arXiv subjects

Anne Juel

Publications and source records attributed to Anne Juel.

33 records · Page 2Linked to original sources

arXiv2020

Sorting of capsules according to their stiffness: from principle to application

We assess experimentally the ability of a simple flow-based sorting device, recently proposed numerically by [Zhu et al., Soft Matter, 2014, 10, 7705-7711], to separate capsules according to their stiffness. The device consists of a single pillar with a half-cylinder cross-section which partially obstructs a flow channel so that initially centred, propagating capsules deform and circumvent the obstacle into an expanding channel (or diffuser). We perform experiments with millimetric capsules of fixed size which indicate that the deviation of the capsule in the diffuser varies monotonically with a capillary number - the ratio of viscous to elastic stresses - where the elastic stresses are measured independently to include the effects of pre-inflation, membrane thickness and material properties. We find that soft capsules with resistance to deformation differing by a factor of 1.5 can be reliably separated in the diffuser but that experimental variability increases significantly with capsule stiffness. We extend the study to populations of microcapsules with size polydispersity. We find that the combined effects of increasing capsule deformability and relative constriction of the device with increasing capsule size enable the tuning of the imposed flow so that capsules can be separated based on their shear modulus but irrespectively of their size.

cond-mat.soft↗

arXiv2020

Self-assembly of coated microdroplets at the sudden expansion of a microchannel

We report observations of the self-assembly of coated droplets into regular clusters at the sudden expansion of a microfluidic channel. A double emulsion consisting of a regular train of coated microdroplets was created upstream of the channel expansion, so that the inter-drop distance, droplet length, velocity and coating thickness could be varied by imposing different inlet pressures, albeit not independently. Provided that the enlarged channel remains sufficiently confined to prohibit propagation in double file, droplets can assemble sequentially into regular linear clusters at the expansion. Droplets join a cluster via the coalescence of their coating film with that of the group ahead. This coalescence occurs when the droplets approach each other to within a critical distance at the expansion, enabled by hydrodynamic interactions within the train. Clusters comprising a finite number of droplets are obtained because reconfiguration of the droplet assembly during coalescence increases the distance to the following droplet. Decreasing the inter-drop distance increases the cluster size up to a maximum value beyond which continuous clusters form. Formalising these observations in a simple model reveals that clusters of any size are possible but that they occur for increasingly narrow ranges of parameter values. Our experimental observations suggests that background experimental fluctuations limit the maximum discrete cluster size in practice. This method of self-assembly offers a robust alternative to flow focusing for encapsulating multiple cores in a single coating film and the potential to build more complex colloidal building blocks by de-confining the clusters.

cond-mat.soft↗

arXiv2020

The engulfment of aqueous droplets on perfectly wetting oil layers

Place a droplet of mineral oil on water and the oil will spread to cover the water surface in a thin film -- a phenomenon familiar to many, owing to the rainbow-faced puddles left behind leaking buses on rainy days. In this paper we study the everted problem: an aqueous droplet deposited onto a deep layer of silicone oil. As it is energetically favourable for the oil phase to spread to cover the droplet surface completely, the droplet is ultimately engulfed in the oil layer. We present a detailed study of engulfment dynamics, from the instant the droplet first impacts the oil surface until it finally sediments into the less dense oil. We study a broad range of droplet sizes (micrometric to millimetric) and oil kinematic viscosities ($10^2$ to $10^5$ cSt), corresponding to a viscosity-dominated parameter regime with relevance to oil spills. Our investigation primarily examines droplet engulfment dynamics over two distinct stages: a rapid earlier stage in which the droplet is almost entirely submerged, driven by capillary forces in the oil surface, and cloaked by a thin layer of oil; and a much slower later stage in which gravity pulls on the drop adhered to the oil surface, thus driving a peeling flow. This means that gravitational effects are essential to complete the engulfmet of the droplet, even for micrometric droplets. We observe the longest engulfment times for droplets of intermediate size. Experiments at fixed droplet size reveal a power law dependence of engulfment time on oil kinematic viscosity.

