quantum Fisher information (QFI). Discrete variable (DV) quantum states (defined to be a finite superposition of Fock states) are optimised to maximise the QFI for given absorption, revealing a quantum advantage compared to both the coherent state (classical) benchmark and the single-mode squeezed vacuum state. For fixed average energy $\bar{n} \in 2\mathbb{N}$, the Fock state is shown to be optimal for large TPA parameters, while a superposition of vacuum and a particular Fock state is optimal for small absorption for all $\bar{n}$. This differs from single-photon absorption where the Fock state is always optimal. Notably, photon counting is demonstrated to offer optimal or nearly optimal performance compared to the QFI bound for all levels of TPA parameters for the optimised quantum probes. Our findings provide insight into known limiting behaviours of Gaussian probes and their different Fisher information (FI) scalings under photon counting ($\propto \bar{n}^2$ for squeezed vacuum states versus $\bar{n}^3$ for coherent states). The squeezed state outperforms coherent states for small TPA parameters but underperforms in the intermediate regime, becoming comparable in the large absorption limit. This can be explained through fundamental differences between behaviours of even and odd number Fock states: the former's QFI diverges in both large and small absorption limits, while the latter diverges only in the small absorption limit, dominating at intermediate scales.

quant-ph

Quantum synchronization effects induced by strong nonlinearities

A paradigm for quantum synchronization is the quantum analog of the Stuart--Landau oscillator, which corresponds to a van der Pol oscillator in the limit of weak (i.e. vanishingly small) nonlinearity. Due to this limitation, the quantum Stuart--Landau oscillator fails to capture interesting nonlinearity-induced phenomena such as relaxation oscillations. To overcome this deficiency we propose an alternative model which approximates the van der Pol oscillator to finitely large nonlinearities while remaining numerically tractable. This allows us to uncover interesting phenomena in the deep-quantum strongly-nonlinear regime with no classical analog, such as the persistence of amplitude death on resonance. We also report nonlinearity-induced position correlations in reactively coupled quantum oscillators. Such coupled oscillations become more and more correlated with increasing nonlinearity before reaching some maximum. Again, this behavior is absent classically. We also show how strong nonlinearity can enlarge the synchronization bandwidth in both single and coupled oscillators. This effect can be harnessed to induce mutual synchronization between two oscillators initially in amplitude death.

quant-ph