SearcharxivSearch

arXiv subjects

Anthony J. Bennett

Publications and source records attributed to Anthony J. Bennett.

At least 19 recordsLinked to original sources

High-sensitivity silicon nitride microring resonator opto-fluidic sensor

Photonic integrated circuit devices can be used as refractometric opto-fluidic sensors to detect the presence of analytes in solution at low concentrations. In this work, we investigate the refractive index sensitivity of silicon nitride microring resonator based photonic integrated circuit fluidic sensors. The performance of a foundry fabricated sensor is measured over the C-band in the presence of liquid samples achieving a mean sensitivity of 579 nanometres per refractive index unit. This demonstration of a scalable, high-sensitivity opto-fluidic sensor, compatible with recognition marker surface functionalisation, opens the way to applications in environmental and bio-sensing.

physics.optics

The origin and influence of non-cavity modes in a micropillar Bragg microcavity

Controlling the photonic environment of emitters is essential to the design of classical and quantum light sources. We study the case of a dipole-like emitter in a cylindrical pillar etched into a planar Bragg microcavity, which is a common design of quantum-dot single photon source. In addition to the well-known cavity modes created by the high-reflectivity of the Bragg mirrors at small in-plane wavevectors, we show the presence of broad spectral features that play a key role in controlling photon collection efficiency and Purcell enhancement. These non-cavity modes are insensitive to the periodic index modulation of the Bragg reflectors, but arise from the cylindrical pillar geometry, as we show by comparison with simulations of uniform pillars, which reproduce the non-cavity modes. This approach provides a tool for understanding and modelling these often-disregarded decay channels as a function of source height, cavity dimensions and surface layers.

physics.optics

Controlled epitaxy of room-temperature quantum emitters in gallium nitride

The ability to generate quantum light at room temperature on a mature semiconductor platform opens up new possibilities for quantum technologies. Heteroepitaxial growth of gallium nitride on silicon substrates offers the opportunity to leverage existing expertise and wafer-scale manufacturing to integrate bright quantum emitters in this material within cavities, diodes, and photonic circuits. Until now, it has only been possible to grow GaN QEs at uncontrolled depths on sapphire substrates, which is disadvantageous for potential device architectures. Here, we report a method to produce GaN QEs by metal-organic vapor phase epitaxy at a controlled depth in the crystal through the application of silane treatment and subsequent growth of 3D islands. We demonstrate this process on highly technologically relevant silicon substrates, producing room-temperature QEs with a high Debye Waller factor and strongly anti-bunched emission.

cond-mat.mtrl-sci

Tunable multi-photon correlations from a coherently driven quantum dot

Mixing the fields generated by different light sources has emerged as a powerful approach for engineering non-Gaussian quantum states. Understanding and controlling the resulting photon statistics is useful for emerging quantum technologies that are underpinned by interference. In this work, we investigate intensity correlation functions arising from the interference of resonance fluorescence from a quantum emitter with a coherent laser field. We show that the observed bunching behavior results from a subtle interplay between quantum interference and the normalization of the correlation functions. We show that by adjusting the mixing ratio and phase one can achieve full tunability of the second-order correlation, ranging from anti-bunching to bunching. We further extend our analysis to third-order correlation functions, both experimentally and theoretically, to provide new insights into the interpretation of higher-order correlations and offer practical tools for shaping quantum optical fields.

quant-ph

Femtosecond laser-written nano-ablations containing bright antibunched emitters on gallium nitride

Femtosecond laser-writing offers distinct capabilities for fabrication, including three-dimensional, multi-material, and sub-diffraction-limited patterning. In particular, demonstrations of laser-written quantum emitters and photonic devices with superior optical properties have attracted attention. Recently, gallium nitride (GaN) has been reported to host quantum emitters with narrow and bright zero-phonon photoluminescence from ultraviolet to telecom ranges. However, emitters formed during epitaxy are randomly positioned, and until now, it has not been possible to fabricate quantum emitters in ordered arrays. In this paper, we employ femtosecond laser writing to create nano-ablations with sub-diffraction-limited diameter, and use rapid thermal annealing to activate co-located stable emitters. The emitters show MHz antibunched emission with a sharp spectral peak at room temperature. Our study not only presents an efficient approach to laser-written nanofabrication on GaN but also offers a promising pathway for the deterministic creation of quantum emitters in GaN, shedding light on the underlying mechanisms involved.

