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Anjan Barman

Publications and source records attributed to Anjan Barman.

At least 19 recordsLinked to original sources

Tunnel-Barrier-Engineered Ultrafast Demagnetization and Spin Transport in Graphene-Based Heterostructures

Heterostructures combining graphene with 3d transition metal ferromagnets (FMs) enable various spin-based phenomena at ultrafast timescales. However, challenges such as the interfacial impedance mismatch, FM deposition-induced defect generation, and interface modification by interfacial coupling or hybridization can impede their functionalization for spin-orbitronics. In this work, we utilize insulating TiOx barrier layers (BLs) to modify the interfacial spin conductance structurally, disentangle spin pumping and magnetic proximity effects (MPE), and establish external control over ultrafast magnetization dynamics in single-layer graphene/TiOx/Co systems. All-optical time-resolved magneto-optical Kerr effect measurements of femtosecond to nanosecond spin dynamics reveal systematic tunability of ultrafast magnetic parameters via barrier engineering. The thickness-dependent damping modulation in Co indicates strong spin pumping, with interfacial spin transparency close to half its physical limit in the presence of an ultrathin BL, where MPE is eliminated. Our results show that appropriately chosen ultrathin BLs can prevent interfacial alterations from ferromagnetic metals, facilitating efficient spin detection in graphene and enhancing control over spin angular momentum dissipation in graphene/FM interfaces.

cond-mat.mes-hall

Magnetic Charge State Controlled Spin-Wave Dynamics in Nanoscale Three-Dimensional Artificial Spin Ice

Three-dimensional (3D) magnetic nanostructures offer a versatile platform for exploring complex spin textures and spin-wave (SW) dynamics, with implications in next-generation spintronic and magnonic technologies. Advances in 3D nanofabrication have allowed a wide-range of structures and phenomena to be realized. Whilst the study of simple cylindrical magnetic nanowires allows the realization of ultrafast domain walls and a spin Cherenkov effect, placing such wires of complex cross-section into 3D arrangements allows one to produce magnetic metamaterials, known as artificial spin-ice (ASI), where the overall ground state and spin dynamics are governed by magnetostatic interactions between elements. Here, using Brillouin Light Scattering (BLS) we demonstrate the direct detection of magnetic charged states in a 3D-ASI system. The measured spin-wave modes in 3D-ASI are found to be directly controlled by the local magnetic charge configuration and the direction of the applied magnetic field. Micromagnetic simulations provide insight into the spatially selective excitation of spin waves and the evolution of magnetic microstates, uncovering a direct link to the field-dependent characteristics of the spin-wave spectrum. These findings make 3D-ASI architectures a promising system to realize reconfigurable, low-power magnonic devices with engineered collective dynamics.

cond-mat.mes-hall

Optical excitation and detection of high-frequency Sezawa modes in Si/SiO2 system decorated with Ni80Fe20 nanodot arrays

Surface acoustic waves have emerged as one of the potential candidates for the development of next-generation wave-based information and computing technologies. For practical devices, it is essential to develop the excitation techniques for different types of surface acoustic waves, especially at higher microwave frequencies, and to tailor their frequency versus wave vector characteristics. We show that this can be done by using ultrashort laser pulses incident on the surface of a multilayer decorated with a periodic array of metallic nanodots. Specifically, we study surface acoustic waves in the dielectric substrate Si/SiO2 decorated with a square lattice of thin Ni80Fe20 (Py) dots. Using a femtosecond laser-based optical pump-probe measurement, we detect a number of high-frequency phononic modes. By performing finite element simulations, we identify them as Sezawa modes from the second and third Brillouin zone in addition to the modes confined within the Py dots. The frequency of the Sezawa modes strongly depends on the period of the Py dots and varies in the range between 5 to 15 GHz. Both types of waves cover the same frequency range for Py dots with period less than 400 nm, providing a promising system for magnetoelastic studies.

