arXiv subjects

Anjan Soumyanarayanan

Publications and source records attributed to Anjan Soumyanarayanan.

At least 19 recordsLinked to original sources

arXiv2026

Electrical manipulation and detection of perpendicular altermagnetic order via proximitized Dirac semimetal

Altermagnets, which combine antiferromagnetic-like magnetic compensation with ferromagnetic-like broken time-reversal symmetry, hold great promise for high-density and ultrafast spintronic applications. However, the detection and switching of perpendicular altermagnetic order are fundamentally constrained by magnetic symmetry, restricting both fundamental studies and practical implementation. We realize robust electrical reading and deterministic switching of perpendicular altermagnetic order by designing a Dirac semimetal/altermagnet heterostructure of PtTe2/CrSb. This engineered interface enables anomalous Hall readout via altermagnetic proximity effect and delivers efficient spin-orbit torque for manipulating the epitaxial perpendicular Neel vector in CrSb. These findings significantly broaden the functional scope of altermagnetic heterostructures and pave the way for highly scalable altermagnetic memory.

cond-mat.mtrl-sci↗

arXiv2025

Real-time dynamics of VCMA-assisted switching of magnetic tunnel junctions

Voltage control of magnetic anisotropy (VCMA) induced by charge accumulation is typically considered as an ultrafast process, enabling energy-efficient and high-speed magnetization switching in spintronic devices. In this work, we investigate the real-time dynamics of VCMA-assisted switching of magnetic tunnel junctions via relaxation in a magnetic field. We show that device-dependent charging effects and magnetic granularity in the free layer limit the switching speed at applied voltages close to the critical switching threshold. Increasing the voltage or the applied magnetic field reduces the incubation delay and total switching time to below a few ns. Micromagnetic simulations incorporating the finite charging times of the tunnel junction and the granularity of the magnetic film reproduce the experimental results, providing critical insights into optimizing VCMA-driven magnetization control for memory and logic applications.

physics.app-ph↗

arXiv2025

Magnon-mediated perpendicular magnetization switching by topological crystalline insulator SnTe with high spin Hall conductivity

Magnons possess the ability to transport spin angular momentum in insulating magnetic materials, a characteristic that sets them apart from traditional electronics where power consumption arises from the movement of electrons. However, the practical application of magnon devices demands room temperature operation and low switching power of perpendicular magnetization. Here we demonstrate the low-power manipulation of perpendicular magnetization via magnon torques in SnTe/NiO/CoFeB devices at room temperature. Topological crystalline insulator SnTe exhibits a high spin Hall conductivity of $σ_s \approx 6.1\times 10^4 (\hbar/2e)\cdot (Ω\cdot m)^{-1}$, which facilitates the generation of magnon currents in an antiferromagnetic insulator NiO. The magnon currents traverse the 20-nm-thick NiO layer and subsequently exert magnon torques on the adjacent ferromagnetic layer, leading to magnetization switching. Notably, we achieve a 22-fold reduction in power consumption in SnTe/NiO/CoFeB heterostructures compared to Bi2Te3/NiO/CoFeB control samples. Our findings establish the low-power perpendicular magnetization manipulation through magnon torques, significantly expanding the range of topological materials with practical applications.

cond-mat.mtrl-sci↗

arXiv2025

Zero Field Antiferromagnetically Coupled Skyrmions and their Field-Driven Uncoupling in Composite Chiral Multilayers

Antiferromagnetic (AF) skyrmions are topological spin structures with fully compensated, net-zero magnetization. Compared to their ferromagnetic (FM) skyrmion counterparts, their reduced stray field and enhanced electrical response can enable linear, high-throughput current-driven motion. However, their bubble-like character in conventional bilayer AFs limits their stability to fluctuations, leading to deformation and annihilation. Here we present the engineering of a composite AF chiral multilayer, wherein the interplay of AF and FM interlayer couplings generates compensated skyrmions with compact structures. High-resolution magnetic imaging and micromagnetic simulations show that the internal exchange field stabilizes AF skyrmions at zero external field with characteristics comparable to FM counterparts at 100 mT. Quantitative analyses establish their decoupling above the exchange field, yielding independent, spatially segregated textures in constituent chiral layers. This work provides a foundation to develop AF spin-textures with enhanced immunity, compatible with efficient readout and manipulation, with relevance to unconventional computing.

