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Annica M. Black-Schaffer

Publications and source records attributed to Annica M. Black-Schaffer.

At least 37 records · Page 2Linked to original sources

Electric field controlled second-order anomalous Hall effect in altermagnets

Altermagnets are a recently discovered class of compensated magnets with momentum-dependent spin splittings and unusual transport properties, even without a net magnetization. In the presence of combined four-fold rotation and time-reversal ($C_4\mathcal{T}$) symmetry, linear and also second-order, driven by a Berry curvature dipole, anomalous Hall responses are forbidden in any pure $d$-wave altermagnet. Nevertheless, here we find that the nontrivial quantum metric of the occupied Bloch states allows for an electric field induced Berry curvature dipole, which generates a strong and tunable second-order Hall current, enabling it to be switched on or off by simply adjusting the relative orientation between the symmetry-reducing dc field and the ac probe field. Specifically, we investigate the electric field induced second-order anomalous Hall response in a two-dimensional Rashba-coupled hybrid altermagnet that interpolates between $d_{x^2-y^2}$ ($B_{1g}$) and $d_{xy}$ ($B_{2g}$) altermagnet symmetry, motivated by recent proposals for mixed-symmetry states. Crucially, the nonlinear signal is highly sensitive to the underlying symmetry of the altermagnetic order at specific doping levels, offering a purely electrical method to distinguish distinct altermagnetic orders. Our results position hybrid altermagnets as a promising platform for controllable nonlinear transport and spintronic applications.

cond-mat.mes-hall↗

Buckling and flat bands in twisted bilayer graphene

Magic-angle twisted bilayer graphene (TBG) with its flat bands provides a rich platform for exploring emergent electronic orders. Similarly, periodically buckled monolayer graphene has been proposed as a tunable alternative for realizing flat bands. Here, we investigate the combined effect of buckling and twisting in bilayer graphene. We find that periodic buckling in large-angle TBG initially enhances band flattening compared to monolayer graphene, but for sufficiently strong buckling, it instead increases the band dispersion. This occurs both because of the presence of interlayer coupling, which reduces the in-plane kinetic energy, and due to the opening of a gap at the Dirac point resulting from inversion-symmetry breaking. Additionally, we find that buckling-induced band flattening competes with twist-induced band flattening. While the former breaks sublattice symmetry, generating a sublattice polarization, the latter prefers to preserve it. This prevents buckling from generating even flatter bands at the magic angle. Nevertheless, we find that buckled TBG can exhibit flatter bands than pristine TBG over a wide range of twist angles, with a flatness similar to that of pristine magic-angle TBG.

cond-mat.mes-hall↗

Diamagnetic Meissner response of odd-frequency superconducting pairing from quantum geometry

We investigate the role of quantum geometry in the Meissner response for odd-frequency superconducting pairs in multiband systems. Odd-frequency pairing is traditionally associated with a paramagnetic Meissner response, which raises questions about the stability of the superconducting phase, especially in multiband systems where odd-frequency pairing is ubiquitous. Using analytical calculations in a general two-band, we show that the quantum geometric contribution to the Meissner response from odd-frequency pairs is always diamagnetic for its interband processes, while intraband processes always yield a paramagnetic response. With odd-frequency pairing itself generated by interband pairing, an overall diamagnetic response may often be anticipated. We confirm these results with numerical calculations of models with both flat and dispersive bands. In flat band systems, where geometric effects dominate, the diamagnetic odd-frequency response can even exceed the even-frequency contribution, making odd-frequency pairs the primary source of the diamagnetic Meissner response. In a dispersive two-band system with finite quantum geometry, we similarly find a robust diamagnetic contribution from odd-frequency pairing, even when the total response turns paramagnetic due to even-frequency contributions. These results establish that quantum geometry stabilizes odd-frequency superconductivity and also identify flat-band materials as candidates for realizing odd-frequency superconductivity with a diamagnetic Meissner effect.

cond-mat.supr-con↗

Conditions for orbital selective altermagnetism in Sr$_2$RuO$_4$: tight binding model, similarities with cuprates and implications on superconductivity