cond-mat.mtrl-sci

Spin Pumping in Magnetostrictive Galfenol Interfaced with Ta

In view of their advantages for memory and storage applications, the quest to find suitable magnetic thin film heterostructures that can exhibit strong spin pumping effect persists in the scientific community. Here, the spin pumping phenomenon is investigated in Ta/Galfenol (FeGa) thin film heterostructures by systematically varying the thickness of the heavy metallic Ta underlayer (UL). The films exhibit soft magnetic property with a bcc-phase with a notably low Gilbert damping obtained for FeGa on Si (100). The precessional magnetization dynamics of Ta/FeGa films are explored using time-resolved magneto-optical Kerr effect magnetometry, revealing the presence of a resonant Kittel mode and additional strain-induced modes. The lowest value of effective Gilbert damping in Ta/FeGa is obtained as ~ 0.015, which rises by ~ 65 % as the thickness of UL increases. Spin pumping and two-magnon scattering mechanisms are validated using a ballistic spin transport model. An overall effective spin mixing conductance value of ~ 5.48 $\times$ 10$^{15}$ cm$^{-2}$ is found, which is the highest value ever reported in magnetostrictive Galfenol films. Additionally, micromagnetic simulations are performed to understand the effect of tilted magnetic anisotropy on the formation of magnetic modes in these films. These findings in FeGa films establish it as an effective spin source material and offer innovative ideas to control spin-wave propagation and diverse applications in straintronics.

cond-mat.mtrl-sci

Spin Hall Nano-Antenna

The spin Hall effect is a celebrated phenomenon in spintronics and magnetism that has found numerous applications in digital electronics (memory and logic), but very few in analog electronics. Practically, the only analog application in widespread use is the spin Hall nano-oscillator (SHNO) that delivers a high frequency alternating current or voltage to a load. Here, we report its analogue - a spin Hall nano-antenna (SHNA) that radiates a high frequency electromagnetic wave (alternating electric/magnetic fields) into the surrounding medium. It can also radiate an acoustic wave in an underlying substrate if the nanomagnets are made of a magnetostrictive material. That makes it a dual electromagnetic/acoustic antenna. The SHNA is made of an array of ledged magnetostrictive nanomagnets deposited on a substrate, with a heavy metal nanostrip underlying/overlying the ledges. An alternating charge current passed through the nanostrip generates an alternating spin-orbit torque in the nanomagnets via the spin Hall effect which makes their magnetizations oscillate in time with the frequency of the current, producing confined spin waves (magnons), which radiate electromagnetic waves (photons) in space with the same frequency as the ac current. Despite being much smaller than the radiated wavelength, the SHNA surprisingly does not act as a point source which would radiate isotropically. Instead, there is clear directionality (anisotropy) in the radiation pattern, which is frequency-dependent. This is due to the (frequency-dependent) intrinsic anisotropy in the confined spin wave patterns generated within the nanomagnets, which effectively endows the "point source" with internal anisotropy.

cond-mat.mes-hall

Anomalous Inverse Spin Hall Effect (AISHE) due to Unconventional Spin Currents in Ferromagnetic Films with Tailored Interfacial Magnetic Anisotropy

A single layer ferromagnetic film magnetized in the plane of an ac current flow, exhibits a characteristic Hall voltage with harmonic and second harmonic components, which is attributed to the presence of spin currents with polarization non-collinear with the magnetization. A set of 30 nm thick permalloy (Py) films used in this study are deposited at an oblique angle with respect to the substrate plane which induces an in-plane easy axis in the magnetization of the initial nucleating layers of the films which is distinct from the overall bulk magnetic properties of the film. This unusual magnetic texture provides a platform for the direct detection of inverse spin Hall effect in Hall bar shaped macroscopic devices at room temperatures which we denote as Anomalous Inverse Spin Hall Effect (AISHE). Control samples fabricated by normal deposition of permalloy with slow rotation of substrate shows significant reduction of the harmonic Hall signal that further substantiates the model. The analysis of the second harmonic Hall signal corroborates the presence of spin-orbit torque arising from the unconventional spin-currents in the single-layer ferromagnets.

cond-mat.mes-hall

Tripartite Phonon-Magnon-Plasmon Coupling, Parametric Amplification, and Formation of a Phonon-Magnon-Plasmon Polariton in a Two-Dimensional Periodic Array of Magnetostrictive/Plasmonic Bilayered Nanodots

Coupling between spin waves (SWs) and other types of waves in nanostructured magnetic media has garnered increased attention in recent years because of the rich physics and the potential to produce disruptive technologies. Among this family of intriguing phenomena, we recently reported a new one: coupling between SWs and hybridized phonon-plasmon waves, resulting in tripartite coupling of magnons, phonons, and plasmons. Here, this acousto-plasmo-magnonic phenomenon is studied in a two-dimensional periodic array of bilayered [Co/Al] nanodots on a silicon substrate, where the Co is a magnetostrictive constituent responsive to magneto-elastic coupling and the Al acts as a source of surface plasmons. Time-resolved magneto-optical-Kerr-effect microscopy revealed parametric amplification and strong coupling between two spin wave modes mediated by a hybrid phonon-plasmon wave. The strong coupling forms a new quasi-particle: the phonon-plasmonmagnon polariton.