physics.optics

Enhanced quantum magnetometry with a laser-written integrated photonic diamond chip

An ensemble of negatively charged nitrogen-vacancy centers in diamond can act as a precise quantum sensor even under ambient conditions. In particular, to optimize thier sensitivity, it is crucial to increase the number of spins sampled and maximize their coupling to the detection system, without degrading their spin properties. In this paper, we demonstrate enhanced quantum magnetometry via a high-quality buried laser-written waveguide in diamond with a 4.5 ppm density of nitrogen-vacancy centers. We show that the waveguide-coupled nitrogen-vacancy centers exhibit comparable spin coherence properties as that of nitrogen-vacancy centers in pristine diamond using time-domain optically detected magnetic resonance spectroscopy. Waveguide-enhanced magnetic field sensing is demonstrated in a fiber-coupled integrated photonic chip, where probing an increased volume of high-density spins results in 63 pT$.$Hz $^{-1/2}$ of DC-magnetic field sensitivity and 20 pT$.$Hz $^{-1/2}$ of AC magnetic field sensitivity. This on-chip sensor realizes at least an order of magnitude improvement in sensitivity compared to the conventional confocal detection setup, paving the way for microscale sensing with nitrogen-vacancy ensembles.

quant-ph

Measuring photon correlation using imperfect detectors

Single-photon detectors are ``blind" after the detection of a photon, and thereafter display a characteristic recovery in efficiency, during which the number of undetected photons depends on the statistics of the incident light. We show how the efficiency-recovery, photon statistics and intensity have an interdependent relationship which suppresses a detector's ability to count photons and measure correlations. We also demonstrate this effect with an experiment using $n$ such detectors to determine the $n^{\mathrm{th}}$ order correlation function with pseudothermal light.

quant-ph

Determining Strain Components in a Diamond Waveguide from Zero-Field ODMR Spectra of NV$^{-}$ Center Ensembles

The negatively charged nitrogen-vacancy (NV$^{-}$) center in diamond has shown great potential in nanoscale sensing and quantum information processing due to its rich spin physics. An efficient coupling with light, providing strong luminescence, is crucial for realizing these applications. Laser-written waveguides in diamond promote NV$^{-}$ creation and improve their coupling to light but, at the same time, induce strain in the crystal. The induced strain contributes to light guiding but also affects the energy levels of NV$^{-}$ centers. We probe NV$^{-}$ spin states experimentally with the commonly used continuous-wave zero-field optically detected magnetic resonance (ODMR). In our waveguides, the ODMR spectra are shifted, split, and consistently asymmetric, which we attribute to the impact of local strain. To understand these features, we model ensemble ODMR signals in the presence of strain. By fitting the model results to the experimentally collected ODMR data, we determine the strain tensor components at different positions, thus determining the strain profile across the waveguide. This shows that zero-field ODMR spectroscopy can be used as a strain imaging tool. The resulting strain within the waveguide is dominated by a compressive axial component transverse to the waveguide structure, with a smaller contribution from vertical and shear strain components.

cond-mat.mes-hall

Vector Magnetometry Using Shallow Implanted NV Centers in Diamond with Waveguide-Assisted Dipole Excitation and Readout