The vibrational modes in Sr$_2$RuO$_4$ easily induce octahedral rotations without tilting. Being on the verge of a magnetic instability, such propensity of octahedral rotation may also produce magnetic fluctuations. In this work, we analyze the long-range magnetic phase diagram incorporating such octahedral rotations and demonstrate the possibility of an altermagnetic phase in Sr$_2$RuO$_4$. Using ab-initio calculations, we first study single layer Sr$_2$RuO$_4$ with octahedral rotations, obtaining an orbital-selective $g$-wave altermagnetic phase. We further provide an effective $t_{2g}$ tight-binding model, demonstrating that the $g$-wave altermagnetism is primarily a product of second and third nearest neighbor interorbital hybridizations between the $γz$ ($γ=x,y$) orbitals, but only a much longer range intraorbital hybridization in the $xy$ orbitals, establishing a strong orbital-selectiveness for the altermagnetism. Notably, by replacing the $xy$ orbital with the $x^2-y^2$ orbital, a similar tight-biding model may be used to investigate the hole-doped cuprate superconductors. We then study bulk Sr$_2$RuO$_4$, where we find the altermagnetic phase as the magnetic ground state for a range of finite octahedral rotations. In the bulk, interlayer hopping breaks some of the symmetries of the $g$-wave altermagnet, resulting in a $d_{xy}$-wave altermagnet, still with orbital selectiveness. We also include relativistic effects through spin-orbit coupling and obtain that an effective staggered Dzyaloshinskii-Moriya interaction generates weak ferromagnetism. Finally, we discuss the implications of the altermagnetic order on the intrinsic superconductivity of Sr$_2$RuO$_4$. Assuming in-plane and intraorbital pairing, the altermagnetism favors spin-singlet $d_{x^2-y^2}$-wave or $g$-wave pairing, or (nematic or chiral) combinations thereof.

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Impurity strength-temperature phase diagram with phase crystals and competing time-reversal symmetry breaking states in nodal $d$-wave superconductors

Phase crystals are a class of nonuniform superconducting ground states characterized by spontaneous phase gradients of the superconducting order parameter. These phase gradients nonlocally drive periodic currents and magnetic fields, thus breaking both time-reversal symmetry and continuous translational symmetry. The phase crystal instability is generally triggered by negative and inhomogeneous superfluid stiffness. Several scenarios have been identified that can realize phase crystals, especially flat bands at specific edges of unconventional nodal superconductors. Motivated by omnipresent disorder in all materials, we employ the ${t}$-matrix approach within the quasiclassical theory of superconductivity to study the emergence of phase crystals at edges of a nodal $d$-wave superconductor. We quantify the full phase diagram as a function of the impurity scattering energy and the temperature, with full self-consistency in the impurity self energies, the superconducting order parameter, and the vector potential. We find that the phase crystal survives even up to $\sim 40-50\%$ of the superconducting critical impurity strength in both the Born and unitary scattering limits. Finally, we show how mesoscopic finite-size effects induce a competition with a state still breaking time-reversal symmetry but with translationally invariant edge currents.

cond-mat.supr-con↗

Designing edge currents using mesoscopic patterning in chiral d-wave superconductors

Chiral superconductors are topological as characterized by a finite Chern number and chiral edge modes. Direct fingerprints of chiral superconductivity are thus often taken to be spontaneous edge currents with associated magnetic signatures. However, a number of recent theoretical studies have shown that the total edge current along semi-infinite edges is greatly reduced or even vanishes in many scenarios for all pairing symmetries except chiral $p$-wave, thus impeding experimental detection. We demonstrate how mesoscopic finite-sized samples can be designed to give rise to a shape- and size-dependent strong enhancement of the chiral edge currents and their generated orbital magnetic moment and magnetic fields. In particular, we find that low rotational symmetry systems, such as pentagons and hexagons, give rise to the largest currents, while circular disks also generate large currents but in the opposite direction. We estimate the resulting magnetic fields to be as large as $0.01-0.5$ mT, with a magnetic moment approaching $μ_B/2$ per Cooper pair (Bohr magneton $μ_B$). The current and magnetic signatures diverge with shrinking system sizes, eventually cut off by finite-size suppression of chiral superconductivity. We extract the full phase diagram as a function of temperature and system size for different geometries, including competing superconducting orders. In geometries strongly suppressing only one of the $d$-wave components, we find an additional heat capacity jump, as large as $10\%$ of the bulk normal-superconducting transition, marking the transition between a chiral and a nodal $d$-wave state. This further acts as an indirect signature of chiral superconductivity. Our results are relevant for system sizes on the order of tens to hundreds of coherence lengths, and highlight mesoscopic patterning as a viable route to experimentally identify chiral $d$-wave superconductivity.

