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Antonio H. Castro Neto

Publications and source records attributed to Antonio H. Castro Neto.

At least 37 records · Page 2Linked to original sources

Optical conductivity study of screening of many-body effects in graphene interfaces

Theoretical studies have shown that electron-electron (e-e) and electron-hole (e-h) interactions play important roles in many observed quantum properties of graphene making this an ideal system to study many body effects. In this report we show that spectroscopic ellipsometry can enable us to measure this interactions quantitatively. We present spectroscopic data in two extreme systems of graphene on quartz (GOQ), an insulator, and graphene on copper (GOC), a metal which show that for GOQ, both e-e and e-h interactions dominate while for GOC e-h interactions are screened. The data further enables the estimation of the strength of the many body interaction through the effective fine structure constant, $α_{g}^{*}$. The $α_{g}^{*}$ for GOQ indicates a strong correlation with an almost energy independent value of about 1.37. In contrast, $α_{g}^{*}$ value of GOC is photon energy dependent, is almost two orders of magnitude lower at low energies indicating very weak correlation.

cond-mat.mes-hall↗

Magnetic states and optical properties of single-layer carbon-doped hexagonal boron nitride

We show that carbon-doped hexagonal boron nitride (h-BN) has extraordinary properties with many possible applications. We demonstrate that the substitution-induced impurity states, associated with carbon atoms, and their interactions dictate the electronic structure and properties of C-doped h-BN. Furthermore, we show that stacking of localized impurity states in small C clusters embedded in h-BN forms a set of discrete energy levels in the wide gap of h-BN. The electronic structures of these C clusters have a plethora of applications in optics, magneto-optics, and opto-electronics.

cond-mat.mes-hall↗

Atomically thin boron nitride: a tunnelling barrier for graphene devices

We investigate the electronic properties of heterostructures based on ultrathin hexagonal boron nitride (h-BN) crystalline layers sandwiched between two layers of graphene as well as other conducting materials (graphite, gold). The tunnel conductance depends exponentially on the number of h-BN atomic layers, down to a monolayer thickness. Exponential behaviour of I-V characteristics for graphene/BN/graphene and graphite/BN/graphite devices is determined mainly by the changes in the density of states with bias voltage in the electrodes. Conductive atomic force microscopy scans across h-BN terraces of different thickness reveal a high level of uniformity in the tunnel current. Our results demonstrate that atomically thin h-BN acts as a defect-free dielectric with a high breakdown field; it offers great potential for applications in tunnel devices and in field-effect transistors with a high carrier density in the conducting channel.

cond-mat.mes-hall↗

Near-field spectroscopy of silicon dioxide thin films

We analyze the results of scanning near-field infrared spectroscopy performed on thin films of a-SiO2 on Si substrate. The measured near-field signal exhibits surface-phonon resonances whose strength has a strong thickness dependence in the range from 2 to 300 {nm}. These observations are compared with calculations in which the tip of the near-field infrared spectrometer is modeled either as a point dipole or an elongated spheroid. The latter model accounts for the antenna effect of the tip and gives a better agreement with the experiment. Possible applications of the near-field technique for depth profiling of layered nanostructures are discussed.

cond-mat.mes-hall↗

Electronic doping of graphene by deposited transition metal atoms

We perform a phenomenological analysis of the problem of the electronic doping of a graphene sheet by deposited transition metal atoms, which aggregate in clusters. The sample is placed in a capacitor device such that the electronic doping of graphene can be varied by the application of a gate voltage and such that transport measurements can be performed via the application of a (much smaller) voltage along the graphene sample, as reported in the work of Pi et al. [Phys. Rev. B 80, 075406 (2009)]. The analysis allows us to explain the thermodynamic properties of the device, such as the level of doping of graphene and the ionisation potential of the metal clusters in terms of the chemical interaction between graphene and the clusters. We are also able, by modelling the metallic clusters as perfect conducting spheres, to determine the scattering potential due to these clusters on the electronic carriers of graphene and hence the contribution of these clusters to the resistivity of the sample. The model presented is able to explain the measurements performed by Pi et al. on Pt-covered graphene samples at the lowest metallic coverages measured and we also present a theoretical argument based on the above model that explains why significant deviations from such a theory are observed at higher levels of coverage.