On-chip magnetic field sensing with Nitrogen-Vacancy (NV) centers in diamond requires scalable integration of 3D waveguides into diamond substrates. Here, we develop a sensing array device with an ensemble of shallow implanted NV centers integrated with arrays of laser-written waveguides for excitation and readout of NV signals. Our approach enables an easy-to-operate on-chip magnetometer with a pixel size proportional to the Gaussian mode area of each waveguide. The performed continuous wave optically detected magnetic resonance on each waveguide gives an average dc-sensitivity value of $195 \pm 3 {nT}/\sqrt{Hz}$, which can be improved with lock-in-detection or pulsed-microwave sequences. We apply a magnetic field to separate the four NV crystallographic orientations of the magnetic resonance and then utilize a DC current through a straight wire antenna close to the waveguide to prove the sensor capabilities of our device. We reconstruct the complete vector magnetic field in the NV crystal frame using three different NV crystallographic orientations. By knowing the polarization axis of the waveguide mode, we project the magnetic field vector into the lab frame.

quant-ph

Laser-written waveguide-integrated coherent spins in diamond

Quantum emitters, such as the negatively charged nitrogen-vacancy center in diamond, are attractive for quantum technologies such as nano-sensing, quantum information processing, and as a non-classical light source. However, it is still challenging to position individual emitters in photonic structures whilst preserving the spin coherence properties of the defect. In this paper, we investigate single and ensemble waveguide-integrated nitrogen-vacancy centers in diamond fabricated by femtosecond laser writing followed by thermal annealing. Their spin coherence properties are systematically investigated and are shown to be comparable to native nitrogen-vacancy centers in diamond. This method paves the way for the fabrication of coherent spins integrated within photonic devices.

quant-ph

Probing Purcell enhancement and photon collection efficiency of InAs quantum dots at nodes of the cavity electric field

The interaction of excitonic transitions with confined photonic modes enables tests of quantum physics and design of efficient optoelectronic devices. Here we study how key metrics such as Purcell factor, beta-factor and collection efficiency are determined by the non-cavity modes which exist in real devices, taking the well-studied micropillar cavity as an example. Samples with dots at different positions in the cavity field allow us to quantify the effect of the non-cavity modes and show that the zero-phonon line and the phonon-assisted emission into the cavity mode HE11 is suppressed by positioning dots at the field node.

cond-mat.mes-hall

Photo-dynamics of quantum emitters in aluminum nitride

Aluminum nitride is a technologically important wide bandgap semiconductor which has been shown to host bright quantum emitters. In this paper, we probe the photodynamics of quantum emitters in aluminum nitride using photon emission correlations and time-resolved spectroscopy. We identify that each emitter contains as many as 6 internal energy levels with distinct laser power-dependent behaviors. Power-dependent shelving and de-shelving processes, such as optically induced ionization and recombination are considered, indicating complex optical dynamics associated with the spontaneous and optically pumped transitions. State population dynamics simulations qualitatively explain the temporal behaviours of the quantum emitters, revealing that those with pump-dependent de-shelving processes can saturate at significantly higher intensities, resulting in bright room-temperature quantum light emission.

physics.optics

Direct-write projection lithography of quantum dot micropillar single photon sources

We have developed a process to mass-produce quantum dot micropillar cavities using direct-write lithography. This technique allows us to achieve high volume patterning of high aspect ratio pillars with vertical, smooth sidewalls maintaining a high quality factor for diameters below 2.0 $μ$m. Encapsulating the cavities in a thin layer of oxide (Ta$_2$O$_5$) prevents oxidation in the atmosphere, preserving the optical properties of the cavity over months of ambient exposure. We confirm that single dots in the cavities can be deterministically excited to create high purity indistinguishable single photons with interference visibility $(96.2\pm0.7)\%$.

physics.app-ph

Bullseye dielectric cavities for photon collection from a surface-mounted quantum-light-emitter