cond-mat.supr-con↗

Electric field induced second-order anomalous Hall transport in unconventional Rashba systems

Nonlinear responses in transport experiments may unveil information and generate new phenomena in materials that are not accessible at linear order due to symmetry constraints. While the linear anomalous Hall response strictly requires the absence of time-reversal symmetry, the second-order, thus nonlinear, Hall response needs broken inversion symmetry. Recently, much effort has been made to obtain a second-order Hall voltage in response to a longitudinal ac driving current, both to obtain information about band geometric quantities and for its useful technological applications, including rectification and frequency doubling. Typically, additional material engineering is required in noncentrosymmetric systems to obtain second-order responses since it obeys a stringent crystallographic symmetry constraint. To circumvent this, an alternative route is to apply a dc electric field. In this Letter, we uncover an electric field induced second-order anomalous Hall effect in inversion-broken systems possessing experimentally accessible unconventional Rashba bands. We establish that the quantum metric, a geometrical feature of electronic wave functions providing information on the nontrivial structure of Bloch bands, is responsible for providing the nonlinear Hall response

cond-mat.mes-hall↗

Local and energy-resolved topological invariants for Floquet systems

Periodically driven systems offer a perfect breeding ground for out-of-equilibrium engineering of topological boundary states at zero energy ($0$-mode), as well as finite energy ($π$-mode), with the latter having no static analog. The Floquet operator and the effective Floquet Hamiltonian, which encapsulate the stroboscopic features of the driven system, capture both spectral and localization properties of the $0$- and $π$-modes but sometimes fail to provide complete topological characterization, especially when $0$- and $π$-modes coexist. In this work, we utilize the spectral localizer, a powerful local probe that can provide numerically efficient, spatially local, and energy-resolved topological characterization. In particular, we apply the spectral localizer to the effective Floquet Hamiltonian for driven one- and two-dimensional topological systems with no or limited symmetries and are able to assign topological invariants, or local markers, that characterize the $0$- and the $π$-boundary modes individually and unambiguously. Due to the spatial resolution, we also demonstrate that the extracted topological invariants are suitable for studying driven disordered systems and can even capture disorder-induced phase transitions.

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Competing magnetic states on the surface of multilayer ABC-stacked graphene

We study interaction-mediated magnetism on the surface of ABC-multilayer graphene driven by its zero-energy topological flat bands. Using the random-phase approximation we treat onsite Hubbard repulsion and find multiple competing magnetic states, due to both intra- and inter-valley scattering, with the latter causing an enlarged magnetic unit cell. At half-filling and when the Hubbard repulsion is weak, we observe two different ferromagnetic orders. Once the Hubbard repulsion becomes more realistic, new ferrimagnetic orders arise with distinct incommensurate intra- or inter-valley scattering vectors depending on interaction strength and doping, leading to a multitude of competing magnetic states.

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Mixed higher-order topology and nodal and nodeless flat band topological phases in a superconducting multiorbital model

We investigate the topological phases that appear in an orbital version of the Benalcazar-Bernevig-Hughes (BBH) model in the presence of conventional spin-singlet $s$-wave superconductivity and with the possibility of tuning an in-plane magnetic field. We chart out the phase diagram by considering different boundary conditions, with the topology of the individual phases further examined by considering both the Wannier and entanglement spectra, as well as the Majorana polarization. For weak to moderate values of magnetic field and superconducting pairing amplitude, we find a second-order topological superconductor phase with eight zero-energy corner modes. Further increasing field or pairing, half of the corner states can be turned into zero-energy edge-localized modes, thus forming a type of hybrid-order phase. Then, we find two different putative first-order topological phases, a nodal and a nodeless phase, both with zero-energy flat bands localized along mirror-symmetric open edges. For the nodal phase, the flat bands are localized between the nodes in reciprocal space, while in the nodeless phase, with its a full bulk gap, the zero-energy boundary flat band spans the whole Brillouin zone.

