arXiv subjects

Antoine Riaud

Publications and source records attributed to Antoine Riaud.

At least 19 recordsLinked to original sources

arXiv2024

Implementation of two-dimensional selective acoustic tweezers merely using four straight interdigitated transducers:a numerical proof of concept of radiation field synthesis by pulsed acoustic waves

Selective acoustic tweezers can focus the acoustic radiation force on a single particle to manipulate it without affecting its neighbors. This has long required highly complex hardware. In this numerical study, we show that pulsed acoustic waves can be used for the selective manipulation of particles using only two pairs of orthogonal transducers. While these tweezers are well-known for their ability to manipulate arrays of particles, we show that selectivity can be achieved by using sequences of acoustic pulses to iteratively construct a combined acoustic potential focused only on the target particle.

physics.flu-dyn↗

arXiv2023

Numerical simulation of the radiation force from transient acoustic fields: Application to laser-guided acoustic tweezers

Using pulsed acoustic waves could provide a superior selectivity for microscale acoustic tweezers. However, the theory for the radiation force of pulsed acoustic waves has only been recently derived and no numerical implementations are available. In this paper, we present a finite-element implementation of this model to simulate the transient acoustic radiation force on small spheres. We use the model to simulate laser-guided acoustic tweezers and optimize their performance. By enabling numerical simulations of the transient radiation force, this work may accelerate the rational design of pulse-based high-selectivity acoustic tweezers devices.

physics.flu-dyn↗

arXiv2022

Skipping the boundary layer: high-speed droplet-based immunoassay using Rayleigh acoustic streaming

Acoustic mixing of droplets is a promising way to implement biosensors that combine high speed and minimal reagent consumption. To date, this type of droplet mixing is driven by a volume force resulting from the absorption of high-frequency acoustic waves in the bulk of the fluid. Here, we show that the speed of these sensors is limited by the slow advection of analyte to the sensor surface due to the formation of a hydrodynamic boundary layer. We eliminate this hydrodynamic boundary layer by using much lower ultrasonic frequencies to excite the droplet, which drives a Rayleigh streaming that behaves essentially like a slip velocity. Three-dimensional simulations show that this provides a threefold speedup compared to Eckart streaming. Experimentally, we shorten a SARS-CoV-2 antibody immunoassay from 20 min to 40 s.

physics.flu-dyn↗

arXiv2022

Effect of viscosity on surface acoustic wave driven collective particle dynamics in sessile droplets: nebula, black holes and white dwarfs

Surface acoustic waves (SAW) can concentrate micro-particles in droplets within seconds. Yet, the mechanism is not clear and existing explanations fail by several orders of magnitude. In this paper, we analyze the effect of fluid viscosity and particle size on SAW-driven collective particle dynamics in droplets. In most of our experiments, the particles do not aggregate but instead remain away from the droplet center, thereby forming "black holes". We show that the black holes are due to steric hindrance wherein the poloidal streamlines that should drive particles to the center of the droplet come too close to the solid, so that the particles carried along these streamlines touch the solid wall on the edge of the black hole before reaching the center of the droplet. The size of these black holes is correlated with the size of the aggregates formed in less viscous droplets. This suggests a common formation mechanism for black holes and white dwarfs (aggregates). In the former, the particles touching the solid would be washed away by the fluid, whereas in the latter the particles would remain in contact with the solid and roll to the center of the droplet where an aggregate is formed. We also discuss the stability conditions of the aggregate at the bottom of the droplet. The concept of hydrodynamic shielding is then used to concentrate 1 $μ$m particles using 10 $μ$m beads as shields.

physics.flu-dyn↗

arXiv2022

Laser-guided acoustic tweezers

Acoustic tweezers can manipulate microscopic objects and cells independently of the optical, magnetic and electrical properties of the objects or their medium. However, because ultrasonic waves are attenuated within few millimeters, existing devices must synthesize intricate and powerful acoustic fields in a very narrow footprint immediately close to the manipulated object. Here we show that the design of microscale acoustic tweezers can be considerably simplified by taking advantage of the nonlinear nature of the acoustic trapping force. In our experiment, a featureless piezoelectric crystal coated with a photoacoustic conversion layer is hit by an electric pulse and a spatially modulated laser pulse to generate synchronized electro- and photo- acoustic waves. Interference between these waves creates a hybrid acoustic trapping force 30 times stronger than the laser pulse alone but with the same spatial information. By disentangling the tradeoff between spatial resolution and trapping force that has long held back the development of acoustic tweezers, this field hybridization strategy opens new avenues for cell manipulation in organ on chip and organ printing.