cond-mat.mtrl-sci↗

arXiv2024

Chiral damping of magnons

Chiral magnets have garnered significant interest due to the emergence of unique phenomena prohibited in inversion-symmetric magnets. While the equilibrium characteristics of chiral magnets have been extensively explored through the Dzyaloshinskii-Moriya interaction (DMI), non-equilibrium properties like magnetic damping have received comparatively less attention. We present the inaugural direct observation of chiral damping through Brillouin light scattering (BLS) spectroscopy. Employing BLS spectrum analysis, we independently deduce the Dzyaloshinskii-Moriya interaction (DMI) and chiral damping, extracting them from the frequency shift and linewidth of the spectrum peak, respectively. The resulting linewidths exhibit clear odd symmetry with respect to the magnon wave vector, unambiguously confirming the presence of chiral damping. Our study introduces a novel methodology for quantifying chiral damping, with potential ramifications on diverse nonequilibrium phenomena within chiral magnets.

cond-mat.mtrl-sci↗

arXiv2023

Stability and Character of Zero Field Skyrmionic States in Hybrid Magnetic Multilayer Nanodots

Ambient magnetic skyrmions stabilized in multilayer nanostructures are of immense interest due to their relevance to magnetic tunnel junction (MTJ) devices for memory and unconventional computing applications. However, existing skyrmionic nanostructures built using conventional metallic or oxide multilayer nanodots are unable to concurrently fulfill the requirements of nanoscale skyrmion stability and feasibility of all-electrical readout and manipulation. Here, we develop a few-repeat hybrid multilayer platform consisting of metallic [Pt/CoB/Ir]3 and oxide [Pt/CoB/MgO] components that are coupled to evolve together as a single, composite stack. Zero-field (ZF) skyrmions with sizes as small as 50 nm are stabilized in the hybrid multilayer nanodots, which are smoothly modulated by up to 2.5x by varying CoB thickness and dot sizes. Meanwhile, skyrmion multiplets are also stabilized by small bias fields. Crucially, we observe higher order 'target' skyrmions with varying magnetization rotations in moderately-sized, low anisotropy nanodots. These results provide a viable route to realize long-sought skyrmionic MTJ devices and new possibilities for multi-state skyrmionic device concepts.

cond-mat.mtrl-sci↗

arXiv2023

Quantifying the magnetic interactions governing chiral spin textures using deep neural networks

The interplay of magnetic interactions in chiral multilayer films gives rise to nanoscale topological spin textures, which form attractive elements for next-generation computing. Quantifying these interactions requires several specialized, time-consuming, and resource-intensive experimental techniques. Imaging of ambient domain configurations presents a promising avenue for high-throughput extraction of the parent magnetic interactions. Here we present a machine learning-based approach to determine the key interactions -- symmetric exchange, chiral exchange, and anisotropy -- governing chiral domain phenomenology in multilayers. Our convolutional neural network model, trained and validated on over 10,000 domain images, achieved $R^2 > 0.85$ in predicting the parameters and independently learned physical interdependencies between them. When applied to microscopy data acquired across samples, our model-predicted parameter trends are consistent with independent experimental measurements. These results establish ML-driven techniques as valuable, high-throughput complements to conventional determination of magnetic interactions, and serve to accelerate materials and device development for nanoscale electronics.

