arXiv subjects

Anshuman Kumar

Publications and source records attributed to Anshuman Kumar.

At least 37 records · Page 2Linked to original sources

arXiv2024

Quantum emitters in bilayer hexagonal boron nitride

Hexagonal boron nitride (hBN) has been experimentally shown to exhibit room-temperature single-photon emission. This emission is attributed to defect states in the wide band-gap of hBN, which allow new optical transitions between these dispersion-less defect levels. In this work, we study the new spectral features introduced by interacting atomic defects in consecutive layers of bilayer hBN. Density Functional theory simulations have been carried out to calculate the energy band structure, frequency-dependent complex dielectric functions, and Kohn-Sham states to demonstrate and understand the cause of the emission enhancements. We found that placing colour centres in the vicinity of each other in bilayer hBN introduces new polarization dependent spectral features, with strong dependence on the distance and relative orientation between atomic defects. Our results provide a pathway to engineering single photon emission in hBN via inter-defect interaction.

cond-mat.mtrl-sci↗

arXiv2024

Focused ion beam polishing based optimization of high-Q silica microdisk resonators

Whispering gallery mode (WGM) microdisk resonators are promising optical devices that confine light efficiently and enable enhanced nonlinear optical effects. This work presents a novel approach to reduce sidewall roughness in SiO\textsubscript{2} microdisk resonators using focused ion beam (FIB) polishing. The microdisks, with varying diameter ranging from 5 to 20 $μ$m are fabricated using a multi-step fabrication scheme. However, the etching process introduces significant sidewall roughness, which increases with decreasing microdisk radius, degrading the resonators' quality. To address this issue, a FIB system is employed to polish the sidewalls, using optimized process parameters to minimize Ga ion implantation. White light interferometry measurements reveal a significant reduction in surface roughness from 7 nm to 20 nm for a 5 $μ$m diameter microdisk, leading to a substantial enhancement in the scattering quality factor (Qss) from $3\times 10^2$ to $2\times 10^6$. These findings demonstrate the effectiveness of FIB polishing in improving the quality of microdisk resonators and open up new possibilities for the fabrication of advanced photonic devices.

physics.optics↗

arXiv2024

Twisted hyperbolic van der Waals crystals for full Stokes mid-infrared polarization detection

Investigating the polarization properties of light in the mid-infrared (mid-IR) spectrum is crucial for molecular sensing, biomedical diagnostics, and IR imaging system technologies. Traditional methods, limited by bulky size and intricate fabrication, utilize large rotating optics for full Stokes polarization detection, impeding miniaturization and accuracy. Van der Waals materials (vdW) based devices can address these challenges due to their lithography-free fabrication, ease of integration with chip-scale platforms and room-temperature operation. This study introduces a chip-integrated polarimeter device leveraging the in-plane biaxial hyperbolic vdW crystal properties for mid-infrared light manipulation. The spatial division measurement scheme incorporates six meticulously designed linear and circular polarization filters, achieving high extinction ratios exceeding 30 dB and transmittance surpassing 50%, with fabrication tolerance of film thickness up to 100 nm. The proposed device represents a significant advancement in polarimetric detection, providing a compact, cost-effective solution and opens new avenues for on-chip mid-IR polarimetric detection in next-generation ultra-compact optical systems.

physics.optics↗

arXiv2024

Deep learning-based variational autoencoder for classification of quantum and classical states of light

Advancements in optical quantum technologies have been enabled by the generation, manipulation, and characterization of light, with identification based on its photon statistics. However, characterizing light and its sources through single photon measurements often requires efficient detectors and longer measurement times to obtain high-quality photon statistics. Here we introduce a deep learning-based variational autoencoder (VAE) method for classifying single photon added coherent state (SPACS), single photon added thermal state (SPACS), mixed states between coherent/SPACS and thermal/SPATS of light. Our semisupervised learning-based VAE efficiently maps the photon statistics features of light to a lower dimension, enabling quasi-instantaneous classification with low average photon counts. The proposed VAE method is robust and maintains classification accuracy in the presence of losses inherent in an experiment, such as finite collection efficiency, non-unity quantum efficiency, finite number of detectors, etc. Additionally, leveraging the transfer learning capabilities of VAE enables successful classification of data of any quality using a single trained model. We envision that such a deep learning methodology will enable better classification of quantum light and light sources even in the presence of poor detection quality.

quant-ph↗

arXiv2024

Interplay of plasmonics and strain for Hexagonal Boron Nitride emission engineering