physics.flu-dyn↗

arXiv2021

Contactless generation and trapping of hydrodynamic knots in sessile droplets by acoustic screw dislocations

Hydrodynamics knots are not only promising elementary structures to study mass and momentum transfer in turbulent flows, but also potent analogs for other topological problems arising in particle physics. However, experimental studies of knots are highly challenging due to the limited control over knot generation and difficult observation of the resulting fast-paced multiscale flow evolution. In this paper, we propose using acoustic streaming to tie hydrodynamic knots in fluids. The method is contactless, almost instantaneous and is relatively insensitive to viscosity. Importantly, it allows starting from quite arbitrary three dimensional flow structures without relying on external boundary conditions. We demonstrate our approach by using an acoustic screw dislocation to tie a knot in a sessile droplet. We observe an inversion of the knot chirality (measured by the hydrodynamic helicity) as the topological charge of the screw dislocation is increased. Combined with recent progress in acoustic field synthesis, this work opens a window to study more complex hydrodynamic knot topologies at a broader range of space and timescales.

physics.flu-dyn↗

arXiv2020

Hydrodynamic constraints on the energy efficiency of droplet electricity generators

Electric energy generation from falling droplets has seen a hundred-fold rise in efficiency over the past year. However, even these newest devices can only extract a small portion of the droplet energy. In this paper, we theoretically investigate the contributions of hydrodynamic and electric losses in limiting the efficiency of droplet electricity generators (DEG). Noting that the electro-mechanical energy conversion occurs during the recoil that immediately follows droplet impact, we identify three limits on existing droplet electric generators: (i) the impingement velocity is limited in order to maintain the droplet integrity; (ii) much of droplet mechanical energy is squandered in overcoming viscous shear force with the substrate; (iii) insufficient electrical charge of the substrate. Of all these effects, we found that up to 83% of the total energy available was lost by viscous dissipation during spreading. Minimizing this loss by using cascaded DEG devices to reduce the droplet kinetic energy may increase future devices efficiency beyond 10%.

physics.flu-dyn↗

arXiv2020

Acoustic radiation force on small spheres due to transient acoustic fields

Acoustic radiation force is a net force experienced by an object under the action of an acoustic wave. Most theoretical models require the acoustic wave to be periodic, if not purely monofrequency, and are therefore irrelevant for the study of acoustic radiation force due to acoustic pulses. Here, we introduce the concept of finite-duration pulses, which is the most general condition to derive the acoustic radiation force. In the case of small spheres, we extend the Gor'kov to formula to unsteady acoustic fields such as traveling pulses and interfering wave packets. In the latter case, our study suggests that the concept of acoustic contrast is also relevant to express the acoustic radiation force. For negative acoustic contrast particles, the acoustic trapping region narrows with shorter pulses, whereas positive contrast particles (such as biological cells) can fall in secondary traps when the pulse width deviates from an optimal value. This theoretical insight may help to improve the selectivity of pulsed acoustic tweezers.

physics.flu-dyn↗

arXiv2020

Observation of contact angle hysteresis due to inhomogeneous electric fields

Static contact angle hysteresis (CAH) is widely attributed to surface roughness and chemical contamination. In the latter case, chemical defects create free-energy barriers that prevent the contact line motion. Electrowetting studies have demonstrated the similar ability of electric fields to alter the surface free-energy landscape. Yet, the increase of apparent static CAH by electric fields remains unseen. Here, we report the observation and theoretical analysis of electrowetting hysteresis. This phenomenon enables the continuous and dynamic control of CAH, not only for fundamental studies but also to manufacture sticky-on-demand surfaces for sample collection.

physics.flu-dyn↗

arXiv2019

High-Performance Logic and Memory Devices Based on a Dual-Gated MoS2 Architecture

In this work, we demonstrate a dual-gated (DG) MoS2 field effect transistors (FETs) in which the degraded switching performance of multilayer MoS2 can be compensated by the DG structure. It produces large current density (>100 μA/μm for a monolayer), steep subthreshold swing (SS) (~100 mV/dec for 5 nm thickness), and high on/off current ratio (greater than 107 for 10 nm thickness). Such DG structure not only improves electrostatic control but also provides an extra degree of freedom for manipulating the threshold voltage (VTH) and SS by separately tuning the top and back gate voltages, which are demonstrated in a logic inverter. Dynamic random access memory (DRAM) has a short retention time because of large OFF-state current in the Si MOSFET. Based on our DG MoS2-FETs, and a DRAM unit cell with a long retention time of 1260 ms are realized. A large-scale isolated MoS2 DG-FETs based on CVD-synthesized continuous films is also demonstrated, which shows potential applications for future wafer-scale digital and low-power electronics.