cond-mat.mtrl-sci↗

arXiv2023

All-Electrical Skyrmionic Bits in a Chiral Magnetic Tunnel Junction

Topological spin textures such as magnetic skyrmions hold considerable promise as robust, nanometre-scale, mobile bits for sustainable computing. A longstanding roadblock to unleashing their potential is the absence of a device enabling deterministic electrical readout of individual spin textures. Here we present the wafer-scale realization of a nanoscale chiral magnetic tunnel junction (MTJ) hosting a single, ambient skyrmion. Using a suite of electrical and multi-modal imaging techniques, we show that the MTJ nucleates skyrmions of fixed polarity, whose large readout signal - 20-70% relative to uniform states - corresponds directly to skyrmion size. Further, the MTJ exploits complementary mechanisms to stabilize distinctly sized skyrmions at zero field, thereby realizing three nonvolatile electrical states. Crucially, it can write and delete skyrmions using current densities 1,000 times lower than state-of-the-art. These results provide a platform to incorporate readout and manipulation of skyrmionic bits across myriad device architectures, and a springboard to harness chiral spin textures for multi-bit memory and unconventional computing.

cond-mat.mes-hall↗

arXiv2023

Quantifying symmetric exchange in ultrathin ferromagnetic films with chirality

The symmetric (Heisenberg) exchange interaction is fundamental to magnetism and assumes critical importance in designing magnetic materials for novel emergent phenomena and device applications. However, quantifying exchange is extremely challenging for ultrathin ($\sim$ 1 nm) magnetic films, as techniques and approximations reliably used for bulk materials are largely inapplicable in the two-dimensional (2D) limit. Here we present and contrast the measurement of exchange stiffness, $A$, by several methods on a series of five Co/Pt-based ultrathin ($1-2$ nm) films. We compare results from (a) spin-wave spectroscopy by Brillouin light scattering (BLS), (b) three analytical models describing the temperature dependence of magnetization obtained by magnetometry, (c) microscopic domain periodicity measurements and simulations, and (d) ab initio density functional theory (DFT) calculations. While different methods present some qualitatively consistent trends across samples, we note, for any given sample, considerable differences (up to $5\times$) in the absolute values of $A$ across the techniques, consistent with discrepancies of $A$ reported in literature for nominally similar samples. We analyze possible sources of the discrepancies across various methods, notably including their relationship to the spin-wave dispersion, and the wave-vector ranges probed. We compare the strengths and limitations of the techniques, and outline directions for their future use in characterizing exchange interactions in ultrathin films.

cond-mat.mtrl-sci↗

arXiv2023

Tailoring Zero-Field Magnetic Skyrmions in Chiral Multilayers by a Duet of Interlayer Exchange Couplings

Magnetic skyrmions have emerged as promising elements for encoding information towards biomimetic computing applications due to their pseudoparticle nature and efficient coupling to spin currents. A key hindrance for skyrmionic devices is their instability against elongation at zero magnetic field (ZF). Prevailing materials approaches focussed on tailoring skyrmion energetics have found ZF configurations to be highly sensitive, which imposes significant growth constraints and limits their device scalability. Here we propose that designer ZF skyrmion configurations can be robustly stabilized within chiral multilayer stacks by exploiting a duet of interlayer exchange couplings (IECs). Microscopic imaging experiments show that varying the two IECs enables the coarse and fine-tuning of ZF skyrmion stability and density. Micromagnetic simulations reveal that the duo-IEC approach is distinguished by its influence on the kinetics of skyrmion nucleation, in addition to the ability to tailor energetics, resulting in a substantially expanded parameter space, and enhanced stability for individual ZF skyrmions. Our work underscores the importance of IEC as a means of stabilizing and controlling ZF skyrmions, paving the way to scalable skyrmion-based devices.

cond-mat.mtrl-sci↗

arXiv2022

Chiral Spin Textures for Next-Generation Memory and Unconventional Computing

The realization of chiral spin textures - comprising myriad distinct, nanoscale arrangements of spins with topological properties - has established pathways for engineering robust, energy-efficient and scalable elements for non-volatile nanoelectronics. Particularly, current-induced manipulation of spin textures in nanowire racetracks and tunnel junction based devices are actively investigated for applications in memory, logic and unconventional computing. In this article, we paint a background on the progress of spin textures, as well as the relevant state-of-the-art techniques used for their development. In particular, we clarify the competing energy landscape of chiral spin textures, such as skyrmions and chiral domain walls, to tune their size, density and zero-field stability. Next, we discuss the spin texture phenomenology and their response to extrinsic factors arising from geometric constraints, inter-wire interactions and thermal-electrical effects. Finally, we reveal promising chiral spintronic memory and neuromorphic devices, and discuss emerging material and device engineering opportunities.