cond-mat.mes-hall

Enhancement of spin to charge conversion efficiency at the topological surface state by inserting normal metal spacer layer in the topological insulator based heterostructure

We report efficient spin to charge conversion (SCC) in the topological insulator (TI) based heterostructure ($BiSbTe_{1.5}Se_{1.5}/Cu/Ni_{80}Fe_{20}$) by using spin-pumping technique where $BiSbTe_{1.5}Se_{1.5}$ is the TI and $Ni_{80}Fe_{20}$ is the ferromagnetic layer. The SCC, characterized by inverse Edelstein effect length ($\lambda_{IEE}$) in the TI material gets altered with an intervening Copper (Cu) layer and it depends on the interlayer thickness. The introduction of Cu layer at the interface of TI and ferromagnetic metal (FM) provides a new degree of freedom for tuning the SCC efficiency of the topological surface states. The significant enhancement of the measured spin-pumping voltage and the linewidth of ferromagnetic resonance (FMR) absorption spectra due to the insertion of Cu layer at the interface indicates a reduction in spin memory loss at the interface that resulted from the presence of exchange coupling between the surface states of TI and the local moments of ferromagnetic metal. The temperature dependence (from 8K to 300K) of the evaluated $\lambda_{IEE}$ data for all the trilayer systems, TI/Cu/FM with different Cu thickness confirms the effect of exchange coupling between the TI and FM layer on the spin to charge conversion efficiency of the topological surface state.

cond-mat.mes-hall

Spin-wave spectral analysis in crescent-shaped ferromagnetic nanorods

The research on the properties of spin waves (SWs) in three-dimensional nanosystems is an innovative idea in the field of magnonics. Mastering and understanding the nature of magnetization dynamics and binding of SWs at surfaces, edges, and in-volume parts of three-dimensional magnetic systems enables the discovery of new phenomena and suggests new possibilities for their use in magnonic and spintronic devices. In this work, we use numerical methods to study the effect of geometry and external magnetic field manipulations on the localization and dynamics of SWs in crescent-shaped (CS) waveguides. It is shown that changing the magnetic field direction in these waveguides breaks the symmetry and affects the localization of eigenmodes with respect to the static demagnetizing field. This in turn has a direct effect on their frequency. Furthermore, CS structures were found to be characterized by significant saturation at certain field orientations, resulting in a cylindrical magnetization distribution. Thus, we present chirality-based nonreciprocal dispersion relations for high-frequency SWs, which can be controlled by the field direction (shape symmetry) and its amplitude (saturation).

cond-mat.mes-hall

Investigation of Ultrafast Demagnetization and Gilbert Damping and their Correlation in Different Ferromagnetic Thin Films Grown Under Identical Conditions

Following the demonstration of laser-induced ultrafast demagnetization in ferromagnetic nickel, several theoretical and phenomenological propositions have sought to uncover its underlying physics. In this work we revisit the three temperature model (3TM) and the microscopic three temperature model (M3TM) to perform a comparative analysis of ultrafast demagnetization in 20-nm-thick cobalt, nickel and permalloy thin films measured using an all-optical pump-probe technique. In addition to the ultrafast dynamics at the femtosecond timescales, the nanosecond magnetization precession and damping are recorded at various pump excitation fluences revealing a fluence-dependent enhancement in both the demagnetization times and the damping factors. We confirm that the Curie temperature to magnetic moment ratio of a given system acts as a figure of merit for the demagnetization time, while the demagnetization times and damping factors show an apparent sensitivity to the density of states at the Fermi level for a given system. Further, from numerical simulations of the ultrafast demagnetization based on both the 3TM and the M3TM, we extract the reservoir coupling parameters that best reproduce the experimental data and estimate the value of the spin flip scattering probability for each system. We discuss how the fluence-dependence of inter-reservoir coupling parameters so extracted may reflect a role played by nonthermal electrons in the magnetization dynamics at low laser fluences.

cond-mat.str-el

Spin Dynamics in Patterned Magnetic Multilayers with Perpendicular Magnetic Anisotropy