cond-mat.supr-con↗

Josephson effect in a Fibonacci quasicrystal

Quasiperiodicity has recently been proposed to enhance superconductivity and its proximity effect. At the same time, there has been significant experimental progress in the fabrication of quasiperiodic structures, also in reduced dimensions. Motivated by these developments, we use microscopic tight-binding theory to investigate the DC Josephson effect through a ballistic Fibonacci chain attached to two superconducting leads. The Fibonacci chain is one of the most studied examples of quasicrystals, hosting a rich multifractal spectrum, containing topological gaps with different winding numbers. We study how the Andreev bound states (ABS), current-phase relation, and the critical current depend on the quasiperiodic degrees of freedom, from short to long junctions. While the current-phase relation shows a traditional $2π$ sinusoidal or sawtooth profile, we find that the ABS obtain quasiperiodic oscillations and that the Andreev reflection is qualitatively altered, leading to quasiperiodic oscillations in the critical current as a function of junction length. Surprisingly, despite earlier proposals of quasiperiodicity enhancing superconductivity compared to crystalline junctions, we do not in general find that it enhances the critical current. However, we find significant current enhancement for reduced interface transparency due to the modified Andreev reflection. Furthermore, by varying the chemical potential, e.g. by an applied gate voltage, we find a fractal oscillation between superconductor-normal metal-superconductor (SNS) and superconductor-insulator-superconductor (SIS) behavior. Finally, we show that the winding of the subgap states leads to an equivalent winding in the critical current, such that the winding numbers, and thus the topological invariant, can be determined.

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Perfect superconducting diode effect in altermagnets

We investigate intrinsic superconducting diode effect in the unconventional superconducting state of $d$-wave altermagnets. We find large diode efficiencies in the wide-reaching finite-momentum pairing regimes of the phase diagram. Remarkably, even perfect diode efficiency of 100% can be obtained in the presence of an external magnetic field. We attribute the largest efficiencies to competition between multiple zero-momentum (BCS) and finite-momentum superconducting states, which is connected to a topological nodal-to-nodeless transition in altermagnets with magnetic field, making our results applicable to a wide range of altermagnets.

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Constraints on superconducting pairing in altermagnets

Superconductivity in the recently discovered altermagnetic materials hosts large prospects for both fundamental physics and technological applications. In this work we show that a characteristic spin-sublattice locking in altermagnets puts severe constraints on possible superconducting pairing. In particular, we uncover that the most common form of superconductivity, uniform $s$-wave spin-singlet pairing is not possible to achieve in altermagnets. Considering an effective model for a $d_{x^2-y^2}$-wave altermagnet on a square lattice, we instead find that the most likely forms of spin-singlet pairing have $d_{x^2-y^2}$- or extended $s$-wave symmetry. We also find that the simplest form of equal-spin-triplet $p$-wave pairing is not allowed, but it can only exist as a mixed-spin-triplet $p$-wave state. We verify these constraints on pairing within an interaction-induced model of altermagnetism, where we also establish their validity for finite-momentum pairing. Additionally we discuss the possible pairing symmetries for odd-frequency superconducting pairing. Due to the generality of our results, they are applicable to both intrinsic superconductivity and proximity-induced superconductivity in altermagnet-superconductor hybrid junctions.

cond-mat.supr-con↗

Enhanced quantum metric due to vacancies in graphene

Random vacancies in a graphene monolayer induce defect states that are known to form a narrow impurity band centered around zero energy at half-filling. We use a space-resolved formulation of the quantum metric and establish a strong enhancement of the electronic correlations in this impurity band. The enhancement is primarily due to strong correlations between pairs of vacancies situated on different sublattices at anomalously large spatial distances. We trace the strong enhancement to both the multifractal vacancy wave functions, which ties the system exactly at the Anderson insulator transition for all defect concentrations, and preserving the chiral symmetry.