cond-mat.str-el↗

Selected Topics in Graphene physics

Graphene research is currently one of the largest fields in condensed matter. Due to its unusual electronic spectrum with Dirac-like quasiparticles, and the fact that it is a unique example of a metallic membrane, graphene has properties that have no match in standard solid state textbooks. In these lecture notes, I discuss some of these properties that are not covered in detail in recent reviews. We study the particular aspects of the physics/chemistry of carbon that influence the properties of graphene; the basic features of graphene's band structure including the pi and sigma bands; the phonon spectra in free floating graphene; the effects of a substrate on the structural properties of graphene; and the effect of deformations in the propagation of electrons. The objective of these notes is not to provide an unabridged theoretical description of graphene but to point out some of the peculiar aspects of this material.

cond-mat.mtrl-sci↗

The Carbon New Age

Graphene has been considered by many as a revolutionary material with electronic and structural properties that surpass conventional semiconductors and metals. Due to its superlative qualities, graphene is being considered as the reference material for a post-CMOS technology. Furthermore, graphene is also quite unusual electronically since its electric carriers behave as if they were massless and relativistic, the so-called Dirac particles. Because of its exotic electronic properties, theorists are being forced to revisit the conceptual basis for the theory of metals. Hence, graphene seems to be unveiling a new era in science and technology with still unseen consequences.

cond-mat.mtrl-sci↗

All-graphene integrated circuits via strain engineering

We propose a route to all-graphene integrated electronic devices by exploring the influence of strain on the electronic structure of graphene. We show that strain can be easily tailored to generate electron beam collimation, 1D channels, surface states and confinement, the basic elements for all-graphene electronics. In addition this proposal has the advantage that patterning can be made on substrates rather than on the graphene sheet, thereby protecting the integrity of the latter.

cond-mat.mes-hall↗

Conductance quantization and transport gap in disordered graphene nanoribbons

We study numerically the effects of edge and bulk disorder on the conductance of graphene nanoribbons. We compute the conductance suppression due to localization induced by edge scattering. We find that even for weak edge roughness, conductance steps are suppressed and transport gaps appear. These gaps are approximately inversely proportional to the nanoribbon width. On/off conductance ratios grow exponentially with the nanoribbon length. Our results impose severe limitations to the use of graphene in ballistic nanowires.

cond-mat.mes-hall↗

Adatoms in Graphene

We review the problem of adatoms in graphene under two complementary points of view, scattering theory and strong correlations. We show that in both cases impurity atoms on the graphene surface present effects that are absent in the physics of impurities in ordinary metals. We discuss how to observe these unusual effects with standard experimental probes such as scanning tunneling microscopes, and spin susceptibility.

cond-mat.mtrl-sci↗

Double Exchange Model at Low Densities: Magnetic Polarons and Coulomb Suppressed Phase Separation

We consider the double exchange model at very low densities. The conditions for the formation of self-trapped magnetic polarons are analyzed using an independent polaron model. The issue of phase separation in the low density region of the temperature-density phase diagram is discussed. We show how electrostatic and localization effects can lead to the substantial suppression of the phase separated regime. By examining connections between the resulting phase and the polaronic phase, we conclude that they reflect essentially the same physical situation of a ferromagnetic droplet containing one single electron. In the ultra diluted regime, we explore the possible stabilization of a Wigner crystal of magnetic polarons. Our results are compared with the experimental evidence for a polaronic phase in europium hexaboride, and we are able to reproduce the experimental region of stability of the polaronic phase. We further demonstrate that phase-separation is a general feature expected in metallic ferromagnets whose bandwidth depends on the magnetization.

cond-mat.str-el↗

Conductivity and Fano factor in disordered graphene

Using the recursive Green's function method, we study the problem of electron transport in a disordered single-layer graphene sheet. The conductivity is of order $e^2/h$ and its dependence on the carrier density has a scaling form that is controlled solely by the disorder strength and the ratio between the sample size and the correlation length of the disorder potential. The shot noise Fano factor is shown to have a narrow dip near the neutrality point for weak disorder and to develop a nearly doping independent behavior at strong disorder. Our results are in good qualitative and quantitative agreement with experiments and provide a way for extracting microscopic information about the magnitude of extrinsic disorder in graphene.