In the realm of quantum information and sensing, there has been substantial interest in the single-photon emission associated with defects in hexagonal boron nitride (hBN). With the goal of producing deterministic emission centers, in this work, we present a platform for engineering emission in hBN integrated with gold truncated nanocone structures. Our findings highlights that, the activation of emission is due to the truncated gold nanocones. Furthermore, we measure the quantum characteristics of this emission and find that while our system demonstrates support for single-photon emission, the origin of this emission remains ambiguous. Specifically, it is unclear whether the emission arises from defects generated by the induced strain or from alternative defect mechanisms. This uncertainty stems from the fluorescence properties inherent to gold, complicating our definitive attribution of the quantum emission source. To provide a rigorous theoretical foundation, we elucidate the effects of strain via the Kirchhoff-Love theory. Additionally, the enhancements observed due to plasmonic effects are comprehensively explained through the resolution of Maxwell's equations. This study will be useful for the development of deterministic and tunable single photonic sources in two dimensional materials and their integration with plasmonic platforms.

physics.optics↗

arXiv2024

Emission engineering in monolithically integrated silicon nitride microring resonators

Monolithic integration of solid-state color centers with photonic elements of the same material is a promising approach to overcome the constraints of fabrication complexity and coupling losses in traditional hybrid integration approaches. A wide band-gap, low-loss silicon nitride (SiN) platform is a mature technology, having CMOS compatibility, widely used in hybrid integrated photonics and optoelectronics. However, it has been shown that certain growth conditions enable the SiN material to host color centers, whose origin is currently under investigation. In this work, we have engineered a novel technique for the efficient coupling of these intrinsic emitters into the whispering gallery modes (WGMs) of the SiN microring cavity -- which has not been explored previously. We have engineered a subwavelength-sized notch into the rim of the SiN microring structure, to optimize the collection efficiency of the cavity-coupled enhanced photoluminescence (PL) spectra at room temperature. The platform presented in this work will enable the development of monolithic integration of color centers with nanophotonic elements for application to quantum photonic technologies.

cond-mat.mtrl-sci↗

arXiv2023

Exceptional point sensing via energy loss profile in a non-Hermitian system

The heightened sensitivity observed in non-Hermitian systems at exceptional points (EPs) has garnered significant attention. Typical EP sensor implementations rely on precise measurements of spectra and importantly, for real time sensing measurements, the EP condition ceases to hold as the perturbation increases over time, thereby preventing the use of high sensitivity at the EP point. In this work, we present an new approach to EP sensing which goes beyond these two traditional constraints. Firstly, instead of measuring the spectra, our scheme of EP based sensing is based on the observation of decay length of the optical mode in finite size gratings, which is validated via coupled mode theory as well as full wave electrodynamic simulations. Secondly, for larger perturbation strengths, the EP is spectrally shifted instead of being destroyed -- this spectral shift of the EP is calibrated and using this look-up table, we propose continuous real time detection by varying the excitation laser wavelength. As a proof of principle of our technique, we present an application to the sensing of coronavirus particles, which shows unprecedented limit of detection. These findings will contribute to the expanding field of exceptional point based sensing technologies for real time applications beyond spectral measurements.

physics.optics↗

arXiv2023

Accelerating Quantum Optimal Control of Multi-Qubit Systems with Symmetry-Based Hamiltonian Transformations

We present a novel, computationally efficient approach to accelerate quantum optimal control calculations of large multi-qubit systems used in a variety of quantum computing applications. By leveraging the intrinsic symmetry of finite groups, the Hilbert space can be decomposed and the Hamiltonians block-diagonalized to enable extremely fast quantum optimal control calculations. Our approach reduces the Hamiltonian size of an $n$-qubit system from 2^n by 2^n to O(n by n) or O((2^n / n) by (2^n / n)) under Sn or Dn symmetry, respectively. Most importantly, this approach reduces the computational runtime of qubit optimal control calculations by orders of magnitude while maintaining the same accuracy as the conventional method. As prospective applications, we show that (1) symmetry-protected subspaces can be potential platforms for quantum error suppression and simulation of other quantum Hamiltonians, and (2) Lie-Trotter-Suzuki decomposition approaches can generalize our method to a general variety of multi-qubit systems.

quant-ph↗

arXiv2023

Polaritons in photonic hypercrystals of van der Waals materials

In-plane Hyperbolic Phonon polaritons (HPhPs) are quasiparticles formed via coupling of photons and optical phonons in in-plane hyperbolic materials and offer unique applications in sensing, thermal emitters and high resolution imaging. However, the large momentum mismatch between photons and these in-plane HPhPs has restricted their technological potential as most experimental demonstration rely on sophisticated and expensive near field detection schemes. In this work, using the example of $α-$MoO$_3$, we demonstrate that by constructing photonic hypercrystals of this material, one can not only excite these in-plane HPhPs in the far field but also tune the far field response via twisting the hypercrystal lattice with respect the lattice of $α-$MoO$_3$. Our findings will pave the way for the development of practical in-plane HPhP devices as well as provide access to new fundamental physics of such materials via conventional and well developed far field measurement techniques.