physics.flu-dyn↗

arXiv2020

The life and fate of a bubble in a geometrically-perturbed Hele-Shaw channel

Motivated by the desire to understand complex transient behaviour in fluid flows, we study the dynamics of an air bubble driven by the steady motion of a suspending viscous fluid within a Hele-Shaw channel with a centred depth perturbation. Using both experiments and numerical simulations of a depth-averaged model, we investigate the evolution of an initially centred bubble of prescribed volume as a function of flow rate and initial shape. The experiments exhibit a rich variety of organised transient dynamics, involving bubble break up as well as aggregation and coalescence of interacting neighbouring bubbles. The long-term outcome is either a single bubble or multiple separating bubbles, positioned along the channel in order of increasing velocity. Up to moderate flow rates, the life and fate of the bubble are reproducible and can be categorised by a small number of characteristic behaviours that occur in simply-connected regions of the parameter plane. Increasing the flow rate leads to less reproducible time evolutions with increasing sensitivity to initial conditions and perturbations in the channel. Time-dependent numerical simulations that allow for break up and coalescence are found to reproduce most of the dynamical behaviour observed experimentally including enhanced sensitivity at high flow rate. An unusual feature of this system is that the set of steady and periodic solutions can change during temporal evolution because both the number of bubbles and their size distribution evolve due to break up and coalescence events. Calculation of stable and unstable solutions in the single- and two-bubble cases reveals that the transient dynamics are orchestrated by weakly-unstable solutions of the system termed edge states that can appear and disappear as the number of bubbles changes.

physics.flu-dyn↗

arXiv2019

Dynamics of front propagation in a compliant channel

Front-propagating systems provide some of the most fundamental physical examples of interfacial instability and pattern formation. However, their nonlinear dynamics are rarely addressed. Here, we present an experimental study of air displacing a viscous fluid within a collapsed, compliant channel - a model system for pulmonary airway reopening. We show that compliance induces fingering instabilities absent in the rigid channel and we present the first experimental observations of the counter-intuitive 'pushing' behaviour previously predicted numerically, for which a reduction in air pressure results in faster flow. We find that pushing modes are unstable and moreover, that the dynamics of the air-fluid front involves a host of transient finger shapes over a significant range of experimental parameters.

physics.flu-dyn↗

arXiv2019

Self-similar and disordered front propagation in a radial Hele-Shaw channel with time-varying cell depth

The displacement of a viscous fluid by an air bubble in the narrow gap between two parallel plates can readily drive complex interfacial pattern formation known as viscous fingering. We focus on a modified system suggested recently by [1], in which the onset of the fingering instability is delayed by introducing a time-dependent (power-law) plate separation. We perform a complete linear stability analysis of a depth-averaged theoretical model to show that the plate separation delays the onset of non-axisymmetric instabilities, in qualitative agreement with the predictions obtained from a simplified analysis by [1]. We then employ direct numerical simulations to show that in the parameter regime where the axisymmetrically expanding air bubble is unstable to nonaxisymmetric perturbations, the interface can evolve in a self-similar fashion such that the interface shape at a given time is simply a rescaled version of the shape at an earlier time. These novel, self-similar solutions are linearly stable but they only develop if the initially circular interface is subjected to unimodal perturbations. Conversely, the application of non-unimodal perturbations (e.g. via the superposition of multiple linearly unstable modes) leads to the development of complex, constantly evolving finger patterns similar to those that are typically observed in constant-width Hele-Shaw cells. [1] Z. Zheng, H. Kim, and H. A. Stone, Controlling viscous fingering using time-dependent strategies, Phys. Rev. Lett. 115, 174501 (2015).