Coupling light from a point source to a propagating mode is an important problem in nano-photonics and is essential for many applications in quantum optics. Circular "bullseye" cavities, consisting of concentric rings of alternating refractive index, are a promising technology that can achieve near-unity coupling into a first lens. Here we design a bullseye structure suitable for enhancing the emission from dye molecules, 2D materials and nano-diamonds positioned on the surface of these cavities. A periodic design of cavity, meeting the Bragg scattering condition, achieves a Purcell factor of 22.5 and collection efficiency of 80 %. We also tackle the more challenging task of designing a cavity for coupling to a low numerical aperture fibre in the near field. Using an iterative procedure, we show that apodized (non-periodic) rings can achieve a collection efficiency that exceeds the periodic Bragg cavity.

physics.optics

Room-Temperature Quantum Emitter in Aluminum Nitride

A device that is able to produce single photons is a fundamental building block for a number of quantum technologies. Significant progress has been made in engineering quantum emission in the solid state, for instance, using semiconductor quantum dots as well as defect sites in bulk and two-dimensional materials. Here we report the discovery of a room-temperature quantum emitter embedded deep within the band gap of aluminum nitride. Using spectral, polarization, and photon-counting time-resolved measurements we demonstrate bright ($>10^5$ counts per second), pure ($g^{(2)}(0) < 0.2$), and polarized room-temperature quantum light emission from color centers in this commercially important semiconductor.

physics.app-ph

Design of free-space couplers for suspended triangular nano-beam waveguides

Photonic waveguides with triangular cross section are being investigated for material systems such as diamond, glasses and gallium nitride, which lack easy options to create conventional rectangular nanophotonic waveguides. The design rules for optical elements in these triangular waveguides, such as couplers and gratings, are not well established. Here we present simulations of elements designed to couple light into, and out of, triangular waveguides from the vertical direction, which can be implemented with current angled-etch fabrication technology. The devices demonstrate coupling efficiencies approaching \unit{50}{\%} for light focused from a high numerical aperture objective. The implementation of such couplers will enable fast and efficient testing of closely spaced integrated circuit components.

physics.optics

Room temperature coherent control of protected qubit in hexagonal boron nitride

Spin defects in foils of hexagonal boron nitride are an attractive platform for magnetic field imaging, since the probe can be placed in close proximity to the target. However, as a III-V material the electron spin coherence is limited by the nuclear spin environment, with spin echo coherence time of $\sim100~\mathrm{ns}$ at room temperature accessible magnetic fields. We use a strong continuous microwave drive with a modulation in order to stabilize a Rabi oscillation, extending the coherence time up to $\sim4~\mathrm{μs}$, which is close to the 10-$\mathrm{μs}$ electron spin lifetime in our sample. We then define a protected qubit basis, and show full control of the protected qubit. The coherence times of a superposition of the protected qubit can be as high as $0.8~\mathrm{μs}$. This work establishes that boron vacancies in hexagonal boron nitride can have electron spin coherence times that are competitive with typical NV-centers in small nanodiamonds under ambient conditions.

cond-mat.mtrl-sci

Two-Photon Interference of Single Photons from Dissimilar Sources

Entanglement swapping and heralding are at the heart of many protocols for distributed quantum information. For photons, this typically involves Bell state measurements based on two-photon interference effects. In this context, hybrid systems that combine high rate, ultra-stable and pure quantum sources with long-lived quantum memories are particularly interesting. Here, we develop a theoretical description of pulsed two-photon interference of photons from dissimilar sources to predict the outcomes of second-order cross-correlation measurements. These are directly related to, and hence used to quantify, photon indistinguishability. We study their dependence on critical system parameters such as quantum state lifetime and frequency detuning, and quantify the impact of emission time jitter, pure dephasing and spectral wandering. Our results show that for fixed lifetime of emitter one, for each frequency detuning there is an optimal lifetime of emitter two that leads to highest photon indistinguishability. Expectations for different hybrid combinations involving III-V quantum dots, color centers in diamond, 2D materials and atoms are quantitatively compared for real-world system parameters. Our work both provides a theoretical basis for the treatment of dissimilar emitters and enables assessment of which imperfections can be tolerated in hybrid photonic quantum networks.

quant-ph