The magnetization dynamics in nanostructures has been extensively studied in the last decades, and nanomagnetism has evolved significantly over that time, discovering new effects, developing numerous applications, and identifying promising new directions. This includes magnonics, an emerging research field oriented on the study of spin-wave dynamics and their applications. In this context, thin ferromagnetic films with perpendicular magnetic anisotropy (PMA) offer interesting opportunities to study spin waves, in particular, due to out-of-plane magnetization in remanence or at relatively weak external magnetic fields. This is the only magnetization configuration offering isotropic in-plane spin-wave propagation within the sample plane, the forward volume magnetostatic spin-wave geometry. The isotropic dispersion relation is highly important in designing signal-processing devices, offering superior prospects for direct replicating various concepts from photonics into magnonics. Analogous to photonic or phononic crystals, which are the building blocks of optoelectronics and phononics, magnonic crystals are considered as key components in magnonics applications. Arrays of nanodots and structured ferromagnetic thin films with a periodic array of holes, popularly known as antidot lattices based on PMA multilayers have been recently studied. Novel magnonic properties related to propagating spin-wave modes, exploitation of the band gaps, and confined modes, were demonstrated. Also, the existence of nontrivial magnonic band topologies has been shown. Moreover, the combination of PMA and Dzyaloshinskii-Moriya interaction leads to the formation of chiral magnetization states, including Néel domain walls, skyrmions, and skyrmionium states.

cond-mat.mtrl-sci

Spin Wave Electromagnetic Nano-Antenna Enabled by Tripartite Phonon-Magnon-Photon Coupling

We investigate tripartite coupling between phonons, magnons and photons in a periodic array of elliptical magnetostrictive nanomagnets delineated on a piezoelectric substrate to form a two-dimensional two-phase multiferroic crystal. A surface acoustic wave (phonons) of 5 - 35 GHz frequency launched into the substrate causes the magnetizations of the nanomagnets to precess at the frequency of the wave, giving rise to spin waves (magnons). The spin waves, in turn, radiate electromagnetic waves (photons) into the surrounding space at the surface acoustic wave frequency. Here, the phonons couple into magnons, which then couple into photons. This tripartite phonon-magnon-photon coupling is exploited to implement an extreme sub-wavelength electromagnetic antenna whose measured radiation efficiency and antenna gain exceed the theoretical limits for traditional antennas by more than two orders of magnitude at some frequencies. Micro-magnetic simulations are in excellent agreement with experimental observations and provide insight into the spin wave modes that couple into radiating electromagnetic modes to implement the antenna.

cond-mat.mes-hall

Mechanism of Spin-Orbit Torques in Platinum Oxide Systems

Spin-Orbit Torque (SOT) Magnetic Random-Access Memories (MRAM) have shown promising results towards the realization of fast, non-volatile memory systems. Oxidation of the heavy-metal (HM) layer of the SOT-MRAM has been proposed as a method to increase its energy efficiency. But the results are widely divergent due to the difficulty in controlling the HM oxidation because of its low enthalpy of formation. Here, we reconcile these differences by performing a gradual oxidation procedure, which allows correlating the chemical structure to the physical properties of the stack. As an HM layer, we chose Pt because of the strong SOT and the low enthalpy of formation of its oxides. We find evidence of an oxide inversion layer at the FM/HM interface: the oxygen is drawn into the FM, while the HM remains metallic near the interface. We further demonstrate that the oxygen migrates in the volume of the FM layer rather than being concentrated at the interface. Consequently, we find that the intrinsic magnitude of the SOT is unchanged compared to the fully metallic structure. The previously reported apparent increase of SOTs is not intrinsic to platinum oxide and instead arises from systemic changes produced by oxidation.

cond-mat.mes-hall

Comparison of Spin-Wave Modes in Connected and Disconnected Artificial Spin Ice Nanostructures Using Brillouin Light Scattering Spectroscopy

Artificial spin ice systems have seen burgeoning interest due to their intriguing physics and potential applications in reprogrammable memory, logic and magnonics. Integration of artificial spin ice with functional magnonics is a relatively recent research direction, with a host of promising results. As the field progresses, direct in-depth comparisons of distinct artificial spin systems are crucial to advancing the field. While studies have investigated the effects of different lattice geometries, little comparison exists between systems comprising continuously connected nanostructures, where spin-waves propagate via dipole-exchange interaction, and systems with nanobars disconnected at vertices where spin-wave propagation occurs via stray dipolar-field. Gaining understanding of how these very different coupling methods affect both spin-wave dynamics and magnetic reversal is key for the field to progress and provides crucial system-design information including for future systems containing combinations of connected and disconnected elements. Here, we study the magnonic response of two kagome spin ices via Brillouin light scattering, a continuously connected system and a disconnected system with vertex gaps. We observe distinct high-frequency dynamics and magnetization reversal regimes between the systems, with key distinctions in spin-wave localization and mode quantization, microstate-trajectory during reversal and internal field-profiles. These observations are pertinent for the fundamental understanding of artificial spin systems and broader design and engineering of reconfigurable functional magnonic crystals.