physics.app-ph↗

arXiv2019

MoS$_2$ Dual-gate Transistors with Electrostatically Doped Contacts

Two-dimensional (2D) transition metal dichalcogenides (TMDs) such as molybdenum disulfide (MoS2) have been intensively investigated because of their exclusive physical properties for advanced electronics and optoelectronics. In the present work, we study the MoS2 transistor based on a novel tri-gate device architecture, with dual-gate (Dual-G) in the channel and the buried side-gate (Side-G) for the source/drain regions. All gates can be independently controlled without interference. For a MoS2 sheet with a thickness of 3.6 nm, the Schottky barrier (SB) and non-overlapped channel region can be effectively tuned by electrostatically doping the source/drain regions with Side-G. Thus, the extrinsic resistance can be effectively lowered, and a boost of the ON-state current can be achieved. Meanwhile, the channel control remains efficient under the Dual-G mode, with an ON-OFF current ratio of 3E7 and subthreshold swing of 83 mV/decade. The corresponding band diagram is also discussed to illustrate the device operation mechanism. This novel device structure opens up a new way toward fabrication of high-performance devices based on 2D-TMDs.

physics.app-ph↗

arXiv2019

Mechanical characterization of cells and microspheres sorted by acoustophoresis with in-line resistive pulse sensing

Resistive Pulse Sensing (RPS) is a key label-free technology to measure particles and single-cell size distribution. As a growing corpus of evidence supports that cancer cells exhibit distinct mechanical phenotypes from healthy cells, expanding the method from size to mechanical sensing could represent a pertinent and innovative tool for cancer research. In this paper, we infer the cells compressibility by using acoustic radiation pressure to deflect flowing cells in a microchannel, and use RPS to sense the subpopulations of cells and particles at each acoustic power level. We develop and validate a linear model to analyze experimental data from a large number of particles. This high-precision linear model is complemented by a more robust (yet less detailed) statistical model to analyze datasets with fewer particles. Compared to current acoustic cell phenotyping apparatus based on video cameras, the proposed approach is not limited by the optical diffraction, frame rate, data storage or processing speed, and may ultimately constitute a step forward towards point-of-care acousto-electrical phenotyping and acoustic phenotyping of nanoscale objects such as exosomes and viruses.

physics.bio-ph↗

arXiv2019

On-demand contact line pinning during droplet evaporation

Depending on the contact line motion, colloid-rich drolets evaporation can leave a ring-like or a spot-like residue. Herein, we determine this outcome by controlling the contact line motion using coplanar direct current electrowetting-on-dielectrics (DC-EWOD). Combined with theoretical calculations of the droplet shape and its evaporation rate, the time-dependent actuation voltage is first derived from experiments and simulations. Thanks to the additional control over the contact angle, the contact line can be maintained in pinned state even on surfaces that exhibit little contact angle hysteresis such as homogenous flat Teflon coatings. In the absence of EWOD control, polystyrene particles and Escherichia coli suspended in the droplet formed a dot-like pattern at the center of the initial contact, whereas application of the mechanism resulted in ring-like patterns of a controllable radius. Unlike chemically or structurally patterned substrates, the contact line could recover its mobility at any preset time before reaching the control limit, which is useful to accurately and consistently fabricate self-assembled nanostructures of desired patterns on different surfaces.

physics.flu-dyn↗

arXiv2019

Trajectory of particles exposed to a tilted-angle washboard potential: application to high-throughput acoustophoresis in microchannels

A wide variety of tilted washboard potentials based on acoustic waves, electric fields, optical patterns and so on have been applied to sort particles in microchannels. In this paper, we present a theoretical analysis of the particles trajectory in a washboard potential making a tilt angle $θ$ with the flow. Depending on the sorting to drag force ratio $ε$, we identified a transition threshold $ε= \cos(θ)$ between two distinct regimes of particles motion: drift and locked modes. In drift mode, the particles follow an oscillating trajectory which slope is given by $\frac{ε^2}{2}\tan(θ)$, while in locked mode the trajectory slope is given by $1/\tan(θ)$. These theoretical predictions agree quantitatively well with previously published experimental data and may help in the design of high-performance microfluidic sorting devices.

physics.flu-dyn↗

arXiv2018

Folding a focalized acoustical vortex on a flat holographic transducer: miniaturized selective acoustical tweezers