nlin.PS↗

arXiv2017

Bubble propagation in Hele-Shaw channels with centred constrictions

We study the propagation of finite bubbles in a Hele-Shaw channel, where a centred occlusion (termed a rail) is introduced to provide a small axially-uniform depth constriction. For bubbles wide enough to span the channel, the system's behaviour is similar to that of semi-infinite fingers and a symmetric static solution is stable. Here, we focus on smaller bubbles, in which case the symmetric static solution is unstable and the static bubble is displaced towards one of the deeper regions of the channel on either side of the rail. Using a combination of experiments and numerical simulations of a depth-averaged model, we show that a bubble propagating axially due to a small imposed flow rate can be stabilised in a steady symmetric mode centred on the rail through a subtle interaction between stabilising viscous forces and destabilising surface tension forces. However, for sufficiently large capillary numbers Ca, the ratio of viscous to surface tension forces, viscous forces in turn become destabilising thus returning the bubble to an off-centred propagation regime. With decreasing bubble size, the range of Ca for which steady centred propagation is stable decreases, and eventually vanishes through the coalescence of two supercritical pitchfork bifurcations. The depth-averaged model is found to accurately predict all the steady modes of propagation observed experimentally, and provides a comprehensive picture of the underlying steady bifurcation structure. However, for sufficiently large imposed flow rates, we find that initially centred bubbles do not converge onto a steady mode of propagation. Instead they transiently explore weakly unstable steady modes, an evolution which results in their break-up and eventual settling into a steady propagating state of changed topology.

physics.flu-dyn↗

arXiv2017

Controlling droplet spreading with topography

We present a novel experimental system that can be used to study the dynamics of picoliter droplet spreading over substrates with topographic variations. We concentrate on spreading of a droplet within a recessed stadium-shaped pixel, with applications to the manufacture of POLED displays, and find that the sloping side wall of the pixel can either locally enhance or hinder spreading depending on whether the topography gradient ahead of the contact line is positive or negative. Locally enhanced spreading occurs via the formation of thin pointed rivulets along the side walls of the pixel through a mechanism similar to capillary rise in sharp corners. We demonstrate that a thin-film model combined with an experimentally measured spreading law, which relates the speed of the contact line to the contact angle, provides excellent predictions of the evolving liquid morphologies. We also show that the spreading can be adequately described by a Cox-Voinov law for the majority of the evolution. The model does not include viscous effects and hence, the timescales for the propagation of the thin pointed rivulets are not captured. Nonetheless, this simple model can be used very effectively to predict the areas covered by the liquid and may serve as a useful design tool for systems that require precise control of liquid on substrates.

physics.flu-dyn↗

arXiv2016

Viscous fingering and dendritic growth under an elastic membrane

We investigate the viscous fingering instability that arises when air is injected from the end of an oil-filled, compliant channel. We show that induced axial and transverse depth gradients foster novel pattern formation. Moreover, the steady propagation of the interface allows us to elucidate the nonlinear saturation of a fingering pattern first observed in a time-evolving system (Pihler-Puzovic et al. PRL 108, 074502, 2012): the wavelength is set by the viscous fingering mechanism, but the amplitude is inversely proportional to the tangent of the compliant wall's inclination angle.

physics.flu-dyn↗

arXiv2016

Reopening modes of a collapsed elasto-rigid channel

Motivated by the reopening mechanics of strongly collapsed airways, we study the steady propagation of an air finger through a collapsed oil-filled channel with a single compliant wall. In a previous study using fully-compliant elastic tubes, a `pointed' air finger was found to propagate at high speed and low pressure, which may enable rapid reopening of highly collapsed airways with minimal tissue damage (Heap & Juel 2008). In this paper, we identify the selection mechanism of that pointed finger, which remained unexplained, by conducting an experimental study in a rigid rectangular Hele-Shaw channel with an elastic top boundary. The constitutive behaviour of this elasto-rigid channel is broadly similar to that of an elastic tube, but unlike the tube the channel's cross-section adopts self-similar shapes from the undeformed state to the point of first near wall contact. The simplification of the vessel geometry enables the systematic investigation of the reopening dynamics in terms of initial collapse. We find that for low levels of initial collapse, a single centred symmetric finger propagates in the channel and its shape is set by the tip curvature. As the level of collapse increases, the channel cross-section develops a central region of near opposite wall contact, and the finger shape evolves smoothly towards a `flat-tipped' finger whose geometry is set by the strong depth gradient near the channel walls. We show that the flat-tipped mode of reopening is analogous to the pointed finger observed in tubes. Its propagation is sustained by the vessel's extreme cross-sectional profile at high collapse, while vessel compliance stabilises it. A simple scaling argument based on the dissipated power reveals that this reopening mode is preferred at higher propagation speeds when it becomes favourable to displace the elastic channel wall rather than the viscous fluid.