cond-mat.mes-hall

Straintronics: Manipulating the Magnetization of Magnetostrictive Nanomagnets with Strain for Energy-Efficient Applications

The desire to perform information processing, computation, communication, signal generation and related tasks, while dissipating as little energy as possible, has inspired many ideas and paradigms. One of the most powerful among them is the notion of using magnetostrictive nanomagnets as the primitive units of the hardware platforms and manipulating their magnetizations with electrically generated static or time varying mechanical strain to elicit myriad functionalities. This approach has two advantages. First, information can be retained in the devices after powering off since the nanomagnets are non-volatile unlike charge-based devices such as transistors. Second, the energy expended to perform a given task is exceptionally low since it takes very little energy to alter magnetization states with strain. This field is now known as "straintronics", in analogy with electronics, spintronics, valleytronics, etc. We review the recent advances and trends in straintronics, including digital information processing (logic), information storage (memory), domain wall devices operated with strain, control of skyrmions with strain, non-Boolean computing and machine learning with straintronics, signal generation (microwave sources) and communication (ultra-miniaturized acoustic and electromagnetic antennas) implemented with strained nanomagnets, hybrid straintronics-magnonics, and interaction between phonons and magnons in straintronic systems. We identify key challenges and opportunities, and lay out pathways to advance this field to the point where it might become a mainstream technology for energy-efficient systems.

cond-mat.mes-hall

Applications of Nanomagnets as Dynamical Systems

When magnets are fashioned into nanoscale elements, they exhibit a wide variety of phenomena replete with rich physics and the lure of tantalizing applications. In this topical review, we discuss some of these phenomena, especially those that have come to light recently, and highlight their potential applications. We emphasize what drives a phenomenon, what undergirds the dynamics of the system that exhibits the phenomenon, how the dynamics can be manipulated, and what specific features can be harnessed for technological advances. For the sake of balance, we point out both advantages and shortcomings of nanomagnet based devices and systems predicated on the phenomena we discuss. Where possible, we chart out paths for future investigations that can shed new light on an intriguing phenomenon and/or facilitate both traditional and non-traditional applications.

cond-mat.mes-hall

Observation of Coherent Spin Waves in a Three-Dimensional Artificial Spin Ice Structure

Harnessing high-frequency spin dynamics in three-dimensional (3D) nanostructures may lead to paradigm-shifting, next generation devices including high density spintronics and neuromorphic systems. Despite remarkable progress in fabrication, the measurement and interpretation of spin dynamics in complex 3D structures remain exceptionally challenging. Here we take a first step and measure coherent spin waves within a 3D artificial spin ice (ASI) structure using Brillouin light scattering. The 3D-ASI was fabricated by using a combination of two-photon lithography and thermal evaporation. Two spin-wave modes were observed in the experiment whose frequencies showed a monotonic variation with the applied field strength. Numerical simulations qualitatively reproduced the observed modes. The simulated mode profiles revealed the collective nature of the modes extending throughout the complex network of nanowires while showing spatial quantization with varying mode quantization numbers. The study shows a well-defined means to explore high-frequency spin dynamics in complex 3D spintronic and magnonic structures.

cond-mat.mes-hall

Structural Phase Dependent Giant Interfacial Spin Transparency in W/CoFeB Thin Film Heterostructure

Pure spin current has transfigured the energy-efficient spintronic devices and it has the salient characteristic of transport of the spin angular momentum. Spin pumping is a potent method to generate pure spin current and for its increased efficiency high effective spin-mixing conductance (Geff) and interfacial spin transparency (T) are essential. Here, a giant T is reported in Sub/W(t)/Co20Fe60B20(d)/SiO2(2 nm) heterostructures in β-tungsten (β-W) phase by employing all-optical time-resolved magneto-optical Kerr effect technique. From the variation of Gilbert damping with W and CoFeB thicknesses, the spin diffusion length of W and spin-mixing conductances are extracted. Subsequently, T is derived as 0.81 \pm 0.03 for the β-W/CoFeB interface. A sharp variation of Geff and T with W thickness is observed in consonance with the thickness-dependent structural phase transition and resistivity of W. The spin memory loss and two-magnon scattering effects are found to have negligible contributions to damping modulation as opposed to spin pumping effect which is reconfirmed from the invariance of damping with Cu spacer layer thickness inserted between W and CoFeB. The observation of giant interfacial spin transparency and its strong dependence on crystal structures of W will be important for pure spin current based spin-orbitronic devices.

cond-mat.mtrl-sci