cond-mat.mtrl-sci↗

arXiv2022

Targeted Writing and Deleting of Magnetic Skyrmions in Two-Terminal Nanowire Devices

Controllable writing and deleting of nanoscale magnetic skyrmions are key requirements for their use as information carriers for next-generation memory and computing technologies. While several schemes have been proposed, they require complex fabrication techniques or precisely tailored electrical inputs, which limits their long-term scalability. Here we demonstrate an alternative approach for writing and deleting skyrmions using conventional electrical pulses within a simple, two-terminal wire geometry. X-ray microscopy experiments and micromagnetic simulations establish the observed skyrmion creation and annihilation as arising from Joule heating and Oersted field effects of the current pulses, respectively. The unique characteristics of these writing and deleting schemes, such as spatial and temporal selectivity, together with the simplicity of the 2-terminal device architecture, provide a flexible and scalable route to the viable applications of skyrmions.

cond-mat.mtrl-sci↗

arXiv2022

Unveiling the emergent traits of chiral spin textures in magnetic multilayers

Magnetic skyrmions are topologically wound nanoscale textures of spins whose ambient stability and electrical manipulation in multilayer films have led to an explosion of research activities. While past efforts focused predominantly on isolated skyrmions, recently ensembles of chiral spin textures, consisting of skyrmions and magnetic stripes, were shown to possess rich interactions with potential for device applications. However, several fundamental aspects of chiral spin texture phenomenology remain to be elucidated, including their domain wall structure, thermodynamic stability, and morphological transitions. Here we unveil the evolution of these textural characteristics on a tunable multilayer platform - wherein chiral interactions governing spin texture energetics can be widely varied - using a combination of full-field electron and soft X-ray microscopies with numerical simulations. With increasing chiral interactions, we demonstrate the emergence of Néel helicity, followed by a marked reduction in domain compressibility, and finally a transformation in the skyrmion formation mechanism. Together with an analytical model, these experiments establish a comprehensive microscopic framework for investigating and tailoring chiral spin texture character in multilayer films.

cond-mat.mes-hall↗

arXiv2022

Thermal evolution of skyrmion formation mechanism in chiral multilayer films

Magnetic skyrmions form in chiral multilayers from the shrinking or fission of elongated stripe textures. Here we report an experimental and theoretical study of the temperature dependence of this stripe-to-skyrmion transition in Co/Pt-based multilayers. Field-reversal magnetometry and Lorentz microscopy experiments over 100 - 350 K establish the increased efficacy of stripe-to-skyrmion fission at higher temperatures - driven primarily by the thermal evolution of key magnetic interactions - thereby enhancing skyrmion density. Atomistic calculations elucidate that the energy barrier to fission governs the thermodynamics of the skyrmion formation. Our results establish a mechanistic picture of the stripe-to-skyrmion transition and advance the use of thermal knobs for efficient skyrmion generation.

cond-mat.mes-hall↗

arXiv2021

Coexisting charge-ordered states with distinct driving mechanisms in monolayer VSe$_2$

Thinning crystalline materials to two dimensions (2D) creates a rich playground for electronic phases, including charge, spin, superconducting, and topological order. Bulk materials hosting charge density waves (CDWs), when reduced to ultrathin films, have shown CDW enhancement and tunability. However, charge order confined to only 2D remains elusive. Here we report a distinct charge ordered state emerging in the monolayer limit of $1T$-VSe$_2$. Systematic scanning tunneling microscopy experiments reveal that bilayer VSe$_2$ largely retains the bulk electronic structure, hosting a tri-directional CDW. However, monolayer VSe$_2$ -- consistently across distinct substrates -- exhibits a dimensional crossover, hosting two CDWs with distinct wavelengths and transition temperatures. Electronic structure calculations reveal that while one CDW is bulk-like and arises from the well-known Peierls mechanism, the other is decidedly unconventional. The observed CDW-lattice decoupling and the emergence of a flat band suggest that the new CDW could arise from enhanced electron-electron interactions in the 2D limit. These findings establish monolayer-VSe$_2$ as a host of coexisting charge orders with distinct origins, and enable the tailoring of electronic phenomena via emergent interactions in 2D materials.