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Topological superconductivity in Fibonacci quasicrystals

We investigate the properties of a Fibonacci quasicrystal (QC) arrangement of a one-dimensional topological superconductor, such as a magnetic atom chain deposited on a superconducting surface. We uncover a general mutually exclusive competition between the QC properties and the topological superconducting phase with Majorana bound states (MBS): there are no MBS inside the QC gaps and the MBS never behaves as QC subgap states, and likewise, no critical, or winding, QC subgap states exist inside the topological superconducting gaps. Surprisingly, despite this competition, we find that the QC is still highly beneficial for realizing topological superconductivity with MBS. It both leads to additional large nontrivial regions with MBS in parameter space, that are topologically trivial in crystalline systems, and increases the topological gap protecting the MBS. We also find that shorter approximants of the Fibonacci QC display the largest benefits. As a consequence, our results promote QCs, and especially their short approximants, as an appealing platform for improved experimental possibilities to realize MBS as well as generally highlights the fundamental interplay between different topologies.

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Majorana zero-modes in a dissipative Rashba nanowire

Condensed matter systems are continuously subjected to dissipation, which often has adverse effects on quantum phenomena. We focus on the impact of dissipation on a superconducting Rashba nanowire. We reveal that the system can still host Majorana zero-modes (MZMs) with a finite lifetime in the presence of dissipation. Most interestingly, dissipation can also generate two kinds of dissipative boundary states: four robust zero-modes (RZMs) and two MZMs, in the regime where the non-dissipative system is topologically trivial. The MZMs appear via bulk gap closing and are topologically characterized by a winding number. The RZMs are not associated with any bulk states and possess no winding number, but their emergence is instead tied to exceptional points. Further, we confirm the stability of the dissipation-induced RZMs and MZMs in the presence of random disorder. Our study paves the way for both realizing and stabilizing MZMs in an experimental setup, driven by dissipation.

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Distinct quasiparticle interference patterns for surface impurity scattering on various Weyl semimetals

We examine the response of the Fermi arc in the context of quasi-particle interference (QPI) with regard to a localized surface impurity on various three-dimensional Weyl semimetals (WSMs). Our study also reveals the variation of the local density of states (LDOS), obtained by Fourier transforming the QPI profile, on the two-dimensional surface. We use the $T$-matrix formalism to numerically (analytically and numerically) capture the details of the momentum space scattering in QPI (real space decay in LDOS), considering relevant tight-binding lattice and/or low-energy continuum models modeling a range of different WSMs. In particular, we consider multi-WSM (mWSM), hosting multiple Fermi arcs between two opposite chirality Weyl nodes (WNs), where we find a universal $1/r$-decay ($r$ measuring the radial distance from the impurity core) of the impurity-induced LDOS, irrespective of the topological charge. Interestingly, the inter-Fermi arc scattering is only present for triple WSMs, where we find an additional $1/r^3$-decay as compared to double and single WSMs. The untilted single (double) [triple] WSM shows a straight-line (leaf-like) [oval-shaped] QPI profile. The above QPI profiles are canted for hybrid WSMs where type-I and type-II Weyl nodes coexist, however, hybrid single WSM demonstrates strong non-uniformity, unlike the hybrid double and triple WSMs. We also show that the chirality and the positions of the Weyl nodes imprint marked signatures in the QPI profile. This allows us to distinguish between different WSMs, including the time-reversal-broken WSMs from the time-reversal-invariant WSM, even though both of the WSMs can host two pairs of Weyl nodes. Our study can thus shed light on experimentally obtainable complex QPI profiles and help differentiate different WSMs and their surface band structures.

cond-mat.mes-hall↗

Zero-field finite-momentum and field-induced superconductivity in altermagnets

We explore the possibilities for spin-singlet superconductivity in newly discovered altermagnets. Investigating $d$-wave altermagnets, we show that finite-momentum superconductivity can easily emerge in altermagnets even though they have no net magnetization, when the superconducting order parameter also has $d$-wave symmetry with nodes coinciding with the altermagnet nodes. Additionally, we find a rich phase diagram when both altermagnetism and an external magnetic field are considered, including superconductivity appearing at high magnetic fields from a parent zero-field normal state.

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