physics.optics↗

arXiv2023

An electroplating-based plasmonic platform for giant emission enhancement in monolayer semiconductors

Two dimensional semiconductors have attracted considerable attention owing to their exceptional electronic and optical characteristics. However, their practical application has been hindered by the limited light absorption resulting from their atomically thin thickness and low quantum yield. A highly effective approach to manipulate optical properties and address these limitations is integrating subwavelength plasmonic nanostructures with these monolayers. In this study, we employed electron beam lithography and electroplating technique to fabricate a gold nanodisc (AuND) array capable of enhancing the photoluminescence (PL) of monolayer MoS$_2$ giantly. Monolayer MoS$_2$ placed on the top of the AuND array yields up to 150-fold PL enhancement compared to that on a gold film. We explain our experimental findings based on electromagnetic simulations.

physics.optics↗

arXiv2022

A universal and stable metasurface for photonic quasi bound state in continuum coupled with two dimensional semiconductors

Strong coupling of excitons to optical cavity modes is of immense importance to understanding the fundamental physics of quantum electrodynamics at the nanoscale as well as for practical applications in quantum information technologies. There have been several attempts at achieving strong coupling between excitons in two dimensional semiconductors such as transition metal dichalcogenides (TMDCs) and photonic quasi-bound states in the continuum (BICs). We identify two gaps in the platforms for achieving strong coupling between TMDC excitons and photonic quasi-BICs: firstly, in the studies so far, different cavity architectures have been employed for coupling to different TMDCs. This would mean that typically, the fabrication process flow for the cavities will need to be modified as one moves from one TMDC to the other, which can limit the technological progress in the field. Secondly, there has been no discussion of the impact of fabrication imperfections in the studies on strong coupling of these subsystems so far. In this work, we address these two questions by optimizing a cavity with the same architecture which can couple to the four typical TMDCs (MoS$_2$, WS$_2$, MoSe$_2$, WSe$_2$) and perform a detailed investigation on the fabrication tolerance of the associated photonic quasi-BICs and their impact on strong coupling.

physics.optics↗

arXiv2022

Electroplating based engineering of plasmonic nanorod metamaterials for biosensing applications

Sensing lower molecular weight in a diluted solution using a label-free biosensor is challenging and requires a miniaturized plasmonic structure, e.g., a vertical Au nanorod (AuNR) array based metamaterials. The sensitivity of a sensor mainly depends on transducer properties and hence for instance, the AuNR array geometry requires optimization. Physical vapour deposition methods (e.g., sputtering and e-beam evaporation) require a vacuum environment to deposit Au, which is costly, time-consuming, and thickness-limited. On the other hand, chemical deposition, i.e., electroplating deposit higher thickness in less time and at lower cost, becomes an alternative method for Au deposition. In this work, we present a detailed optimization for electroplating based fabrication of these metamaterials. We find that slightly acidic (6.0 < pH < 7.0) gold sulfite solution supports immersion deposition, which should be minimized to avoid uncontrolled Au deposition. Immersion deposition leads to plate-like (for smaller radius AuNR) or capped-like, i.e., mushroom (for higher radius AuNR) structure formation. The electroplating time and DC supply are the tuning parameters that decide the geometry of the vertically aligned AuNR array in area-dependent electroplating deposition. This work will have implications for developing plasmonic metamaterial based sensors.

physics.app-ph↗

arXiv2022

A low cost plasmonic platform for photon emission engineering of two dimensional semiconductors

Although the field of 2D materials has democratized materials science by making high quality samples accessible cheaply, due to the atomically thin nature of these systems, an integration with nanostructures is almost always required to obtain a significant optical response. Traditionally, these nanostructures are fabricated via electron beam lithography or focused ion beam milling, which are expensive and large area fabrication can be further time consuming. In order to overcome this problem, we report the integration of 2D semiconductors on a cost-effective and large area fabricated nanocone platform. We show that the plasmon modes of our nanocone structures lead to photoluminescence (PL) enhancement of monolayer WSe$_2$ by about eight to ten times compared to the non-plasmonic case, consistent with finite-difference time-domain simulations. Excitation power-dependent measurements reveal that our nanocone platform enables a versatile route to engineering the relative exciton trion contributions to the emission.

physics.optics↗

arXiv2022

A photonic integrated chip platform for interlayer exciton valley routing

Interlayer excitons in two dimensional semiconductor heterostructures show suppressed electron-hole overlap resulting in longer radiative lifetimes as compared to intralyer excitons. Such tightly bound interlayer excitons are relevant for important optoelectronic applications including light storage and quantum communication. Their optical accessibility is, however, limited due to their out-of-plane transition dipole moment. In this work, we design a CMOS compatible photonic integrated chip platform for enhanced near field coupling of these interlayer excitons with the whispering gallery modes of a microresonator, exploiting the high confinement of light in a small modal volume and high quality factor of the system. Our platform allows for highly selective emission routing via engineering an asymmetric light transmission which facilitates efficient readout and channeling of the excitonic valley state from such systems.