cond-mat.str-el↗

arXiv2021

Intermixing Induced Anisotropy Variations in CoB-based Chiral Multilayer Films

We examine the atomic intermixing phenomenon in three distinct amorphous CoB-based multilayer thin film platforms - Pt/CoB/Ir, Ir/CoB/Pt and Pt/CoB/MgO - which are shown to stabilise room-temperature chiral magnetic textures. Intermixing occurs predominantly between adjacent metallic layers. Notably, it is stack-order dependent, and particularly extensive when Ir sits atop CoB. Intermixing induced variations in magnetic properties are ascribed to the formation of magnetic dead layer arising from CoIr alloying in the metallic stacks. It also produces systematic variations in saturation magnetization, by as much as 30%, across stacks. Crucially, the resulting crossover CoB thickness for the transition from perpendicular to in-plane magnetic anisotropy differs by more than 2x across the stacks. Finally, with thermal annealing treatment over moderate temperatures of 150-300 degree Celsius, the magnetic anisotropy increases monotonically across all stacks, coupled with discernibly larger Hc for the metallic stacks. These are attributed to thermally induced CoPt alloying and MgO crystallization in the metallic and oxide stacks, respectively. Remarkably, the CoB in the Pt/CoB/MgO stacks retains its amorphous nature after annealing. Our results set the stage for harnessing the collective attributes of amorphous CoB-based material platforms and associated annealing processes for modulating magnetic interactions, enabling the tuning of chiral magnetic texture properties in ambient conditions.

cond-mat.mtrl-sci↗

arXiv2021

Visualizing the strongly reshaped skyrmion Hall effect in multilayer wire devices

Magnetic skyrmions are nanoscale spin textures touted as next-generation computing elements. When subjected to lateral currents, skyrmions move at considerable speeds. Their topological charge results in an additional transverse deflection known as the skyrmion Hall effect (SkHE). While promising, their dynamic phenomenology with current, skyrmion size, geometric effects and disorder remain to be established. Here we report on the ensemble dynamics of individual skyrmions forming dense arrays in Pt/Co/MgO wires by examining over 20,000 instances of motion across currents and fields. The skyrmion speed reaches 24 m/s in the plastic flow regime and is surprisingly robust to positional and size variations. Meanwhile, the SkHE saturates at $\sim 22^\circ$, is substantially reshaped by the wire edge, and crucially increases weakly with skyrmion size. Particle model simulations suggest that the SkHE size dependence - contrary to analytical predictions - arises from the interplay of intrinsic and pinning-driven effects. These results establish a robust framework to harness SkHE and achieve high-throughput skyrmion motion in wire devices.

cond-mat.mes-hall↗

arXiv2021

Skyrmion generation from irreversible fission of stripes in chiral multilayer films

Competing interactions produce finite-size textures in myriad condensed matter systems, typically forming elongated stripe or round bubble domains. Transitions between stripe and bubble phases, driven by field or temperature, are expected to be reversible in nature. Here we report on the distinct character of the analogous transition for nanoscale spin textures in chiral Co/Pt-based multilayer films, known to host Néel skyrmions, using microscopy, magnetometry, and micromagnetic simulations. Upon increasing field, individual stripes fission into multiple skyrmions, and this transition exhibits a macroscopic signature of irreversibility. Crucially, upon field reversal, the skyrmions do not fuse back into stripes, with many skyrmions retaining their morphology down to zero field. Both the macroscopic irreversibility and the microscopic zero-field skyrmion density are governed by the thermodynamic material parameter determining chiral domain stability. These results establish the thermodynamic and microscopic framework underlying ambient skyrmion generation and stability in chiral multilayer films and provide immediate directions for their functionalization in devices.

cond-mat.mtrl-sci↗