Acoustical tweezers based on focalized acoustical vortices hold the promise of precise contactless 3D manipulation of millimeter down to sub-micrometer particles, microorganisms and cells with unprecedented combined selectivity and trapping force. Yet, the widespread dissemination of this technology has been hindered by severe limitations of current systems in terms of performance and/or miniaturization and integrability. In this paper, we unleash the potential of focalized acoustical vortices by developing the first flat, compact, single-electrodes focalized acoustical tweezers. These tweezers rely on holographic Archimedes-Fermat spiraling transducers obtained by folding a spherical acoustical vortex on a flat piezoelectric substrate. We demonstrate the ability of these tweezers to grab and displace micrometric objects in a standard microfluidic environment with unique selectivity. The simplicity of this system and its scalability to higher frequencies opens tremendous perspectives in microbiology, microrobotics and microscopy.

physics.class-ph↗

arXiv2016

Influence of viscosity on acoustic streaming in sessile droplets: an experimental and a numerical study with a Streaming Source Spatial Filtering (SSSF) method

When an acoustic wave travels in a lossy medium such as a liquid, it progressively transfers its pseudo-momentum to the fluid, which results in a steady acoustic streaming. Remarkably, the phenomenon involves a balance between sound attenuation and shear, such that viscosity vanishes in the final expression of the velocity field. For this reason, the effect of viscosity has long been ignored in acoustic streaming experiments. Here, we show experimentally that the viscosity plays a major role in cavities such as the streaming induced by surface acoustic waves in sessile droplets. We develop a numerical model based on the spatial filtering of the streaming source term to compute the induced flow motion with dramatically reduced computational requirements. We evidence that acoustic fields in droplets are a superposition of a chaotic field and a few powerful caustics. It appears that the caustics drive the flow, which allows a qualitative prediction of the flow structure. Finally, we reduce the problem to two dimensionless numbers related to the surface and bulk waves attenuation and simulate hemispherical sessile droplets resting on a lithium niobate substrate for a range of parameters. Even in such a baseline configuration, we observe at least four distinct flow regimes. For each of them, we establish a correlation of the average streaming speed in the droplet, which is increasingly dependent on the bulk wave attenuation as the viscosity increases. These correlations extend our results to a wide range of fluids and actuation frequencies.

physics.flu-dyn↗

arXiv2016

SAW synthesis with IDTs array and the inverse filter: toward a versatile SAW toolbox for microfluidics and biological applications

Surface acoustic waves (SAWs) are versatile tools to manipulate fluids at small scales for microfluidics and bio- logical applications. A non-exhaustive list of operations that can be performed with SAW includes sessile droplet displacement, atomization, division and merging but also the actuation of fluids embedded in microchannels or the manipulation of suspended particles. However, each of these operations requires a specific design of the wave generation system, the so-called interdigitated transducers (IDTs). Depending on the application, it might indeed be necessary to generate focused or plane, propagating or standing, aligned or shifted waves. Furthermore, the possibilities offered by more complex wave-fields such as acoustical vortices for particle tweezing and liquid twisting cannot be explored with classical IDTs. In this paper, we show that the inverse filter technique coupled with an interdigitated transducers array (IDTA) enables to synthesize all classical wave-fields used in microfluidics and biological applications with a single multi- function platform. It also enables to generate swirling SAWs, whose potential for the on-chip synthesis of tailored acoustical vortices has been demonstrated lately. The possibilities offered by this platform is illustrated by performing successively many operations on sessile droplets with the same system.

physics.flu-dyn↗

arXiv2015

Taming the degeneration of Bessel beams at anisotropic-isotropic interface: toward 3D control of confined vortical waves

Despite their self-reconstruction properties in heterogeneous media, Bessel beams are known to degenerate when they are refracted from an isotropic to an anisotropic medium. In this paper, we study the converse situation wherein an anisotropic Bessel beam is refracted into an isotropic medium. It is shown that these anisotropic Bessel beams also degenerate, leading to confined vortical waves that may serve as localized particle trap for acoustical tweezers. The linear nature of this degeneration allows the 3D control of this trap position by wavefront correction. Theory is confronted to experiments performed in the field of acoustics. A swirling surface acoustic wave is synthesized at the surface of a piezoelectric crystal by a MEMS integrated system and radiated inside a miniature liquid vessel. The wavefront correction is operated with inverse filter technique. This work opens perspectives for contactless on-chip manipulation devices.

physics.flu-dyn↗