physics.flu-dyn↗

arXiv2013

Wrinkly fingers: the interaction between fluid- and solid-based instabilities in elastic-walled Hele-Shaw cells

In this fluid dynamics video, we study a two-phase flow in an elastic Hele-Shaw cell that involves two distinct fluid- and solid-based instabilities: viscous fingering and sheet buckling. We show that the relative importance of the two instabilities is controlled by a single non-dimensional parameter, which provides a measure of the elasticity of the flexible wall. We employ numerical simulations to show that for relatively stiff [soft] walls, the system's behaviour is dominated by viscous fingering [sheet buckling]. Strong interactions between the two instabilities arise in an intermediate regime and lead to the development of extremely complex fingering and buckling patterns.

physics.flu-dyn↗

arXiv2013

Squeezing through: capsule or bubble?

In this fluid dynamics video, we compare the deformation of two flexible particles as they propagate through a sudden constriction of a liquid filled channel under constant-flux flow: a gas bubble, and a capsule formed by encapsulating a liquid droplet in a cross-linked polymeric membrane. Both bubble and capsule adopt highly contorted configurations as they squeeze through the constriction, exhibit broadly similar features over a wide range of flow rates, and rupture for sufficiently high flow rates. However, at flow rates prior to rupture, certain features of the deformation allow bubble and capsule to be distinguished: bubbles exhibit a tip-streaming singularity associated with critical thinning of the rear of the bubble, while the capsule membrane wrinkles under large compressive stresses induced by the constriction.

physics.flu-dyn↗

arXiv2002

Fluctuations and Pinch-Offs Observed in Viscous Fingering

Our experiments on viscous (Saffman-Taylor) fingering in Hele-Shaw channels reveal several phenomena that were not observed in previous experiments. At low flow rates, growing fingers undergo width fluctuations that intermittently narrow the finger as they evolve. The magnitude of these fluctuations is proportional to Ca^{-0.64}, where Ca is the capillary number, which is proportional to the finger velocity. This relation holds for all aspect ratios studied up to the onset of tip instabilities. At higher flow rates, finger pinch-off and reconnection events are observed. These events appear to be caused by an interaction between the actively growing finger and suppressed fingers at the back of the channel. Both the fluctuation and pinch-off phenomena are robust but not explained by current theory.

cond-mat.soft↗

arXiv2001

Fluctuations in viscous fingering

Our experiments on viscous (Saffman-Taylor) fingering in Hele-Shaw channels reveal finger width fluctuations that were not observed in previous experiments, which had lower aspect ratios and higher capillary numbers Ca. These fluctuations intermittently narrow the finger from its expected width. The magnitude of these fluctuations is described by a power law, Ca^{-0.64}, which holds for all aspect ratios studied up to the onset of tip instabilities. Further, for large aspect ratios, the mean finger width exhibits a maximum as Ca is decreased instead of the predicted monotonic increase.

cond-mat.soft↗

arXiv1999

Surface tension-driven convection patterns in two liquid layers

Two superposed liquid layers display a variety of convective phenomena that are inaccessible in the traditional system where the upper layer is a gas. We consider several pairs of immiscible liquids. Once the liquids have been selected, the applied temperature difference and the depths of the layers are the only independent control parameters. Using a perfluorinated hydrocarbon and silicone oil system, we have made the first experimental observation of convection with the top plate hotter than the lower plate. Since the system is stably stratified, this convective flow is solely due to thermocapillary forces. We also have found oscillatory convection at onset in an acetonitrile and n-hexane system heated from below.

patt-sol↗