cond-mat.mes-hall↗

Metallic Continuum Quantum Ferromagnets at Finite Temperature

We study via renormalization group (RG) and large N methods the problem of continuum SU(N) quantum Heisenberg ferromagnets (QHF) coupled to gapless electrons. We establish the phase diagram of the dissipative problem and investigate the changes in the Curie temperature, magnetization, and magnetic correlation length due to dissipation and both thermal and quantum fluctuations. We show that the interplay between the topological term (Berry's phase) and dissipation leads to non-trivial effects for the finite temperature critical behavior.

cond-mat.str-el↗

P-wave pairing and ferromagnetism in the metal-insulator transition in two dimensions

Based on recent experimental evidence for a spin polarized ground state in the insulating phase of the two-dimensional electron system, we propose that ferromagnetic spin fluctuations lead to an attractive interaction in the triplet channel and cause p-wave pairing in the conducting phase. We use the Landau Fermi liquid phenomenology to explain how the enhanced spin susceptibility near the critical density yields an attractive potential, in a similar mechanism to superfluidity in $^3$He. As the density is decreased, the p-wave order parameter undergoes a transition from a unitary to a nonunitary state, in which it coexists with ferromagnetism for a range of densities. As the density is further reduced, the pairing amplitude vanishes and the system is described by a ferromagnetic insulator. Thus, we find two quantum critical points as a function of density associated with the polarization of the paired state and ferromagnetism. We explain the magnetotransport measurements in parallel and perpendicular magnetic fields and propose a shot noise experiment to measure the pair charge.

cond-mat.str-el↗

Droplets in Disordered Metallic Quantum Critical Systems

We present a field theory for a structurally disordered magnetic system coupled to a metallic environment near a quantum critical point. We show that close to the magnetic quantum critical point droplets are formed due to the disorder and undergo dissipative quantum dynamics. We show that the problem has a characteristic energy scale, the droplet Kondo temperature, that determines the crossover energy scale from weak to strong coupling. Our results have direct significance for the Griffiths-McCoy singularities of itinerant magnets.

cond-mat.str-el↗

Stripes, Vibrations and Superconductivity

We propose a model of a spatially modulated collective charge state of superconducting cuprates. The regions of higher carrier density (stripes) are described in terms of Luttinger liquids and the regions of lower density as a two-dimensional interacting bosonic gas of d_{x^2-y^2} hole pairs. The interactions among the elementary excitations are repulsive and the transition to the superconducting state is driven by decay processes. Vibrations of the CCS and the lattice, although not participating directly in the binding mechanism, are fundamental for superconductivity. The superfluid density and the lattice have a strong tendency to modulation implying a still unobserved dimerized stripe phase in cuprates. The phase diagram of the model has a crossover from 1D to 2D behavior and a pseudogap region where the amplitude of the order parameters are finite but phase coherence is not established. We discuss the nature of the spin fluctuations and the unusual isotope effect within the model.

cond-mat.supr-con↗

CDW, Superconductivity and Anomalous Metallic Behavior in 2D Transition Metal Dichalcogenides

We propose a theory for quasi-two-dimensional transition metal dichalcogenides that provides a unified microscopic picture of the charge density wave (CDW) and superconducting phases. We show, based on the electron-phonon coupling and Fermi surface topology, that a CDW order parameter with six-fold symmetry and nodes (f-wave) gives a consistent description of the available experimental data. The elementary excitations in the CDW phase are Dirac electrons. The superconducting state has its origin on the attractive interaction mediated by phonons. The theory predicts strong deviations from Fermi liquid theory in the CDW phase.

cond-mat.str-el↗

Pairing, Stripes, Lattice Distortions and Superconductivity in Cuprate Oxides

We propose a model for a spatially modulated collective state of superconducting cuprates in which the electronic properties vary locally in space. In this model the regions of higher hole density (called stripes) are described as Luttinger liquids and the regions of lower density (antiferromagnetic ladders) as an interacting bosonic gas of d$_{x^2-y^2}$ hole pairs. We show that the transition to the superconducting state is topological and driven by decay processes among these elementary excitations in the presence of vibrations.

cond-mat.supr-con↗