physics.optics↗

arXiv2022

Gate tunable light-matter interaction in natural biaxial hyperbolic van der Waals heterostructures

The recent discovery of natural biaxial hyperbolicity in van der Waals crystals, such as $α$-MoO$_3$, has opened up new avenues for mid-IR nanophotonics due to their deep subwavelength phonon-polaritons. However, a significant challenge is the lack of active tunability of these hyperbolic phonon polaritons. In this work, we investigate heterostructures of graphene and $α$-MoO$_3$ for actively tunable hybrid plasmon phonon polariton modes via electrostatic gating in the mid-infrared spectral region. We observe a unique propagation direction dependent hybridization of graphene plasmon polaritons with hyperbolic phonon polaritons for experimentally feasible values of graphene chemical potential. We further report an application to tunable valley quantum interference in this system with a broad operational bandwidth due to the formation of these hybrid modes. This work presents a lithography-free alternative for actively tunable, anisotropic spontaneous emission enhancement using a sub-wavelength thick naturally biaxial hyperbolic materials.

physics.optics↗

arXiv2021

Terahertz Nonlinear Optics in Two-dimensional Semi-Hydrogenated SiB

Phase transition and current of planar clusters with loops of Josephson $π$ junction is of great importance for application in the adiabatic quantum computation devices (AQC). Each $π$-ring possesses an orbital moment with a current. The orientation of these orbital moments is altered by self-interactions and controlled with a bias current. In the current research, we construct the phase diagram of semi-hydrogenated SiB (H-SiB) semiconductor using a two-dimensional (2D) Ising model with considering nearest-neighbor and diagonal interactions of spin planes on the on the hexagonal lattice. Our findings reveal that by decreasing temperature, two phase transitions of order and disorder occur and at low temperatures a glassy state appears, where this model maps to spin qubit. We theoretically study the magnetostriction effect by considering of laser electromagnetic field coupled to the spin planes of electric polarization of magnetic insulator for both unstrained and strained H-SiB monolayers. The dynamic of laser-spin coupling and spin current shows nonlinear optical effects and high-harmonic generation (HHG) under both terahertz (THz) and gigahertz (GHz) electromagnetic waves. The findings of this research open an avenue for experimentalists how to detect HHG in the topological insulators, Dirac systems, Mott insulators, and superconducting memories.

cond-mat.mes-hall↗

arXiv2021

Engineering Purcell factor anisotropy for dark and bright excitons in two dimensional semiconductors

Tightly bound dark excitons in atomically thin semiconductors can be used for various optoelectronic applications including light storage and quantum communication. Their optical accessibility is however limited due to their out-of-plane transition dipole moment. We thus propose to strengthen the coupling of dark excitons in two dimensional materials with out-of-plane resonant modes of a cavity at room temperature, by engineering the anisotropy in the Purcell factor. A silica micro-disk characterised by high confinement of light in small modal volume, high Q-factor and free spectral range is used to couple to the excitons in monolayer transition metal dichalcogenides. We show numerically that the tapering of sidewalls of the micro-disk is an extremely versatile route for achieving the selective coupling of whispering gallery modes to light emitted from out-of-plane dipoles to the detriment of that from in-plane ones for four representative monolayer transition metal dichalcogenides.

physics.optics↗

arXiv2021

High temperature mid-IR polarizer via natural in-plane hyperbolic Van der Waals crystals

Integration of conventional mid to long-wavelength infrared polarizers with chip-scale platforms is restricted by their bulky size and complex fabrication. Van der Waals materials based polarizer can address these challenges due to its non-lithographic fabrication, ease of integration with chip-scale platforms, and room temperature operation. In the present work, mid-IR optical response of the sub-wavelength thin films of $α$-MoO$_3$ is investigated for application towards high temperature mid-IR transmission and reflection type thin film polarizer. To our knowledge, this is the first report of above room temperature mid-IR optical response of $α$-MoO$_3$ to determine the thermal stability of the proposed device. We find that our $α$-MoO$_3$ based polarizer retains high extinction ratio with peak value exceeding 10 dB, up to a temperature of 140$^{\circ}$C. We explain our experimental findings by natural in-plane hyperbolic anisotropy of $α$-MoO$_3$ in the mid-IR, high temperature X-ray diffraction and Raman spectroscopic measurements. This work opens up new avenues for naturally in-plane hyperbolic van der Waals thin-films to realize sub-wavelength IR optical components without lithographic constraints.

cond-mat.mtrl-sci↗